Hydrogen storage: based on hydrogenation and dehydrogenation reactions of small molecules
Gespeichert in:
| Weitere Verfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin
De Gruyter
[2019]
|
| Schlagworte: | |
| Online-Zugang: | http://www.degruyter.com/search?f_0=isbnissn&q_0=9783110534603&searchTitles=true Inhaltsverzeichnis |
| Beschreibung: | XIV, 377 Seiten Illustrationen, Diagramme |
| ISBN: | 9783110534603 |
Internformat
MARC
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Datensatz im Suchindex
| _version_ | 1804178504136261632 |
|---|---|
| adam_text | CONTENTS
PREFACE* V
LIST OF CONTRIBUTING AUTHORS * XIII
THOMAS ZELL AND ROBERT LANGER
1 INTRODUCTION: HYDROGEN STORAGE AS SOLUTION FOR A CHANGING ENERGY
LANDSCAPE * 1
1.1 INTRODUCTION * 1
1.2 CURRENT ENERGY LANDSCAPE - US STATISTICS * 2
1.3 ENERGY STORAGE SYSTEMS * 5
1.3.1 LARGE SCALE CENTRALIZED ENERGY STORAGE * 6
1.3.2 SMALLER SCALE GRIDS AND DISTRIBUTED ENERGY STORAGE SYSTEMS * 7
1.4 ENERGY TRANSPORTATION * 9
1.5 H2 STORAGE - PRODUCTION OF HYDROGEN * 10
1.6 EFFICIENCIES OF HYDROGEN ECONOMY * 12
1.7 HYDROGEN STORAGE - WHY HYDROGEN? * 13
1.8 DEMANDS ON HYDROGEN STORAGE SYSTEMS * 15
1.9 CLASSIFICATION OF HYDROGEN STORAGE SYSTEMS * 16
1.10 PHYSICAL METHODS FOR HYDROGEN STORAGE * 17
1.10.1 COMPRESSING GASEOUS HYDROGEN (CGH2) * 17
1.10.2 LIQUID HYDROGEN (LH2)
-----
20
1.11 MATERIAL BASED METHODS FOR HYDROGEN STORAGE * 20
1.11.1 HYDROGEN STORAGE BY ABSORPTION ON SOLIDS WITH LARGE SURFACE AREA
*
1.12 CHEMICAL METHODS FOR HYDROGEN STORAGE * 22
1.12.1 HYDRIDE MATERIALS * 22
1.12.2 HYDROGENATION AND DEHYDROGENATION REACTIONS OF SMALL
MOLECULES * 24
REFERENCES * 26
THOMAS SCHAUB
2 C02-BASED HYDROGEN STORAGE: C02 HYDROGENATION TO FORMIC ACID,
FORMALDEHYDE AND METHANOL
* 35
2.1 INTRODUCTION
-----
35
2.2 METHANOL * 37
2.2.1 HETEROGENEOUS CATALYZED HYDROGENATION TO METHANOL AND
REFORMING * 37
2.2.2 HOMOGENEOUS CATALYZED HYDROGENATION TO METHANOL AND
REFORMING * 40
2.3 FORMIC ACID
------
42
2.3.1 C02 HYDROGENATION TO FORMIC ACID * 42
2.3.2 HYDROGEN GENERATION FROM FORMIC ACID
-----
44
2.3.3 H2 STORAGE IN INTEGRATED SYSTEMS VIA FORMIC ACID/FORMATES
-----
46
2.4 FORMALDEHYDE
-----
47
2.4.1 C02 HYDROGENATION TO FORMALDEHYDE
-----
48
2.4.2 HYDROGEN GENERATION FROM FORMALDEHYDE * 50
2.5 CONCLUSION
-----
51
REFERENCES * 52
THOMAS ZELL AND ROBERT LANGER
3 C02-BASED HYDROGEN STORAGE - FORMIC ACID DEHYDROGENATION
-----
57
3.1 INTRODUCTION
-----
57
3.2 THE CONCEPT OF FORMIC ACID (FA) AS HYDROGEN STORAGE COMPOUND
-----
58
3.3 SELECTED CATALYTIC PROCESSES FOR THE HYDROGEN GENERATION FROM FA *
62
3.4 MAIN GROUP COMPOUNDS AS CATALYSTS FOR FA DEHYDROGENATION
-----
62
3.5 NOBLE METAL CATALYSTS FOR FA DEHYDROGENATION
-----
65
3.6 BASE-METAL CATALYSTS FOR FA DEHYDROGENATION * 71
3.7 HETEROGENEOUS CATALYSTS FOR FA DEHYDROGENATION * 79
3.8 CATALYTIC SYSTEMS FOR THE REVERSIBLE STORAGE OF H2 IN FA
-----
82
3.9 CONCLUSIONS AND OUTLOOK-------87
REFERENCES
-----
88
MONICA TRINCADO, HANSJOERG GRUETZMACHER AND MARTIN H. G. PRECHTL
4 C02-BASED HYDROGEN STORAGE - HYDROGEN GENERATION FROM
FORMALDEHYDE/WATER
