Perovskite silicon tandem solar cells: two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Stuttgart
Fraunhofer Verlag
[2020]
|
| Schriftenreihe: | Solare Energie- und Systemforschung/Solar energy and system research
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | 172 Seiten Illustrationen, Diagramme 21 cm x 14.8 cm |
| ISBN: | 383961662X 9783839616628 |
Internformat
MARC
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| 100 | 1 | |a Bett, Alexander Jürgen |d 1988- |e Verfasser |0 (DE-588)1214769675 |4 aut | |
| 245 | 1 | 0 | |a Perovskite silicon tandem solar cells |b two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |c Alexander Jürgen Bett |
| 264 | 1 | |a Stuttgart |b Fraunhofer Verlag |c [2020] | |
| 264 | 4 | |c © 2020 | |
| 300 | |a 172 Seiten |b Illustrationen, Diagramme |c 21 cm x 14.8 cm | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 0 | |a Solare Energie- und Systemforschung/Solar energy and system research | |
| 502 | |b Dissertation |c Albert-Ludwigs-Universität freiburg |d 2020 | ||
| 650 | 0 | 7 | |a Perowskit |0 (DE-588)4173836-6 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Solarzelle |0 (DE-588)4181740-0 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Mehrfach-Solarzelle |0 (DE-588)4674119-7 |2 gnd |9 rswk-swf |
| 653 | |a Halbleitertechnologen | ||
| 653 | |a Perovskite | ||
| 653 | |a Tandem Solar Cell | ||
| 653 | |a Thermalization | ||
| 653 | |a low-temperature process | ||
| 653 | |a silicon heterojunction solar cells | ||
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
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| 710 | 2 | |a Fraunhofer-Institut für Solare Energiesysteme |0 (DE-588)2081865-8 |4 isb | |
| 710 | 2 | |a Fraunhofer IRB-Verlag |0 (DE-588)4786605-6 |4 pbl | |
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Datensatz im Suchindex
| _version_ | 1804182112559955968 |
|---|---|
| adam_text | TABLE
OF
CONTENTS
ABSTRACT
....................................................................................................................................................
3
GERMAN
SUMMARY
I
DEUTSCHE
ZUSAMMENFASSUNG
..............................................................................
5
1
INTRODUCTION
....................................................................................................................................
11
1.1
MOTIVATION
...............................................................................................................................
11
1.1.1
PHOTOVOLTAICS
..............................................................................................................
11
1.1.2
SILICON-BASED
TANDEM
SOLAR
CELLS
............................................................................
12
1.2
CHALLENGES
AND
OBJECTIVES
OF
THE
THESIS
...............................................................................
15
1.3
STRUCTURE
OF
THE
THESIS
............................................................................................................
16
2
THEORETICAL
BACKGROUND
................................................................................................................
19
2.1
PEROVSKITE
SOLAR
CELLS
............................................................................................................
19
2.1.1
PROPERTIES
OF
PEROVSKITE
MATERIALS
.............................................................................
19
2.1.2
SOLAR
CELL
ARCHITECTURES
............................................................................................
22
2.1.3
HYSTERESIS
...................................................................................................................
24
2.2
PEROVSKITE
SILICON
TANDEM
SOLAR
CELLS
.................................................................................
26
2.2.1
FUNDAMENTALS
OF
TANDEM
SOLAR
CELLS
.......................................................................
26
2.2.2
STATE
OF
THE
ART
AT
THE
BEGINNING
OF
THIS
WORK
.........................................................
28
2.2.3
INTERCONNECTION
LAYER
.................................................................................................
29
2.2.4
FRONT
SIDE
CONTACT
.....................................................................................................
30
2.2.5
CURRENT
PEROVSKITE
SILICON
TANDEM
SOLAR
CELL
RESULTS
.............................................32
3
METHODS
...........................................................................................................................................
37
3.1
SAMPLE
F
ABRICATION
................................................................................................................
37
3.1.1
SILICON
BOTTOM
SOLAR
CELLS
.......................................................................................
37
3.1.2
PEROVSKITE
TOP
SOLAR
CELLS
.......................................................................................
39
3.2
CHARACTERIZATION
.....................................................................................................................
