Molecular magnets: physics and applications
Gespeichert in:
| Weitere Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
Springer
2014
|
| Schriftenreihe: | NanoScience and Technology
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XVI, 395 S. Ill., graph. Darst. |
| ISBN: | 3642406084 9783642406089 |
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CONTENTS
PART I TUNNELING OF SINGLE MOLECULE MAGNETS
1 FROM QUANTUM RELAXATION TO RESONANT SPIN TUNNELING 3
JAVIER TEJADA
1.1 HISTORIC NOTES 3
1.2 EARLY EXPERIMENTS ON MAGNETIC TUNNELING AT THE UNIVERSITY
OF BARCELONA 5
1.3 EXPERIMENTS ON MN-12 8
1.4 CONCLUSION 12
REFERENCES 13
2 QUANTUM TUNNELING OF THE COLLECTIVE SPINS OF SINGLE-MOLECULE
MAGNETS: FROM EARLY STUDIES TO QUANTUM COHERENCE 17
BERNARD BARBARA
2.1 INTRODUCTION 17
2.2 PREHISTORY AND HISTORY 18
2.2.1 MICRO-SQUID MEASUREMENTS 22
2.2.2 MNI2-AC, THE FIRST SINGLE MOLECULAR MAGNET 22
2.3 QUANTUM TUNNELING IN SINGLE MOLECULE MAGNETS 24
2.3.1 SINGLE MOLECULE MAGNETS: BASIC PROPERTIES 24
2.3.2 FIRST EVIDENCES 26
2.3.3 MAIN EVIDENCES 28
2.4 THEORY AND COMPARISONS WITH EXPERIMENTS 33
2.4.1 RESONANCE CONDITIONS 33
2.4.2 QUANTUM FLUCTUATIONS AND BARRIER ERASING 34
2.4.3 TUNNEL SPLITTINGS, SPIN-PARITY AND OBSERVATION OF MQTM 34
2.4.4 QUANTUM TUNNELING AND SPIN-BATH 36
2.5 QUANTUM TUNNELING AND COHERENCE IN SINGLE ION MAGNETS . 44
2.5.1 FIRST EVIDENCE OF MQTM IN SIMS AND COMPARISON
WITH SMMS 44
2.5.2 FIRST EVIDENCE OF MQCM IN SIMS, PAVING THE WAY
FOR SMMS 47
IX
HTTP://D-NB.INFO/1037896580
X CONTENTS
2.6 QUANTUM COHERENCE IN SINGLE MOLECULE MAGNETS 50
2.7 CONCLUSION AND PERSPECTIVES 54
REFERENCES 55
3 SPIN L\INNELING IN MAGNETIC MOLECULES THAT HAVE FULL OR PARTIAL
MECHANICAL FREEDOM 61
EUGENE M. CHUDNOVSKY
3.1 INTRODUCTION 61
3.2 NANOMECHANICS OF A TWO-STATE SPIN SYSTEM ROTATING ABOUT
A FIXED AXIS 64
3.2.1 QUANTUM MECHANICS OF A TWO-STATE SPIN SYSTEM 64
3.2.2 RENORMALIZATION OF THE SPIN TUNNEL SPLITTING
IN A NANO-OSCILLATOR 65
3.3 FREE QUANTUM ROTATOR WITH A TWO-STATE MACROSPIN 67
3.3.1 ANOMALOUS COMMUTATION RELATIONS 67
3.3.2 ROTATING TWO-STATE SPIN SYSTEM 70
3.3.3 GROUND STATE 72
3.4 CONCLUSIONS 74
REFERENCES 75
4 A MICROSCOPIC AND SPECTROSCOPIC VIEW OF QUANTUM TUNNELING
OF MAGNETIZATION 77
JUNJIE LIU, ENRIQUE DEL BARCO, AND STEPHEN HILL
4.1 SPIN HAMILTONIAN 77
4.1.1 GIANT-SPIN APPROXIMATION HAMILTONIAN 78
4.1.2 MULTI-SPIN HAMILTONIAN 82
4.2 QUANTUM TUNNELING OF MAGNETIZATION IN HIGH-SYMMETRY MN3
SINGLE-MOLECULE MAGNETS 83
4.2.1 THE MNI SINGLE-MOLECULE MAGNET 84
4.2.2 QTM SELECTION RULES IN MN.I 85
4.2.3 THE INFLUENCE OF DISORDER ON QTM 88
4.2.4 BERRY PHASE INTERFERENCE IN TRIGONAL SYMMETRY 92
