Frontiers and advances in molecular spectroscopy:
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| Format: | Buch |
| Sprache: | English |
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Amsterdam ; Oxford ; Cambridge, MA
Elsevier
[2018]
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| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | xxi, 763 Seiten Illustrationen, Diagramme |
| ISBN: | 9780128112205 |
Internformat
MARC
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| 245 | 1 | 0 | |a Frontiers and advances in molecular spectroscopy |c edited by Jaan Laane |
| 264 | 1 | |a Amsterdam ; Oxford ; Cambridge, MA |b Elsevier |c [2018] | |
| 300 | |a xxi, 763 Seiten |b Illustrationen, Diagramme | ||
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Datensatz im Suchindex
| _version_ | 1804178429327704064 |
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| adam_text | Contents
Contributors xvii
Preface xix
1 Stark-Induced Adiabatic Passage Processes to
Selectively Prepare Vibrationally Excited Single and
Superposition of Quantum States i
Nandini Mukherjee, William E Perreault and Richard N Zare
1 Introduction 2
1 1 How Can a Large Ensemble of Molecular Targets be
Prepared in a Selected Highly Vibrationally Excited Quantum
State With Rotational (J, M) Quantum Number Precision? 2
2 Theory of Stark-Induced Adiabatic Raman Passage 5
2 1 Schrödinger Equation for Stimulated Raman Pumping 5
2 2 Density Matrix Equation 8
2 3 Saturation of Raman Pumping in a High-Pressure Gas Cell 9
2 4 Bloch Vector Model for Stark-Induced Adiabatic Passage 9
2 5 Rabi Oscillations 11
2 6 Coherent Population Return is a Problem for Stark-Induced
Population Transfer 12
2 7 How Do We Accomplish Stark-Induced Adiabatic Passage
Using Pulsed Excitation? 13
3 Theoretical Simulation of SARP for H2 v=0-»v=1 Transitions 14
3 1 SARP is a Threshold Phenomenon 15
4 Experimental Demonstration of SARP Preparing Single and
Superpositions of Quantum States 16
4 1 Preparation of a Bi-Axial Superposition State Within a Single
Rovibrational H2 (v= 1,7=2) Eigenstate 18
4 2 Demonstration That SARP is a Robust Technique for
Preparing a Desired Rovibrational M-Quantum State 21
5 SARP Excitation of a High Vibrational (v=4) Level 23
6 Vibrational Ladder Climbing Using Multicolor SARP 26
6 1 How Do We Prepare A Diatomic Molecule in An
Arbitrary High Vibrational Level? 28
6 2 Theory of Four-Photon Three-Color SARP 29
6 3 Vibrational Ladder Climbing of H2 Using Three-Color SARP 31
v
vi Contents
6 4 Preparation of H2 (v=6, J—0) Using Three-Color SARP 32
6 5 Preparation of a Pair of Loosely Bound H Atoms Using
Four-Color Ladder SARP 34
7 Other Related Adiabatic Passage Processes 36
7 1 Stimulated Raman Adiabatic Passage 36
7 2 High Vibrational Excitation Using STIRAP 38
7 3 Multicolor STIRAP to Prepare High Vibrational States 38
7 4 Stark-Chirped Rapid Adiabatic Passage 40
8 Concluding Remarks 42
Acknowledgments 43
References 43
2 Advances in Two-Dimensional Correlation
Spectroscopy (2DCOS) 47
Isao Noda
1 Introduction 47
2 Generalized 2D Correlation Analysis 48
2 1 Perturbation-Induced Dynamic Spectra 48
2 2 2D Correlation Analysis of Dynamic Spectra 50
2 3 Matrix Notation for 2DCOS 51
2 4 Unevenly Sampled Dynamic Spectra 52
3 Interpreting 2D Correlation Spectra 53
3 1 Simulated Model Spectra 53
3 2 Properties of Synchronous Spectrum 54
3 3 Properties of Asynchronous Spectrum 55
4 Illustrative Example of 2DCOS Application 56
