Verfügbarkeit: Towards advanced photon management - singlet fission and beyond

Towards advanced photon management - singlet fission and beyond: = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus

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Bibliographische Detailangaben
1. Verfasser:	Zirzlmeier, Johannes (VerfasserIn)
Format:	Abschlussarbeit Buch
Sprache:	English
Veröffentlicht:	Erlangen ; Nürnberg [2018]
Schlagworte:	Quantenoptik Singulettzustand Photon Hochschulschrift
Online-Zugang:	Inhaltsverzeichnis Inhaltsverzeichnis
Beschreibung:	xiii, 242 Seiten Illustrationen, Diagramme 30 cm

Internformat

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Datensatz im Suchindex

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adam_text	TABLE OF CONTENTS ABSTRACT......................................................................................................................I KURZZUSAMMENFASSUNG........................................................................................... V TABLE OF CONTENTS....................................................................................................XI 1 INTRODUCTION.......................................................................................................1 1.1 NEXT GENERATION PHOTOVOLTAICS..................................................................1 1.2 MOLECULAR ELECTRONICS..................................................................................5 2 THEORETICAL CONSIDERATIONS............................................................................. 9 2.1 FUNDAMENTAL PHOTOPHYSICAL PROCESSES...................................................9 2.1.1 THE J ABLONSKI DIAGRAM......................................................................9 2.1.2 ENERGY TRANSFER.................................................................................11 2.2 SINGLET EXCITON FISSION ............................................................................ 12 2.2.1 BASIC DESCRIPTION...............................................................................13 2.2.2 HISTORICAL OVERVIEW ........................................................................... 14 2.2.3 APPLICATIONS OF SINGLET FISSION - SOLAR ENERGY CONVERSION ............ 15 2.2.4 SINGLET FISSION MECHANISMS.............................................................16 2.2.5 SINGLET FISSION MATERIALS...................................................................17 2.3 TWO-PHOTON ABSORPTION........................................................................... 18 3 BUILDING BLOCKS...............................................................................................21 3.1 ACENES..................................................................................................... 21 3.1.1 PENTACENE AND FUNCTIONALIZED DERIVATIVES.......................................22 3.1.2 PENTACENE DIMERS ............................................................................. 24 3.2 SUBPHTHALOCYANINES................................................................................ 28 3.3 OLIGOYNES.................................................................................................29 4 RESULTS........................................................................................................... 33 4.1 SPIN DYNAMICS AND SINGLET FISSION IN PENTACENE MONOMERS .............. 33 4.1.1 SPIN DYNAMICS IN PENTACENE MONOMERS ......................................... 34 4.1.2 UNSYMMETRICAL PENTACENES - INTERMOLECULAR SINGLET FISSION ....... 39 4.2 SINGLET FISSION IN PENTACENE DIMERS......................................................43 4.2.1 PHENYLENE TETHERED PENTACENE DIMERS.........................................45 4.2.2 CROSS-CONJUGATED PENTACENE DIMERS ............................................. 50 4.2.3 1,3-DIETHYNYLADAMANTYL TETHERED PENTACENE DIMER ...................... 54 4.2.4 (1,4-DIETHYNYL)BICYCLO[2.2.2]OCTANE TETHERED PENTACENE DIMER... 60 4.2.5 TWO-PHOTON ABSORPTION IN PENTACENE DIM ERS..................................65 4.2.6 SINGLET FISSION IN PENTACENE DIMERS FOR PHOTOVOLTAICS ..................... 68 4.2.7 SUBPHTHALOCYANINE-PENTACENE DIMER CONJUGATES ........................ 71 4.3 PUSH-PULL INTERACTIONS IN A SUBPHTHALOCYANINE DIMER..........................75 4.4 SPECTROSCOPIC CHARACTERIZATION OF TWO SERIES OF OLIGOYNES...............78 5 SUMMARY.........................................................................................................83 6 ACKNOWLEDGEMENTS ....................................................................................... 