4.3 QUANTUM TUNNELING OF MAGNETIZATION IN THE HIGH-SYMMETRY NI4
SINGLE-MOLECULE MAGNET 93
4.3.1 THE NI4 SINGLE-MOLECULE MAGNET 93
*-- 4.3.2 QUANTUM TUNNELING OF MAGNETIZATION IN THE NI4 SMM . . 96
4.3.3 DISORDER 98
4.4 QUANTUM TUNNELING OF MAGNETIZATION IN LOW-SYMMETRY MN4
SINGLE-MOLECULE MAGNETS 99
4.4.1 THE MN4 SINGLE-MOLECULE MAGNETS 99
4.4.2 EPR AND QTM SPECTROSCOPY IN MN4 SMMS WITH AND
WITHOUT SOLVENT 100
4.4.3 BERRY PHASE INTERFERENCE IN
MN4
-BET 103
4.5 SUMMARY AND OUTLOOK 106
REFERENCES 108
CONTENTS XI
PART II BEYOND SINGLE MOLECULES
5 MAGNETIC AVALANCHES IN MOLECULAR MAGNETS 113
MYRIAM P. SARACHIK
5.1 BACKGROUND 113
5.2 TEMPERATURE-DRIVEN MAGNETIC DEFLAGRATION 116
5.2.1 AVALANCHE IGNITION 117
5.2.2 AVALANCHE SPEED 120
5.3 COLD DEFLAGRATION 123
5.4 SUMMARY AND OUTLOOK FOR THE FUTURE 124
REFERENCES 125
6 THEORY OF DEFLAGRATION AND FRONTS OF T\INNELING IN MOLECULAR
MAGNETS 129
D.A. GARANIN
6.1 INTRODUCTION 129
6.2 MAGNETIC DEFLAGRATION 132
6.2.1 IGNITION OF DEFLAGRATION 134
6.2.2 DEFLAGRATION FRONTS 135
6.3 FRONTS OF TUNNELING 139
6.3.1 TUNNELING EFFECTS IN THE RELAXATION RATE 139
6.3.2 DIPOLAR FIELD IN MOLECULAR MAGNETS 143
6.3.3 FRONTS OF TUNNELING AT T = 0 147
6.3.4 ID THEORY OF QUANTUM DEFLAGRATION 151
6.3.5 3D THEORY OF QUANTUM DEFLAGRATION 154
6.4 DISCUSSION 156
REFERENCES 157
7 DIPOLAR MAGNETIC ORDER IN CRYSTALS OF MOLECULAR NANOMAGNETS . . 161
FERNANDO LUIS
7.1 INTRODUCTION 161
7.2 THEORETICAL BACKGROUND 165
7.2.1 SPIN HAMILTONIAN 165
7.2.2 MEAN-FIELD APPROXIMATIONS 166
7.3 DIPOLAR ORDER VS. SINGLE-MOLECULE MAGNET BEHAVIOR 168
7.3.1 MAGNETIC ORDER AND RELAXATION TOWARDS THERMAL
EQUILIBRIUM 168
7.3.2 INFLUENCE OF DIPOLAR INTERACTIONS ON MAGNETIC RELAXATION
AND SPIN TUNNELING 169
7.3.3 EXPERIMENTAL DETERMINATION OF THE AVERAGE INTERACTION
FIELDS 170
7.4 DIPOLAR ORDER OF MOLECULAR NANOMAGNETS WITH LOW MAGNETIC
ANISOTROPY. FERROMAGNETISM IN MNFI 172
7.5 DIPOLAR ORDER IN A TRANSVERSE MAGNETIC FIELD. FERROMAGNETISM
IN MNI2
ACETATE 175
7.5.1 MAGNETIC ORDERING VIA PURE QUANTUM TUNNELING 175
XII CONTENTS
7.5.2 QUANTUM ANNEALING 175
7.5.3 THE QUANTUM ISING MODEL 176
7.5.4 MAGNETIC ORDER IN MN12 ACETATE 177
7.6 MAGNETIC ORDER AND QUANTUM PHASE TRANSITION IN FES 181
7.7 CONCLUSIONS AND OUTLOOK 186
REFERENCES 187
8 SINGLE-CHAIN MAGNETS 191
DANTE GATTESCHI AND ALESSANDRO VINDIGNI
8.1 INTRODUCTION 191
8.2 THERMAL EQUILIBRIUM AND SLOW DYNAMICS IN IDEAL SCMS . 194
8.3 TAILORING SCMS BY BUILDING-BLOCK APPROACH 198
8.4 REALISTIC SPIN HAMILTONIANS FOR SINGLE-CHAIN MAGNETS 201
8.5 GLAUBER MODEL AND SINGLE-CHAIN MAGNETS 206
8.6 GLAUBER MODEL FOR FINITE CHAINS 211
