Environmental organic chemistry:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Hoboken, New Jersey
Wiley
[2017]
|
| Ausgabe: | Third edition |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | xvii, 1005 Seiten Illustrationen, Diagramme |
| ISBN: | 1118767233 9781118767238 |
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Datensatz im Suchindex
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| adam_text |
Titel: Environmental organic chemistry
Autor: Schwarzenbach, René P
Jahr: 2017
V
Contents
Preface xiii
About the Companion Website xvii
1 General Topic and Overview 1
1.1 Introduction / 2
1.2 Assessing Organic Chemicals in the Environment / 4
1.3 What is This Book All About? / 7
1.4 Bibliography / 14
PARTI
Background Knowledge 17
2 Background Knowledge on Organic Chemicals 19
2.1 The Makeup of Organic Compounds / 20
2.2 Intermolecular Forces Between Uncharged Molecules / 37
2.3 Questions and Problems / 40
2.4 Bibliography / 43
3 The Amazing World of Anthropogenic Organic Chemicals 45
3.1 Introduction / 47
3.2 A Lasting Global Problem: Persistent Organic Pollutants (POPs) / 47
3.3 Natural but Nevertheless Problematic: Petroleum Hydrocarbons / 48
3.4 Notorious Air and Groundwater Pollutants: Organic Solvents / 53
3.5 Safety First: Flame Retardants All Around Us / 56
3.6 How to Make Materials "Repellent": Polyfluorinated Chemicals
(PFCs) / 58
3.7 From Washing Machines to Surface Waters: Complexing Agents,
Surfactants, Whitening Agents, and Corrosion Inhibitors / 60
3.8 Health, Well-Being, and Water Pollution: Pharmaceuticals and
Personal Care Products / 63
3.9 Fighting Pests: Herbicides, Insecticides, and Fungicides / 65
3.10 Our Companion Compounds: Representative Model Chemicals / 69
3.11 Questions/72
3.12 Bibliography / 73
vi
Contents
4 Background Thermodynamics, Equilibrium Partitioning and Acidity
Constants 81
4.1 Important Thermodynamic Functions / 83
4.2 Using Thermodynamic Functions to Quantify
Equilibrium Partitioning / 89
4.3 Organic Acids and Bases I: Acidity Constant and Speciation in
Natural Waters / 98
4.4 Organic Acids and Bases II: Chemical Structure
and Acidity Constant / 107
4.5 Questions and Problems / 116
4.6 Bibliography / 119
5 Earth Systems and Compartments 121
5.1 Introduction /123
5.2 The Atmosphere / 125
5.3 Surface Waters and Sediments /131
5.4 Soil and Groundwater / 148
5.5 Biota/154
5.6 Questions / 155
5.7 B ibliography / 15 8
6 Environmental Systems: Physical Processes and Mathematical
Modeling 165
6.1 Systems and Models / 167
6.2 Box Models: A Concept for a Simple World / 174
6.3 When Space Matters: Transport Processes /191
6.4 Models in Space and Time / 196
6.5 Questions and Problems / 203
6.6 Bibliography / 211
PARTII
Equilibrium Partitioning in Well-Defined Systems 213
7 Partitioning Between Bulk Phases: General Aspects and Modeling
Approaches 215
7.1 Introduction / 216
7.2 Molecular Interactions Governing Bulk Phase Partitioning
of Organic Chemicals / 217
7.3 Quantitative Approaches to Estimate Bulk Phase Partition
Constants/Coefficients: Linear Free Energy Relationships (LFERs) / 225
7.4 Questions / 232
7.5 Bibliography / 234
Contents vii
8 Vapor Pressure (p*) 237
8.1 Introduction and Theoretical Background / 238
8.2 Molecular Interactions Governing Vapor Pressure and Vapor
Pressure Estimation Methods / 246
8.3 Questions and Problems / 253
8.4 Bibliography / 257
9 Solubility (Cand Activity Coefficient (y™1) in Water; Air-Water
Partition Constant (A,aw) 259
9.1 Introduction and Thermodynamic Considerations / 261
9.2 Molecular Interactions Governing the Aqueous Activity
