Molecular water oxidation catalysis: a key topic for new sustainable energy conversion schemes
Gespeichert in:
| Weitere Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Chichester [u.a.]
Wiley
2014
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis Klappentext |
| Beschreibung: | Includes bibliographical references and index Weitere Ausgabe: Online version : Molecular water oxidation catalysis |
| Beschreibung: | XIII, 265 S. Ill., graph. Darst. |
| ISBN: | 9781118413371 9781118698624 |
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| 300 | |a XIII, 265 S. |b Ill., graph. Darst. | ||
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Datensatz im Suchindex
| _version_ | 1804152291916251136 |
|---|---|
| adam_text | Contents
Fl·
List of Contributors
xi
Preface
xv
1.
Structural Studies of Oxomanganese Complexes for
Water Oxidation Catalysis
1
Ivan
Rivolta,
Gary W. Brudvig, and Victor S. Batista
1.1
Introduction
1
1.2
Structural Studies of the OEC
2
1.3
The Dark-Stable State of the OEC
4
1.4
В
iomimetic Oxomanganese Complexes
6
1.5
Base-Assisted
О
-O
Bond Formation
7
1.6
Biomimetic Mn Catalysts for Artificial Photosynthesis
8
1.7
Conclusion
11
Acknowledgments
12
References
12
2.
О
-O
Bond Formation by
a Heme
Protein: The Unexpected
Efficiency of Chlorite Dismutase
15
Jennifer L. DuBois
2.1
Introduction
15
2.2
Origins of 02-EvoIving Chlorite Dismutases (Clds)
15
2.3
Major Structural Features of the Proteins and their Active Sites
16
2.4
Efficiency, Specificity, and Stability
20
2.5
Mechanistic Insights from Surrogate Reactions with Peracids and
Peroxide
22
2.6
Possible Mechanisms
23
2.7
Conclusion
25
Acknowledgements
25
References
25
3.
Ru-Based Water Oxidation Catalysts
29
Laia Francas,
Roger Bofill, Jordi
García-Antón,
Lluis Escriche,
Xavier
Sala
and
Antoni
Höbet
3.
1 Introduction
29
3.2
Proton-Coupled Electron Transfer (PCET)
and Water Oxidation
Thermodynamics
3
1
vi
Contents
3.3
O-O
Bond Formation Mechanisms
33
3.4
Polynuclear Ru Water Oxidation Catalysts
34
3.5
Mononuclear Ru WOCs
40
3.6
Anchored Molecular Ru WOCs
42
3.7
Light-Induced Ru WOCs
43
3.8
Conclusion
45
Acknowledgments
46
References
46
4.
Towards the Visible Light-Driven Water Splitting Device: Ruthenium
Water Oxidation Catalysts with Carboxy late-Containing Ligands
51
Lele
Duan,
Lianpeng
Tong,
and Licheng Sun
4.1
Introduction
51
4.2
Binuclear Ru Complexes
52
4.3
Mononuclear Ru Complexes
54
4.3.1
Ru-O2N-N3 Analogs
55
4.3.2
RU-O2N2-N2 Analogs
57
4.4
Homogeneous Light-Driven Water Oxidation
68
4.4.1
The Three-Component System
68
4.4.2
The Supramolecular Assembly Approach
69
4.5
Water Oxidation Device
72
4.5.1
Electrochemical Water Oxidation Anode
72
4.5.2
Photo-Anode for Water Oxidation
74
4.6
Conclusion
75
References
75
5.
Water Oxidation by Ruthenium Catalysts with Non-Innocent Ligands
77
Tohru
Wada, Koji
Тапака,
James
T.
Muckerman, and Etsuko Fujita
5.1
Introduction
77
5.2
Water Oxidation Catalyzed by Dinuclear Ruthenium Complexes with
NILs
81
5.3
Water Oxidation by Intramolecular
О
-O
Coupling with
[Ru£(//-Ci)(bpy)2(btpyan)]3+
85
5.4
Mononuclear Ru-Aqua Complexes with a Dioxolene Ligand
91
5.4.1
Structural Characterization
91
5.4.2
Theoretical and Electrochemical Characterization
96
5.5
Mechanistic Investigation of Water Oxidation by Dinuclear Ru
Complexes with NILs: Characterization of Key Intermediates
101
References
107
6.
