Electron photoemission from sodium and carbon clusters:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
2013
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| Schlagworte: | |
| Online-Zugang: | Volltext Volltext http://d-nb.info/1036774864/34 Inhaltsverzeichnis |
| Beschreibung: | 180 S. Ill., graph. Darst. 21 cm |
Internformat
MARC
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| 100 | 1 | |a Wopperer, Philipp |e Verfasser |0 (DE-588)1038651190 |4 aut | |
| 245 | 1 | 0 | |a Electron photoemission from sodium and carbon clusters |c vorgelegt von Philipp Wopperer |
| 264 | 1 | |c 2013 | |
| 300 | |a 180 S. |b Ill., graph. Darst. |c 21 cm | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 502 | |a Erlangen-Nürnberg, Univ., Diss., 2013 | ||
| 650 | 0 | 7 | |a Dichtefunktionalformalismus |0 (DE-588)4258514-4 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Ionisation |0 (DE-588)4135379-1 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Photoelektronenspektroskopie |0 (DE-588)4174491-3 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Cluster |0 (DE-588)4010318-3 |2 gnd |9 rswk-swf |
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
| 689 | 0 | 0 | |a Cluster |0 (DE-588)4010318-3 |D s |
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Datensatz im Suchindex
| _version_ | 1804151349423636480 |
|---|---|
| adam_text | CONTENTS
1 INTRODUCTION 25
2 MANY-BODY THEORY IN CLUSTER PHYSICS 29
2.1 IONIC BACKGROUND 30
2.2 ELECTRON DYNAMICS: DENSITY-FUNCTIONAL THEORY 33
2.2.1 STATIONARY DENSITY-FUNCTIONAL THEORY 33
2.2.2 LOCAL-DENSITY APPROXIMATION 36
2.2.3 SELF-INTERACTION CORRECTION 37
2.2.4 TIME-DEPENDENT DENSITY-FUNCTIONAL THEORY 38
2.3 SUMMARY 39
3 EXCITATION AND ANALYSIS TOOLS 41
3.1 GAUGES AND DIPOLE APPROXIMATION 41
3.2 PULSE PROFILE 43
3.3 DETERMINATION OF THE EMITTED DENSITY 44
3.4 DETERMINATION OF PHOTOANGULAR DISTRIBUTIONS 46
3.5 DETERMINATION OF PHOTOELECTRON SPECTRA 47
3.6 INTEGRATED PHOTOELECTRON SPECTRA 49
3.7 COMBINED DETERMINATION OF PES AND PAD 50
4 AVERAGING METHODS 53
4.1 THE ANISOTROPY PARAMETER 53
4.2 THE ANALYTICAL AVERAGING SCHEME 55
4.2.1 THE EULER ANGLES 55
4.2.2 NOTATION 56
4.2.3 DERIVATION IN FIRST-ORDER PERTURBATION THEORY 58
4.2.4 TRANSFORMATION INTO CARTESIAN COORDINATES 60
4.2.5 PROCEDURE 61
4.3 DIRECT AVERAGING SCHEMES 62
5 FIRST RESULTS 65
5.1 EXAMPLE: NAS SPHERICAL JELLIUM 65
5.2 ONE-PHOTON PROCESSES IN SMALL SODIUM CLUSTERS 68
21
HTTP://D-NB.INFO/1038651255
CONTENTS
5.3 IONIZATION BEYOND THE LINEAR REGIME 74
5.3.1 RESONANT EMISSION BELOW THE IONIZATION THRESHOLD 74
5.3.2 CONVERGENCE TESTS OF THE DIRECT AVERAGING SCHEME 79
5.4 SUMMARY 82
6 FREQUENCY DEPENDENCE OF PAD IN SMALL SODIUM CLUSTERS 85
6.1 PERTURBATIVE APPROACHES 86
6.1.1 BETHE-COOPER-ZARE FORMULA 86
6.1.2 APPROXIMATIONS FOR THE OUTGOING WAVE 87
6.2 STATIC RESULTS FOR NAG SPHERICAL JELLIUM 89
6.2.1 HARMONIC OSCILLATOR MODEL 89
6.2.2 STATIC RESULTS WITH SELF-CONSISTENT WAVEFUNCTIONS 90
6.3 TIME-DEPENDENT SPHERICAL JELLIUM CALCULATIONS 100
6.4 ROLE OF DEFORMATION 100
6.4.1 TRENDS IN STATIC PLANE WAVE APPROXIMATION 100
6.4.2 TIME-DEPENDENT CALCULATIONS 103
6.5 STATIC AND TIME-DEPENDENT RESULTS FOR NAF 105
6.6 SUMMARY 108
7 BUCKMINSTERFULLERENE 111
7.1 BASIC PROPERTIES 113
7.1.1 IONIC STRUCTURE 113
7.1.2 ELECTRONIC STRUCTURE, IONIZATION POTENTIAL, AND GAPS .... 113
7.1.3 DIPOLE RESPONSE 116
7.2 AVERAGING AND INTEGRATION SCHEME 120
7.3 PHOTOEMISSION IN ONE-PHOTON DOMAIN 121
7.3.1 FIRST RESULTS - VELOCITY MAPS 121
7.3.2 SYSTEMATICS WITH FREQUENCY 126
7.4 MULTIPHOTON DOMAIN 127
7.4.1 SYSTEMATICS WITH INTENSITY 127
7.4.2 SYSTEMATICS WITH FREQUENCY 131
7.5 COMPARISON WITH EXPERIMENT 132
7.6 SUMMARY 134
8 CARBON CHAINS 137
8.1 IONIC AND ELECTRONIC STRUCTURE 138
8.2 DIPOLE RESPONSE 140
8.3 PLASMON-ENHANCED PHOTOEMISSION 141
9 CONCLUSION 147
22
CONTENTS
APPENDIX
A ANGULAR MOMENTUM AND ROTATIONS 155
A.L EULER ANGLES AND ROTATION OPERATORS 155
A.1.1 WIGNER 3J-SYMBOLS 156
A.1.2 TRANSFORMATION OF LST-ORDER TENSORS 157