Coefficient and the Air-Water Partition Constant / 267
9.3 LFERs for Estimating Air-Water Partition Constants and
Aqueous Activity Coefficients/Aqueous Solubilities / 270
9.4 Effect of Temperature, Dissolved Salts, and pH on the Aqueous
Activity Coefficient/Aqueous Solubility and on the Air-Water
Partition Constant / 272
9.5 Questions and Problems / 282
9.6 Bibliography / 285
10 Organic Liquid-Air and Organic Liquid-Water Partitioning 289
10.1 Introduction / 291
10.2 Thermodynamic Considerations and Comparisons of Different
Organic Solvents / 291
10.3 The Octanol-Water System: The Atom/Fragment Contribution
Method for Estimation of the Octanol-Water Partition
Constant / 298
10.4 Partitioning Involving Organic Solvent-Water Mixtures / 301
10.5 Evaporation and Dissolution of Organic Compounds
from Organic Liquid Mixtures-Equilibrium
Considerations / 307
10.6 Questions and Problems / 311
10.7 Bibliography / 317
11 Partitioning of Nonionic Organic Compounds Between Well-Defined
Surfaces and Air or Water 321
11.1 Introduction / 322
11.2 Adsorption from Air to Weil-Defined Surfaces / 322
11.3 Adsorption from Water to Inorganic Surfaces / 335
11.4 Questions and Problems / 342
11.5 Bibliography / 345
viii
Contents
PART III
Equilibrium Partitioning in Environmental Systems
349
General Introduction to Sorption Processes
351
13
14
15
12.1 Introduction / 352
12.2 Sorption Isotherms and the Solid-Water Equilibrium Distribution
Coefficient (Kki) / 354
12.3 Speciation (Sorbed versus Dissolved or Gaseous), Retardation,
and Sedimentation / 360
12.4 Questions and Problems / 366
12.5 Bibliography / 368
Sorption from Water to Natural Organic Matter (NOM) 369
13.1 The Structural Diversity of Natural Organic Matter Present in
Aquatic and Terrestrial Environments / 371
13.2 Quantifying Natural Organic Matter-Water Partitioning
of Neutral Organic Compounds / 376
13.3 Sorption of Organic Acids and Bases to Natural Organic Matter / 388
13.4 Questions and Problems / 392
13.5 Bibliography / 397
Sorption of Ionic Organic Compounds to Charged Surfaces 405
14.1 Introduction / 407
14.2 Cation and Anion Exchange Capacities of Solids in Water / 408
14.3 Ion Exchange: Nonspecific Adsorption of Ionized Organic
Chemicals from Aqueous Solutions to Charged Surfaces / 414
14.4 Surface Complexation: Specific Bonding of Organic Compounds
with Solid Phases in Water / 426
14.5 Questions and Problems / 432
14.6 Bibliography / 436
Aerosol-Air Partitioning: Dry and Wet Deposition of Organic
Pollutants 441
15.1 Origins and Properties of Atmospheric Aerosols / 442
15.2 Assessing Aerosol-Air Partition Coefficients (Ä",-PMa) / 445
15.3 Dry and Wet Deposition / 453
15.4 Questions and Problems / 459
15.5 Bibliography / 464
Equilibrium Partitioning From Water and Air to Biota 469
16.1 Introduction / 471
16.2 Predicting Biota-Water and Biota-Air Equilibrium Partitioning / 471
16.3 Bioaccumulation and Biomagnification in Aquatic Systems / 485
16.4 Bioaccumulation and Biomagnification in Terrestrial Systems / 498
Contents ix
16.5 Baseline Toxicity (Narcosis) / 503 16.6 Questions and Problems / 507 16.7 Bibliography / 514
PART IV Mass Transfer Processes in Environmental Systems 523
17 Random Motion, Molecular and Turbulent Diffusivity 17.1 Random Motion / 526 17.2 Molecular Diffusion / 534 17.3 Other Random Transport Processes in the Environment / 545 17.4 Questions and Problems / 550 17.5 Bibliography / 557 525
18 Transport at Boundaries 18.1 The Role of Boundaries in the Environment / 560 18.2 Bottleneck Boundaries / 562 18.3 Wall Boundaries / 567 18.4 Hybrid Boundaries / 572 18.5 Questions and Problems / 577 18.6 Bibliography / 580 559
