Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process:
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| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
2014
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| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XXI, 146 S. Ill., graph. Darst. |
Internformat
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Datensatz im Suchindex
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| adam_text | CONTENTS
LIST OF FIGURES XI
LIST OF TABLES XV
LIST OF SYMBOLS AND ABBREVIATIONS XVII
CHAPTER 1 INTRODUCTION 1
1.1 OXIDATIVE COUPLING OF METHANE 3
1.2 TECHNOLOGIES OF CO2 CAPTURE 7
1.2.1 PHYSICAL ABSORPTION PROCESS 7
1.2.2 CHEMICAL ABSORPTION PROCESS 9
1.2.3 ADSORPTION PROCESS 11
1.2.4 MEMBRANE PROCESS 13
1.3 MOTIVATION AND MAIN TASK IN THIS WORK 15
1.3.1 MOTIVATION OF THIS WORK 15
1.3.2 MAIN RESEARCH WORKS 17
CHAPTER 2 MEMBRANE-BASED GAS SEPARATION
TECHNOLOGY IN OCM PROCESS 19
2.1 DEVELOPMENT OF MEMBRANE SEPARATION 19
2.2 CLASSIFICATION OF MEMBRANE 20
2.3 GAS SEPARATION 22
2.3.1 FUNDAMENTALS OF GAS SEPARATION 22
2.3.2 MECHANISMS OF GAS SEPARATION 23
2.3.3 DRIVING FORCE OF GAS PERMEATION 25
2.3.4 INHERENT PROPERTY OF DENSE MEMBRANE: PERMEABILITY 27
2.3.5 INDICATOR OF SEPARATION PERFORMANCE 29
2.3.6 STRUCTURES OF MEMBRANE MODULES 29
2.3.7 APPLICATIONS OF MEMBRANE-BASE GAS SEPARATION 32
2.4 MEMBRANE-BASED CO2 REMOVAL TECHNOLOGY 34
2.4.1 MEMBRANES FOR CO2 SEPARATION 34
HTTP://D-NB.INFO/1050942655
2.4.2 MEMBRANE MODULES IN OCM MINI-PLANT 36
CHAPTER 3 SIMULATIVE INVESTIGATION OF MEMBRANE-
BASED GAS SEPARATION FOR COZ REMOVAL IN
OCM MINI-PLANT 39
3.1 DESCRIPTION OF MODELLED MEMBRANE MODULE 40
3.2 MODELLING OF GAS PERMEATION PROCESS IN OCM MINI-PLANT 41
3.2.1 PERMEATION FLUX IN DENSE MEMBRANE 42
3.2.2 OVERALL PERMEANCE OF MEMBRANE 44
3.2.3 GOVERNING EQUATIONS OF PERMEATION PROCESS 47
3.2.4 MODELLING OF STANDARD MEMBRANE MODULE IN OCM MINI-PLANT 49
3.2.4.1 GAS PERMEATION MODEL FOR MEMBRANE MODULE IN OCM MINI-
PLANT 49
3.2.4.2 ASPEN CUSTOM MODELER FOR PROGRAMMING 51
3.3
SIMULATIONS OF
MEMBRANE-BASED
CO2
REMOVAL
IN OCM
PROCESS 52
3.3.1 INDEPENDENCE OF DISCRETIZATION 53
3.3.2 ORIGINAL SCHEME: SINGLE MEMBRANE MODULE 54
3.3.2.1 VERIFICATION OF MATHEMATICAL MODEL 55
3.3.2.2 INFLUENCE OF OPERATIONAL PRESSURE 58
3.3.2.3 INFLUENCE OF OPERATIONAL FEED FLOW RATE 60
3.3.2.4 SEPARATION PERFORMANCE LIMITATION OF SINGLE MODULE 62
3.3.2.5 SUMMARY 63
3.3.3 INVESTIGATION OF MULTI-STEP MEMBRANE CASCADE FOR CO2 REMOVAL
64
3.3.3.1 DESIGN OF EFFECTIVE AREA FOR PEO MODULE 66
3.3.3.2 DESCRIPTION OF THREE TYPES OF MULTI-STEP MEMBRANE CASCADES
68
3.3.3.3 ANALYSIS OF RESULTS 70
3.3.3.4 SUMMARY 72
3.3.4 IMPROVED SCHEME: PI-PEO MEMBRANE CASCADE IN OCM MINI-
PLANT 72
3.3.4.1 INFLUENCE OF OPERATING CONDITIONS 72
3.3.4.2 COMPARISON OF SEPARATION FOR DIFFERENT CO2 COMPOSITIONS IN
FEED STREAM 76
3.3.4.3 IMPROVEMENT OF PI-PEO CASCADE IN COMPARISON WITH SINGLE
PI MODULE 77
3.4 CONCLUSIONS
79
CHAPTER 4 EXPERIMENTAL INVESTIGATION OF C0
2
REMOVAL
VIA MEMBRANE SYSTEM IN OCM MINI-PLANT 81
4.1 DESCRIPTION OF PREVIOUS MEMBRANE SYSTEM IN OCM MINI-PLANT 82
4.2 DESIGN OF PI-PEO MEMBRANE CASCADE IN OCM MINI-PLANT 83
4.2.1 SCHEMATIC DIAGRAM OF MEMBRANE CASCADE 83
4.2.2 REQUIRED EQUIPMENTS AND DEVICES 86
4.3 CONTROL SYSTEM 89
4.4 PRESSURE AND TIGHTNESS TEST 91
4.5 EXPERIMENT OPERATION 92
4.6 EXPERIMENTS OF STAND-ALONE PEO MODULE 93
4.7 EXPERIMENTS OF PI-PEO MEMBRANE CASCADE 95
4.8 SUMMARY 97
CHAPTER 5 EVALUATION OF MEMBRANE CASCADE FOR
ASSIST-REMOVAL OF C0
2
IN OCM PROCESS 99
5.1 ENERGETIC EVALUATION OF MEMBRANE CASCADE IN OCM MINI-PLANT 99
5.1.1 PREVIOUS EXPERIMENTAL STUDY OF ENERGY IN OCM MINI-PLANT 100
5.1.2 EVALUATION OF BENEFITS FROM MEMBRANE CASCADE 101
5.2 PRELIMINARY ECONOMIC ANALYSIS OF MEMBRANE CASCADE IN OCM PLANT
ON LARGE SCALE 104
5.3 SUMMARY 107
CHAPTER 6 CONCLUSIONS AND FUTURE WORKS 109