-----
95
4.1 INTRODUCTION
-----
95
4.2 PRODUCTION OF FORMALDEHYDE AND RELATED TECHNOLOGIES
-----
99
4.2.1 FORMALDEHYDE PRODUCTION AND METABOLISM BY BIOLOGICAL SYSTEMS
-----
99
4.2.2 INDUSTRIAL PRODUCTION OF FORMALDEHYDE
----
100
4.2.3 RELATED TECHNOLOGIES FOR FORMALDEHYDE SYNTHESIS
-----
101
4.3 AQUEOUS FORMALDEHYDE AS HYDROGEN AND ENERGY CARRIER
-----
105
4.3.1 BASE PROMOTED DEHYDROGENATION * 105
4.3.2 METAL CATALYZED DEHYDROGENATION * 107
4.4 FUTURE PERSPECTIVES
-----
118
REFERENCES
-----
120
MONICA TRINCADO AND MATTHIAS VOGT
5 C02-BASED HYDROGEN STORAGE - HYDROGEN LIBERATION FROM METHANOL/
WATER MIXTURES AND FROM ANHYDROUS METHANOL * 125
5.1 INTRODUCTION
-----
125
5.2 PRODUCTION OF METHANOL
-----
127
5.2.1 INDUSTRIAL BULK PRODUCTION
------
127
5.2.2 EXPERIMENTAL APPROACHES TOWARD THE FORMATION OF METHANOL * 128
5.3 AQUEOUS METHANOL AS HYDROGEN AND ENERGY CARRIER * 135
5.3.1 BIOLOGICAL SYSTEMS * 136
5.3.2 HYDROGEN PRODUCTION FROM AQUEOUS METHANOL IN ARTIFICIAL SYSTEMS *
138
5.4 OUTLOOK * 165
5.4.1 HYDROGEN AS SUSTAINABLE ENERGY CARRIER AND METHANOL AS HYDROGEN
STORAGE MATERIAL * 165
5.4.2 DEHYDROGENATION OF METHANOL * 166
REFERENCES * 168
ANDRES SUAREZ
6 HYDROGENATION OF CARBONYL COMPOUNDS OF RELEVANCE TO HYDROGEN
STORAGE IN ALCOHOLS * 183
6.1 INTRODUCTION * 183
6.2 HYDROGENATION OF KETONES * 185
6.2.1 GENERAL CONSIDERATIONS * 185
6.2.2 RUTHENIUM AND OSMIUM CATALYSTS * 186
6.2.3 IRIDIUM CATALYSTS * 191
6.2.4 NON-NOBLE METAL CATALYSTS * 193
6.3 HYDROGENATION OF ESTERS * 195
6.3.1 GENERAL CONSIDERATIONS * 195
6.3.2 RUTHENIUM AND OSMIUM CATALYSTS * 197
6.3.3 IRIDIUM CATALYSTS * 206
6.3.4 NON-NOBLE METAL CATALYSTS * 207
6.4 HYDROGENATION OF AMIDES * 211
6.4.1 GENERAL CONSIDERATIONS * 211
6.4.2 RUTHENIUM CATALYSTS
-----
212
6.4.3 NON-NOBLE METAL CATALYSTS * 216
6.5 HYDROGENATION OF CARBOXYLIC ACIDS * 219
6.5.1 GENERAL CONSIDERATIONS * 219
6.5.2 NOBLE METAL CATALYSTS * 220
6.5.3 NON-NOBLE METAL CATALYSTS * 222
6.6 CONCLUSIONS AND OUTLOOK * 223
REFERENCES * 223
JESUS CAMPOS
7 DEHYDROGENATION OF ALCOHOLS AND POLYOLS FROM A HYDROGEN
PRODUCTION PERSPECTIVE
* 231
7.1 INTRODUCTION
-----
231
7.2 GENERAL PERSPECTIVE ON ACCEPTORLESS ALCOHOL DEHYDROGENATION
REACTIONS * 234
7.3 ETHANOL DEHYDROGENATION * 245
7.4 GLYCEROL DEHYDROGENATION * 254
7.5 SUGARS AND SUGAR ALCOHOL DEHYDROGENATION * 258
7.6 CONCLUSION
-----
262
REFERENCES * 263
MORAN FELLER
8 HYDROGENATION OF NITRILES AND IMINES FOR HYDROGEN STORAGE * 271
8.1 INTRODUCTION * 271
8.2 CATALYTIC HYDROGENATION OF NITRILES * 273
8.2.1 NITRILE HYDROGENATION - SELECTIVITY ISSUES AND HOMOGENEOUS
RU-BASED CATALYSTS * 273
8.2.2 HOMOGENEOUS EARTH-ABUNDANT METALS-BASED CATALYSTS * 278
8.2.3 HETEROGENEOUS METALS-BASED CATALYSTS * 281
8.3 IMINE HYDROGENATION * 284
8.4 CONCLUSIONS
-----
285
REFERENCES * 286
DANIEL L. J. BROERE
9 TRANSITION METAL-CATALYZED DEHYDROGENATION OF AMINES * 295
9.1 INTRODUCTION * 295
9.2 CATALYTIC DEHYDROGENATION OF AMINES * 297
9.2.1 PRIMARY AMINES TO IMINES AND SECONDARY AMINES * 297
9.2.2 SELECTIVE CATALYTIC DEHYDROGENATION OF PRIMARY AMINES TO NITRILES
* 303
