Colloidal quantum dot optoelectronics and photovoltaics:
"Capturing the most up-to-date research in colloidal quantum dot (CQD) devices, this book is written in an accessible style by the world's leading experts. The application of CQDs in solar cells, photodetectors and light-emitting diodes (LEDs) has developed rapidly over recent years, promi...
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Cambridge
Cambridge Univ. Press
2013
|
| Ausgabe: | 1. publ. |
| Schlagworte: | |
| Online-Zugang: | Cover Inhaltsverzeichnis |
| Zusammenfassung: | "Capturing the most up-to-date research in colloidal quantum dot (CQD) devices, this book is written in an accessible style by the world's leading experts. The application of CQDs in solar cells, photodetectors and light-emitting diodes (LEDs) has developed rapidly over recent years, promising to transform the future of clean energy, communications, and displays. This complete guide to the field provides researchers, students and practitioners alike with everything they need to understand these developments, and begin contributing to future applications. Introductory chapters summarise the fundamental physics and chemistry, whilst later chapters review the developments that have propelled the field forwards, systematically working through key device advances. The science of CQD films is explained through the latest physical models of semiconductor transport, trapping, and recombination, whilst the engineering of organic and inorganic multilayered materials is shown to have enabled major advances in the brightness and efficiency of CQD LEDs"-- |
| Beschreibung: | XIV, 314 S. Ill., graph. Darst. |
| ISBN: | 9780521198264 |
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Datensatz im Suchindex
| _version_ | 1818149202767642624 |
|---|---|
| adam_text |
Contents
List of contributors page
xi
Preface
xiii
Engineering colloidal quantum dots: synthesis, surface chemistry, and
self-assembly
1
Maryna I. Bodnarchuk and
Maksym
V. Kovalenko
1.1
Colloidal synthesis of inorganic nanocrystals and quantum dots
1
1.1.1
Introductory remarks
:
history and terminology
1
1.1.2
Basics of the surfactant-assisted colloidal synthesis of NC
quantum dots
2
1.2
Long-range ordered NC solids
7
1.2.1
Single-component NC superlattices
7
1.2.2
Multicomponent NC superlattices
9
1.2.3
Shape-directed self-assembly of NCs
13
1.3
Surface chemistry
-
a gateway to applications of NCs
16
1.3.1
Organic capping ligands
16
1.3.2
Complete removal of organic ligands and inorganic surface
functionalization
19
References
20
Aqueous based colloidal quantum dots for optoelectronics
30
Vladimir Lesnyak and Nikolai Gaponik
2.1
Introduction
30
2.2
Aqueous colloidal synthesis of semiconductor NCs
32
2.2.1
ZnXNCs
32
2.2.2
Alloyed ZnSe based NCs
34
2.2.3
CdXNCs
35
2.2.4
Core/shell CdTe based NCs
36
2.2.5
Alloyed CdTe based NCs
37
2.2.6
CdSe, CdSe/CdS NCs
39
2.2.7
HgXandPbXNCs
39
vi
Contents
2.2.7.1
HgXNCs
40
2.2.7.2
PbX NCs
40
2.3
Assemblies and functional
architectures
of
NCs
41
2.3.1
LbL
assembly technique
43
2.3.2
Assembly of NCs on micro-and nano-beads
46
2.3.3
Covalent coupling of NCs
47
2.3.4
Controllable aggregation
48
2.3.5
Nanowires and nanosheets
49
2.3.6
Nanocrystal based gels and aerogels
49
2.4
Conclusions and outlook
50
References
5
1
Electronic structure and optical transitions in colloidal
semiconductor nanocrystals
59
Todd D. Krauss and Jeffrey J. Peterson
3.1
Introduction
59
3.2
Foundational concepts
60
3.3
A simple model
65
3.4
Experimental evidence for quantum confinement
67
3.5
Engineered quantum dot structures
71
3.6
Advanced theoretical treatments
73
3.7
Atomistic approaches
76
3.8
Current challenges and future outlook
80
References
8
1
Charge and energy transfer in polymer/nanocrystal blends: physics and devices
87
Kevin M. Noone and David S. Ginger
4.1
Introduction
87
4.2
A brief history of QD/polymer optoelectronics
88
4.2.1
Quantum dot light emitting diodes (QD-LEDs)
-
size-tunable
emission across the spectrum
88
4.2.2
Quantum dot photovoltaics (QD-PV) and photodetectors
