Selectivity in the Synthesis of Cyclic Sulfonamides: Application in the Synthesis of Natural Products
Gespeichert in:
| 1. Verfasser: | |
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| Format: | Abschlussarbeit Elektronisch E-Book |
| Sprache: | English |
| Veröffentlicht: |
Cham [u.a.]
Springer
2014
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| Schriftenreihe: | Springer Theses
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| Schlagworte: | |
| Online-Zugang: | UBT01 Volltext Inhaltsverzeichnis Abstract |
| Beschreibung: | 1 Online-Ressource |
| ISBN: | 9783319103389 |
| DOI: | 10.1007/978-3-319-10338-9 |
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Datensatz im Suchindex
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| adam_text | SELECTIVITY IN THE SYNTHESIS OF CYCLIC SULFONAMIDES
/ GEOGHEGAN, KIMBERLY
: 2014
TABLE OF CONTENTS / INHALTSVERZEICHNIS
INTRODUCTION
REGIOSELECTIVITY IN THE HECK (MIZOROKI-HECK) REACTION
WAGNER-MEERWEIN REARRANGEMENT OF CYCLIC SULFONAMIDES
AN INVESTIGATION INTO THE ONE-POT HECK OLEFINATION-HYDROGENATION
REACTION
DOUBLE REDUCTION OF CYCLIC AROMATIC SULFONAMIDES
EXPERIMENTAL
DIESES SCHRIFTSTUECK WURDE MASCHINELL ERZEUGT.
SELECTIVITY IN THE SYNTHESIS OF CYCLIC SULFONAMIDES
/ GEOGHEGAN, KIMBERLY
: 2014
ABSTRACT / INHALTSTEXT
IN THE AREA OF ORGANIC CHEMISTRY ONE MAJOR CHALLENGE WE ARE CURRENTLY
FACED WITH IS HOW TO ASSEMBLE POTENTIALLY USEFUL MOLECULES IN NEW WAYS
THAT GENERATE MOLECULAR COMPLEXITY AND IN SEQUENCES THAT ARE AS
EFFICIENT AS POSSIBLE. OUR EFFORTS IN THIS REGARD, SPECIFICALLY FOR THE
PREPARATION OF AMINO CONTAINING COMPOUNDS INCORPORATING AN AROMATIC
RING, ARE DESCRIBED IN THIS DOCTORAL THESIS. WE DISCOVERED AN
INTERESTING REGIOSELECTIVITY IN AN INTRAMOLECULAR HECK REACTION, WHICH
WE STUDIED FOR A SERIES OF SUBSTRATES THAT ARE UNBIASED IN TERMS OF THE
SIZE OF THE NEWLY FORMED RING, WHERE VERY HIGH LEVELS OF SELECTIVITY IN
RELATION TO THE NEW CARBON-CARBON BOND ARE TYPICALLY OBSERVED. DFT
CALCULATIONS WERE PERFORMED TO ATTEMPT TO SHED LIGHT ON THE REACTION
SEQUENCE. THIS REGIOSELECTIVE HECK REACTION, COMBINED WITH THE REDUCTIVE
REMOVAL OF THE TEMPORARY AMINO-PROTECTING GROUP, ALLOWED US TO
SYNTHESIZE THE SCELETIUM ALKALOIDS: MESEMBRANE, MESEMBRANOL AND
MESEMBRINE
DIESES SCHRIFTSTUECK WURDE MASCHINELL ERZEUGT.
|
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| spelling | Geoghegan, Kimberly Verfasser aut Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products Kimberly Geoghegan Cham [u.a.] Springer 2014 1 Online-Ressource txt rdacontent c rdamedia cr rdacarrier Springer Theses Zugl.: Dublin, University College, Diss. Chemie Chemistry Chemistry, Organic Catalysis (DE-588)4113937-9 Hochschulschrift gnd-content Erscheint auch als Druckausgabe 978-3-319-10337-2 https://doi.org/10.1007/978-3-319-10338-9 Verlag Volltext Springer Fremddatenuebernahme application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027498943&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Springer Fremddatenuebernahme application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027498943&sequence=000003&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Abstract |
| spellingShingle | Geoghegan, Kimberly Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products Chemie Chemistry Chemistry, Organic Catalysis |
| subject_GND | (DE-588)4113937-9 |
| title | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products |
| title_auth | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products |
| title_exact_search | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products |
| title_full | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products Kimberly Geoghegan |
| title_fullStr | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products Kimberly Geoghegan |
| title_full_unstemmed | Selectivity in the Synthesis of Cyclic Sulfonamides Application in the Synthesis of Natural Products Kimberly Geoghegan |
| title_short | Selectivity in the Synthesis of Cyclic Sulfonamides |
| title_sort | selectivity in the synthesis of cyclic sulfonamides application in the synthesis of natural products |
| title_sub | Application in the Synthesis of Natural Products |
| topic | Chemie Chemistry Chemistry, Organic Catalysis |
| topic_facet | Chemie Chemistry Chemistry, Organic Catalysis Hochschulschrift |
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