Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale:
Gas hydrates are crystalline solids composed of water and gas molecules. They are stable at elevated pressure and low temperatures. Therefore, natural gas hydrate deposits occur at continental margins, permafrost areas, deep lakes, and deep inland seas. During hydrate formation, the water molecules...
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| Format: | Abschlussarbeit Elektronisch E-Book |
| Sprache: | English |
| Veröffentlicht: |
Potsdam
2016
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| Zusammenfassung: | Gas hydrates are crystalline solids composed of water and gas molecules. They are stable at elevated pressure and low temperatures. Therefore, natural gas hydrate deposits occur at continental margins, permafrost areas, deep lakes, and deep inland seas. During hydrate formation, the water molecules rearrange to form cavities which host gas molecules. Due to the high pressure during hydrate formation, significant amounts of gas can be stored in hydrate structures. The water-gas ratio hereby can reach up to 1:172 at 0°C and atmospheric pressure. Natural gas hydrates predominantly contain methane. Because methane constitutes both a fuel and a greenhouse gas, gas hydrates are a potential energy resource as well as a potential source for greenhouse gas. This study investigates the physical properties of methane hydrate bearing sediments on a laboratory scale. To do so, an electrical resistivity tomography (ERT) array was developed and mounted in a large reservoir simulator (LARS). For the first time, the ERT array was applied to hydrate saturated sediment samples under controlled temperature, pressure, and hydrate saturation conditions on a laboratory scale. Typically, the pore space of (marine) sediments is filled with electrically well conductive brine. Because hydrates constitute an electrical isolator, significant contrasts regarding the electrical properties of the pore space emerge during hydrate formation and dissociation. Frequent measurements during hydrate formation experiments permit the recordings of the spatial resistivity distribution inside LARS. Those data sets are used as input for a new data processing routine which transfers the spatial resistivity distribution into the spatial distribution of hydrate saturation. Thus, the changes of local hydrate saturation can be monitored with respect to space and time. This study shows that the developed tomography yielded good data quality and resolved even small amounts of hydrate saturation inside the sediment sample. The conversion algorithm transforming the spatial resistivity distribution into local hydrate saturation values yielded the best results using the Archie-var-phi relation. This approach considers the increasing hydrate phase as part of the sediment frame, metaphorically reducing the sample’s porosity. In addition, the tomographical measurements showed that fast lab based hydrate formation processes cause small crystallites to form which tend to recrystallize. Furthermore, hydrate dissociation experiments via depressurization were conducted in order to mimic the 2007/2008 Mallik field trial. It was observed that some patterns in gas and water flow could be reproduced, even though some setup related limitations arose. In two additional long-term experiments the feasibility and performance of CO2-CH4 hydrate exchange reactions were studied in LARS. The tomographical system was used to monitor the spatial hydrate distribution during the hydrate formation stage. During the subsequent CO2 injection, the tomographical array allowed to follow the CO2 migration front inside the sediment sample and helped to identify the CO2 breakthrough. |
| Beschreibung: | Enthält 4 Zeitschriftenaufsätze |
| Beschreibung: | 1 Online-Ressource (X, 125 Seiten) Illustrationen, Diagramme |
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| 245 | 1 | 0 | |a Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |c von Mike Priegnitz |
| 246 | 1 | 3 | |a Entwicklung geophysikalischer Methoden zur Charakterisierung von Methanhydrat-Reservoiren im Labormaßstab |
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| 520 | 1 | |a Gas hydrates are crystalline solids composed of water and gas molecules. They are stable at elevated pressure and low temperatures. Therefore, natural gas hydrate deposits occur at continental margins, permafrost areas, deep lakes, and deep inland seas. During hydrate formation, the water molecules rearrange to form cavities which host gas molecules. Due to the high pressure during hydrate formation, significant amounts of gas can be stored in hydrate structures. The water-gas ratio hereby can reach up to 1:172 at 0°C and atmospheric pressure. Natural gas hydrates predominantly contain methane. Because methane constitutes both a fuel and a greenhouse gas, gas hydrates are a potential energy resource as well as a potential source for greenhouse gas. This study investigates the physical properties of methane hydrate bearing sediments on a laboratory scale. To do so, an electrical resistivity tomography (ERT) array was developed and mounted in a large reservoir simulator (LARS). For the first time, the ERT array was applied to hydrate saturated sediment samples under controlled temperature, pressure, and hydrate saturation conditions on a laboratory scale. Typically, the pore space of (marine) sediments is filled with electrically well conductive brine. Because hydrates constitute an electrical isolator, significant contrasts regarding the electrical properties of the pore space emerge during hydrate formation and dissociation. Frequent measurements during hydrate formation experiments permit the recordings of the spatial resistivity distribution inside LARS. Those data sets are used as input for a new data processing routine which transfers the spatial resistivity distribution into the spatial distribution of hydrate saturation. Thus, the changes of local hydrate saturation can be monitored with respect to space and time. This study shows that the developed tomography | |
