Atmospheric aerosols: properties and climate impacts
Gespeichert in:
1. Verfasser: | |
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Format: | Buch |
Sprache: | English |
Veröffentlicht: |
Dordrecht [u.a]
Springer
2015
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Schlagworte: | |
Online-Zugang: | Inhaltsverzeichnis |
Beschreibung: | This book is an updated and extended tranlation |
Beschreibung: | XVII, 311 S. Ill., graph. Darst. |
ISBN: | 9789401796484 |
Internformat
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245 | 1 | 0 | |a Atmospheric aerosols |b properties and climate impacts |c Olivier Boucher |
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adam_text | Contents
1 Generał Introduction ................................................ 1
1.1 The Climate System............................................. 1
1.2 The Atmosphere ................................................ 2
1.3 Energy Budget and Atmospheric Composition...................... 3
1.4 The Water Cycle................................................ 4
1.5 Aerosols and Climate Change.................................... 5
1.6 Outline of this Textbook....................................... 7
References.......................................................... 8
Further Reading (Textbooks and Articles)............................ 8
2 Atmospheric Aerosols................................................. 9
2.1 Definitions.................................................... 9
2.2 Sources of Aerosols and Aerosol Precursors .................. 12
2.2.1 Marine Aerosols......................................... 12
2.2.2 Desert Dust............................................. 12
2.2.3 Volcanic Aerosols....................................... 13
2.2.4 Biogenic Aerosols....................................... 14
2.2.5 Biomass Burning Aerosols ............................... 15
2.2.6 Aerosols from Fossil Fuel Combustion ................... 15
2.3 Spatial and Temporal Aerosol Distributions.................... 15
2.4 Aerosol-Cloud-Radiation Interactions.......................... 17
2.5 Climate Effects of Aerosols................................... 21
References......................................................... 24
Further Reading (Textbooks and Articles)........................... 24
3 Physical, Chemical and Optical Aerosol Properties................... 25
3.1 Fine, Accumulation and Coarse Modes........................... 25
3.2 Size Distribution............................................. 26
3.3 Chemical Composition.......................................... 29
3.3.1 Aerosol Mixture......................................... 29
3.3.2 Inorganic Aerosols...................................... 30
3.3.3 Black Carbon Aerosols................................... 30
ix
x Contents
3.3.4 Organic Aerosols .......................................... 31
3.3.5 Geographic Distribution of Aerosol Chemical Composition 31
3.4 Refractive Index ................................................. 32
3.5 Deliquescence, Efflorescence and Hysteresis....................... 36
3.6 Definition of Aerosol Optical Properties.......................... 36
3.6.1 Absorption and Scattering Cross Sections................... 36
3.6.2 Phase Function............................................. 38
3.6.3 Upscatter Fractions........................................ 38
3.7 Calculation of Aerosol Optical Properties ........................ 40
3.7.1 Mie Theory................................................. 40
3.7.2 Extinction, Scattering and Absorption...................... 41
3.7.3 Optical Depth and Angstrom Coefficient..................... 43
3.8 Optical Properties of Nonspherical Aerosols....................... 45
3.9 Aerosols and Atmospheric Visibility............................... 45
References............................................................. 48
Further Reading (Textbooks and Articles)............................... 49
4 Aerosol Modelling....................................................... 51
4.1 Introduction...................................................... 51
4.2 Emissions......................................................... 52
4.2.1 Generalities............................................... 52
4.2.2 Fossil Fuels, Biofuels, and Other Anthropogenic Sources . . 53
4.2.3 Vegetation Fires .......................................... 54
4.2.4 Sea Spray.................................................. 55
4.2.5 Desert Dust................................................ 56
4.2.6 Dimethyl sulphide.......................................... 60
4.2.7 Biogenic Volatile Organic Compounds ....................... 62
4.2.8 Volcanoes.................................................. 63
4.2.9 Resuspension .............................................. 63
4.3 Atmospheric Processes............................................. 65
4.3.1 Nucléation................................................. 65
4.3.2 Condensation of Semi-Volatile Compounds.................... 67
4.3.3 Coagulation................................................ 67
4.3.4 In-Cloud Aerosol Production................................ 68
4.3.5 Wet Deposition............................................. 69