5 Advanced Tools in 2DCOS 61
5 1 Heterocorrelation Analyses 62
5 2 Moving Window 2D Correlation 64
5 3 Two-Dimensional Codistribution (2DCDS) Analysis 66
5 4 Pareto Scaling 69
5 5 Null-Space Projection 71
6 Conclusions 73
References 74
3 Applications of 2D-IR Spectroscopy to Probe the
Structural Dynamics of DNA 77
Gordon Hithell, Lennart A I Ramakers, Glenn A Burley
and Neil T Hunt
1 Introduction 77
2 Methodology 79
2 1 Obtaining 2D-IR Spectra 79
2 2 Spectral Assignment of DNA 2D-IR Spectra 82
3 Advances in Our Understanding of DNA From 2D-IR 86
3 1 Spectroscopy, Coupling, and Vibrational Modes 86
3 2 Dynamics and Solvation 89
Contents vii
3 3 Vibrational Relaxation 92
3 4 Intermolecular Interactions—Duplex Melting 94
3 5 Intermolecular Interactions—Ligand Binding 95
4 Outlook 96
References 96
4 Vibrational Potential Energy Surfaces in Ground
and Excited Electronic States 101
Jaan Laane, Esther J Ocola and Hye J Chun
1 Introduction 101
2 Theory 103
2 1 The Quartic Potential Energy 103
2 2 Calculation of Energy Levels 104
2 3 Kinetic Energy Functions 105
3 Experimental Methods 107
4 Molecules With Intramolecular Jt-Type Hydrogen Bonding 109
4 1 Introduction 109
4 2 3-Cyclopenten-1 -ol 109
4 3 2-lndanol 110
4 4 2-Cyclopenten-1-ol and 2-Cyclohexen-1-ol 111
4 5 3-Cyclopentene-1-Amine and 2-Aminoindan 113
5 1,3-Butadiene 113
6 Pyridine and Fluoropyridines in Electronic Excited States 116
6 1 Pyridine-do and-dö 116
6 2 Fluoropyridines 116
7 Spiro and Bicyclic Molecules 117
7 1 4-Silaspiro(3,3)heptane (SSH) 117
7 2 2-Cyclopenten-1-one Ethylene Ketal (CEK) 118
7 3 2,4,7-Trioxa[3 3 0]octane (247TOO) 122
8 trans- and c/s-Stilbenes 123
9 Bicyclic Aromatics 126
9 1 Indan and Related Molecules 126
9 2 Other Bicyclic Aromatics 131
10 Cyclic Ketones 134
11 Conclusion 136
Acknowledgments 137
References 137
5 Structures and Dipole Moments of Molecules
in Their Electronically Excited States 143
Michael Schmitt and Leo Meerts
1 Introduction 144
2 Permanent Dipole Moments and Transition Dipoles 147
3 The Stark Effect 149
3 1 First Order Stark Effect 150
3 2 Second Order Stark Effect 150
viii Contents
4 Hamiltonian for the Evaluation of Rovibronic Stark Spectra 151
4 1 The Rigid Rotor Hamiltonian for Asymmetric Tops 151
4 2 The Centrifugal Distortion Hamiltonian for Asymmetric Tops 151
4 3 The Stark Hamiltonian for Asymmetric Tops 152
5 Selection Rules 153
6 Theory of Evolutionary Algorithms for the Assignment and Fit of
Spectra 155
6 1 The Genetic Algorithm 157
6 2 The Evolutionary Strategy 157
6 3 The Fitness Function for the Analysis of Spectra 159
7 Experimental Set-Up 160
7 1 Rotationally Resolved Electronic Stark Spectroscopy 160
7 2 Excited State Dipole Moments From Experiments
in the Time Domain 164
8 Excited State Dipole Moments From Rotationally Resolved
Stark Spectroscopy 165
8 1 The Additivity of Excited State Dipole Moments 170
8 2 The Direction of Excited State Dipole Moments 177
8 3 State Labeling Using Excited State Dipole Moments 181
8 4 Comparison of Excited State Dipole Moments From Gas
Phase and Condensed Phase Experiments 183
Acknowledgments 184
References 186
6 Two-Color Pulsed-Field lonization-Photoelectron
Spectroscopy: A Quest to Benchmark State-of-the-Art
ab initio Quantum Electronic Structure Calculations
of Spectroscopic and Energetic Properties for
Transition Metal-Containing Species 195
Zhihong Luo, Yih-Chung Chang, Chow-Sing Lam,
