Many-electron electrochemical processes: reactions in molten salts, room-temperature ionic liquids and ionic solutions
Gespeichert in:
| Hauptverfasser: | , , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Heidelberg [u.a.]
Springer
2013
|
| Schriftenreihe: | Monographs in electrochemistry
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XIX, 167 S. Ill., graph. Darst. 235 mm x 155 mm |
| ISBN: | 9783642357695 |
Internformat
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Datensatz im Suchindex
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| adam_text |
IMAGE 1
CONTENTS
1 MANY-ELECTRON ELECTROCHEMICAL SYSTEMS: CONCEPTS AND DEFINITIONS 1 1.1
DEFINITION OF A STEPWISE ELECTROCHEMICAL PROCESS 1
1.2 STEPWISE MANY-ELECTRON PROCESS: PROBLEM OF KINETIC DESCRIPTION. 4
1.3 ELECTRODE FILM SYSTEMS. FORMATION, GENERAL PROPERTIES,
CLASSIFICATION 6
1.4 VELIKANOV'S POLYFUNCTIONAL CONDUCTOR 7
1.5 CLASSIFICATION OF FILM SYSTEMS. PROCESSES IN CHEMICAL FILM SYSTEMS 8
1.5.1 PROCESSES IN CHEMICAL FILM SYSTEMS 8
1.6 MACROKINETICS OF PROCESSES IN FILM SYSTEMS: GENERAL PRINCIPLES OF
THEORETICAL MODELLING 12
1.6.1 MATHEMATICAL MODELS OF PHYSICO-CHEMICAL PROCESSES USING AN
APPROACH BASED ON THE BIFURCATION THEORY . 13
REFERENCES 17
2 MANY-ELECTRON SYSTEMS AT EQUILIBRIUM 21
2.1 GENERAL FORMULATION 21
2.2 EXPERIMENTAL METHODS: EQUILIBRIUM CONDITIONS 24
2.2.1 SOLUBILITY OF METALS IN MOLTEN SALT MEDIA 24
2.2.2 POTENTIOMETRY 27
2.3 EXPERIMENTAL METHODS: NERNSTIAN STATIONARY CONDITIONS 31
2.3.1 GENERAL NOTIONS AND VALIDITY CONDITIONS 31
2.3.2 STATIONARY POTENTIAL 32
2.3.3 VOLTAMMETRY AT STATIONARY CONDITIONS (POLAROGRAPHY). 35
2.4 EXPERIMENTAL METHODS: NONSTATIONARY NERNSTIAN CONDITIONS. 39
2.4.1 APPLICABILITY 39
2.4.2 CHRONOAMPEROMETRY 39
2.4.3 CHRONOPOTENTIOMETRY 40
2.5 INSTEAD OF CONCLUSIONS: MORE ABOUT "SYSTEM" AND "NON-SYSTEM"
ELECTROCHEMISTRY 48
REFERENCES 50
XVII
HTTP://D-NB.INFO/1028418477
IMAGE 2
XVIII
CONTENTS
3 PHENOMENOLOGY OF ELECTROCHEMICAL KINETICS 51
3.1 DIAGNOSTICS OF INTERVALENT REACTIONS 51
3.2 ELECTROCHEMICAL REDUCTION OF GERMANIUM COMPOUNDS IN FLUORIDE MELTS
54
3.3 EXPERIMENTAL STUDY OF MANY-ELECTRON KINETICS: GENERAL RULES AND
RECOMMENDATIONS 61
3.4 SOME DATA ON THE ELECTROREDUCTION MECHANISMS OF POLYVALENT SPECIES
IN IONIC MELTS 63
3.5 DISPUTABLE PROBLEMS OF MANY-ELECTRON KINETICS 66
REFERENCES 68
4 ELECTRODE FILM SYSTEMS: EXPERIMENTAL EVIDENCES 71
4.1 ION-METAL FILM SYSTEMS IN PROCESSES OF ELECTRODEPOSITION AND
ELECTROREFINEMENT OF POLYVALENT METALS 71
4.2 ION-SEMICONDUCTOR FILM SYSTEMS 80
4.3 DIELECTRIC FILM SYSTEMS 81
REFERENCES 87
5 DYNAMICS OF A NON-EQUILIBRIUM ELECTROCHEMICAL SYSTEM 89
5.1 COUPLING IN ELECTROCHEMICAL SYSTEMS: ELECTROCHEMICAL DECOMPOSITION
OF MIXED CONDUCTOR 89
5.1.1 THE MATHEMATICAL MODEL 90
5.1.2 EXPERIMENT AND ITS ANALYSIS 91
5.2 COUPLING IN ELECTROCHEMICAL SYSTEMS: ELECTROREFINING OF POLYVALENT
METALS IN A LONG-TERM CONTINUOUS PROCESS 97
5.2.1 SIMPLEST LINEAR MODEL 99
5.2.2 NON-LINEAR MATHEMATICAL MODEL 100
5.3 THERMOKINETIC MODELS OF DYNAMICS IN PHYSICO-CHEMICAL SYSTEMS:
THERMAL SELF-DESTRUCTION OF LITHIUM POWER SOURCES WITH HIGH ENERGY
DENSITY 104
5.3.1 A MODEL OF CHEMICAL POWER SOURCE (CPS) SELF-DISCHARGE 105
5.3.2 CONDITIONS OF CPS STABILITY DURING STORAGE 108
5.4 THERMOKINETIC MODEL OF ELECTROLYSIS IN THE CONDITIONS OF ANODE
EFFECT 113
5.4.1 THEORY 113
5.4.2 EXPERIMENTAL VERIFICATION 119
APPENDIX A. DERIVATION OF THE DIFFERENTIAL EQUATIONS (5.11) AND (5.12)