45
3.2.1
CURRENT-VOLTAGE
MEASUREMENTS
.................................................................................
45
3.2.2
SUNS
K
OC
MEASUREMENTS
.............................................................................................50
3.2.3
SPECTRAL
ELLIPSOMETRY
................................................................................................
50
3.2.4
REFLECTANCE
AND
TRANSMITTANCE
MEASUREMENTS
........................................................52
3.2.5
FURTHER
CHARACTERIZATION
METHODS
............................................................................
53
7
4
OPTIMIZATION
OF
PEROVSKITE
SOLAR
CELLS
FOR
APPLICATION
IN
TANDEM
DEVICES
.............
55
4.1
LOW-TEMPERATURE
PROCESS
FOR
PEROVSKITE
SOLAR
CELLS
................................................
55
4.1.1
DEGRADATION
OF
BOTTOM
SOLAR
CELLS
DUE
TO
HIGH
TEMPERATURES
.....................
56
4.1.2
OPTIMIZATION
OF
LOW-TEMPERATURE
PROCESSES
FOR
TIO
X
..................................
59
4.1.3
COMPARISON
BETWEEN
HIGH-
AND
LOW-TEMPERATURE
PROCESS
..........................
64
4.1.4
TIO
X
AND
SNO
X
ELECTRON
CONTACTS
DEPOSITED
BY
ATOMIC
LAYER
DEPOSITION
......
65
4.1.5
SUMMARY
AND
CONCLUSION
.................................................................................
68
4.2
HIGH-BANDGAP
PEROVSKITE
ABSORBER
AND
PASSIVATING
ELECTRON
CONTACT
....................
69
4.2.1
MIXED
CATION
MIXED
HALIDE
PEROVSKITE
...........................................................
69
4.2.2
PASSIVATING
ELECTRON
CONTACT
.............................................................................
70
4.2.3
SUMMARY
AND
CONCLUSION
.................................................................................
72
4.3
HOLE
CONTACTS
FOR
PEROVSKITE
SOLAR
CELLS
.....................................................................
72
4.3.1
SCREENING
OF
HOLE
CONTACT
MATERIALS
...............................................................
73
4.3.2
OPTIMIZATION
OF
CUSCN
....................................................................................
75
4.3.3
SUMMARY
AND
CONCLUSION
.................................................................................
76
4.4
SEMI-TRANSPARENT
PEROVSKITE
SOLAR
CELLS
.....................................................................
77
4.4.1
PROCESS
OPTIMIZATION
FOR
ITO
DIRECTLY
SPUTTERED
ON
SPIRO-OMETAD
.......
78
4.4.2
BUFFER
LAYERS
BETWEEN
ITO
AND
SPIRO-OMETAD
..........................................
82
4.4.3
OPTICAL
IMPROVEMENT
..........................................................................................
83
4.4.4
FOUR-TERMINAL
TANDEM
PERFORMANCE
ESTIMATION
...........................................
90
4.4.5
SUMMARY
AND
CONCLUSION
.................................................................................
91
4.5
PEROVSKITE
SOLAR
CELL
PERFORMANCE
EVOLUTION
.............................................................
92
5
MONOLITHIC
PEROVSKITE
SILICON
TANDEM
SOLAR
CELLS
.........................................................
99
5.1
SILICON
BOTTOM
SOLAR
CELLS
.............................................................................................
99
5.2
FIRST
TANDEM
SOLAR
CELLS
.............................................................................................
101
5.2.1
SOLAR
CELL
ARCHITECTURE
.....................................................................................
101
5.2.2
RESULTS
AND
DISCUSSION
.....................................................................................
102
5.3
TANDEM
SOLAR
CELLS
WITH
ADVANCED
STRUCTURE
..........................................................
103
5.3.1
SOLAR
CELL
ARCHITECTURE
.....................................................................................
103
5.3.2
SPATIALLY
RESOLVED
PHOTOLUMINESCENCE
IMAGING
...........................................
104
5.3.3
SOLAR
CELL
RESULTS
.............................................................................................
106
5.3.4
CALLAB
PV
CELLS
MEASUREMENTS
AND
SPECTROMETRIC
CHARACTERIZATION
.......