Recent Advances in the Field of
Iridium-Catalyzed
Molecular
Water Oxidation
113
James A. Woods, Stefan
Bernhard,
and Martin
Albrecht
6.1
introduction
113
6.2
Bernhard
2008 [ 111 114
6.3
Crabtree
2009
6.4
Crabtree
2010
6.5
Macchioni
2010
6.6
Albrecht/Bernhard 2010
6.7
Hetterscheid/Reek 2011
6.8
Crabtree 2011
6.9
Crabtree 2011
6.10
Lin
2011
6.11
Macchioni
2011
6.12
Grotjahn
2011
6.13
Fukuzumi
2011
6.14
Lin
2012
6.15
Crabtree
2012
6.16
Albrecht/Bernhard 2012
6.17
Crabtree
2012
6.18
Beller
2012
6.19
Lin
2012
6.20
Lloblet and
Macchioni
2012
6.21
Analysis
Contents
vii
115
116
117
117
118
119
120
120
122
123
123
124
125
125
126
127
128
129
130
References
131
7.
Complexes
of
First
Row
d-Block Metals:
Manganese
135
Philipp
Kurz
7.1
Background
135
7.2
Oxidation States of Manganese in an Aqueous Environment
137
7.3
Dinuclear Manganese Complexes: Syntheses and Structures
138
7.4
Redox
and Acid-Base Chemistry of Mn2-^-WDL Systems
139
7.5
Mn2 Systems: Oxygen Evolution (but not Water Oxidation) Catalysis
142
7.6
Mn2 Complexes/the
OEC/Ru2
Catalysts: A Comparison
144
7.7
Heterogeneous Water Oxidation Catalysis by Mn>2 Systems
146
7.8
Conclusion
148
Acknowledgements
148
References
149
8.
Molecular Water Oxidation Catalysts from Iron
153
W. Chadwick Ellis, Neal D. McDaniel, and Stefan
Bernhard
8.1
Introduction
153
8.2
Fe-Tetrasulfophthalocyanine
154
8.3
Fe-TAML
155
8.4
Fe-mcp
157
8.5
Fe2O3 as a Microheterogeneous Catalyst
158
8.6
Conclusion
160
References
í
61
viii Contents
9.
Water Oxidation by Co-Based Oxides with Molecular Properties
163
Marcel Risch,
Katharina
Klingan,
¡velina
Zaharieva, and
Holger
Dau
9.1
Introduction
163
9.2
CoCat Formation
164
9.3
Structure and Structure-Function Relations
166
9.4
Functional Characterization
173
9.5
Directly Light-Driven Water Oxidation
175
References
180
10.
Developing Molecular Copper Complexes for Water Oxidation
187
Shoshanna M. Barnett, Christopher R.
Waidmann,
Margaret L.
Scheuermann,
Jared C. Nesvet, Karen Goldberg and James M. Mayer
10.1
Introduction
187
10.2
A Biomimetic Approach
188
10.2.1
Thermochemistry: Developing Oxidant/Base Combinations as
PCET Reagents
189
10.2.2
Copper Complexes with Alkylamine Ligands
190
10.2.3
Copper Complexes with
Anionie
Ligands
195
10.2.4
Lessons Learned: Thermochemical Insights and Oxidant/Base
Compatibility
198
10.3
An Aqueous System: Electrocatalysis with (bpy)Cu(II) Complexes
198
10.3.1
System Selection: bpy
+
Cu
199
10.3.2
Observing Electrocatalysis
199
10.3.3
Catalyst Turnover Number and Turnover Frequency
201
10.3.4
Catalyst Speciation: Monomer, Dimer, or Nanoparticles?
203
10.4
Conclusion
206
Acknowledgement
206
References
207
11.
Polyoxometalate Water Oxidation Catalytic Systems
211
Jordan M. Sumliner, James W. Vickers, Hongjin
Lv,
Yurii V. Geletii, and
Craig
L
Hill
11.1
Introduction
211
11.2
Recent POM WOCs
214
11.3
Assessing POM WOC Reactivity
220
11.4
The Ru(bpy)32+/S2O82-System
221
11.5
Ru(bpy)33+ as an
Oxidant
for POM WOCs
222
11.6
Additional Aspects of WOC System Stability
224
11.7
Techniques for Assessing POM WOC Stability
224
11.8
Conclusion
227
Acknowledgments
228
References
228
Contents ix
12. Quantum Chemical
Characterization of Water Oxidation Catalysts
233
Pere
Miró,
Mehmed
Z.
