On the Role of Spin States in Organic Semiconductor Devices: = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen
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| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
Würzburg
2016
|
| Subjects: | |
| Online Access: | Volltext http://d-nb.info/1122436076/34 Inhaltsverzeichnis |
| Physical Description: | V, 158 Seiten Illustrationen, Diagramme |
| Format: | Langzeitarchivierung gewährleistet, LZA |
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MARC
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| 245 | 1 | 0 | |a On the Role of Spin States in Organic Semiconductor Devices |b = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |c vorgelegt von Stefan Kilian Väth aus Würzburg ; Gutachter: Prof. Dr. Vladimir Dyakonov, Prof. Dr. Jean Geurts |
| 246 | 1 | 1 | |a Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| 264 | 1 | |a Würzburg |c 2016 | |
| 300 | |a V, 158 Seiten |b Illustrationen, Diagramme | ||
| 336 | |b txt |2 rdacontent | ||
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| 338 | |b nc |2 rdacarrier | ||
| 502 | |b Dissertation |c Julius-Maximilians-Universität Würzburg |d 2016 | ||
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| 546 | |a Zusammenfassung in deutscher und englischer Sprache | ||
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Record in the Search Index
| _version_ | 1804177012159414272 |
|---|---|
| adam_text | ON THE ROLE OF SPIN STATES IN
ORGANIC SEMICONDUCTOR DEVICES
DISSERTATION ZUR ERLANGUNG DES
NATURWISSENSCHAFTLICHEN DOKTORGRADES
DER JULIUS-MAXIMILIANS-UNIVERSITAET WUERZBURG
VORGELEGT VON
STEFAN KILIAN VAETH
AUS WUERZBURG
WUERZBURG 2016
C ONTENTS
1. INTRODUCTION 1
2. ORGANIC PHOTOVOLTAICS 5
2.1. ORGANIC SEMICONDUCTORS
......................................................................................
5
2.2. THE EMERGENCE OF ORGANIC
PHOTOVOLTAICS......................................................... 7
2.3. FUNDAMENTAL PROCESSES IN ORGANIC BULK HETEROJUNCTION SOLAR CELLS
.... 9
2.4. J-V-CHARACTERISTICS AND SOLAR CELL PARAMETERS
...................................................
14
2.5. MORPHOLOGY OF BULK HETEROJUNCTION SOLAR C E L L S
................................................
16
3. ELECTRON PARAMAGNETIC RESONANCE 19
3.1. THE ELECTRON S P IN
......................................................................................................19
3.2. THE SPIN H A M ILTO N IA N
............................................................................................
20
3.2.1. THE ELECTRON ZEEMAN IN TE R A C TIO N
............................................................21
3.2.2. THE ELECTRON-EXCHANGE IN TE R A CTIO N
.........................................................22
3.2.3. THE ZERO FIELD
INTERACTION...........................................................................23
3.2.4. DISTANCE DEPENDENCY OF
INTERACTIONS......................................................25
3.3. ELECTRON PARAMAGNETIC RESONANCE T H E O R Y
.........................................................27
3.4. OPTICALLY DETECTED MAGNETIC RESONANCE T H
EORY................................................31
3.4.1. TRIPLET-TRIPLET AN N IH ILATION
........................................................................32
3.4.2. SPIN-DEPENDENT RECOMBINATION MODEL
................................................ 33
3.5. ELECTRICALLY DETECTED MAGNETIC RESONANCE T H E O R Y
..........................................
35
3.5.1. SPIN-DEPENDENT RECOM
BINATION...............................................................35
3.5.2. SPIN-DEPENDENT
TRANSPORT........................................................................36
3.5.3. DETECTION M O D E S
.........................................................................................
36
4. EXPERIMENTAL SECTION 39
4.1. M
ATERIALS....................................................................................................................
39
4.1.1. DONOR-MATERIALS . .
.
..........................................................
39
4.1.2. ACCEPTOR-M
ATERIALS.......................................................................................41
4.2. SAMPLE PREPARATION
......................................
43
4.3. THE X-BAND EPR S P ECTROM
ETER.............................................................................48
4.3.1. CONTINUOUS WAVE E P R
.................................................................................50
4.3.2. PHOTOLUMINESCENCE DETECTED MAGNETIC R ESONANCE
..............................