-
converting photons to electrons
90
4.2.2.1
QD-PVs
90
4.2.2.2
Quantum dot photodetectors
93
4.3
The QD-organic interface
-
ligands and more
96
4.3.1
Ligands
96
4.3.2
Energetics
98
4.3.2.1
Charge transfer and
Förster
resonance energy transfer
(FRET) in QD-LEDs
99
4.3.2.2
Type II heterojunctions and charge transfer in QD-PVs
99
4.4
Conclusion and future outlook
104
References
105
Contents
vii
Multiple
exciten
generation in semiconductor quantum dots and
electronically coupled quantum dot arrays for application to third-generation
photovoltaic solar cells
112
Matthew
С
Beard, Joey M. Luther, and Arthur J. Nozik
5.1
Introduction
112
5.2
Relaxation dynamics of photogenerated electron-hole pairs in QDs
115
5.2.1
Transient absorption spectroscopy
(ТА)
117
5.3
Multiple exciton generation (MEG)
121
5.3.1
MEG in QDs
121
5.3.2
MEG controversy and role of photocharging
125
5.3.3
MEG efficiency and comparison to impact ionization in bulk
semiconductors
128
5.4
QD solar cells
131
5.4.1
MEG photocurrent and determination of the internal quantum
efficiency (IQE) in QD solar cells
133
5.5
QD arrays
136
5.5.1
MEG in PbSe QD arrays
137
5.6
Conclusions
140
References
141
Colloidal quantum dot light emitting devices
148
Vanessa Wood, Matthew Panzer, Seth-Coe Sullivan, and Vladimir Bulovic
6.1
Introduction
148
6.2
Why QDs for
LEDs? 148
6.2.1
Saturated colors
148
6.2.2
Solution processable
150
6.2.3
Stability
150
6.3
QD and device physics influencing LED performance
151
6.3.1
Quantifying the luminescence efficiency
151
6.3.2
QD surface states
152
6.3.3
QD charging
153
6.3.4
Charge transport in QD films
154
6.3.5
Field driven luminescence quenching
154
6.3.6
Isolating the effects of charge and field
155
6.4
Characterizing QD-LEDs
157
6.5
QD-LEDs based on optical downconversion
160
6.6
QD-LEDs based on organic charge transport layers
161
6.6.1
Deposition of QDs: spin casting, phase separation, and
microcontact
printing
161
6.6.2
Operation of colloidal QD-LEDs
163
6.7
QD-LEDs with inorganic charge transport layers
165
6.7.1
Reasons for inorganic charge transport layers
165
viii Contents
6.7.2
Fabrication
ofall
inorganic QD-LEDs
165
6.7.3
Operation of QD-LED with inorganic charge transport
layers
166
6.7.4
Improving the efficiency of QD-LEDs with inorganic charge
transport layers
167
6.8
Future
work
167
References
168
7
Colloidal quantum dot photodetectors
173
Gerasimos Konstantatos
7.1
Introduction
173
7.1.1
Applications of top-surface photodetectors
173
7.1.2
Colloidal quantum dots (CQDs) for light detection
174
7.2
Fundamentals of photodetectors
175
7.2.1
Types of photodetectors
175
7.2.2
Figures of merit
176
7.3
Prior art in solution-processed photodetectors
177
7.4
Solution-processed QD photoconductors
179
7.4.1
Photoconductive gain and noise in PbS QD photodetectors
179
7.4.2
Visible-wavelength and multispectral photodetection
183
7.4.3
Control of temporal response in photoconductive detectors via
trap state engineering
185
7.5
CQD based
phototransistors
187
7.6
CQD
photodiodes
190
7.7
Conclusions
-
summary
193
References
195
8
Optical gain and lasing in colloidal quantum dots
199
Sjoerd Hoogland
8.1
Introduction
199
8.2
Optical properties of colloidal nanocrystal quantum dots
200
8.3
Carrier dynamics in colloidal quantum dots
202
8.3.1
Auger recombination
205
8.3.2
Poisson
statistics and state filling
206
8.4
Gain in solid state nanocrystal quantum dot films
207
8.4.1
Amplified spontaneous emission
(ASE)
208
8.4.2
Variable strip length (VSL) for optical gain measurements
209
8.4.3
Experimental techniques for waveguide loss measurement in
colloidal quantum dot films
209
8.4.4
Modal gain in visible colloidal quantum dots based on cadmium
chalcogenides
211
8.4.5
Modal gain in infrared colloidal quantum dots based on lead
chalcogenides
213
Contents ix
8.5
Spectral
and temporal characteristics of optical gain in nanocrystal
quantum dots
214
8.5.1
Visible colloidal quantum dots based on cadmium chalcogenides
214
8.5.2
Infrared colloidal quantum dots based on lead chalcogenides
