Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces:
Saved in:
| Main Author: | |
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| Format: | Thesis Book |
| Language: | English |
| Published: |
2012
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| Subjects: | |
| Online Access: | https://nbn-resolving.org/urn:nbn:de:bvb:384-opus4-22817 Volltext Inhaltsverzeichnis |
| Physical Description: | V, 198 S. Ill., graph. Darst. |
Staff View
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| 245 | 1 | 0 | |a Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces |c vorgelegt von Christoph Richter |
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Record in the Search Index
| _version_ | 1804150329738002432 |
|---|---|
| adam_text | IMAGE 1
CONTENTS
1. INTRODUCTION 1
1.1. LAALOS AND SRTIOS: TWO BAND INSULATORS AND THEIR INTERFACE 2
1.1.1. LAALOA: LANTHANUM ALUMINATE 2
1.1.2. SRTIC 3: STRONTIUM TITANATE 2
1.1.3. A CONDUCTING INTERFACE BETWEEN TWO INSULATORS 4
2. EXPERIMENTAL CONCEPT, METHODS AND SETUP 9
2.1. EXPERIMENTAL METHODS 11
2.1.1. SAMPLE GROWTH AND MORPHOLOGICAL CHARACTERIZATION 11
2.1.2. TUNNELING SPECTROSCOPY 11
2.1.3. CANTILEVER-BASED TORQUE MAGNETOMETRY 14
2.2. EXPERIMENTAL CONCEPT AND SAMPLE DESIGN 16
2.2.1. LAO-STO DIRECT MAGNETIZATION MEASUREMENT 16
2.2.2. LAO-STO LOW-ENERGY TUNNELING SPECTROSCOPY 16
2.2.3. PLANAR TUNNEL DEVICE CONCEPT 17
2.2.4. TUNNEL-ELECTRODE MATERIAL CONSTRAINTS 17
2.2.5. TUNNEL DEVICE LAYOUT 18
2.3. SAMPLE PREPARATION 22
2.3.1. TI02-TERMINATED SRTIOS SUBSTRATE 22
.2.3.2. PLD-GROWN LAA103 FILM 23
2.3.3. PATTERNED LAA103-SRTI03 INTERFACES 25
2.3.4. SPUTTERED AU TOP-ELECTRODE 25
2.3.5. AU-TUNNEL-ELECTRODE PATTERNING 25
2.3.6. LAA103-SRTI03-INTERFACE CONTACTS 26
2.3.7. WIRE-BONDING 26
2.4. PRELIMINARY CHARACTERIZATION OF TUNNEL-JUNCTIONS 28
2.4.1. TEM RESULTS OF AU-LAO-STO JUNCTIONS 29
2.4.2. NORMAL CONDUCTIVITY OF AU-COVERED LAO-STO INTERFACES 31 2.4.3.
TRANSPORT PROPERTIES AT MILLIKELVIN TEMPERATURES 32
2.4.4. CONCLUSION 35
3. LAO-STO TUNNELING SPECTROSCOPY 37
3.1. TUNNELING ON A MICROVOLT SCALE: THE SUPERCONDUCTING GAP 38
3.1.1. TEMPERATURE DEPENDENCE OF TUNNEL SPECTRA 38
3.1.2. TEMPERATURE DEPENDENCE OF THE SUPERCONDUCTING GAP 42
3.1.3. DOPING (GATE-VOLTAGE) DEPENDENCY OF THE GAP 45
3.1.4. SUMMARY 51