8.7 BEYOND THE GLAUBER MODEL 215
8.8 CONCLUSION AND PERSPECTIVES 217
REFERENCES 218
9 MAGNETISM OF METAL PHTHALOCYANINES 221
JUAN BARTOLOME, CARLOS MONTON, AND IVAN K. SCHULLER
9.1 INTRODUCTION 221
9.2 SOLID STATE MPCS 222
9.3 MPC THIN FILMS 229
9.4 MPC MOLECULES ADSORBED ON SUBSTRATES 234
9.5 PERSPECTIVES OF MPCS 239
REFERENCES 242
PART III APPLICATIONS
10 POTENTIALITIES OF MOLECULAR NANOMAGNETS FOR INFORMATION
TECHNOLOGIES 249
MARCO AFFRONTE AND FILIPPO TROIANI
10.1 INTRODUCTION 249
10.2 CLASSICAL AND QUANTUM BITS 251
10.3 ISSUES, TRENDS AND BENCHMARKS OF INFORMATION TECHNOLOGIES . . 257
10.4 QUANTUM COMPUTATION 262
10.5 CONCLUSIONS AND FUTURE DIRECTIONS 270
REFERENCES 270
11 MOLECULAR MAGNETS FOR QUANTUM INFORMATION PROCESSING 275
KEVIN VAN HOOGDALEM, DIMITRIJE STEPANENKO, AND DANIEL LOSS
11.1 INTRODUCTION 275
11.2 ENCODING OF QUBITS IN MOLECULAR MAGNETS 278
11.3 SINGLE-QUBIT ROTATIONS AND THE SPIN-ELECTRIC EFFECT 280
11.4 TWO-QUBIT GATES 286
11.5 DECOHERENCE IN MOLECULAR MAGNETS 288
11.6 INITIALIZATION AND READ-OUT 291
CONTENTS XIII
11.7 GROVER'S ALGORITHM USING MOLECULAR MAGNETS 292
REFERENCES 294
12 SINGLE-MOLECULE SPINTRONICS 297
ENRIQUE BURZURF AND HERRE S.J. VAN DER ZANT
12.1 INTRODUCTION 297
12.1.1 HOW TO DETECT SPIN IN MAGNETIC MOLECULES? 298
12.2 COULOMB BLOCKADE 299
12.3 SPECTROSCOPY OF MAGNETIC SPIN STATES 301
12.3.1 WEAK COUPLING: SET EXCITATIONS 302
12.3.2 INTERMEDIATE COUPLING: INELASTIC SPIN-FLIP CO-TUNNELING
PROCESS 303
12.3.3 KONDO CORRELATIONS 304
12.3.4 GROUND STATE TO GROUND STATE: GATE SPECTROSCOPY . 305
12.3.5 SUMMARY 307
12.4 FABRICATION OF A SPIN TRANSISTOR 307
12.4.1 ELECTRON-BEAM LITHOGRAPHY 307
12.4.2 ELECTROMIGRATION 309
12.4.3 PRELIMINARY CHARACTERIZATION 310
12.5 A PRACTICAL EXAMPLE. THE FE4 SINGLE-MOLECULE MAGNET 310
12.5.1 WHY THE FE4 SINGLE-MOLECULE MAGNET? 310
12.5.2 SPIN EXCITATIONS: INELASTIC SPIN FLIP SPECTROSCOPY . 312
12.5.3 GATE-VOLTAGE SPECTROSCOPY 313
12.5.4 KONDO EXCITATIONS AND HIGH-SPIN STATE 314
12.6 FUTURE DIRECTIONS 315
12.6.1 QUANTUM TUNNELING OF THE MAGNETIZATION AND BERRY PHASE 315
12.6.2 FERROMAGNETIC ELECTRODES 316
12.6.3 SPIN CROSSOVER MOLECULES 316
REFERENCES 317
13 MOLECULAR QUANTUM SPINTRONICS USING SINGLE-MOLECULE MAGNETS . 319
MARC GANZHORN AND WOLFGANG WERNSDORFER
13.1 INTRODUCTION 319
13.2 MOLECULAR NANOMAGNETS FOR MOLECULAR SPINTRONICS 320
13.3 INTRODUCTION TO MOLECULAR SPINTRONICS 321
13.3.1 DIRECT COUPLING SCHEME 322
13.3.2 INDIRECT COUPLING SCHEME 324
13.3.3 MAGNETIC TORQUE DETECTOR OR PROBING VIA MECHANICAL
MOTION 325
13.3.4 NANOSQUID OR PROBING VIA MAGNETIC FLUX 327
13.4 MAGNETISM OF THE TBPC2 MOLECULAR NANOMAGNET 328
