Small organic molecules on surfaces: fundamentals and applications
Gespeichert in:
| Weitere Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
Springer
2013
|
| Schriftenreihe: | Springer Series in Materials Science
173 |
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XV, 323 S. Ill., graph. Darst. |
| ISBN: | 9783642338472 |
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IMAGE 1
CONTENTS
PART I THEORY
1 THE STRUCTURE OF MOLECULAR ORBITALS INVESTIGATED BY ANGLERESOLVED
PHOTOEMISSION 3
PETER PUSCHNIG, GEORG KOLLER, CLAUDIA DRAXL, AND MICHAEL G. RAMSEY 1.1
INTRODUCTION 4
1.2 THEORY 5
1.2.1 ONE-STEP MODEL OF PHOTOEMISSION 5
1.3 PHOTOEMISSION EXPERIMENTS 9
1.4 RESULTS 9
1.4.1 DETERMINATION OF MOLECULAR ORIENTATIONS 10
1.4.2 IDENTIFICATION OF MOLECULAR ORBITALS 13
1.4.3 RECONSTRUCTION OF MOLECULAR ORBITALS IN REAL SPACE . 17
1.5 CONCLUSION 21
REFERENCES 21
PART II GROWTH MODEL AND INTERFACES
2 PRE-NUCLEATION AND GROWTH OF SELF-ASSEMBLING ORGANIC MOLECULE CRYSTALS
27
A.J. FLEMING AND M.G. RAMSEY 2.1 EXPERIMENTAL METHODOLOGY 30
2.2 PEEM PHOTOEMISSION INTENSITY TIME PLOTS 32
2.3 NUCLEATION MECHANISM OF 6P ON CU (110) 2X1-0 35
2.4 NUCLEATION MECHANISM OF 6P ON CU (110) 37
2.5 6P CONDENSATION AT STEPS DURING PRE-NUCLEATION DEPOSITION PERIOD FOR
6P ON CU (110) 39
2.6 SPONTANEOUS DEWETTING DURING POST-NUCLEATION DEPOSITION PERIOD 41
2.7 PEEM MEASUREMENT OF DIFFUSION ANISOTROPY 42
2.8 DIRECT EVIDENCE OF THE FORMATION OF (20-3) CRITICAL NUCLEI ON CU
(110) 44
VII
HTTP://D-NB.INFO/1025651529
IMAGE 2
VIII CONTENTS
2.9 NUCLEATION DENSITIES OF (20-3) CRITICAL NUCLEI ON CU (110) AND CU
( 1 1 0 ) 2 X 1 - 0 4 6
2.10 CONCLUSIONS 47
REFERENCES 48
3 ORGANIC-ORGANIC HETEROEPITAXY-THE METHOD OF CHOICE TO T\INE OPTICAL
EMISSION OF ORGANIC NANO-FIBERS? 49
CLEMENS SIMBRUNNER, GERARDO HERNANDEZ-SOSA, MARTIN OEHZELT, ROLAND
RESEL, FRANCESCO QUOCHI, DIMITRII NABOK, TATJANA DJURIC, LORENZ ROMANER,
PETER PUSCHNIG, CLAUDIA DRAXL, INGO SALZMANN,
GIINTHER SCHWABEGGER, IRENE WATZINGER, MICHELE SABA, ANDREA MURA,
GIOVANNI BONGIOVANNI, AND HELMUT SITTER 3.1 INTRODUCTION 50
3.2 SHEET SILICATE SUBSTRATES 53
3.2.1 DIOCTAHEDRAL PHYLLOSILICATES (MUSCOVITE MICA, PYROPHYLLITE) 55
3.2.2 TRIOCTAHEDRAL PHYLLOSILICATES (PHLOGOPITE MICA, TALC). 56 3.2.3
FRESHLY CLEAVED MICA SURFACES 57
3.3 EPITAXIAL GROWTH OF ROD-LIKE MOLECULES ON SHEET SILICATES . 59
3.3.1 PARA-HEXAPHENYL 59
3.3.2 SEXITHIOPHENE 62
3.3.3 GROWTH MODEL OF ROD-LIKE MOLECULES ON SHEET SILICATES 65 3.4
ORGANIC HETERO-EPITAXY OF NANO-FIBERS 68
3.5 SUMMARY 74
REFERENCES 75
4 EHRLICH-SCHWOEBEL BARRIERS AND ISLAND NUCLEATION IN ORGANIC THIN-FILM
GROWTH 79
CHRISTIAN TEICHERT, GREGOR HLAWACEK, ADOLF WINKLER, PETER PUSCHNIG, AND
CLAUDIA DRAXL 4.1 INTRODUCTION 80
4.2 EXPERIMENTAL 82
4.3 STEP-EDGE BARRIERS IN ORGANIC THIN-FILM GROWTH 82
4.3.1 FORMATION OF TERRACED GROWTH MOUNDS 83
4.3.2 LEVEL-DEPENDENT EHRLICH-SCHWOEBEL BARRIERS 90
4.4 ISLAND NUCLEATION IN ORGANIC THIN-FILM GROWTH 95
4.4.1 ATOMISTIC NUCLEATION THEORY AND DESORPTION RATE DEPENDENCE OF FILM
FORMATION 96
4.4.2 SCALING THEORIES FOR THE ISLAND-SIZE DISTRIBUTION AND THE
CAPTURE-ZONE DISTRIBUTION 99
4.4.3 DISCUSSION OF THE CRITICAL ISLAND SIZE AND MOLECULAR ORIENTATION
100
4.5 SUMMARY AND OUTLOOK 104
REFERENCES 105
IMAGE 3
CONTENTS IX
5 IN-SITU OBSERVATION OF ORGANIC THIN FILM GROWTH ON GRAPHENE . 1 07
GREGOR HLAWACEK, FAWAD S. KHOKHAR, RAOUL VAN GASTEL, HAROLD J.W.