108
5.3.5
SUMMARY
AND
DISCUSSION
................................................................................
114
5.3.6
RECOMMENDATIONS
FOR
FURTHER
IMPROVEMENT
.................................................
116
8
5.4
TANDEM
SOLAR
CELLS
WITH
SPIRO-TTB
AS
FRONT
HOLE
CONTACT
.....................................
117
5.4.1
SOLAR
CELL
ARCHITECTURE
...................................................................................
118
5.4.2
RESULTS
AND
DISCUSSION
.....................................................................................
119
5.4.3
POTENTIAL
FOR
FURTHER
IMPROVEMENT
..................................................................
123
5.5
CONCLUSION
....................................................................................................................
124
6
SUMMARY
AND
OUTLOOK
........................................................................................................
127
6.1
SUMMARY
......................................................................................................................
127
6.2
OUTLOOK
..........................................................................................................................
129
REFERENCES
....................................................................................................................................
131
PUBLICATIONS
..................................................................................................................................
159
JOURNAL
PAPERS
.........................................................................................................................
159
CONTRIBUTIONS
TO
CONFERENCES
AND
WORKSHOPS
....................................................................
160
LIST
OF
SYMBOLS
............................................................................................................................
163
LIST
OF
ABBREVIATIONS
..................................................................................................................
167
ACKNOWLEDGEMENTS
.....................................................................................................................
171
9
|
| adam_txt |
TABLE
OF
CONTENTS
ABSTRACT
.
3
GERMAN
SUMMARY
I
DEUTSCHE
ZUSAMMENFASSUNG
.
5
1
INTRODUCTION
.
11
1.1
MOTIVATION
.
11
1.1.1
PHOTOVOLTAICS
.
11
1.1.2
SILICON-BASED
TANDEM
SOLAR
CELLS
.
12
1.2
CHALLENGES
AND
OBJECTIVES
OF
THE
THESIS
.
15
1.3
STRUCTURE
OF
THE
THESIS
.
16
2
THEORETICAL
BACKGROUND
.
19
2.1
PEROVSKITE
SOLAR
CELLS
.
19
2.1.1
PROPERTIES
OF
PEROVSKITE
MATERIALS
.
19
2.1.2
SOLAR
CELL
ARCHITECTURES
.
22
2.1.3
HYSTERESIS
.
24
2.2
PEROVSKITE
SILICON
TANDEM
SOLAR
CELLS
.
26
2.2.1
FUNDAMENTALS
OF
TANDEM
SOLAR
CELLS
.
26
2.2.2
STATE
OF
THE
ART
AT
THE
BEGINNING
OF
THIS
WORK
.
28
2.2.3
INTERCONNECTION
LAYER
.
29
2.2.4
FRONT
SIDE
CONTACT
.
30
2.2.5
CURRENT
PEROVSKITE
SILICON
TANDEM
SOLAR
CELL
RESULTS
.32
3
METHODS
.
37
3.1
SAMPLE
F
ABRICATION
.
37
3.1.1
SILICON
BOTTOM
SOLAR
CELLS
.
37
3.1.2
PEROVSKITE
TOP
SOLAR
CELLS
.
39
3.2
CHARACTERIZATION
.
45
3.2.1
CURRENT-VOLTAGE
MEASUREMENTS
.
45
3.2.2
SUNS
K
OC
MEASUREMENTS
.50
3.2.3
SPECTRAL
ELLIPSOMETRY
.
50
3.2.4
REFLECTANCE
AND
TRANSMITTANCE
MEASUREMENTS
.52
3.2.5
FURTHER
CHARACTERIZATION
METHODS
.
53
7
4
OPTIMIZATION
OF
PEROVSKITE
SOLAR
CELLS
FOR
APPLICATION
IN
TANDEM
DEVICES
.
55
4.1
LOW-TEMPERATURE
PROCESS
FOR
PEROVSKITE
SOLAR
CELLS
.
55
4.1.1
DEGRADATION
OF
BOTTOM
SOLAR
CELLS
DUE
TO
HIGH
TEMPERATURES
.
56
4.1.2
OPTIMIZATION
OF
LOW-TEMPERATURE
PROCESSES
FOR
TIO
X
.