218
8.6
Colloidal nanocrystal lasers
221
8.6.1
Microcapillary resonators
223
8.6.2
Microsphere resonators
224
8.6.3
Distributed feedback resonators
225
8.6.4
Microtoroid resonators
225
8.6.5
Other resonators
226
8.7
Future prospects
226
8.7.1
Single exciton gain
226
References
229
9
Heterojunction solar cells based on colloidal quantum dots
233
Jeffrey J. Urban and Delia J. Milliron
9.1
Introduction
233
9.2
Chemistry ofCQDs for solar cells
234
9.3
Physics of CQDs for solar cells
238
9.3.1
Electronic structure evolution in low dimensional systems
238
9.3.2
Fundamentals of light-matter interactions in QDs
240
9.3.3
Selection rules and the complications of
Я
241
9.4
Optical and electronic properties of CQD films for solar cells
241
9.5
Device physics and design of CQD heterojunction solar cells
246
9.6
Technology and scientific outlook
250
References
251
10
Solution-processed infrared quantum dot solar cells
256
Jiang Tang and Edward H. Sargent
10.1
Introduction
256
10.2
Infrared CQDs for the full absorption of solar spectrum
257
10.2.1
Bandgap
engineering for the broadband solar spectrum match
257
10.2.2
Light absorption in CQD film
260
10.3
Semiconductor solar cell fundamentals
260
10.3.1
Fundamentals of
p
-η
junction
260
10.3.2
Fundamentals of solar cells
263
10.3.3
Implications for CQD solar cell optimization
264
10.4
Electrical properties of CQD films
265
10.4.1
Measurements of electrical properties of CQD films
265
10.4.2
Transport in CQD film
269
10.4.3
CQD passivation
272
10.4.4
CQD film doping
275
10.4.5
Dielectric constant of CQD film
276
Contents
10.5
Progress
in CQD solar
cell performance
276
10.5.1 Schottky solar
cells
276
10.5.2 Heterojunction solar
cells
279
10.6 Device
stability
283
10.7
Perspectives and conclusions
285
References
286
11
Semiconductor quantum dot sensitized TiO2 mesoporous solar cells
292
Lioz Etgar, Hyo Joong Lee, Sang II Seok,
Md. K.
Nazeeruddin, and Michael
Grätzel
11.1
Introduction
292
11.2
Mesoscopic PbS quantum dot/TiC^ heterojunction solar cells
294
11.2.1
Solid-state PbS/TiO2 heterojunction solar cell
299
11.3
QD/TÍO2
mesoporous solar cell using the
SILAR
process
301
11.4
Cobalt complex-based
redox
couples in
CQD-TÍO2
mesoporous
solar cells
305
References 30X
Index
310 |
| any_adam_object | 1 |
| author_GND | (DE-588)1049310497 |
| building | Verbundindex |
| bvnumber | BV041546748 |
| classification_rvk | UH 5600 VE 8000 ZN 5000 ZP 3730 |
| ctrlnum | (OCoLC)869867097 (DE-599)GBV742034526 |
| discipline | Chemie / Pharmazie Physik Elektrotechnik / Elektronik / Nachrichtentechnik Energietechnik |
| edition | 1. publ. |
| format | Book |
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Press</subfield><subfield code="c">2013</subfield></datafield><datafield tag="300" ind1=" " ind2=" "><subfield code="a">XIV, 314 S.</subfield><subfield code="b">Ill., graph. Darst.</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="b">n</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="b">nc</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1="1" ind2=" "><subfield code="a">"Capturing the most up-to-date research in colloidal quantum dot (CQD) devices, this book is written in an accessible style by the world's leading experts. The application of CQDs in solar cells, photodetectors and light-emitting diodes (LEDs) has developed rapidly over recent years, promising to transform the future of clean energy, communications, and displays. This complete guide to the field provides researchers, students and practitioners alike with everything they need to understand these developments, and begin contributing to future applications. Introductory chapters summarise the fundamental physics and chemistry, whilst later chapters review the developments that have propelled the field forwards, systematically working through key device advances. 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| genre | (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV041546748 |
| illustrated | Illustrated |
| indexdate | 2024-12-11T13:03:17Z |
