Reduction of methane emissions from landfills: processes, measures and monitoring strategies
Gespeichert in:
| 1. Verfasser: | |
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| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Hamburg
Verein zur Förderung der Bodenkunde in Hamburg
2014
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| Schriftenreihe: | Hamburger bodenkundliche Arbeiten
75 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | 191 S. Ill., graph. Darst. |
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Titel: Reduction of methane emissions from landfills
Autor: Röwer, Inga Ute
Jahr: 2014
Table of contents
List of figures.11
List of tables.13
List of abbreviations.14
Summary.15
Zusammenfassung.21
Author's contribution.27
1 Introduction.29
2 Research background.33
2.1 Gas transport in soils.33
2.2 Fluxes to be considered.35
2.2.1 Methane loads to be treated.35
2.2.2 Methane oxidation.36
2.2.3 Methane emission.39
2.2.4 Modeling landfill gas fluxes.39
2.3 Methane oxidation systems.41
2.3.1 Fields of application.41
2.3.2 Existing guidelines.41
2.3.3 Application and examples for methane oxidation systems-----------------------------------41
2.4 Monitoring techniques and strategies.43
2.4.1 Detection of methane emission.:.43
2.4.2 Quantification of emission.44
2.4.3 Quantification of methane oxidation.44
3 Intention of the research.47
3.1 Baseline study: Driving factors for the spatial variability of methane oxidation
in an old landfill cover soil [landfill K).47
3.2 Field trial I: Design, Implementation and Monitoring of Methane oxidation
windows on an old landfill [landfill K).47
3.3 Field trial II: Gas fluxes in an optimized methane oxidation cover
(Wieringermeer landfill).48
3.4 Analysis of the chamber measurement methodology and emission monitoring
strategy.49
3.5 Laboratory study: Quantification of the share of respirative carbon dioxide
during methane oxidation by means of 13C labeled methane.50
4 Study sites and setup of field trials.51
4.1 Field trial I: Old cover of landfill Kand methane oxidation window test cells.51
4.1.1 Old municipal landfill K.51
4.1.2 Methane oxidation windows.54
4.2 Field trial 11: Methane oxidation cover test cells on Wieringermeer landfill.57
5 Methods.61
5.1 General description of methods.61
5.1.1 Standard soil physical and chemical measurement procedures.61
5.1.2 Soil moisture and temperature.62
5.1.3 Penetration resistance.62
5.1.4 Emission measurement.63
5.1.5 Soil gas phase composition measurement.66
5.1.6 Calculation of methane oxidation efficiency.67
5.1.7 Methane oxidation activity tests.68
5.1.8 Estimation of diffusive and advective flux.69
5.1.9 Stable isotope analysis.69
5.2 Experiments and monitoring campaigns.72
5.2.1 Baseline study: Drivers for methane oxidation rate in a cover soil of an old
landfill (Landfill K).72
5.2.2 Field Trial I: Performance of methane oxidation windows.73
5.2.3 Field trial II: Performance of an optimized methane oxidation cover
(Wieringermeer landfill).76
5.3 Laboratory experiment on the quantification of the share of respirative
carbon dioxide during methane oxidation by means of 13C labeled methane.77
5.3.1 Sampling.77
5.3.2 Experiment to determine reaction kinetics.78
5.3.3 Incubation to determine the respiratory share of carbon dioxide.78
5.3.4 Soil physical parameters.78
5.3.5 Stable isotope analysis.78
6 Results.79
6.1 Baseline study: Driving factors for the spatial variability of methane oxidation
in an old landfill cover soil.79
6.1.1 Spatial variability of soil gas composition, and soil properties.79
6.1.2 Variability of methane oxidation rate.81
6.1.3 Influence of soil properties on spatial patterns of gas concentration and
methane oxidation rate.82
6.2 Field trial I: Methane oxidation windows on an old landfill (landfill K).86
6.2.1 Construction of the windows and initial soil properties.86
6.2.2 Soil properties three years after construction.88
6.2.3 Gas transport parameters.95
6.2.4 Horizontal gas distribution at the window base and at the surface.99
6.2.5 Vertical stratification of aeration and the methane oxidation process.104
6.2.6 Methane load to the windows, oxidation efficiency, and emission.106
6.2.7 Change in relationship between methane load, oxidation and emission_108
6.2.8 Greenhouse gas balance and emission avoidance.Ill
6.3 Field trial II: Gas fluxes in a methane oxidation cover optimized for methane
oxidation and water infiltration control (Wieringermeer landfill).113
6.3.1 Soil properties.113
6.3.2 Exclusion of cell G from the considerations on methane oxidation.118
6.3.3 Emission variability due to environmental factors.119
6.3.4 Oxidation efficiency and carbon balance.121
6.3.5 Spatial gas flux patterns.122
6.4 Analysis of the chamber measurement methodology and the emission
monitoring strategy.125
6.4.1 Impact of the chamber measurement itself on the measured fluxes.125
