Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Karlsruhe
KIT Scientific Publ.
2012
|
| Schriftenreihe: | Karlsruher mineralogische und geochemische Hefte
38 |
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XIII, 263 S. Ill., graph. Darst., Kt. |
| ISBN: | 9783866448278 3866448279 |
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CONTENTS
ACKNOWLEDGEMENTS I
ABSTRACT VII
ZUSAMMENFASSUNG XI
1 AIRBORNE PARTICULATE MATTER 1
1.1 BASIC PRINCIPLES AND DEFINITIONS 1
1.2 AIR POLLUTION IN A HISTORICAL PERSPECTIVE 4
1.3 IMPACTS ON HUMAN HEALTH AND THE ENVIRONMENT 4
1.3.1 HEALTH IMPACTS 4
1.3.2 ENVIRONMENTAL IMPACTS 8
1.4 URBAN AIR QUALITY STUDIES 9
1.5 SCOPE OF THE PRESENT WORK 10
2 STUDY AREA 13
2.1 BEIJING AND ITS SURROUNDINGS 13
2.2 METEOROLOGY 14
2.3 REGIONAL GEOLOGY 18
3 METHODOLOGY 19
3.1 SAMPLING SITES AND SAMPLING PROCEDURE 19
3.1.1 LOCATION AND DESCRIPTION OF THE SAMPLING SITES 19
3.1.2 ACTIVE SAMPLING 19
3.1.3 PASSIVE SAMPLING 22
3.2 CHEMICAL-PHYSICAL ANALYSES 23
3.2.1 GRAVIMETRIC ANALYSIS 23
3.2.2 ACID DIGESTION 23
HTTP://D-NB.INFO/102158424X
IV
CONTENTS
3.2.3 WATER-SOLUBLE IONS 23
3.2.4 SEQUENTIAL EXTRACTION PROCEDURE 24
3.2.5 OPTICAL OIL-IMMERSION TECHNIQUE FOR BC 25
3.2.6 QUANTITATIVE OPTICAL MICROSCOPY 26
3.2.7 SCANNING ELECTRON MICROSCOPY 27
3.2.8 SYNCHROTRON RADIATION BASED /X-XRF ANALYSES 27
3.3 STATISTICAL METHODS 28
3.3.1 DESCRIPTIVE STATISTICS 28
3.3.2 Z-TRANSFORMATION 28
3.3.3 FACTOR ANALYSIS 28
3.4 ENRICHMENT FACTORS 29
4 SPATIO-TEMPORAL VARIABILITY 31
4.1 INTRODUCTION 31
4.2 RESULTS FROM LONG-TERM WEEKLY SAMPLING 32
4.2.1 ENRICHMENT FACTORS 32
4.2.2 MASS AND ELEMENT CONCENTRATIONS 34
4.2.3 WATER-SOLUBLE IONS 39
4.2.4 BLACK CARBON 44
4.2.5 PASSIVELY SAMPLED ATMOSPHERIC PARTICLES 45
4.3 RESULTS FROM SHORT-TERM 24-HOURLY SAMPLING 48
4.3.1 MASS AND ELEMENT CONCENTRATIONS 48
4.3.2 BLACK CARBON 51
4.3.3 PASSIVELY SAMPLED ATMOSPHERIC PARTICLES 51
4.4 DISCUSSION 52
4.4.1 SPATIAL VARIATIONS 52
4.4.2 TEMPORAL VARIATIONS AND THE INFLUENCING FACTORS 56
4.4.3 ACIDITY 64
4.4.4 GEOGENIC
VERSUS
ANTHROPOGENIC PARTICLES 66
4.4.5 COMPARISON WITH OTHER CITIES 71
4.5 SUMMARY AND CONCLUSIONS 72
5 MOBILITY OF TRACE METALS 77
5.1 INTRODUCTION 77
5.2 RESULTS 79
5.2.1 MASS CONCENTRATIONS 79
5.2.2 ELEMENT CONCENTRATIONS IN THE FOUR DIFFERENT FRACTIONS . . 81
5.2.3 COMPARISON WITH RESULTS OF TOTAL DIGESTION 89
CONTENTS V
5.3 DISCUSSION 91
5.3.1 TEMPORAL VARIABILITY OF TRACE METAL MOBILITY 91
5.3.2 HEALTH IMPACT ASSESSMENT 95
5.3.3 COMPARISON WITH OTHER STUDIES 96
5.3.4 SOURCE APPORTIONMENT 99
5.4 SUMMARY AND CONCLUSIONS 115
6 OLYMPIC SUMMER GAMES 2008 117
6.1 INTRODUCTION 117
6.2 MITIGATION MEASURES 118
6.3 RESULTS 120
6.3.1 TOTAL SUSPENDED PARTICLES 120