Kai-Chung Lau and Cheuk-Yiu Ng
1 Introduction 196
2 Experimental Considerations 199
2 1 Two-Color VIS-UV Laser PIE and PFI-PE Measurements 199
3 Theoretical Approaches 201
3 1 Coupled-Cluster Theory 201
3 2 CBS Extrapolation Approximation 202
3 3 Corrections to the CCSDTQ/CBS Method 203
4 Experimental Results 204
4 1 Diatomic MX/MX+ Systems 204
4 2 Triatomic Systems 232
5 Comparison of Experimental and Theoretical Results 235
5 1 IE Values for M-Containing Species 236
5 2 Bond Lengths and Vibrational Frequencies of M-Containing
Cationic Species 239
5 3 D0(M+-X)-D0(M-X) Values for MX/MX Systems 241
5 4 Comparison of Experimental and Theoretical D0 Values 243
Contents ix
6 Summary and Future Perspective 244
Acknowledgments 245
References 246
Further Reading 249
Advances in Far-Ultraviolet Spectroscopy in the
Solid and Liquid States 251
Yusuke Morisawa, Ichiro Tanabe and Yukihiro Ozaki
1 Introduction 251
2 Principle and Brief History of FUV Spectroscopy 253
3 Advantages of FUV Spectroscopy for Studies
of Condensed Matter 254
4 Instrumentation of FUV Spectroscopy for Liquid and
Solid Samples 255
5 Applications of FUV Spectroscopy 256
6 FUV Spectroscopy of Molecules in the Gas Phase 256
7 FUV Spectroscopy of Molecules in the Rare Gas Matrices 258
8 FUV Spectroscopy of Organic Liquids and Solids Another
Possibility ATR-FUV Spectra of Organic 258
8 1 ATR-FUV Spectra of Alkanes in Liquid and Solid Phase 259
8 2 Changes of Electronic States of n-Tetradecane During
Liquid-Solid Phase Transition 259
8 3 ATR-FUV Spectra of Amides 264
8 4 ATR-FUV Spectra of Nylons 264
9 ATR-FUV Spectroscopy of Water and Aqueous Solutions 267
10 FUV Spectroscopy of Inorganic Semiconductor Powders 271
10 1 Spectral Measurements of Semiconductor Powders by
ATR-FUV Spectrometer System 271
10 2 Electronic Structures and Photocatalytic Activities
of Ti02 Modified With Metal Nanoparticles 273
11 Future Prospects 280
References 281
Further Reading 285
Development of Sub-10 fs Visible-NIR, UV and
DUV Pulses and Their Applications to Ultrafast
Spectroscopy 287
Takayoshi Kobayashi, Atsushi Yabushita and Yuichiro Kida
1 Basics of Nonlinear Optical Processes 287
1 1 Nonlinear Optical Processes and Nonlinear Susceptibilities 287
1 2 OPA 290
2 Visible Ultrashort Pulse Generation by Noncollinear Optical
Parametric Amplifier 292
2 1 Ultrafast Time-Resolved Spectroscopy by Visible Ultrashort
Laser Pulse 295
2 2 UV and DUV (Pulse and Spectroscopy) 296
References 304
x Contents
9 Biomedical Applications of Surface-Enhanced Raman
Scattering Spectroscopy 307
Rui Wang; Hyangah Chon, Sangyeop Lee, Juhui Ko, Joonki Hwang,
Namhyun Choi, Ziyi Cheng, Xiaokun Wang and Jaebum Choo
1 Introduction 307
2 SERS-Based Assay Using Two-Dimensional Cold-Patterned
Substrates 308
3 SERS-Based Assay Using Magnetic Bead-Based Assay
Platform 310
4 Application of Microfluidics for SERS-Based Bioassays 313
5 Application of SERS-Based Lateral Flow Assay Strips for
Biomedical Diagnostics 318
6 Summary 323
Acknowledgments 323
References 323
10 SERS Biomedical Applications: Diagnostics, Forensics,
and Metabolomics 327
Wijamunidurage R Premasiri, Ying Chen, Jennifer Fore,
Amy Brodeur and Lawrence D Ziegler
1 introduction 328
1 1 Biomedical Applications and Vibrational Spectroscopy 328
1 2 Surface Enhanced Raman Spectroscopy (SERS)—Brief
Introduction 329
1 3 Advantages of SERS for Biomedical Analyses 330
2 Brief Summary of SERS Experimental Considerations 330