| 520 | 1 | |a yielded good data quality and resolved even small amounts of hydrate saturation inside the sediment sample. The conversion algorithm transforming the spatial resistivity distribution into local hydrate saturation values yielded the best results using the Archie-var-phi relation. This approach considers the increasing hydrate phase as part of the sediment frame, metaphorically reducing the sample’s porosity. In addition, the tomographical measurements showed that fast lab based hydrate formation processes cause small crystallites to form which tend to recrystallize. Furthermore, hydrate dissociation experiments via depressurization were conducted in order to mimic the 2007/2008 Mallik field trial. It was observed that some patterns in gas and water flow could be reproduced, even though some setup related limitations arose. In two additional long-term experiments the feasibility and performance of CO2-CH4 hydrate exchange reactions were studied in LARS. The tomographical system was used to monitor the spatial hydrate distribution during the hydrate formation stage. During the subsequent CO2 injection, the tomographical array allowed to follow the CO2 migration front inside the sediment sample and helped to identify the CO2 breakthrough. | |
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| spelling | Priegnitz, Mike Verfasser (DE-588)1100702911 aut Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale von Mike Priegnitz Entwicklung geophysikalischer Methoden zur Charakterisierung von Methanhydrat-Reservoiren im Labormaßstab Potsdam 2016 1 Online-Ressource (X, 125 Seiten) Illustrationen, Diagramme txt rdacontent c rdamedia cr rdacarrier Enthält 4 Zeitschriftenaufsätze Dissertation Universität Potsdam 2015 Kumulative Dissertation Gas hydrates are crystalline solids composed of water and gas molecules. They are stable at elevated pressure and low temperatures. Therefore, natural gas hydrate deposits occur at continental margins, permafrost areas, deep lakes, and deep inland seas. During hydrate formation, the water molecules rearrange to form cavities which host gas molecules. Due to the high pressure during hydrate formation, significant amounts of gas can be stored in hydrate structures. The water-gas ratio hereby can reach up to 1:172 at 0°C and atmospheric pressure. Natural gas hydrates predominantly contain methane. Because methane constitutes both a fuel and a greenhouse gas, gas hydrates are a potential energy resource as well as a potential source for greenhouse gas. This study investigates the physical properties of methane hydrate bearing sediments on a laboratory scale. To do so, an electrical resistivity tomography (ERT) array was developed and mounted in a large reservoir simulator (LARS). For the first time, the ERT array was applied to hydrate saturated sediment samples under controlled temperature, pressure, and hydrate saturation conditions on a laboratory scale. Typically, the pore space of (marine) sediments is filled with electrically well conductive brine. Because hydrates constitute an electrical isolator, significant contrasts regarding the electrical properties of the pore space emerge during hydrate formation and dissociation. Frequent measurements during hydrate formation experiments permit the recordings of the spatial resistivity distribution inside LARS. Those data sets are used as input for a new data processing routine which transfers the spatial resistivity distribution into the spatial distribution of hydrate saturation. Thus, the changes of local hydrate saturation can be monitored with respect to space and time. This study shows that the developed tomography yielded good data quality and resolved even small amounts of hydrate saturation inside the sediment sample. The conversion algorithm transforming the spatial resistivity distribution into local hydrate saturation values yielded the best results using the Archie-var-phi relation. This approach considers the increasing hydrate phase as part of the sediment frame, metaphorically reducing the sample’s porosity. In addition, the tomographical measurements showed that fast lab based hydrate formation processes cause small crystallites to form which tend to recrystallize. Furthermore, hydrate dissociation experiments via depressurization were conducted in order to mimic the 2007/2008 Mallik field trial. It was observed that some patterns in gas and water flow could be reproduced, even though some setup related limitations arose. In two additional long-term experiments the feasibility and performance of CO2-CH4 hydrate exchange reactions were studied in LARS. The tomographical system was used to monitor the spatial hydrate distribution during the hydrate formation stage. During the subsequent CO2 injection, the tomographical array allowed to follow the CO2 migration front inside the sediment sample and helped to identify the CO2 breakthrough. Methanhydrate (DE-588)1052298168 gnd rswk-swf Physikalische Eigenschaft (DE-588)4134738-9 gnd rswk-swf Sediment (DE-588)4054079-0 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Methanhydrate (DE-588)1052298168 s Physikalische Eigenschaft (DE-588)4134738-9 s Sediment (DE-588)4054079-0 s DE-604 Schicks, Judith Maria 1969- (DE-588)121849112 dgs https://nbn-resolving.org/urn:nbn:de:kobv:517-opus4-89321 Resolving-System kostenfrei Volltext https://publishup.uni-potsdam.de/opus4-ubp/frontdoor/index/index/docId/8932 Verlag kostenfrei Volltext |
| spellingShingle | Priegnitz, Mike Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale Methanhydrate (DE-588)1052298168 gnd Physikalische Eigenschaft (DE-588)4134738-9 gnd Sediment (DE-588)4054079-0 gnd |
| subject_GND | (DE-588)1052298168 (DE-588)4134738-9 (DE-588)4054079-0 (DE-588)4113937-9 |
| title | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |
| title_alt | Entwicklung geophysikalischer Methoden zur Charakterisierung von Methanhydrat-Reservoiren im Labormaßstab |
| title_auth | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |
| title_exact_search | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |
| title_full | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale von Mike Priegnitz |
| title_fullStr | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale von Mike Priegnitz |
| title_full_unstemmed | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale von Mike Priegnitz |
| title_short | Development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |
| title_sort | development of geophysical methods to characterize methane hydrate reservoirs on a laboratory scale |
| topic | Methanhydrate (DE-588)1052298168 gnd Physikalische Eigenschaft (DE-588)4134738-9 gnd Sediment (DE-588)4054079-0 gnd |
| topic_facet | Methanhydrate Physikalische Eigenschaft Sediment Hochschulschrift |
| url | https://nbn-resolving.org/urn:nbn:de:kobv:517-opus4-89321 https://publishup.uni-potsdam.de/opus4-ubp/frontdoor/index/index/docId/8932 |
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