91 7 LIST OF ABBREVIATIONS ...................................................................................... 93 8 TABLE OF FIGURES.............................................................................................99 9 REFERENCES................................................................................................... 101 10 CURRICULUM V ITAE ...................................................................................... 115 11 PUBLICATIONS AND CONFERENCE CONTRIBUTIONS ............................................ 117 12 APPENDIX - SELECTED PUBLICATIONS AND MANUSCRIPTS ............................. 121 12.1 PENTACENE APPENDED TO A TEMPO STABLE FREE RADICAL: THE EFFECT OF MAGNETIC EXCHANGE COUPLING ON PHOTOEXCITED PENTACENE .......... 127 12.2 SINGLET FISSION IN PENTACENE DIMERS..................................................134 12.3 SOLUTION-BASED INTRAMOLECULAR SINGLET FISSION IN CROSS-CONJUGATED PENTACENE DIMERS.................................................. ......................................... 140 12.4 UNIFIED MODEL FOR SINGLET FISSION WITHIN A NON-CONJUGATED COVALENT PENTACENE DIM ER.............................................................................................. 151 12.5 EVIDENCE FOR CHARGE-TRANSFER MEDIATION IN THE PRIMARY EVENTS OF SINGLET FISSION IN A WEAKLY COUPLED PENTACENE DIM ER...............................159 12.6 TWO-PHOTON ABSORPTION IN PENTACENE DIMERS: THE IMPORTANCE OF THE SPACER USING BYCONVERSION AS AN INDIRECT ROUTE TO SINGLET FISSION .... 180 12.7 SINGLET FISSION FOR PHOTOVOLTAICS WITH 130% INJECTION EFFICIENCY .... 184 12.8 PANCHROMATIC RESPONSE - TUNING AND CONTROLLING INTRAMOLECULAR FOERSTER RESONANCE ENERGY TRANSFER AND SINGLET FISSION .............................. 191 12.9 A PUSH-PULL UNSYMMETRICAL SUBPHTHALOCYANINE DIM ER ...................... 211 12.10 REASSESSING THE OPTICAL GAP AND THE FUNDAMENTAL GAP IN OLIGOYNES AND CARBYNE................................................................................
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author	Zirzlmeier, Johannes
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spelling	Zirzlmeier, Johannes Verfasser aut Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus vorgelegt von Johannes Zirzlmeier Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus Erlangen ; Nürnberg [2018] xiii, 242 Seiten Illustrationen, Diagramme 30 cm txt rdacontent n rdamedia nc rdacarrier Dissertation Friedrich-Alexander-Universität Erlangen-Nürnberg 2018 Quantenoptik (DE-588)4047990-0 gnd rswk-swf Singulettzustand (DE-588)4310962-7 gnd rswk-swf Photon (DE-588)4045922-6 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Photon (DE-588)4045922-6 s Singulettzustand (DE-588)4310962-7 s Quantenoptik (DE-588)4047990-0 s DE-604 B:DE-101 application/pdf http://d-nb.info/1164197878/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030593976&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Zirzlmeier, Johannes Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus Quantenoptik (DE-588)4047990-0 gnd Singulettzustand (DE-588)4310962-7 gnd Photon (DE-588)4045922-6 gnd
subject_GND	(DE-588)4047990-0 (DE-588)4310962-7 (DE-588)4045922-6 (DE-588)4113937-9
title	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus
title_alt	Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus
title_auth	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus
title_exact_search	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus
title_full	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus vorgelegt von Johannes Zirzlmeier
title_fullStr	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus vorgelegt von Johannes Zirzlmeier
title_full_unstemmed	Towards advanced photon management - singlet fission and beyond = Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus vorgelegt von Johannes Zirzlmeier
title_short	Towards advanced photon management - singlet fission and beyond
title_sort	towards advanced photon management singlet fission and beyond photonenmanagement fur fortgeschrittene uber die singulettspaltung und daruber hinaus
title_sub	= Photonenmanagement für Fortgeschrittene - über die Singulettspaltung und darüber hinaus
topic	Quantenoptik (DE-588)4047990-0 gnd Singulettzustand (DE-588)4310962-7 gnd Photon (DE-588)4045922-6 gnd
topic_facet	Quantenoptik Singulettzustand Photon Hochschulschrift
url	http://d-nb.info/1164197878/04 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030593976&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
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