9.2.3 CATALYTIC DEHYDROGENATION OF N-HETEROCYCLES * 306
9.3 CONCLUSIONS * 318
REFERENCES * 319
ZHUOFENG KE, YINWU LI, CHENG HOU AND YAN LIU
10 HOMOGENEOUSLY CATALYZED HYDROGENATION AND DEHYDROGENATION
REACTIONS - FROM A MECHANISTIC POINT OF VIEW * 327
10.1 INTRODUCTION * 328
10.2 NON-COOPERATION MECHANISMS * 330
10.2.1 OXIDATIVE ADDITION/REDUCTIVE ELIMINATION MECHANISM * 330
10.2.2 O-BOND METATHESIS MECHANISM * 332
10.3 LB-TM COOPERATION MECHANISMS * 333
10.3.1 N-TYPE LB-TM COOPERATION MECHANISM * 334
10.3.2 N-TYPE LB-TM COOPERATION MECHANISM: (DE)AROMATIZATION/
TAUTOMERIZATION * 338
10.3.3 O-TYPE LB-TM COOPERATION MECHANISM * 339
10.3.4 LIGAND-INNOCENT NON-LB-TM COOPERATION MECHANISM
-----
340
10.4 LA-TM COOPERATION MECHANISM
-----
340
10.4.1 P-TYPE LA-TM COOPERATION MECHANISMS
----
342
10.4.2 O-TYPE LA-TM COOPERATION MECHANISM * 344
10.4.3 N*-TYPE LA-TM COOPERATION MECHANISM * 345
10.4.4 LIGAND-INNOCENT NON-MLC MECHANISM IN LA-TM SYSTEMS
-----
345
10.4.5 HYDROGENATION/DEHYDROGENATION MECHANISM IN LA-TM SYSTEMS * 346
10.5 LA-LB COOPERATION (FLP) MECHANISM
-----
348
10.5.1 H2 ACTIVATION MECHANISMS IN LA-LB COOPERATION SYSTEMS * 348
10.5.2 HYDROGENATION/DEHYDROGENATION REACTION MECHANISMS IN LA-LB
COOPERATION SYSTEMS * 350
10.6 AMBIPHILIC MECHANISM * 351
10.6.1 H2 ACTIVATION MECHANISM IN AMBIPHILIC SYSTEMS * 353
10.6.2 HYDROGENATION MECHANISM VIA AMBIPHILIC COOPERATION * 354
10.7 TM-TM COOPERATION MECHANISM
-----
354
10.7.1 HOMOLYTIC MECHANISM VIA TM-TM COOPERATION
-----
355
10.7.2 HETEROLYTIC MECHANISM VIA TM-TM COOPERATION * 356
10.7.3 OXIDATIVE ADDITION MECHANISM
-----
356
10.7.4 HYDROGENATION/DEHYDROGENATION MECHANISM IN TM-TM SYSTEMS
-----
357
10.8 KEY FACTORS GOVERNING THE MECHANISTIC PREFERENCES * 360
10.8.1 THE ROLE OF THE METAL AND THE LIGAND IN MLC * 360
10.8.2 PROTON SHUTTLE
-----
362
10.9 CONCLUDING REMARKS * 363
REFERENCES
-----
364
INDEX * 369
|
| any_adam_object | 1 |
| author2 | Zell, Thomas Langer, Robert |
| author2_role | edt edt |
| author2_variant | t z tz r l rl |
| author_facet | Zell, Thomas Langer, Robert |
| building | Verbundindex |
| bvnumber | BV044929406 |
| classification_rvk | ZP 4150 VH 8007 |
| ctrlnum | (OCoLC)1083287779 (DE-599)DNB1139380214 |
| discipline | Chemie / Pharmazie Energietechnik |
| format | Book |
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| genre_facet | Aufsatzsammlung |
| id | DE-604.BV044929406 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T08:05:01Z |
| institution | BVB |
| institution_GND | (DE-588)10095502-2 |
| isbn | 9783110534603 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-030322498 |
| oclc_num | 1083287779 |
| open_access_boolean | |
| owner | DE-29T DE-703 DE-1050 DE-83 DE-898 DE-BY-UBR |
| owner_facet | DE-29T DE-703 DE-1050 DE-83 DE-898 DE-BY-UBR |
| physical | XIV, 377 Seiten Illustrationen, Diagramme |
| publishDate | 2019 |
| publishDateSearch | 2019 |
| publishDateSort | 2019 |
| publisher | De Gruyter |
| record_format | marc |