51
4.3.3. ELECTRICALLY DETECTED MAGNETIC R E SO N A N CE
.............................................
52
4.3.4. ELECTROLUMINESCENCE DETECTED MAGNETIC R ESO N A N CE
...........................
53
5. DETECTION OF RESIDUAL IODINE IN PTB7:PCBM BLENDS DUE TO THE ADDITIVE
DIO 55
5.1.
INTRODUCTION...............................................................................................................55
5.2. EXPERIMENTAL D E TA ILS
................................................................................................56
5.3. RESULTS & D IS C U SS IO N
................................................................................................57
5.3.1. SOLAR CELL
PERFORMANCE.................................................................................57
5.3.2. XPS M EASUREM
ENTS.......................................................................................58
5.3.3. LIGHT INDUCED EPR M EASUREM
ENTS............................................................ 60
5.3.4. UPS-AND CELIV M EA SU REM EN
TS............................................................... 62
5.4. C
ONCLUSION..................................................................................................................64
6. TRIPLET EXCITON FORMATION IN P-DTS(FBTTH
2
)
2
PC
7
OBM BASED SMALL-
MOLECULE SOLAR CELLS 65
6.1.
INTRODUCTION...............................................................................................................65
6.2. EXPERIMENTAL D E TA ILS
................................................................................................68
6.3. RESULTS & D IS C U SS IO N
................................................................................................69
6.3.1. SOLAR CELL CHARACTERISTICS AND M ORPHOLOGY
.............................................
70
6.3.2. IDENTIFICATION OF ZERO FIELD SPLITTING PARAMETERS
....................................
72
6.3.3. TRIPLET EXCITONS IN P-DTS(FBTTH
2
)
2
- PC
7
OBM B LE N D S
...........................
74
6.3.4. MOLECULAR ORIENTATION OF P-DTS(FBTTH
2 ) 2
MOLECULES
........................
77
6.4. C
ONCLUSION..................................................................................................................60
7. INFLUENCE OF GALVINOXYL-DOPING ON CHARGE SEPARATION 81
7.1.
INTRODUCTION...............................................................................................................81
7.2. EXPERIMENTAL D E TA ILS
................................................................................................83
7.3. RESULTS & D IS C U SS IO N
................................................................................................83
7.3.1. GALVINOXYL DOPING CONCENTRATION D E P E N D E N C Y
....................................
83
7.3.2. TEMPERATURE D
EPENDENCY...........................................................................85
7.4. C
ONCLUSION..................................................................................................................87
8. QUANTIFYING SPIN-DEPENDENT RECOMBINATION 89
8.1. INTRODUCTION
.............................
89
8.2. EXPERIMENTAL D E TA ILS
................................................................................................91
8.3. RESULTS & D IS C U SS IO N
...............................................................................................
93
8.3.1. EDMR SIGNAL GENESIS
.................................................................................94
8.3.2. OTRACE-EDMR
............................................................................................
98
8.4. C
ONCLUSION................................................................................................................102
9. THE ROLE OF SPIN STATES IN THERMALLY ACTIVATED DELAYED FLUORESCENCE
OLEDS 103
9.1.
INTRODUCTION.............................................................................................................103
9.2. EXPERIMENTAL D E TA ILS
..............................................................................................
106
9.3. RESULTS & D ISC U SSIO N
..............................................................................................
107
9.3.1. EXCIPLEX EM
ISSION........................................................................................
107
9.3.2. PLDM R-M EASUREM
ENTS............................................................................
108
9.3.3. EDM R-M
EASUREMENTS...............................................................................
I L L
9.3.4. ELDM
R-MEASUREMENTS............................................................................