13.4.1 MOLECULAR STRUCTURE 329
13.4.2 SPIN HAMILTONIAN 329
13.4.3 QUANTUM TUNNELING OF MAGNETIZATION AND LANDAU-ZENER
MODEL 332
13.4.4 SPIN-LATTICE RELAXATION 333
XIV
CONTENTS
13.5 MOLECULAR QUANTUM SPINTRONICS WITH A SINGLE TBPC2 335
13.5.1 READ-OUT OF THE ELECTRONIC SPIN 336
13.5.2 READ-OUT OF THE NUCLEAR SPIN 344
13.5.3 COUPLING OF A SINGLE TBPC2 SMM TO A CARBON
NANOTUBE'S MECHANICAL MOTION 354
13.5.4 COUPLING OF A SINGLE TBPC2 SMM TO A QUANTUM DOT. . . 358
13.6 CONCLUSION 360
REFERENCES 361
14 MOLECULE-BASED MAGNETIC COOLERS: MEASUREMENT, DESIGN AND
APPLICATION 365
MARCO EVANGELISTI
14.1 INTRODUCTION 365
14.2 THEORETICAL FRAMEWORK 367
14.3 EXPERIMENTAL EVALUATION OF THE MCE 368
14.3.1 INDIRECT METHODS 368
14.3.2 DIRECT MEASUREMENTS 370
14.4 DESIGNING THE IDEAL REFRIGERANT 373
14.4.1 MAGNETIC ANISOTROPY 374
14.4.2 MAGNETIC INTERACTIONS 375
14.4.3 MAGNETIC DENSITY AND CHOICE OF UNITS 378
14.5 TOWARDS APPLICATIONS: ON-CHIP REFRIGERATION 382
14.6 CONCLUDING REMARKS 385
REFERENCES 385
INDEX 389 |
| any_adam_object | 1 |
| author2 | Bartolomé, Juan |
| author2_role | edt |
| author2_variant | j b jb |
| author_facet | Bartolomé, Juan |
| building | Verbundindex |
| bvnumber | BV041419264 |
| classification_rvk | UM 3130 UP 6800 |
| ctrlnum | (OCoLC)865130800 (DE-599)DNB1037896580 |
| dewey-full | 538.4 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 538 - Magnetism |
| dewey-raw | 538.4 |
| dewey-search | 538.4 |
| dewey-sort | 3538.4 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| format | Book |
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| isbn | 3642406084 9783642406089 |
| language | English |
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| spellingShingle | Molecular magnets physics and applications Molekularer Nanomagnet Molekularer Nanomagnet (DE-588)104638838X gnd |
| subject_GND | (DE-588)104638838X |
| title | Molecular magnets physics and applications |
| title_auth | Molecular magnets physics and applications |
| title_exact_search | Molecular magnets physics and applications |
| title_full | Molecular magnets physics and applications Juan Bartolomé ... eds. |
| title_fullStr | Molecular magnets physics and applications Juan Bartolomé ... eds. |
| title_full_unstemmed | Molecular magnets physics and applications Juan Bartolomé ... eds. |
| title_short | Molecular magnets |
| title_sort | molecular magnets physics and applications |
| title_sub | physics and applications |
| topic | Molekularer Nanomagnet Molekularer Nanomagnet (DE-588)104638838X gnd |
| topic_facet | Molekularer Nanomagnet |
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