| institution | BVB |
| isbn | 9780521198264 |
| language | English |
| lccn | 2013013116 |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-026992595 |
| oclc_num | 869867097 |
| open_access_boolean | |
| owner | DE-29T DE-703 DE-384 DE-11 |
| owner_facet | DE-29T DE-703 DE-384 DE-11 |
| physical | XIV, 314 S. Ill., graph. Darst. |
| publishDate | 2013 |
| publishDateSearch | 2013 |
| publishDateSort | 2013 |
| publisher | Cambridge Univ. Press |
| record_format | marc |
| spelling | Colloidal quantum dot optoelectronics and photovoltaics ed. by Gerasimos Konstantatos ... 1. publ. Cambridge Cambridge Univ. Press 2013 XIV, 314 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier "Capturing the most up-to-date research in colloidal quantum dot (CQD) devices, this book is written in an accessible style by the world's leading experts. The application of CQDs in solar cells, photodetectors and light-emitting diodes (LEDs) has developed rapidly over recent years, promising to transform the future of clean energy, communications, and displays. This complete guide to the field provides researchers, students and practitioners alike with everything they need to understand these developments, and begin contributing to future applications. Introductory chapters summarise the fundamental physics and chemistry, whilst later chapters review the developments that have propelled the field forwards, systematically working through key device advances. The science of CQD films is explained through the latest physical models of semiconductor transport, trapping, and recombination, whilst the engineering of organic and inorganic multilayered materials is shown to have enabled major advances in the brightness and efficiency of CQD LEDs"-- Solarzelle (DE-588)4181740-0 gnd rswk-swf Fotovoltaik (DE-588)4121476-6 gnd rswk-swf Optoelektronik (DE-588)4043687-1 gnd rswk-swf Quantenpunkt (DE-588)4263396-5 gnd rswk-swf Kolloid (DE-588)4164695-2 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Kolloid (DE-588)4164695-2 s Quantenpunkt (DE-588)4263396-5 s Optoelektronik (DE-588)4043687-1 s Solarzelle (DE-588)4181740-0 s DE-604 Fotovoltaik (DE-588)4121476-6 s 1\p DE-604 Konstantatos, Gerasimos Sonstige (DE-588)1049310497 oth http://assets.cambridge.org/97805211/98264/cover/9780521198264.jpg Cover Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026992595&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Colloidal quantum dot optoelectronics and photovoltaics Solarzelle (DE-588)4181740-0 gnd Fotovoltaik (DE-588)4121476-6 gnd Optoelektronik (DE-588)4043687-1 gnd Quantenpunkt (DE-588)4263396-5 gnd Kolloid (DE-588)4164695-2 gnd |
| subject_GND | (DE-588)4181740-0 (DE-588)4121476-6 (DE-588)4043687-1 (DE-588)4263396-5 (DE-588)4164695-2 (DE-588)4143413-4 |
| title | Colloidal quantum dot optoelectronics and photovoltaics |
| title_auth | Colloidal quantum dot optoelectronics and photovoltaics |
| title_exact_search | Colloidal quantum dot optoelectronics and photovoltaics |
| title_full | Colloidal quantum dot optoelectronics and photovoltaics ed. by Gerasimos Konstantatos ... |
| title_fullStr | Colloidal quantum dot optoelectronics and photovoltaics ed. by Gerasimos Konstantatos ... |
| title_full_unstemmed | Colloidal quantum dot optoelectronics and photovoltaics ed. by Gerasimos Konstantatos ... |
| title_short | Colloidal quantum dot optoelectronics and photovoltaics |
| title_sort | colloidal quantum dot optoelectronics and photovoltaics |
| topic | Solarzelle (DE-588)4181740-0 gnd Fotovoltaik (DE-588)4121476-6 gnd Optoelektronik (DE-588)4043687-1 gnd Quantenpunkt (DE-588)4263396-5 gnd Kolloid (DE-588)4164695-2 gnd |
| topic_facet | Solarzelle Fotovoltaik Optoelektronik Quantenpunkt Kolloid Aufsatzsammlung |
| url | http://assets.cambridge.org/97805211/98264/cover/9780521198264.jpg http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026992595&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT konstantatosgerasimos colloidalquantumdotoptoelectronicsandphotovoltaics |