19 Air-Water Exchange 19.1 The Air-Water Interface / 583 19.2 Air-Water Exchange Models / 585 19.3 Measurement of Air-Water Exchange Velocities / 592 19.4 Air-Water Exchange in Flowing Waters / 599 19.5 Questions and Problems / 604 19.6 Bibliography / 613 581
20 Interfaces Involving Solids 20.1 The Sediment-Water Interface / 618 20.2 Transport in Unsaturated Soil / 626 20.3 Questions and Problems / 630 20.4 Bibliography / 634 617
PART V Transformation Processes 635
21 Background Knowledge on Transformation Reactions of Organic
Pollutants 637
21.1 Identifying Reactive Sites Within Organic Molecules / 638
21.2 Thermodynamics of Transformation Reactions / 643
X Contents
21.3 Kinetics of Transformation Reactions / 650
21.4 Questions and Problems / 657
21.5 Bibliography / 661
22 Hydrolysis And Reactions With Other Nucleophiles 663
22.1 Nucleophilic Substitution and Elimination Reactions Involving
Primarily Saturated Carbon Atoms / 665
22.2 Hydrolytic Reactions of Carboxylic and Carbonic Acid
Derivatives / 680
22.3 Enzyme-Catalyzed Hydrolysis Reactions: Hydrolases / 695
22.4 Questions and Problems / 701
22.5 Bibliography / 710
23 Redox Reactions 715
23.1 Introduction / 716
23.2 Evaluating the Thermodynamics of Redox Reactions / 719
23.3 Examples of Chemical Redox Reactions in Natural Systems / 730
23.4 Examples of Enzyme-Catalyzed Redox Reactions / 747
23.5 Questions and Problems / 756
23.6 Bibliography / 765
24 Direct Photolysis in Aquatic Systems 773
24.1 Introduction / 775
24.2 Some Basic Principles of Photochemistry / 776
24.3 Light Absorption by Organic Compounds in Natural
Waters / 788
24.4 Quantum Yield and Rate of Direct Photolysis / 800
24.5 Effects of Solid Sorbents (Particles, Soil Surfaces, Ice) on Direct
Photolysis / 803
24.6 Questions and Problems / 804
24.7 Bibliography / 811
25 Indirect Photolysis: Reactions with Photooxidants in Natural
Waters and in the Atmosphere 815
25.1 Introduction / 816
25.2 Indirect Photolysis in Surface Waters / 817
25.3 Indirect Photolysis in the Atmosphere (Troposphere): Reaction
with Hydroxyl Radical (HO*) / 829
25.4 Questions and Problems / 833
25.5 Bibliography / 838
26
Biotransformations
26.1 Introduction / 847
845
Contents xi
26.2 Some Important Concepts about Microorganisms Relevant
to Biotransformations / 848
26.3 Initial Biotransformation Strategies / 858
26.4 Rates of Biotransformations / 864
26.5 Questions and Problems / 882
26.6 Bibliography / 889
27 Assessing Transformation Processes Using Compound-Specific
Isotope Analysis (CSIA) 897
27.1 Introduction, Methodology, and Theoretical Background / 898
27.2 Using CSIA for Assessing Organic Compound Transformations
in Laboratory and Field Systems / 914
27.3 Questions and Problems / 930
27.4 Bibliography / 936
PART VI
Putting Everything Together 945
28 Exposure Assessment of Organic Pollutants Using Simple Modeling
Approaches 947
28.1 One-Box Model: The Universal Tool for Process Integration / 948
28.2 Assessing Equilibrium Partitioning in Simple
Multimedia Systems / 952
28.3 Simple Dynamic Systems / 956
28.4 Systems Driven by Advection / 960
28.5 Bibliography / 974
Appendix
Index
977
995 |
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| author | Schwarzenbach, René P. 1945- |
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| discipline | Chemie / Pharmazie Allgemeines Chemie Umwelt |
| edition | Third edition |
| format | Book |
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| genre | (DE-588)4123623-3 Lehrbuch gnd-content |
| genre_facet | Lehrbuch |