3.2. TUNNELING ON A MILLIVOLT SCALE: LOW CHEMICAL POTENTIAL AND LO
PHONONS 53
III
HTTP://D-NB.INFO/1038380626
IMAGE 2
CONTENTS
3.2.1. I(V) ASYMMETRY AND CONDUCTION-BAND STRUCTURE 53
3.2.2. PHONON-ASSISTED TUNNELING 55
3.2.3. FORMAL DESCRIPTION OF INELASTIC TUNNELING 57
3.2.4. INELASTIC TUNNELING AND LAO-STO BAND STRUCTURE 61
3.2.5. SUMMARY AND DISCUSSION 65
3.3. TUNNELING ON A VOLT SCALE: BARRIER EFFECTS AND INTERFACE
RESISTIVITY 66 3.3.1. PREREQUISITES 66
3.3.2. RESULTS 68
3.3.3. SUMMARY 70
3.4. SUMMARIZED RESULTS OF TUNNELING EXPERIMENTS 71
4. LAO-STO TORQUE MAGNETOMETRY 73
4.1. MAGNETOMETRY RESULTS 74
4.1.1. NATURE OF THE MAGNETIC ORDERING, TEMPERATURE DEPENDENCE .... 75
4.1.2. ORIENTATION OF THE MAGNETIC MOMENT 75
4.1.3. SUMMARY 77
4.2. COEXISTENT SUPERCONDUCTIVITY AND MAGNETIC ORDER 79
4.3. DISCUSSION OF ELECTRONIC PHASE SEPARATION 81
5. CONCLUSIONS AND OUTLOOK 83
APPENDICES 85
A. WITH OLFETS TOWARDS ALL-OXIDE INTEGRATED CIRCUITS 87
B. NATURE OF THE SUPERCONDUCTING STATE - FITS TO THE TUNNEL-SPECTRA 93
C. IN-GAP FEATURES IN TUNNELING SPECTRA 95
D. ALTERNATIVE GROWTH PROCEDURES; OXIDE INTERFACES RELATED TO LAO-STO
103 D.L. CONDUCTING OXIDE INTERFACES WITHOUT LAA10 3 104
D.L.L. LAVC 3: A MOTT-INSULATOR 106
D.1.2. LAGAC 3: LAALCVS NEAREST RELATIVE 107
D.1.3. DYSCOA: A LA-FREE OXIDE INTERFACE 108
D.L.4. GDTIOA: AN MBE-GROWN INTERFACE 109
D.L.5. OTHER RELATED INTERFACE SYSTEMS 110
D.1.6. SUMMARY 112
D.2. CONDUCTING OXIDE INTERFACES BY MOLECULAR-BEAM EPITAXY 113
D.2.1. PREVIOUS WORK 114
D.2.2. LARGE COMPOSITION SPREAD SAMPLES 115
D.2.3. QUANTITATIVE DETERMINATION OF LAALOA STOICHIOMETRY BY RBS . . .
120 D.2.4. RESULT: NO CONDUCTIVITY IN STOICHIOMETRIC LAO-STO 122
D.2.5. CARRIER DENSITY AND MOBILITY OF MBE SAMPLES 123
D.2.6. SUMMARY AND CONCLUSIONS 126
D.3. HF-FREE TERMINATION-PROCESS FOR HIGH-QUALITY LAO-STO INTERFACES
.... 128
IV
IMAGE 3
CONTENTS
D.3.1. THE ARKANSAS-ETCH 129
D.3.2. SURFACE MORPHOLOGY OF ARKANSAS-ETCHED SUBSTRATES 129
D.3.3. RHEED-CONTROLLED LAALOA FILM GROWTH 129
D.3.4. ELECTRONIC PROPERTIES OF HF-FREE LAA103-SRTI03 INTERFACES ....
130 D.4. THE LAA103-CATI03 INTERFACE 133
D.4.1. MATERIAL PROPERTIES OF CATIC 3 (PEROVSKITE) 133
D.4.2. CHARACTERIZATION OF CATIC 3 SUBSTRATES 134
D.4.3. EPITAXIAL GROWTH OF LAA103 ON CATIC 3 136
D.4.4. ELECTRONIC TRANSPORT PROPERTIES OF LAA103-CATI03 INTERFACES . . .