4.3.6 Dry Deposition............................................. 71
4.3.7 Sedimentation.............................................. 71
4.3.8 Aerosol Transport.......................................... 73
4.4 Modelling Approaches.............................................. 73
4.4.1 Bulk Approach.............................................. 74
4.4.2 Sectional Approach......................................... 74
4.4.3 Modal Approach............................................. 75
4.5 Example: The Sulphur Budget....................................... 77
References............................................................. 80
Further Reading (Textbooks and Articles)............................... 81
Contents
5 Interactions of Radiation with Matter and Atmospheric Radiative
Transfer ............................................................. 83
5.1 Introduction..................................................... 83
5.2 Electromagnetic Radiation........................................ 84
5.2.1 Generalities.............................................. 84
5.2.2 Definitions............................................... 85
5.3 Interactions of Radiation with Matter............................ 87
5.3.1 Matter, Energy and Spectral Lines......................... 88
5.3.2 Intensity of Spectral Lines............................... 92
5.3.3 Spectral Line Profiles.................................... 93
5.3.4 Processes of Interactions of Radiation with Matter........ 96
5.4 Modelling of the Interaction Processes........................... 97
5.4.1 Molecular Absorption Coefficient.......................... 97
5.4.2 Scattering Phase Function................................. 98
5.4.3 Molecular Scattering...................................... 99
5.4.4 Absorption and Scattering by Aerosols ................... 100
5.4.5 Thermal Emission......................................... 102
5.5 Atmospheric Radiative Transfer.................................. 105
5.5.1 Equation of Radiative Transfer........................... 105
5.5.2 Extinction Only.......................................... 107
5.5.3 Scattering Medium........................................ 108
5.5.4 Plane-Parallel Atmosphere................................ 109
5.5.5 Resolution of the Equation of Radiative Transfer......... 110
5.6 Absorption Bands, Energy, and Actinic Fluxes.................... 113
5.6.1 Main Molecular Absorption Bands in the Atmosphere...... 113
5.6.2 Radiative Flux........................................... 115
5.6.3 Two-Flux Method.......................................... 116
5.6.4 Stefan-Boltzmann Law..................................... 117
5.6.5 Radiative Budget ........................................ 117
5.6.6 Actinic Fluxes........................................... 119
5.6.7 Polarization of Radiation................................ 121
References........................................................... 126
Further Reading (Textbooks and Articles)............................ 126 6
6 In Situ and Remote Sensing Measurements of Aerosols................ 129
6.1 Introduction to Aerosol Remote Sensing ......................... 129
6.2 Passive Remote Sensing: Measurement of the Extinction........... 134
6.2.1 General Principles ...................................... 134
6.2.2 Ground-Based Photometry ................................. 135
6.2.3 Spacebome Occultation Measurements....................... 136
6.2.4 Retrieval of Aerosol Size Distribution................... 136
6.3 Passive Remote Sensing: Measurement of the Scattering........... 137
6.3.1 General Principles ...................................... 137
6.3.2 Ground-Based Measurement of Scattered Radiation........ 138
6.3.3 Spacebome Measurements of Scattered Radiation............ 138
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6.4 Measurement of Infrared Radiation......................
6.4.1 General Principles .............................
6.4.2 Spacebome Nadir Measurement of Infrared Radiation
6.4.3 Spacebome Limb Measurement of Infrared Radiation
6.5 Active Remote Sensing: Lidar...........................
6.5.1 General Principles .............................
6.5.2 The Lidar Equation..............................
6.5.3 Raman Lidar.....................................
6.6 In Situ Aerosol Measurements ..........................
6.6.1 Measurement of Aerosol Concentrations...........
6.6.2 Measurement of Aerosol Chemical Composition ....
6.6.3 Measurement of Aerosol Scattering...............
6.6.4 Measurement of Aerosol Absorption...............
6.7 Conclusions............................................
References.......^..........................................
Further Reading (Textbooks and Articles)....................
Aerosol Data Assimilation...................................
7.1 Introduction...........................................
7.2 Basic Principles of Data Assimilation..................
7.3 Applications of Data Assimilation for Aerosols.........
References..................................................
Further Reading (Textbooks and Articles)....................
Aerosol-Radiation Interactions .............................