122
APPENDIX B. APPROXIMATE SOLUTION OF THE NON-LINEAR SECOND-ORDER
DIFFERENTIAL EQUATION BY SMALL-PARAMETER (KRYLOV-BOGOLIUBOV) METHOD 124
REFERENCES 125
6 ELECTROCHEMISTRY OF TI(IV) IN IONIC LIQUIDS 127
6.1 WHAT ARE IONIC LIQUIDS? 127
6.2 SOLUTIONS OF TICL 4 IN L-BUTYL-2,3-DIMETHYL IMIDAZOLIUM AZIDE . . .
128
IMAGE 3
CONTENTS XIX
6.3 SOLUTIONS OF TICL 4 IN L-BUTYL-2,3-DIMETHYL IMIDAZOLIUM
TETRAFLUOROBORATE 135
6.3.1 DILUTED SOLUTION (0.025 MOL L _L TICL 4 IN BMMIMBF4). . . 135
6.3.2 "MEDIUM" CONCENTRATION RANGE 139
6.3.3 "CONCENTRATED" SOLUTIONS 140
6.4 SOLUTIONS OF TIF 4 IN L-BUTYL-2,3-DIMETHYLIMIDAZOLIUM
TETRAFLUOROBORATE 142
6.5 CONCLUSIONS 156
REFERENCES 157
AFTERWORD 159
ABOUT THE AUTHORS 161
ABOUT THE EDITOR 163
INDEX 165 |
| any_adam_object | 1 |
| author | Andriiko, Aleksandr A. Andriyko, Yuriy O. Nauer, Gerhard E. |
| author_facet | Andriiko, Aleksandr A. Andriyko, Yuriy O. Nauer, Gerhard E. |
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| author_sort | Andriiko, Aleksandr A. |
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| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541/.37 |
| dewey-search | 541/.37 |
| dewey-sort | 3541 237 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik Chemie |
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| spelling | Andriiko, Aleksandr A. Verfasser aut Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions Aleksandr A. Andriiko ; Yuriy O. Andriyko ; Gerhard E. Nauer Heidelberg [u.a.] Springer 2013 XIX, 167 S. Ill., graph. Darst. 235 mm x 155 mm txt rdacontent n rdamedia nc rdacarrier Monographs in electrochemistry Sukzessivreaktion (DE-588)4346804-4 gnd rswk-swf Elektrochemische Reaktion (DE-588)4151764-7 gnd rswk-swf Ionische Flüssigkeit (DE-588)7548899-1 gnd rswk-swf Salzschmelze (DE-588)4051454-7 gnd rswk-swf Oxidationszahl (DE-588)4173017-3 gnd rswk-swf Elektrochemische Reaktion (DE-588)4151764-7 s Oxidationszahl (DE-588)4173017-3 s Sukzessivreaktion (DE-588)4346804-4 s Salzschmelze (DE-588)4051454-7 s Ionische Flüssigkeit (DE-588)7548899-1 s DE-604 Andriyko, Yuriy O. Verfasser aut Nauer, Gerhard E. Verfasser aut Erscheint auch als Online-Ausgabe 978-3-642-35770-1 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=4198011&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025933068&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Andriiko, Aleksandr A. Andriyko, Yuriy O. Nauer, Gerhard E. Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions Sukzessivreaktion (DE-588)4346804-4 gnd Elektrochemische Reaktion (DE-588)4151764-7 gnd Ionische Flüssigkeit (DE-588)7548899-1 gnd Salzschmelze (DE-588)4051454-7 gnd Oxidationszahl (DE-588)4173017-3 gnd |
| subject_GND | (DE-588)4346804-4 (DE-588)4151764-7 (DE-588)7548899-1 (DE-588)4051454-7 (DE-588)4173017-3 |
| title | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions |
| title_auth | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions |
| title_exact_search | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions |
| title_full | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions Aleksandr A. Andriiko ; Yuriy O. Andriyko ; Gerhard E. Nauer |
| title_fullStr | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions Aleksandr A. Andriiko ; Yuriy O. Andriyko ; Gerhard E. Nauer |
| title_full_unstemmed | Many-electron electrochemical processes reactions in molten salts, room-temperature ionic liquids and ionic solutions Aleksandr A. Andriiko ; Yuriy O. Andriyko ; Gerhard E. Nauer |
| title_short | Many-electron electrochemical processes |
| title_sort | many electron electrochemical processes reactions in molten salts room temperature ionic liquids and ionic solutions |
| title_sub | reactions in molten salts, room-temperature ionic liquids and ionic solutions |
| topic | Sukzessivreaktion (DE-588)4346804-4 gnd Elektrochemische Reaktion (DE-588)4151764-7 gnd Ionische Flüssigkeit (DE-588)7548899-1 gnd Salzschmelze (DE-588)4051454-7 gnd Oxidationszahl (DE-588)4173017-3 gnd |
| topic_facet | Sukzessivreaktion Elektrochemische Reaktion Ionische Flüssigkeit Salzschmelze Oxidationszahl |
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