3 Infectious Disease Diagnostics: General Introduction 331
4 Urinary Tract Infection Diagnostics 332
4 1 General Introduction 332
4 2 SERS Spectra of UTI Clinical Isolates 333
4 3 SERS UTI Diagnostic Capabilities: Identification and
Antibiotic Susceptibilities 333
5 STD Diagnostics 336
5 1 General Introduction: Chlamydia and Gonorrhea 336
5 2 SERS Spectra of STD Causative Bacteria 338
6 Bacteremia Diagnostics 340
6 1 General Introduction 340
6 2 SERS Detection and Identification of Bacteremia
Developments 340
7 Origins of Bacterial SERS Signals 341
7 1 Chemical/Molecular Origins of the SERS Spectra of
Bacteria 341
7 2 Purines Dominate the Bacterial SERS Spectra 343
7 3 Biochemical Origins of the SERS Spectra of Bacteria 347
7 4 Chemical and Biochemical Origins of SERS Spectra of STD
Pathogens 351
Contents xi
8 Forensics 354
8 1 Introduction 354
8 2 SERS Detection and Identification of Human Body Fluids 355
9 Conclusion 359
Acknowledgments 360
References 360
11 Quantitative Spectrometry of Complex Molecular
Systems by Hypothetical Addition Multivariate
Analysis With Numerical Differentiation (HAMAND) 369
Masahiro Ando, Igor K Lednev and Hiro-o Hamaguchi
1 Introduction 369
2 The Principle of HAMAND 370
3 Mathematical Procedure 371
4 Applications of HAMAND 372
4 1 Solution Sample 372
4 2 Solid Sample 374
4 3 Forensic Sample 375
5 Discussion 377
Acknowledgments 378
References 378
12 Progress in FAST CARS Toward Quantum Biophotonics 379
Dmitri V Voronine, Alexei V Sokolov and Marian O Scully
1 Introduction 379
2 Basic Principles of FAST CARS 380
3 Applications to Biosensing 381
4 Versatile FAST CARS 382
5 Heterodyne Single-Beam FAST CARS Microscopy 385
6 FAST CARS With Surface Enhancement 389
7 Conclusion 390
Acknowledgments 391
References 391
13 Coherent Raman Generation in Solid-State Materials
Using Spatial and Temporal Laser Field Shaping 395
Alexandra A Zhdanova, Miaochan Zhi and Alexei V Sokolov
1 Introduction 395
2 Basic Principles of Molecular Modulation 397
3 Broadband Coherent Light Generation in the Raman-Active
Crystal PbW04 398
3 1 Introduction 398
3 2 Coherent Raman Generation via Two-Color Laser Fields 401
3 3 Coherent Raman Generation via Three-Color Laser Fields 403
3 4 Coherent Raman Generation via Linearly Chirped Pulses 405
xii Contents
4 Using Molecular Modulation to Obtain an Ultrafast Pulse 407
4 1 Introduction 407
4 2 Manipulating Raman Sideband Phase via Commercial
Pulse Shaper 408
4 3 Manipulating Raman Sideband Phase via Spherical
Mirrors 409
5 The Raman Process With Optical Vortices 410
5 1 Introduction 410
5 2 Topological Charge Transfer 412
5 3 Experiments With Single-Charged Pump/Stokes 413
5 4 Experiments With Multiply Charged Pump/Stokes 413
6 Summary 416
References 417
Further Reading 420
14 Vibrational Optical Activity: From Small
Chiral Molecules to Protein Pharmaceuticals
and Beyond 421
Laurence A Nafie
1 Introduction 421
1 1 Overview of VO A History 422
1 2 Overview of the Current State of the Art 425
2 Vibrational Circular Dichroism 427
2 1 Theory 427
2 2 Instrumentation and Measurement 429
2 3 Calculations 432
2 4 Established Applications 433
2 5 Frontiers of VCD 436
3 Raman Optical Activity 440
3 1 Theory 440
3 2 Instrumentation and Measurement 446
3 3 Calculations 448
3 4 Established Applications 449
3 5 Frontiers of ROA 451
4 Complementarity of VCD and ROA 454
5 Conclusions and Summary 454
5 1 VCD Frontiers 455
5 2 ROA Frontiers 455