| spelling | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules edited by Thomas Zell, Robert Langer Berlin De Gruyter [2019] XIV, 377 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Wasserstoffspeicherung (DE-588)4189283-5 gnd rswk-swf Wasserstoff (DE-588)4064784-5 gnd rswk-swf Energiespeicher (DE-588)4152230-8 gnd rswk-swf Wasserstoff-Speicher (DE-588)4480116-6 gnd rswk-swf Wasserstoffenergietechnik (DE-588)4121905-3 gnd rswk-swf Energiespeicher Wasserstoff Wasserstoff-Speicher Dehydrierung (DE-588)4143413-4 Aufsatzsammlung gnd-content Wasserstoffspeicherung (DE-588)4189283-5 s DE-604 Energiespeicher (DE-588)4152230-8 s Wasserstoff (DE-588)4064784-5 s Wasserstoffenergietechnik (DE-588)4121905-3 s Wasserstoff-Speicher (DE-588)4480116-6 s Zell, Thomas edt Langer, Robert edt Walter de Gruyter GmbH & Co. KG (DE-588)10095502-2 pbl Erscheint auch als 9783110536430 Erscheint auch als Online-Ausgabe, pdf 978-3-11-053642-3 Erscheint auch als Online-Ausgabe, epub 978-3-11-053465-8 X:MVB http://www.degruyter.com/search?f_0=isbnissn&q_0=9783110534603&searchTitles=true DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030322498&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules Wasserstoffspeicherung (DE-588)4189283-5 gnd Wasserstoff (DE-588)4064784-5 gnd Energiespeicher (DE-588)4152230-8 gnd Wasserstoff-Speicher (DE-588)4480116-6 gnd Wasserstoffenergietechnik (DE-588)4121905-3 gnd |
| subject_GND | (DE-588)4189283-5 (DE-588)4064784-5 (DE-588)4152230-8 (DE-588)4480116-6 (DE-588)4121905-3 (DE-588)4143413-4 |
| title | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules |
| title_auth | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules |
| title_exact_search | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules |
| title_full | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules edited by Thomas Zell, Robert Langer |
| title_fullStr | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules edited by Thomas Zell, Robert Langer |
| title_full_unstemmed | Hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules edited by Thomas Zell, Robert Langer |
| title_short | Hydrogen storage |
| title_sort | hydrogen storage based on hydrogenation and dehydrogenation reactions of small molecules |
| title_sub | based on hydrogenation and dehydrogenation reactions of small molecules |
| topic | Wasserstoffspeicherung (DE-588)4189283-5 gnd Wasserstoff (DE-588)4064784-5 gnd Energiespeicher (DE-588)4152230-8 gnd Wasserstoff-Speicher (DE-588)4480116-6 gnd Wasserstoffenergietechnik (DE-588)4121905-3 gnd |
| topic_facet | Wasserstoffspeicherung Wasserstoff Energiespeicher Wasserstoff-Speicher Wasserstoffenergietechnik Aufsatzsammlung |
| url | http://www.degruyter.com/search?f_0=isbnissn&q_0=9783110534603&searchTitles=true http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030322498&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT zellthomas hydrogenstoragebasedonhydrogenationanddehydrogenationreactionsofsmallmolecules AT langerrobert hydrogenstoragebasedonhydrogenationanddehydrogenationreactionsofsmallmolecules AT walterdegruytergmbhcokg hydrogenstoragebasedonhydrogenationanddehydrogenationreactionsofsmallmolecules |