59
4.1.3
COMPARISON
BETWEEN
HIGH-
AND
LOW-TEMPERATURE
PROCESS
.
64
4.1.4
TIO
X
AND
SNO
X
ELECTRON
CONTACTS
DEPOSITED
BY
ATOMIC
LAYER
DEPOSITION
.
65
4.1.5
SUMMARY
AND
CONCLUSION
.
68
4.2
HIGH-BANDGAP
PEROVSKITE
ABSORBER
AND
PASSIVATING
ELECTRON
CONTACT
.
69
4.2.1
MIXED
CATION
MIXED
HALIDE
PEROVSKITE
.
69
4.2.2
PASSIVATING
ELECTRON
CONTACT
.
70
4.2.3
SUMMARY
AND
CONCLUSION
.
72
4.3
HOLE
CONTACTS
FOR
PEROVSKITE
SOLAR
CELLS
.
72
4.3.1
SCREENING
OF
HOLE
CONTACT
MATERIALS
.
73
4.3.2
OPTIMIZATION
OF
CUSCN
.
75
4.3.3
SUMMARY
AND
CONCLUSION
.
76
4.4
SEMI-TRANSPARENT
PEROVSKITE
SOLAR
CELLS
.
77
4.4.1
PROCESS
OPTIMIZATION
FOR
ITO
DIRECTLY
SPUTTERED
ON
SPIRO-OMETAD
.
78
4.4.2
BUFFER
LAYERS
BETWEEN
ITO
AND
SPIRO-OMETAD
.
82
4.4.3
OPTICAL
IMPROVEMENT
.
83
4.4.4
FOUR-TERMINAL
TANDEM
PERFORMANCE
ESTIMATION
.
90
4.4.5
SUMMARY
AND
CONCLUSION
.
91
4.5
PEROVSKITE
SOLAR
CELL
PERFORMANCE
EVOLUTION
.
92
5
MONOLITHIC
PEROVSKITE
SILICON
TANDEM
SOLAR
CELLS
.
99
5.1
SILICON
BOTTOM
SOLAR
CELLS
.
99
5.2
FIRST
TANDEM
SOLAR
CELLS
.
101
5.2.1
SOLAR
CELL
ARCHITECTURE
.
101
5.2.2
RESULTS
AND
DISCUSSION
.
102
5.3
TANDEM
SOLAR
CELLS
WITH
ADVANCED
STRUCTURE
.
103
5.3.1
SOLAR
CELL
ARCHITECTURE
.
103
5.3.2
SPATIALLY
RESOLVED
PHOTOLUMINESCENCE
IMAGING
.
104
5.3.3
SOLAR
CELL
RESULTS
.
106
5.3.4
CALLAB
PV
CELLS
MEASUREMENTS
AND
SPECTROMETRIC
CHARACTERIZATION
.
108
5.3.5
SUMMARY
AND
DISCUSSION
.
114
5.3.6
RECOMMENDATIONS
FOR
FURTHER
IMPROVEMENT
.
116
8
5.4
TANDEM
SOLAR
CELLS
WITH
SPIRO-TTB
AS
FRONT
HOLE
CONTACT
.
117
5.4.1
SOLAR
CELL
ARCHITECTURE
.
118
5.4.2
RESULTS
AND
DISCUSSION
.
119
5.4.3
POTENTIAL
FOR
FURTHER
IMPROVEMENT
.
123
5.5
CONCLUSION
.
124
6
SUMMARY
AND
OUTLOOK
.
127
6.1
SUMMARY
.
127
6.2
OUTLOOK
.
129
REFERENCES
.
131
PUBLICATIONS
.
159
JOURNAL
PAPERS
.
159
CONTRIBUTIONS
TO
CONFERENCES
AND
WORKSHOPS
.
160
LIST
OF
SYMBOLS
.
163
LIST
OF
ABBREVIATIONS
.
167
ACKNOWLEDGEMENTS
.
