Verfügbarkeit: Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes

Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes: = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen

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Bibliographische Detailangaben
1. Verfasser:	Halter, Dominik Pascal (VerfasserIn)
Format:	Abschlussarbeit Buch
Sprache:	English
Veröffentlicht:	Erlangen ; Nürnberg [2017]
Schlagworte:	Komplexe Katalysator Aromaten f-Element Hochschulschrift
Online-Zugang:	Inhaltsverzeichnis Inhaltsverzeichnis
Beschreibung:	Enthält Sonderabdrucke
Beschreibung:	xvii, 318 Seiten Illustrationen, Diagramme 21 cm

Internformat

MARC


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Datensatz im Suchindex

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adam_text	CONTENTS ABBREVIATIONS IX CONTENTS XV 1 INTRODUCTION 1 1.1 SMALL MOLECULE ACTIVATION WITH URANIUM IN THE CONTEXT OF GLOBAL CHALLENGES . . 1 1.2 ELECTRONIC INFLUENCES IN /-ELEMENT C H E M IS TRY ......................................................... 10 1.3 PREVIEW ON THE THESIS.................................................................................................. 16 REFERENCES 17 2 ELECTROCHEMICAL AND SYNTHETIC ACCESS TO AN ARENE SUPPORTED U (LL) COMPLEX 28 2.1 INTRODUCTION TO LOW-VALENT U COMPLEXES ............................................................... 28 2.2 RESULTS AND DISCUSSION .............................................................................................. 30 2.3 CONCLUSION........................................................................................................................ 46 2.4 EXPERIMENTAL S E C TIO N ................................................................................................. 46 2.4.1 METHODS, PROCEDURES AND STARTING M ATERIALS ................................................... 46 2.4.2 SYNTHETIC D E TA ILS ............................................................................................... 47 2.4.3 SPECTROSCOPIC D E TA ILS ..................................................................................... 53 2.4.4 ELECTROCHEMICAL D E TA ILS ................................................................. 64 2.4.5 SQUID MAGNETOMETRY D E TA ILS ......................................................................... 66 2.4.6 CRYSTALLOGRAPHIC D E TA ILS......................................................................................69 2.5 ACKNOWLEDGEMENTS ..................................................................................................... 77 REFERENCES 78 3 URANIUM(IV) HALIDE (F*, CL , BR~, AND I ) MONOARENE COMPLEXES 83 3.1 INTRODUCTION TO U(IV) MONOARENE COMPLEXES............................................................ 83 3.2 RESULTS AND DISCUSSION .............................................................................................. 84 3.3 CONCLUSION.................................................................................................................... 95 3.4 EXPERIMENTAL S E C TIO N ................................................................................................. 96 3.4.1 GENERAL CONSIDERATIONS......................................................................................96 3.4.2 SYNTHETIC PROCEDURES..................................................................................... 97 3.4.3 SPECTROSCOPIC D E TA ILS .......................................................................................100 3.4.4 CRYSTALLOGRAPHIC D E TA ILS....................................................................................107 3.5 ACKNOWLEDGEMENTS .......................................................................................................117 REFERENCES 118 4 URANIUM-MEDIATED ELECTROCATALYTIC H_ PRODUCTION FROM WATER 124 4.1 INTRODUCTION TO WATER REDUCTION AND URANIUM CATALYSIS ........................................124 4.2 RESULTS AND DISCUSSION ................................................................................................ 125 4.3 CONCLUSION...................................................................................................................... 142 4.4 EXPERIMENTAL S E C TIO N ................................................................................................. 4.4.1 GENERAL CONSIDERATIONS ................................................................................. 4.4.2 SYNTHETIC PROCEDURES .................................................................................... 4.4.3 SPECTROSCOPIC D E TA ILS .................................................................................... 4.4.4 ELECTROCHEMICAL D E TA ILS ................................................................................. 4.4.5 GAS CHROMATOGRAPHIC D ETAILS........................................................................ 4.4.6 CRYSTALLOGRAPHIC D ETAILS ................................................................................. 4.5 ACKNOWLEDGEMENTS .................................................................................................... REFERENCES 5 THE ROLE OF URANIUM-ARENE BONDING IN H20 REDUCTION CATALYSIS 5.1 INTRODUCTION TO URANIUM-MONOARENE INTERMEDIATES IN CATALYSIS ............................ 5.2 RESULTS AND DISCUSSION .............................................................................................. 5.3 CONCLUSION.................................................................................................................... 