6.4.2 Large emission chamber: Corrections to the emission data.126
6.4.3 Relationship between emission and surface concentration.129
6.4.4 Emission extrapolation from conventionally sized chambers.131
6.5 Laboratory study on the quantification of the share of respirative carbon
dioxide during methane oxidation by means of 13C labeled methane.135
7 Discussion.139
7.1 Driving factors of methane oxidation.139
7.1.1 Variability of methane oxidation rate.139
7.1.2 Influence of soil properties on spatial patterns of gas concentration and
methane oxidation rate.140
7.2 Performance of the methane oxidation windows.143
7.2.1 Conspicuous soil properties of two windows.143
7.2.2 Gas transport parameters.144
7.2.3 Horizontal gas distribution at the window base and at the surface.147
7.2.4 Vertical stratification of aeration and the methane oxidation process.148
7.2.5 Methane oxidation, load to the windows, and emission.150
7.2.6 Change in relationship between methane load, oxidation and emission.152
7.2.7 Greenhouse gas balance and emission avoidance.153
7.3 Performance of the methane oxidation cover.153
7.3.1 Methane oxidation cover properties.153
7.3.2 Oxidation efficiency and carbon balance.154
7.3.3 Spatial gas flux patterns.156
7.3.4 Steps in the design of a methane oxidation cover with capillary barrier.157
7.4 Chamber measurement methodology and emission monitoring strategy.159
7.4.1 Large emission chamber: evaluation.159
7.4.2 Predicting emissions.161
7.4.3 Impact of the chamber measurement itself on the measured fluxes.164
7.5 Quantification of the share of respirative carbon dioxide during methane
oxidation by means of 13C labeled methane.164
8 Conclusions and implications.167
8.1 Driving factors of methane oxidation rate.167
8.2 Performance of the methane oxidation windows.168
8.3 Performance of the methane oxidation cover.170
8.4 Chamber measurement methodology and the emission monitoring strategy .172
8.5 Quantification of the share of respirative carbon dioxide during methane
oxidation by means of 13C labeled methane.173
List of publications.175
Publications.175
Selection of conference proceedings.175
References.177 |
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| spelling | Röwer, Inga Ute Verfasser aut Reduction of methane emissions from landfills processes, measures and monitoring strategies Inga Ute Röwer Hamburg Verein zur Förderung der Bodenkunde in Hamburg 2014 191 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Hamburger bodenkundliche Arbeiten 75 Zugl.: Hamburg, Univ., FB Geowiss., Diss., 2014 Emission (DE-588)4014573-6 gnd rswk-swf Deponie (DE-588)4070300-9 gnd rswk-swf Deponiegas (DE-588)4194273-5 gnd rswk-swf Methan (DE-588)4169678-5 gnd rswk-swf Abfall (DE-588)4000098-9 gnd rswk-swf Methanemission (DE-588)4286529-3 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Abfall (DE-588)4000098-9 s Deponie (DE-588)4070300-9 s Emission (DE-588)4014573-6 s Methanemission (DE-588)4286529-3 s DE-604 Deponiegas (DE-588)4194273-5 s Methan (DE-588)4169678-5 s Hamburger bodenkundliche Arbeiten 75 (DE-604)BV000019547 75 HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027652309&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Röwer, Inga Ute Reduction of methane emissions from landfills processes, measures and monitoring strategies Hamburger bodenkundliche Arbeiten Emission (DE-588)4014573-6 gnd Deponie (DE-588)4070300-9 gnd Deponiegas (DE-588)4194273-5 gnd Methan (DE-588)4169678-5 gnd Abfall (DE-588)4000098-9 gnd Methanemission (DE-588)4286529-3 gnd |
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| title | Reduction of methane emissions from landfills processes, measures and monitoring strategies |
| title_auth | Reduction of methane emissions from landfills processes, measures and monitoring strategies |
| title_exact_search | Reduction of methane emissions from landfills processes, measures and monitoring strategies |
| title_full | Reduction of methane emissions from landfills processes, measures and monitoring strategies Inga Ute Röwer |
| title_fullStr | Reduction of methane emissions from landfills processes, measures and monitoring strategies Inga Ute Röwer |
| title_full_unstemmed | Reduction of methane emissions from landfills processes, measures and monitoring strategies Inga Ute Röwer |
| title_short | Reduction of methane emissions from landfills |
| title_sort | reduction of methane emissions from landfills processes measures and monitoring strategies |
| title_sub | processes, measures and monitoring strategies |
| topic | Emission (DE-588)4014573-6 gnd Deponie (DE-588)4070300-9 gnd Deponiegas (DE-588)4194273-5 gnd Methan (DE-588)4169678-5 gnd Abfall (DE-588)4000098-9 gnd Methanemission (DE-588)4286529-3 gnd |
| topic_facet | Emission Deponie Deponiegas Methan Abfall Methanemission Hochschulschrift |
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