A.2 LEGENDRE POLYNOMIALS AND SPHERICAL HARMONICS 159
B RADIAL SCHRODINGER EQUATION 161
B.L INTRODUCTION 161
B.2 CONTINUUM SOLUTIONS 162
B.2.1 FREE SOLUTION 162
B.2.2 SOLUTION IN SHORT-RANGE POTENTIALS 162
B.2.3 SOLUTION IN LONG-RANGE POTENTIALS 163
B.3 INTEGRALS FOR THE HARMONIC OSCILLATOR MODEL 164
B.4 SPHERICAL BESSEL AND COULOMB FUNCTIONS 165
B.4.1 SPHERICAL BESSEL AND NEUMANN FUNCTIONS 165
B.5 SPHERICAL COULOMB FUNCTIONS 166
B.6 NUMERICAL SOLUTION 166
B.6.1 THE NUMEROV ALGORITHM 166
B.6.2 APPLICATION OF THE NUMEROV ALGORITHM 167
BIBLIOGRAPHY 169
23
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| any_adam_object | 1 |
| author | Wopperer, Philipp |
| author_GND | (DE-588)1038651190 |
| author_facet | Wopperer, Philipp |
| author_role | aut |
| author_sort | Wopperer, Philipp |
| author_variant | p w pw |
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| bvnumber | BV041286845 |
| collection | ebook |
| ctrlnum | (OCoLC)859421809 (DE-599)DNB1038651255 |
| dewey-full | 541.28 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541.28 |
| dewey-search | 541.28 |
| dewey-sort | 3541.28 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik |
| format | Thesis Book |
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| spelling | Wopperer, Philipp Verfasser (DE-588)1038651190 aut Electron photoemission from sodium and carbon clusters vorgelegt von Philipp Wopperer 2013 180 S. Ill., graph. Darst. 21 cm txt rdacontent n rdamedia nc rdacarrier Erlangen-Nürnberg, Univ., Diss., 2013 Dichtefunktionalformalismus (DE-588)4258514-4 gnd rswk-swf Ionisation (DE-588)4135379-1 gnd rswk-swf Photoelektronenspektroskopie (DE-588)4174491-3 gnd rswk-swf Cluster (DE-588)4010318-3 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Cluster (DE-588)4010318-3 s Dichtefunktionalformalismus (DE-588)4258514-4 s Ionisation (DE-588)4135379-1 s Photoelektronenspektroskopie (DE-588)4174491-3 s DE-604 Erscheint auch als Online-Ausgabe urn:nbn:de:bvb:29-opus-47637 https://open.fau.de/handle/openfau/3440 Verlag kostenfrei Volltext https://nbn-resolving.org/urn:nbn:de:bvb:29-opus-47637 Resolvingsystem kostenfrei Volltext http://d-nb.info/1036774864/34 Langzeitarchivierung Nationalbibliothek DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026735911&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Wopperer, Philipp Electron photoemission from sodium and carbon clusters Dichtefunktionalformalismus (DE-588)4258514-4 gnd Ionisation (DE-588)4135379-1 gnd Photoelektronenspektroskopie (DE-588)4174491-3 gnd Cluster (DE-588)4010318-3 gnd |
| subject_GND | (DE-588)4258514-4 (DE-588)4135379-1 (DE-588)4174491-3 (DE-588)4010318-3 (DE-588)4113937-9 |
| title | Electron photoemission from sodium and carbon clusters |
| title_auth | Electron photoemission from sodium and carbon clusters |
| title_exact_search | Electron photoemission from sodium and carbon clusters |
| title_full | Electron photoemission from sodium and carbon clusters vorgelegt von Philipp Wopperer |
| title_fullStr | Electron photoemission from sodium and carbon clusters vorgelegt von Philipp Wopperer |
| title_full_unstemmed | Electron photoemission from sodium and carbon clusters vorgelegt von Philipp Wopperer |
| title_short | Electron photoemission from sodium and carbon clusters |
| title_sort | electron photoemission from sodium and carbon clusters |
| topic | Dichtefunktionalformalismus (DE-588)4258514-4 gnd Ionisation (DE-588)4135379-1 gnd Photoelektronenspektroskopie (DE-588)4174491-3 gnd Cluster (DE-588)4010318-3 gnd |
| topic_facet | Dichtefunktionalformalismus Ionisation Photoelektronenspektroskopie Cluster Hochschulschrift |
| url | https://open.fau.de/handle/openfau/3440 https://nbn-resolving.org/urn:nbn:de:bvb:29-opus-47637 http://d-nb.info/1036774864/34 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026735911&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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