| id | DE-604.BV043643914 |
| illustrated | Illustrated |
| indexdate | 2024-11-26T15:01:25Z |
| institution | BVB |
| isbn | 1118767233 9781118767238 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-029057667 |
| oclc_num | 968684807 |
| open_access_boolean | |
| owner | DE-12 DE-210 DE-19 DE-BY-UBM DE-11 DE-91G DE-BY-TUM DE-29 DE-91 DE-BY-TUM DE-83 |
| owner_facet | DE-12 DE-210 DE-19 DE-BY-UBM DE-11 DE-91G DE-BY-TUM DE-29 DE-91 DE-BY-TUM DE-83 |
| physical | xvii, 1005 Seiten Illustrationen, Diagramme |
| publishDate | 2017 |
| publishDateSearch | 2017 |
| publishDateSort | 2017 |
| publisher | Wiley |
| record_format | marc |
| spelling | Schwarzenbach, René P. 1945- Verfasser (DE-588)1027702562 aut Environmental organic chemistry René P. Schwarzenbach, Philip M. Gschwend, Dieter M. Imboden Third edition Hoboken, New Jersey Wiley [2017] © 2017 xvii, 1005 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Physikalisch-chemische Eigenschaft (DE-588)4369521-8 gnd rswk-swf Umwelt (DE-588)4061616-2 gnd rswk-swf Ökologische Chemie (DE-588)4135167-8 gnd rswk-swf Physikalische Chemie (DE-588)4045959-7 gnd rswk-swf Organische Verbindungen (DE-588)4043816-8 gnd rswk-swf Organische Chemie (DE-588)4043793-0 gnd rswk-swf (DE-588)4123623-3 Lehrbuch gnd-content Ökologische Chemie (DE-588)4135167-8 s Organische Chemie (DE-588)4043793-0 s DE-604 Organische Verbindungen (DE-588)4043816-8 s Physikalisch-chemische Eigenschaft (DE-588)4369521-8 s Physikalische Chemie (DE-588)4045959-7 s Umwelt (DE-588)4061616-2 s 1\p DE-604 2\p DE-604 Gschwend, Philip M. 1951- Sonstige (DE-588)136129900 oth Imboden, Dieter M. 1943- Sonstige (DE-588)172164672 oth HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029057667&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 2\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Schwarzenbach, René P. 1945- Environmental organic chemistry Physikalisch-chemische Eigenschaft (DE-588)4369521-8 gnd Umwelt (DE-588)4061616-2 gnd Ökologische Chemie (DE-588)4135167-8 gnd Physikalische Chemie (DE-588)4045959-7 gnd Organische Verbindungen (DE-588)4043816-8 gnd Organische Chemie (DE-588)4043793-0 gnd |
| subject_GND | (DE-588)4369521-8 (DE-588)4061616-2 (DE-588)4135167-8 (DE-588)4045959-7 (DE-588)4043816-8 (DE-588)4043793-0 (DE-588)4123623-3 |
| title | Environmental organic chemistry |
| title_auth | Environmental organic chemistry |
| title_exact_search | Environmental organic chemistry |
| title_full | Environmental organic chemistry René P. Schwarzenbach, Philip M. Gschwend, Dieter M. Imboden |
| title_fullStr | Environmental organic chemistry René P. Schwarzenbach, Philip M. Gschwend, Dieter M. Imboden |
| title_full_unstemmed | Environmental organic chemistry René P. Schwarzenbach, Philip M. Gschwend, Dieter M. Imboden |
| title_short | Environmental organic chemistry |
| title_sort | environmental organic chemistry |
| topic | Physikalisch-chemische Eigenschaft (DE-588)4369521-8 gnd Umwelt (DE-588)4061616-2 gnd Ökologische Chemie (DE-588)4135167-8 gnd Physikalische Chemie (DE-588)4045959-7 gnd Organische Verbindungen (DE-588)4043816-8 gnd Organische Chemie (DE-588)4043793-0 gnd |
| topic_facet | Physikalisch-chemische Eigenschaft Umwelt Ökologische Chemie Physikalische Chemie Organische Verbindungen Organische Chemie Lehrbuch |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029057667&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT schwarzenbachrenep environmentalorganicchemistry AT gschwendphilipm environmentalorganicchemistry AT imbodendieterm environmentalorganicchemistry |