112
9.4. C
ONCLUSION................................................................................................................116
10.SUMMARY 119
BIBLIOGRAPHY 124
A. PUBLICATIONS AND CONFERENCE CONTRIBUTIONS 153
B. DANKSAGUNG 157
|
| any_adam_object | 1 |
| author | Väth, Stefan Kilian ca. 21. Jh |
| author_GND | (DE-588)1124261591 (DE-588)13030302X (DE-588)1124262113 |
| author_facet | Väth, Stefan Kilian ca. 21. Jh |
| author_role | aut |
| author_sort | Väth, Stefan Kilian ca. 21. Jh |
| author_variant | s k v sk skv |
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| dewey-full | 530 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 530 - Physics |
| dewey-raw | 530 |
| dewey-search | 530 |
| dewey-sort | 3530 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| format | Thesis Book |
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| id | DE-604.BV044018100 |
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| indexdate | 2024-07-10T07:41:18Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-029425683 |
| oclc_num | 967725623 |
| open_access_boolean | 1 |
| owner | DE-384 DE-473 DE-BY-UBG DE-703 DE-1051 DE-824 DE-29 DE-12 DE-91 DE-BY-TUM DE-19 DE-BY-UBM DE-1049 DE-92 DE-739 DE-898 DE-BY-UBR DE-355 DE-BY-UBR DE-706 DE-20 DE-1102 DE-860 DE-2174 |
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| spelling | Väth, Stefan Kilian ca. 21. Jh. Verfasser (DE-588)1124261591 aut On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen vorgelegt von Stefan Kilian Väth aus Würzburg ; Gutachter: Prof. Dr. Vladimir Dyakonov, Prof. Dr. Jean Geurts Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen Würzburg 2016 V, 158 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Dissertation Julius-Maximilians-Universität Würzburg 2016 Langzeitarchivierung gewährleistet, LZA Zusammenfassung in deutscher und englischer Sprache Organischer Halbleiter (DE-588)4172780-0 gnd rswk-swf Elektronenspinresonanz (DE-588)4132116-9 gnd rswk-swf Elektronenspin (DE-588)4151885-8 gnd rswk-swf Polymerhalbleiter (DE-588)4175239-9 gnd rswk-swf Organic Semiconductors Electron Spin Resonance (DE-588)4113937-9 Hochschulschrift gnd-content Organischer Halbleiter (DE-588)4172780-0 s Elektronenspin (DE-588)4151885-8 s DE-604 Polymerhalbleiter (DE-588)4175239-9 s Elektronenspinresonanz (DE-588)4132116-9 s Dyakonov, Vladimir 1963- (DE-588)13030302X dgs Geurts, Jean ca. 21. Jh. (DE-588)1124262113 dgs Erscheint auch als Online-Ausgabe urn:nbn:de:bvb:20-opus-141894 https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-141894 Resolving-System kostenfrei Volltext http://d-nb.info/1122436076/34 Langzeitarchivierung Nationalbibliothek DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029425683&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Väth, Stefan Kilian ca. 21. Jh On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen Organischer Halbleiter (DE-588)4172780-0 gnd Elektronenspinresonanz (DE-588)4132116-9 gnd Elektronenspin (DE-588)4151885-8 gnd Polymerhalbleiter (DE-588)4175239-9 gnd |
| subject_GND | (DE-588)4172780-0 (DE-588)4132116-9 (DE-588)4151885-8 (DE-588)4175239-9 (DE-588)4113937-9 |
| title | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| title_alt | Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| title_auth | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| title_exact_search | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| title_full | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen vorgelegt von Stefan Kilian Väth aus Würzburg ; Gutachter: Prof. Dr. Vladimir Dyakonov, Prof. Dr. Jean Geurts |
| title_fullStr | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen vorgelegt von Stefan Kilian Väth aus Würzburg ; Gutachter: Prof. Dr. Vladimir Dyakonov, Prof. Dr. Jean Geurts |
| title_full_unstemmed | On the Role of Spin States in Organic Semiconductor Devices = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen vorgelegt von Stefan Kilian Väth aus Würzburg ; Gutachter: Prof. Dr. Vladimir Dyakonov, Prof. Dr. Jean Geurts |
| title_short | On the Role of Spin States in Organic Semiconductor Devices |
| title_sort | on the role of spin states in organic semiconductor devices die rolle von spin zustanden in organischen halbleiterbauteilen |
| title_sub | = Die Rolle von Spin Zuständen in organischen Halbleiterbauteilen |
| topic | Organischer Halbleiter (DE-588)4172780-0 gnd Elektronenspinresonanz (DE-588)4132116-9 gnd Elektronenspin (DE-588)4151885-8 gnd Polymerhalbleiter (DE-588)4175239-9 gnd |
| topic_facet | Organischer Halbleiter Elektronenspinresonanz Elektronenspin Polymerhalbleiter Hochschulschrift |
| url | https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-141894 http://d-nb.info/1122436076/34 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029425683&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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