5 3 Chiroptical Spectroscopy Frontiers 456
References 457
15 High-Resolution Laboratory Terahertz Spectroscopy
ana Applications to Astrophysics 471
Stephan Schlemmer
1 Introduction 471
2 Molecules in Astrophysical Observations 474
Contents xiii
2 1 Complex Organic Molecules in Space 474
2 2 Molecular Ions in Space 482
3 Terahertz Absorption Spectroscopy 485
4 Action Spectroscopy of Ions in Cold Traps 489
4 1 UR Infrared Spectroscopy 494
4 2 IR/THz Double Resonance Spectroscopy 496
4 3 Frequency Comb Based Spectra 497
4 4 UR Intensities 503
5 Future Trends in THz Spectroscopy 506
5 1 UR Schemes 506
5 2 Different Experimental Approaches 510
Acknowledgments 516
References 516
16 Studying Interaction, Ion-Pair Formation, and Mixing
Behavior of Protic Ionic Liquids by Means of
Far-Infrared Spectroscopy 527
Ralf Ludwig
1 Introduction 527
2 FIR Spectroscopy 529
3 Protic Ionic Liquids 530
4 The Subtle Balance of Coulomb Interaction, Hydrogen
Bonding and Dispersion Forces 531
4 1 Detecting and Quantifying H-Bonds 531
4 2 Pure Interaction by Removing Reduced Mass Effects 535
4 3 The Influence of Dispersion Forces on the FIR
Spectra 538
4 4 Dispersion Forces Compete With Hydrogen Bonds 542
5 Ion Speciation 546
5 1 Ion Speciation in Water 546
5 2 Ion Pair Formation in Dimethylsulfoxide (DMSO) 549
5 3 Reformation of Contact Ion Pairs With Increasing
Temperature 553
6 Mixing Behavior 558
6 1 Nonideal Mixing Behavior Due to Hydrogen Bonds 558
6 2 Cluster Formation Controls Macroscopic Properties 560
7 Conclusions 563
References 563
17 Advancements In Microwave Spectroscopy 569
Walther Caminati and Jens-Uwe Grabow
1 Introduction 569
2 Technical Advancements 570
2 1 Chiral Discrimination 570
2 2 Diffusion of Chirp- and Tone-Excitation Fourier Transform
Spectrometers 571
xiv Contents
3 Molecular Systems 572
3 1 Chemical Information From MW 572
3 2 Internal Dynamics 585
4 Astrochemistry 591
4 1 Laboratory Investigations 592
4 2 Detection in the Interstellar Space 592
Acknowledgments 593
References 593
18 Nitric Oxide Laser-induced Fluorescence
Imaging Methods and Their Application to Study
High-Speed Flows 599
Rodrigo Sänchez-Gonzälez and Simon W North
1 Introduction 599
2 Nitric Oxide Laser Induced Fluorescence 600
2 1 Temperature Measurements Using NO Fluorescence:
Two-Line NO PLIF 603
2 2 Velocity Measurements Using Molecular Tagging
Techniques: NO Fluorescence MTV 605
3 Experimental Measurements 608
3 1 N02 Photodissociation MTV 608
3 2 Temperature Measurements Using N02 Photodissociation 612
3 3 Simultaneous Measurement of Velocity and Temperature 619
3 4 The Invisible Ink VENOM Variant 623
4 Conclusions 627
References 628
19 Photogeneration of Rare Molecules in Cryogenic
Matrices: Spectroscopists Adventures in Wonderland 631
Rui Fausto
1 Introduction 631
2 Act I —Narrowband IR-lnduced Transformations 635
2 1 Scene 1 1: The Case of 2-Fluorobenzoic Acid 635
2 2 Scene 1 2: Glycolic Acid—Probing Consecutive
Conformational Isomerizations 640
2 3 Scene 1 3: The Genesis of Rare Dimers of Acetic Acid 643
2 4 Scene 1 4: Conformational Switching by Excitation of a
Remote Bond 648
3 Act II —Narrowband UV-Induced Transformations 650
3 1 Scene 11 1: p-Anisaldehyde—Dependence of the
Photostationary State Position on the Wavelength 650
3 2 Scene 11 2: Bond-Shift Isomers of 1,3-Dipolar Species
(Nitrile Imines) 651
3 3 Scene 11 3: Photoproduction of a Rare Spiro-2H-Azirine 654
3 4 Scene 11 4: First Observation of a Nitrene Tunneling Reaction 658