Ertem, Laura
Gagliardi,
and Christopher J. Cramer
12.1
Introduction
233
12.2
Computational Details
235
12.2.1
Density Functional Theory Calculations
235
12.2.2
Multiconfigurational Calculations
236
12.3
Methodology
237
12.3.1
Solvation and Standard Reduction Potentials
237
12.3.2
Multideterminantal State Energies
238
12.4
Water Oxidation Catalysts
238
12.4.1
Ruthenium-Based Catalysts
238
12.4.2
Cobalt-Based Catalysts
245
12.4.3
Iron-Based Catalysts
248
12.5
Conclusion
251
References
252
Index
257
MOLECULAR
WATER
OXIDATION
CATALYSIS
A Key Topic for New Sustainable
Energy Conversion Schemes
Photocatalytic water splitting is a promising strategy for capturing energy
from the sun by coupling light harvesting and the oxidation of water, in order
to create clean hydrogen fuel. Thus a deep knowledge of the water oxidation
catalysis field is essential to be able to come up with useful energy conversion
devices based on sunlight and water splitting.
Molecular Water Oxidation Catalysis: A Key Topic for New Sustainable Energy
Conversion Schemes presents a comprehensive and state-of-the-art overview
of water oxidation catalysis in homogeneous phase, describing in detail the
most important catalysts discovered today based on first- and second-row
transition metals. A strong emphasis is placed on their performance as well
as how they work from a mechaflistic perspective. In addition, a theoretical
description of some of the most relevant catalysts based on DFT is presented,
as well as a description of related natural systems, such as the oxygen evolving
system of photosystem II and the
heme
chlorite-dismutase.
This book is a valuable resource for researchers working on water oxidation
catalysis, solar energy conversion and artificial photosynthesis, as well as for
chemists and materials scientists with a broad interest in new sustainable
energy conversion schemes.
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| publisher | Wiley |
| record_format | marc |
| spelling | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes ed., Antoni Llobet Chichester [u.a.] Wiley 2014 XIII, 265 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Includes bibliographical references and index Weitere Ausgabe: Online version : Molecular water oxidation catalysis Katalytische Oxidation (DE-588)4163425-1 gnd rswk-swf Wasser (DE-588)4064689-0 gnd rswk-swf Energy Harvesting (DE-588)7664612-9 gnd rswk-swf Erneuerbare Energien (DE-588)4068598-6 gnd rswk-swf Katalyse (DE-588)4029921-1 gnd rswk-swf Oxidation (DE-588)4137187-2 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Wasser (DE-588)4064689-0 s Katalytische Oxidation (DE-588)4163425-1 s Energy Harvesting (DE-588)7664612-9 s Erneuerbare Energien (DE-588)4068598-6 s DE-604 Oxidation (DE-588)4137187-2 s Katalyse (DE-588)4029921-1 s 1\p DE-604 Llobet, Antoni 1960- (DE-588)1054344736 edt Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027365806&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027365806&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes Katalytische Oxidation (DE-588)4163425-1 gnd Wasser (DE-588)4064689-0 gnd Energy Harvesting (DE-588)7664612-9 gnd Erneuerbare Energien (DE-588)4068598-6 gnd Katalyse (DE-588)4029921-1 gnd Oxidation (DE-588)4137187-2 gnd |
| subject_GND | (DE-588)4163425-1 (DE-588)4064689-0 (DE-588)7664612-9 (DE-588)4068598-6 (DE-588)4029921-1 (DE-588)4137187-2 (DE-588)4143413-4 |
| title | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes |
| title_auth | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes |
| title_exact_search | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes |
| title_full | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes ed., Antoni Llobet |
| title_fullStr | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes ed., Antoni Llobet |
| title_full_unstemmed | Molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes ed., Antoni Llobet |
| title_short | Molecular water oxidation catalysis |
| title_sort | molecular water oxidation catalysis a key topic for new sustainable energy conversion schemes |
| title_sub | a key topic for new sustainable energy conversion schemes |
| topic | Katalytische Oxidation (DE-588)4163425-1 gnd Wasser (DE-588)4064689-0 gnd Energy Harvesting (DE-588)7664612-9 gnd Erneuerbare Energien (DE-588)4068598-6 gnd Katalyse (DE-588)4029921-1 gnd Oxidation (DE-588)4137187-2 gnd |
| topic_facet | Katalytische Oxidation Wasser Energy Harvesting Erneuerbare Energien Katalyse Oxidation Aufsatzsammlung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027365806&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027365806&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT llobetantoni molecularwateroxidationcatalysisakeytopicfornewsustainableenergyconversionschemes |