171
9 |
| any_adam_object | 1 |
| any_adam_object_boolean | 1 |
| author | Bett, Alexander Jürgen 1988- |
| author_GND | (DE-588)1214769675 |
| author_facet | Bett, Alexander Jürgen 1988- |
| author_role | aut |
| author_sort | Bett, Alexander Jürgen 1988- |
| author_variant | a j b aj ajb |
| building | Verbundindex |
| bvnumber | BV047093244 |
| classification_rvk | ZN 5160 ZP 3730 |
| ctrlnum | (OCoLC)1238066767 (DE-599)DNB1222299542 |
| discipline | Elektrotechnik / Elektronik / Nachrichtentechnik Energietechnik |
| discipline_str_mv | Elektrotechnik / Elektronik / Nachrichtentechnik Energietechnik |
| format | Thesis Book |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV047093244 |
| illustrated | Illustrated |
| index_date | 2024-07-03T16:20:22Z |
| indexdate | 2024-07-10T09:02:22Z |
| institution | BVB |
| institution_GND | (DE-588)2081865-8 (DE-588)4786605-6 |
| isbn | 383961662X 9783839616628 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-032499762 |
| oclc_num | 1238066767 |
| open_access_boolean | |
| owner | DE-29T DE-83 |
| owner_facet | DE-29T DE-83 |
| physical | 172 Seiten Illustrationen, Diagramme 21 cm x 14.8 cm |
| publishDate | 2020 |
| publishDateSearch | 2020 |
| publishDateSort | 2020 |
| publisher | Fraunhofer Verlag |
| record_format | marc |
| series2 | Solare Energie- und Systemforschung/Solar energy and system research |
| spelling | Bett, Alexander Jürgen 1988- Verfasser (DE-588)1214769675 aut Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells Alexander Jürgen Bett Stuttgart Fraunhofer Verlag [2020] © 2020 172 Seiten Illustrationen, Diagramme 21 cm x 14.8 cm txt rdacontent n rdamedia nc rdacarrier Solare Energie- und Systemforschung/Solar energy and system research Dissertation Albert-Ludwigs-Universität freiburg 2020 Perowskit (DE-588)4173836-6 gnd rswk-swf Solarzelle (DE-588)4181740-0 gnd rswk-swf Mehrfach-Solarzelle (DE-588)4674119-7 gnd rswk-swf Halbleitertechnologen Perovskite Tandem Solar Cell Thermalization low-temperature process silicon heterojunction solar cells (DE-588)4113937-9 Hochschulschrift gnd-content Mehrfach-Solarzelle (DE-588)4674119-7 s Perowskit (DE-588)4173836-6 s Solarzelle (DE-588)4181740-0 s DE-604 Fraunhofer-Institut für Solare Energiesysteme (DE-588)2081865-8 isb Fraunhofer IRB-Verlag (DE-588)4786605-6 pbl X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=fb85dfa89f3b4b32a236e706477f3a46&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=032499762&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p vlb 20201127 DE-101 https://d-nb.info/provenance/plan#vlb |
| spellingShingle | Bett, Alexander Jürgen 1988- Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells Perowskit (DE-588)4173836-6 gnd Solarzelle (DE-588)4181740-0 gnd Mehrfach-Solarzelle (DE-588)4674119-7 gnd |
| subject_GND | (DE-588)4173836-6 (DE-588)4181740-0 (DE-588)4674119-7 (DE-588)4113937-9 |
| title | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |
| title_auth | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |
| title_exact_search | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |
| title_exact_search_txtP | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |
| title_full | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells Alexander Jürgen Bett |
| title_fullStr | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells Alexander Jürgen Bett |
| title_full_unstemmed | Perovskite silicon tandem solar cells two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells Alexander Jürgen Bett |
| title_short | Perovskite silicon tandem solar cells |
| title_sort | perovskite silicon tandem solar cells two terminal perovskite silicon tandem solar cells using optimized n i p perovskite solar cells |
| title_sub | two-terminal perovskite silicon tandem solar cells using optimized n-i-p perovskite solar cells |
| topic | Perowskit (DE-588)4173836-6 gnd Solarzelle (DE-588)4181740-0 gnd Mehrfach-Solarzelle (DE-588)4674119-7 gnd |
| topic_facet | Perowskit Solarzelle Mehrfach-Solarzelle Hochschulschrift |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=fb85dfa89f3b4b32a236e706477f3a46&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=032499762&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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