5.4 EXPERIMENTAL S E C TIO N ................................................................................................. 5.4.1 GENERAL CONSIDERATIONS ................................................................................. 5.4.2 SYNTHETIC PROCEDURES .................................................................................... 5.4.3 SPECTROSCOPIC D E TA ILS .................................................................................... 5.4.4 SQUID MAGNETOMETRY D E TA ILS ..................................................................... 5.4.5 ELECTROCHEMICAL D E TA ILS ................................................................................. 5.4.6 CRYSTALLOGRAPHIC D ETAILS................................................................................. 5.4.7 QUANTUM CHEMICAL CALCULATION D ETAILS ........................................................ 5.5 ACKNOWLEDGEMENTS .................................................................................................... REFERENCES 6 ELECTROCATALYTIC H20 REDUCTION WITH /-ELEMENTS: MECHANISTIC INSIGHT AND OVERPOTENTIAL TUNING IN A SERIES OF LANTHANIDE COM PLEXES 6.1 INTRODUCTION TO LANTHANIDE CHEMISTRY AND /-ELEMENT ELECTROCATALYSIS................ 6.2 RESULTS AND DISCUSSION .............................................................................................. 6.3 CONCLUSION.................................................................................................................... 6.4 EXPERIMENTAL S E C TIO N ................................................................................................. 6.4.1 GENERAL CONSIDERATIONS................................................................................. 6.4.2 SYNTHETIC PROCEDURES.................................................................................... 6.4.3 SPECTROSCOPIC D E TA ILS .................................................................................... 6.4.4 ELECTROCHEMICAL D E TA ILS ................................................................................. 6.4.5 GAS CHROMATOGRAPHY D E TA ILS ........................................................................ 6.4.6 SQUID MAGNETOMETRY D E TA ILS ..................................................................... 6.4.7 CRYSTALLOGRAPHIC D ETAILS................................................................................. 6.5 ACKNOWLEDGEMENTS .................................................................................................... REFERENCES 142 142 144 146 150 160 163 169 170 175 175 177 191 192 192 193 196 204 205 208 217 240 241 246 246 247 260 261 261 262 264 271 289 291 296 301 302 7 SUMMARY IN ENGLISH AND IN GERMAN 305 7.1 SUMMARY..........................................................................................................................305 7.2 ZUSAMMENFASSUNG..........................................................................................................311 REFERENCES 317
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author	Halter, Dominik Pascal
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spelling	Halter, Dominik Pascal Verfasser aut Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen vorgelegt von Dominik Pascal Halter Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen Erlangen ; Nürnberg [2017] xvii, 318 Seiten Illustrationen, Diagramme 21 cm txt rdacontent n rdamedia nc rdacarrier Enthält Sonderabdrucke Dissertation Friedrich-Alexander-Universität Erlangen-Nürnberg 2018 Komplexe (DE-588)4133953-8 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf Aromaten (DE-588)4143049-9 gnd rswk-swf f-Element (DE-588)4327313-0 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content f-Element (DE-588)4327313-0 s Aromaten (DE-588)4143049-9 s Komplexe (DE-588)4133953-8 s Katalysator (DE-588)4029919-3 s DE-604 B:DE-101 application/pdf http://d-nb.info/1163046655/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030489668&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Halter, Dominik Pascal Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen Komplexe (DE-588)4133953-8 gnd Katalysator (DE-588)4029919-3 gnd Aromaten (DE-588)4143049-9 gnd f-Element (DE-588)4327313-0 gnd
subject_GND	(DE-588)4133953-8 (DE-588)4029919-3 (DE-588)4143049-9 (DE-588)4327313-0 (DE-588)4113937-9
title	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen
title_alt	Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen
title_auth	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen
title_exact_search	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen
title_full	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen vorgelegt von Dominik Pascal Halter
title_fullStr	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen vorgelegt von Dominik Pascal Halter
title_full_unstemmed	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes = Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen vorgelegt von Dominik Pascal Halter
title_short	Stoichiometric and catalytic small molecule activation with f-element-monoarene complexes
title_sort	stoichiometric and catalytic small molecule activation with f element monoarene complexes stochiometrische und katalytische aktivierung kleiner molekule mit f element monoaren komplexen
title_sub	= Stöchiometrische und katalytische Aktivierung kleiner Moleküle mit f-Element-Monoaren-Komplexen
topic	Komplexe (DE-588)4133953-8 gnd Katalysator (DE-588)4029919-3 gnd Aromaten (DE-588)4143049-9 gnd f-Element (DE-588)4327313-0 gnd
topic_facet	Komplexe Katalysator Aromaten f-Element Hochschulschrift
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