8.1 Introduction...........................................
8.2 Atmospheric Radiative Effects Due to Aerosols .........
8.2.1 Simplified Equation for Scattering Aerosols.....
8.2.2 Simplified Equation for Absorbing Aerosols......
8.2.3 Radiative Transfer Calculations ................
8.2.4 Global Estimates and Sources of Uncertainty.....
8.3 Rapid Adjustments to Aerosol-Radiation Interactions....
8.4 Radiative Impact of Aerosols on Surface Snow and Ice...
References..................................................
Further Reading (Textbooks and Articles)....................
Aerosol-Cloud Interactions .................................
9.1 Introduction...........................................
9.1.1 Cloud Formation.................................
9.1.2 Cloud Distribution..............................
9.1.3 Aerosol-Cloud Interactions......................
9.2 Aerosol Effects on Liquid Clouds.......................
9.2.1 Saturation Pressure of Water Vapour.............
9.2.2 Kelvin Effect...................................
9.2.3 Raoult’s Law....................................
Contents
Xlll
9.2.4 Kohler Theory......................................... 200
9.2.5 Extensions to the Köhler Theory....................... 202
9.2.6 CCN and Supersaturation in the Cloud................... 204
9.2.7 Dynamical and Radiative Effects in Clouds.............. 205
9.2.8 Principle of the Cloud Albedo Effect.................. 205
9.2.9 Observations of the Cloud Albedo Effect............... 206
9.2.10 Adjustments in Liquid Water Clouds.................... 208
9.2.11 Rapid Adjustments Occurring in Liquid Clouds.......... 210
9.3 Aerosols Effects on Mixed-Phased and Ice Clouds............... 212
9.3.1 Elements of Microphysics of Ice Clouds................ 213
9.3.2 Impact of Anthropogenic Aerosols on Ice Clouds........ 214
9.4 Forcing Due to Aerosol-Cloud Interactions..................... 215
9.5 Aerosols, Contrails and Aviation-Induced Cloudiness........... 216
9.5.1 Formation of Condensation Trails....................... 216
9.5.2 Estimate of the Climate Impact of Contrails........... 218
References.......................................................... 221
Further Reading (Textbooks and Articles)............................ 225
10 Climate Response to Aerosol Forcings............................... 227
10.1 Introduction................................................... 227
10.2 Radiative Forcing, Feedbacks and Climate Response.............. 227
10.2.1 Radiative Forcing...................................... 227
10.2.2 Climate Feedbacks...................................... 228
10.2.3 Rapid Adjustments and Effective Radiative Forcing...... 231
10.2.4 Climate Response and Climate Efficacy ................. 234
10.3 Climate Response to Aerosol Forcings........................... 235
10.3.1 Equilibrium Response................................... 235
10.3.2 Past Emissions ........................................ 237
10.3.3 Detection and Attribution of Aerosol Impacts........... 239
10.3.4 Future Emissions Scenarios............................. 240
10.4 Nuclear Winter................................................. 242
References.......................................................... 244
Further Reading (Textbooks and Articles)............................ 246
11 Biogeochemical Effects and Climate Feedbacks of Aerosols........... 247
11.1 Introduction................................................... 247
11.2 Impact of Aerosols on Terrestrial Ecosystems................... 248
11.2.1 Diffuse Radiation and Primary Productivity............. 248
11.2.2 Aerosols as a Source of Nutrients..................... 249
11.2.3 Acidification of Precipitation......................... 250
11.3 Impact of Aerosols on Marine Ecosystems........................ 252
11.4 Aerosols-Atmospheric Chemistry Interactions.................... 253
11.4.1 Interactions with Tropospheric Chemistry............... 253
11.4.2 Impact of Stratospheric Aerosols on the Ozone Layer and
Ultraviolet Radiation................................... 255
XIV
Contents
11.5 Climate Feedbacks Involving Marine Aerosols................... 255
11.5.1 Sulphate Aerosols from DMS Emissions................... 255
1L5.2 Marine Aerosols.......................................... 257
11.5.3 Other Aerosols of Maritime Origin...................... 258
11.6 Climate Feedbacks Involving Continental Aerosols.............. 258
11.6.1 Secondary Organic Aerosols.............................. 259
11.6.2 Primary Aerosols of Biogenic Origin.................... 260
11.6.3 Aerosols from Vegetation Fires......................... 261