141 D.4.5. SUMMARY 149
D.5. CHAPTER SUMMARY AND DISCUSSION 152
E. AFM IMAGES OF MBE-GROWN LAO-STO SAMPLES 155
F. HYSTERETIC MAGNETOTRANSPORT ON MBE-GROWN LAO-STO SAMPLES 159
G. CO-ETCHING TO DETERMINE SHALLOW ETCH STEPS 161
H. CURRICULUM VITAE 163
H.L. LIST OF PUBLICATIONS 165
BIBLIOGRAPHY 169
LIST OF FIGURES 191
LIST OF TABLES 195
ACKNOWLEDGEMENT/DANKSAGUNG 197
V
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| any_adam_object | 1 |
| author | Richter, Christoph 1981- |
| author_GND | (DE-588)1038366712 |
| author_facet | Richter, Christoph 1981- |
| author_role | aut |
| author_sort | Richter, Christoph 1981- |
| author_variant | c r cr |
| building | Verbundindex |
| bvnumber | BV041011821 |
| classification_rvk | UP 3150 UP 3400 UP 7750 |
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| discipline | Physik |
| format | Thesis Book |
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| indexdate | 2024-07-10T00:37:12Z |
| institution | BVB |
| language | English |
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| physical | V, 198 S. Ill., graph. Darst. |
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| spelling | Richter, Christoph 1981- Verfasser (DE-588)1038366712 aut Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces vorgelegt von Christoph Richter 2012 V, 198 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Augsburg, Univ., Diss., 2013 Inelastische Elektronen-Tunnelspektroskopie (DE-588)4161633-9 gnd rswk-swf Lanthanaluminide (DE-588)4760078-0 gnd rswk-swf Strontiumtitanat (DE-588)4183773-3 gnd rswk-swf Physikalische Eigenschaft (DE-588)4134738-9 gnd rswk-swf Übergangsmetalloxide (DE-588)4186583-2 gnd rswk-swf Supraleitung (DE-588)4058651-0 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Übergangsmetalloxide (DE-588)4186583-2 s Physikalische Eigenschaft (DE-588)4134738-9 s Lanthanaluminide (DE-588)4760078-0 s Strontiumtitanat (DE-588)4183773-3 s Inelastische Elektronen-Tunnelspektroskopie (DE-588)4161633-9 s Supraleitung (DE-588)4058651-0 s DE-604 Erscheint auch als Online-Ausgabe urn:nbn:de:bvb:384-opus4-22817 https://nbn-resolving.org/urn:nbn:de:bvb:384-opus4-22817 Resolving-System http://opus.bibliothek.uni-augsburg.de/opus4/frontdoor/index/index/docId/2281 Verlag kostenfrei Volltext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025989393&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Richter, Christoph 1981- Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces Inelastische Elektronen-Tunnelspektroskopie (DE-588)4161633-9 gnd Lanthanaluminide (DE-588)4760078-0 gnd Strontiumtitanat (DE-588)4183773-3 gnd Physikalische Eigenschaft (DE-588)4134738-9 gnd Übergangsmetalloxide (DE-588)4186583-2 gnd Supraleitung (DE-588)4058651-0 gnd |
| subject_GND | (DE-588)4161633-9 (DE-588)4760078-0 (DE-588)4183773-3 (DE-588)4134738-9 (DE-588)4186583-2 (DE-588)4058651-0 (DE-588)4113937-9 |
| title | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces |
| title_auth | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces |
| title_exact_search | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces |
| title_full | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces vorgelegt von Christoph Richter |
| title_fullStr | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces vorgelegt von Christoph Richter |
| title_full_unstemmed | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces vorgelegt von Christoph Richter |
| title_short | Experimental Investigation of Electronic and Magnetic Properties of LaAlO3-SrTiO3 Interfaces |
| title_sort | experimental investigation of electronic and magnetic properties of laalo3 srtio3 interfaces |
| topic | Inelastische Elektronen-Tunnelspektroskopie (DE-588)4161633-9 gnd Lanthanaluminide (DE-588)4760078-0 gnd Strontiumtitanat (DE-588)4183773-3 gnd Physikalische Eigenschaft (DE-588)4134738-9 gnd Übergangsmetalloxide (DE-588)4186583-2 gnd Supraleitung (DE-588)4058651-0 gnd |
| topic_facet | Inelastische Elektronen-Tunnelspektroskopie Lanthanaluminide Strontiumtitanat Physikalische Eigenschaft Übergangsmetalloxide Supraleitung Hochschulschrift |
| url | https://nbn-resolving.org/urn:nbn:de:bvb:384-opus4-22817 http://opus.bibliothek.uni-augsburg.de/opus4/frontdoor/index/index/docId/2281 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025989393&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT richterchristoph experimentalinvestigationofelectronicandmagneticpropertiesoflaalo3srtio3interfaces |