Contents xv
4 Conclusion 662
Acknowledgements 662
References 663
20 Matrix isolation Spectroscopic Studies: Thermal
and Soft Photochemical Bimolecular Reactions 667
Bruce S Ault
1 Introduction and Scope 668
2 Introduction to Matrix Isolation and Experimental Details 669
2 1 Cryogenics and Vacuum Hardware 669
2 2 Preparation of Reactive Intermediates 670
2 3 Applications of Computational Chemistry 673
3 Thermal Reactions and Complex Formation 674
3 1 Hydrogen-Bonded Complexes 674
3 2 Intermediate Lewis Acid-Base Complexes 675
3 3 Reactions of Diborane 676
3 4 Reactions of Chromyl Chloride and Metal Oxo Compounds 677
4 Ozonolysis of Alkenes 679
4 1 c/s-2-Butene 679
4 2 Cyclopentene and Cyclopentadiene 685
4 3 Ethene and Propene 686
4 4 Bicylic Alkenes 687
4 5 1,3- and 1,4-Cyclohexadiene: A Non-Criegee Mechanism 688
5 Reaction of Ozone With Volatile Organometallic
Compounds 691
5 1 Introduction and Dimethylzinc 691
5 2 Dimethylcadmium 693
5 3 Trimethyl Metals 695
5 4 Metallocenes 697
6 Soft Photochemical Reactions 697
6 1 Ozone Reaction With Ferrocene 697
6 2 Electronic Spectroscopy 700
7 Conclusions 704
Acknowledgments 704
References 705
Further Reading 712
21 Theory of Enantiomer-Specific Microwave
Spectroscopy 713
Kevin K Lehmann
1 Introduction 713
2 Stark Induced Chiral Emission 716
2 1 Signals in the Perturbative Limit 716
2 2 High Stark Field Mixing 727
2 3 Effect of Variation in Excitation Strength 730
xvi Contents
3 Three Wave Mixing
3 1 Polarization Calculation
3 2 The Effects of Lack of Phase Matching
4 Some Extensions
5 Conclusions
Acknowledgments
References
731
732
736
738
741
741
741
Index
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| illustrated | Illustrated |
| indexdate | 2024-07-10T08:03:50Z |
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| isbn | 9780128112205 |
| language | English |
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| publisher | Elsevier |
| record_format | marc |
| spelling | Frontiers and advances in molecular spectroscopy edited by Jaan Laane Amsterdam ; Oxford ; Cambridge, MA Elsevier [2018] xxi, 763 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Molekülspektroskopie (DE-588)4128850-6 gnd rswk-swf Molekülspektroskopie (DE-588)4128850-6 s DE-604 Laane, Jaan 1942- (DE-588)12045467X edt HEBIS Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030280705&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Frontiers and advances in molecular spectroscopy Molekülspektroskopie (DE-588)4128850-6 gnd |
| subject_GND | (DE-588)4128850-6 |
| title | Frontiers and advances in molecular spectroscopy |
| title_auth | Frontiers and advances in molecular spectroscopy |
| title_exact_search | Frontiers and advances in molecular spectroscopy |
| title_full | Frontiers and advances in molecular spectroscopy edited by Jaan Laane |
| title_fullStr | Frontiers and advances in molecular spectroscopy edited by Jaan Laane |
| title_full_unstemmed | Frontiers and advances in molecular spectroscopy edited by Jaan Laane |
| title_short | Frontiers and advances in molecular spectroscopy |
| title_sort | frontiers and advances in molecular spectroscopy |
| topic | Molekülspektroskopie (DE-588)4128850-6 gnd |
| topic_facet | Molekülspektroskopie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030280705&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT laanejaan frontiersandadvancesinmolecularspectroscopy |