6.3.2 PM2.5 AND PMJ 129
6.3.3 PASSIVELY SAMPLED ATMOSPHERIC PARTICULATE MATTER . 136
6.4 DISCUSSION 136
6.4.1 EVALUATION OF THE AMOUNT OF PARTICLE REDUCTION IN AUGUST
2008 136
6.4.2 EVALUATION OF THE INFLUENCE OF METEOROLOGICAL CONDITIONS
ON PARTICLE REDUCTION 141
6.4.3 EVALUATION OF THE SOURCES STILL CONTRIBUTING TO PARTICULATE
AIR POLLUTION DURING THE OLYMPIC GAMES 144
6.4.4 EVALUATION OF THE EFFECTIVENESS OF THE APPLIED MITIGATION
MEASURES 157
6.4.5 EVALUATION OF THE INCREASE OF PARTICULATE AIR POLLUTION AF
TER THE OLYMPIC GAMES 158
6.5 SUMMARY AND CONCLUSIONS 161
7 SINGLE ATMOSPHERIC PARTICLES 165
7.1 INTRODUCTION 165
7.2 RESULTS 167
7.2.1 SINGLE PARTICLES ANALYSED BY OPTICAL MICROSCOPY 167
7.2.2 SINGLE PARTICLES ANALYSED BY SEM-EDX 167
7.2.3 SINGLE PARTICLES ANALYSED BY |US-XRF 168
7.3 DISCUSSION 174
7.3.1 COARSE PARTICLES AS SCAVENGER FOR SMALLER TOXIC PARTICLES . 174
7.3.2 ACCELERATED STONE DECAY IN URBAN AREAS 177
7.4 SUMMARY AND CONCLUSIONS 179
VI CONTENTS
EXECUTIVE SUMMARY AND OUTLOOK 181
A TABLES CORRESPONDING TO CHAPTER 4 185
B TABLES CORRESPONDING TO CHAPTER 5 201
C TABLES CORRESPONDING TO CHAPTER 6 209
D TABLES CORRESPONDING TO CHAPTER 7 227
LIST OF FIGURES 229
LIST OF TABLES 239
REFERENCES 245 |
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| spellingShingle | Schleicher, Nina Jasmin Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing Karlsruher mineralogische und geochemische Hefte Geogener Faktor (DE-588)4372241-6 gnd Geochemische Analyse (DE-588)4290341-5 gnd Anthropogenes Aerosol (DE-588)4588624-6 gnd Luftverschmutzung (DE-588)4074381-0 gnd Sandsturm (DE-588)4179066-2 gnd |
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| title | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing |
| title_auth | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing |
| title_exact_search | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing |
| title_full | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing by Nina Jasmin Schleicher |
| title_fullStr | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing by Nina Jasmin Schleicher |
| title_full_unstemmed | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing by Nina Jasmin Schleicher |
| title_short | Chemical, physical and mineralogical properties of atmospheric particulate matter in the megacity Beijing |
| title_sort | chemical physical and mineralogical properties of atmospheric particulate matter in the megacity beijing |
| topic | Geogener Faktor (DE-588)4372241-6 gnd Geochemische Analyse (DE-588)4290341-5 gnd Anthropogenes Aerosol (DE-588)4588624-6 gnd Luftverschmutzung (DE-588)4074381-0 gnd Sandsturm (DE-588)4179066-2 gnd |
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