11.6.4 Desert Dust............................................. 262
11.7 Climate Feedbacks Involving Stratospheric Aerosols............ 264
References.......................................................... 265
Further Reading (Textbooks and Articles)............................ 269
12 Stratospheric Aerosols............................................... 271
12.1 Introduction................................................. 271
12.2 Atmospheric dycle of Stratospheric Aerosols................... 271
12.2.1 Sources of Stratospheric Aerosols...................... 271
12.2.2 Transport in the Stratosphere........................... 273
12.3 Physics and Chemistry of Stratospheric Aerosols................ 275
12.4 Volcanic Aerosol Records....................................... 277
12.4.1 Volcanic Aerosols During the 1750-2010 Period........... 277
12.4.2 A Few Recent Climate-Relevant Eruptions................. 279
12.4.3 Mega-Eruptions ......................................... 281
12.5 Role of Stratospheric Aerosols on the Climate System........... 281
References.......................................................... 284
Further Reading (Textbooks and Articles)............................ 286
13 Aerosol-Based Climate Engineering.................................... 287
13.1 Introduction................................................... 287
13.2 Stratospheric Aerosol Injection................................ 288
13.3 Marine Cloud Brightening....................................... 290
13.4 Role of Rapid Adjustments and Feedbacks ....................... 291
13.5 A Thought on Timescales........................................ 292
References.......................................................... 293
Further Reading (Textbooks and Articles)............................ 294
Appendix A Units and Physical Constants ................................. 295
Appendix B Properties of the Log-Normal Size Distribution................ 297
Appendix C Mie Theory.................................................... 299
Appendix D Radiative Impact of Aerosols on Snow and Ice.................. 305
Index
307
|
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id | DE-604.BV042223489 |
illustrated | Illustrated |
indexdate | 2024-07-10T01:15:43Z |
institution | BVB |
isbn | 9789401796484 |
language | English |
oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-027661949 |
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physical | XVII, 311 S. Ill., graph. Darst. |
publishDate | 2015 |
publishDateSearch | 2015 |
publishDateSort | 2015 |
publisher | Springer |
record_format | marc |
spelling | Boucher, Olivier Verfasser aut Aérosols atmosphériques Atmospheric aerosols properties and climate impacts Olivier Boucher Dordrecht [u.a] Springer 2015 XVII, 311 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier This book is an updated and extended tranlation Atmosphärisches Aerosol (DE-588)4201505-4 gnd rswk-swf Aerosol (DE-588)4000595-1 gnd rswk-swf Klimazeuge (DE-588)4489056-4 gnd rswk-swf Aerosol (DE-588)4000595-1 s Klimazeuge (DE-588)4489056-4 s DE-604 Atmosphärisches Aerosol (DE-588)4201505-4 s Erscheint auch als Online-Ausgabe 978-94-017-9649-1 Digitalisierung UB Augsburg - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027661949&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
spellingShingle | Boucher, Olivier Atmospheric aerosols properties and climate impacts Atmosphärisches Aerosol (DE-588)4201505-4 gnd Aerosol (DE-588)4000595-1 gnd Klimazeuge (DE-588)4489056-4 gnd |
subject_GND | (DE-588)4201505-4 (DE-588)4000595-1 (DE-588)4489056-4 |
title | Atmospheric aerosols properties and climate impacts |
title_alt | Aérosols atmosphériques |
title_auth | Atmospheric aerosols properties and climate impacts |
title_exact_search | Atmospheric aerosols properties and climate impacts |
title_full | Atmospheric aerosols properties and climate impacts Olivier Boucher |
title_fullStr | Atmospheric aerosols properties and climate impacts Olivier Boucher |
title_full_unstemmed | Atmospheric aerosols properties and climate impacts Olivier Boucher |
title_short | Atmospheric aerosols |
title_sort | atmospheric aerosols properties and climate impacts |
title_sub | properties and climate impacts |
topic | Atmosphärisches Aerosol (DE-588)4201505-4 gnd Aerosol (DE-588)4000595-1 gnd Klimazeuge (DE-588)4489056-4 gnd |
topic_facet | Atmosphärisches Aerosol Aerosol Klimazeuge |
url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027661949&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
work_keys_str_mv | AT boucherolivier aerosolsatmospheriques AT boucherolivier atmosphericaerosolspropertiesandclimateimpacts |