6.1 CONCLUSIONS 110
6.1.1 GAS PERMEATION MODEL FOR FLAT-SHEET ENVELOPE MEMBRANE
MODULE 111
6.1.2 C0
2
REMOVAL USING MEMBRANE MODULE 111
6.1.3 ADVANTAGES OF HYBRID PROCESS FOR CO2 REMOVAL IN OCM PROCESS
112
6.2 OUTLOOK TO FUTURE WORKS 112
REFERENCES 115
APPENDIX A SIMULATION RESULTS OF MEMBRANE SYSTEM IN
OCM MINI-PLANT 125
A.1 SIMULATION OF STAND-ALONE PI MEMBRANE MODULE FOR CO2 REMOVAL 126
A.2 SIMULATION OF PI-PI MEMBRANE CASCADE FOR CO2 REMOVAL 128
A.3 SIMULATION OF PI-PEO MEMBRANE CASCADE FOR CO2 REMOVAL 130
A.4 SIMULATION OF PI-PI-PI MEMBRANE CASCADE FOR CO2
REMOVAL 132
APPENDIX B EQUATION OF STATE AND MIXING RULE 135
B.1 STANDARD PENG-ROBINSON EQUATION OF STATE 135
B.2 FUGACITY COEFFICIENT CALCULATED BY EQUATION OF STATE 135
B.3 CHAPMAN-ENSKOG-BROKAW-WIKE MIXING RULE FOR VAPOR VISCOSITY 136
APPENDIX C CALIBRATION OF MASS FLOW METER FR-3 IN
FIGURE 4.2 139
APPENDIX D PARAMETERS IN EQUATION (3-8) 141
APPENDIX E DETAILS OF EQUATION (3-19)
143
|
| any_adam_object | 1 |
| author | Song, Shankui |
| author_GND | (DE-588)1049348737 |
| author_facet | Song, Shankui |
| author_role | aut |
| author_sort | Song, Shankui |
| author_variant | s s ss |
| building | Verbundindex |
| bvnumber | BV041764647 |
| classification_rvk | VN 7190 |
| ctrlnum | (OCoLC)931516457 (DE-599)BVBBV041764647 |
| dewey-full | 661.814 |
| dewey-hundreds | 600 - Technology (Applied sciences) |
| dewey-ones | 661 - Technology of industrial chemicals |
| dewey-raw | 661.814 |
| dewey-search | 661.814 |
| dewey-sort | 3661.814 |
| dewey-tens | 660 - Chemical engineering |
| discipline | Chemie / Pharmazie |
| format | Thesis Book |
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| language | English |
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| spelling | Song, Shankui Verfasser (DE-588)1049348737 aut Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process vorgelegt von Shankui Song Simulation, experiment, and evaluation of membrane-based CO 2 gas separation in the downstream of oxidative coupling of methane process 2014 XXI, 146 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Berlin, Techn. Univ., Diss., 2014 Gastrennung (DE-588)4156082-6 gnd rswk-swf Membranverfahren (DE-588)4231727-7 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Gastrennung (DE-588)4156082-6 s Membranverfahren (DE-588)4231727-7 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027210769&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Song, Shankui Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process Gastrennung (DE-588)4156082-6 gnd Membranverfahren (DE-588)4231727-7 gnd |
| subject_GND | (DE-588)4156082-6 (DE-588)4231727-7 (DE-588)4113937-9 |
| title | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process |
| title_alt | Simulation, experiment, and evaluation of membrane-based CO 2 gas separation in the downstream of oxidative coupling of methane process |
| title_auth | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process |
| title_exact_search | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process |
| title_full | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process vorgelegt von Shankui Song |
| title_fullStr | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process vorgelegt von Shankui Song |
| title_full_unstemmed | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process vorgelegt von Shankui Song |
| title_short | Simulation, experiment, and evaluation of membrane based CO 2 gas separation in the downstream of oxidative coupling of methane process |
| title_sort | simulation experiment and evaluation of membrane based co 2 gas separation in the downstream of oxidative coupling of methane process |
| topic | Gastrennung (DE-588)4156082-6 gnd Membranverfahren (DE-588)4231727-7 gnd |
| topic_facet | Gastrennung Membranverfahren Hochschulschrift |
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