ZANDVLIET, BENE POELSEMA, AND CHRISTIAN TEICHERT 5.1 INTRODUCTION 107
5.2 EXPERIMENTAL 109
5.2.1 LOW ENERGY ELECTRON MICROSCOPY 109
5.2.2 METAL SUPPORTED GRAPHENE 110
5.2.3 PARA-SEXIPHENYL 110
5.3 GRAPHENE ILL
5.3.1 LAY ER-BY-LAYER GROWTH ILL
5.3.2 STRUCTURE OF THE THICKER LAYER 120
5.3.3 STRANSKI-KRASTANOV GROWTH 124
5.4 IRIDIUM) 111} 127
5.4.1 ISLAND GROWTH 127
5.4.2 STEP FLOW GROWTH 131
5.5 SUMMARY 132
REFERENCES 134
6 T\INING ORGANIC ELECTRONICS VIA PHOTOREACTIVE THIN ORGANIC FILMS . 141
MATTHIAS EDLER, THOMAS GRIESSER, GREGOR TRIMMEL, AND WOLFGANG KERN 6.1
INTRODUCTION 142
6.2 EXAMPLES OF PHOTOREACTIONS 144
6.2.1 PHOTO-FRIES REARRANGEMENT OF AROMATIC ESTERS AND AMIDES 144
6.2.2 PHOTOREACTION OF ORTHO-NITROBENZYL ESTER 145
6.3 TUNING OF MATERIAL PARAMETERS 145
6.3.1 REFRACTIVE INDEX CHANGES INDUCED BY THE PHOTO-FRIES REARRANGEMENT
AND RELATED PHOTOREACTIONS 146
6.3.2 TUNING THE CHEMICAL REACTIVITY 150
6.4 INFLUENCE ON EPITAXIAL GROWTH OF SMALL MOLECULES 152
6.5 APPLICATIONS OF PHOTOREACTIVE POLYMER LAYERS IN ORGANIC ELECTRONICS
153
6.5.1 TUNING THE CHARACTERISTICS OF ORGANIC THIN-FILM TRANSISTORS
(OTFTS) 153
6.5.2 APPLICATION OF PHOTOREACTIVE POLYMERIC LAYERS IN OLEDS . 158 6.6
PHOTOREACTIVE SELF-ASSEMBLED MONOLAYERS 159
6.7 SUMMARY 164
REFERENCES 165
PART III ELECTRICAL PROPERTIES
7 EFFECTIVE MEDIUM APPROXIMATION THEORY DESCRIPTION OF CHARGE-CARRIER
TRANSPORT IN ORGANIC FIELD-EFFECT TRANSISTORS . . . 171 IVAN I. FISHCHUK
AND ANDREY KADASHCHUK 7.1 INTRODUCTION 172
7.2 EMA APPROACH TO HOPPING CHARGE TRANSPORT AT LARGE CHARGE-CARRIER
CONCENTRATIONS 174
IMAGE 4
X CONTENTS
7.2.1 GENERAL EMA THEORY FORMULATION 174
7.2.2 SPATIAL ENERGY CORRELATIONS 177
7.3 CALCULATIONS OF THE CHARGE-CARRIER CONCENTRATION AND THE
ELECTRIC-FIELD DEPENDENCES OF THE CHARGE MOBILITY 178
7.3.1 DEPENDENCE OF THE CHARGE MOBILITY ON CARRIER CONCENTRATION 178
7.3.2 DEPENDENCE OF THE CHARGE-CARRIER MOBILITY ON ELECTRIC FIELD 180
7.3.3 CONCEPT OF STRONG LOCAL FIELDS IN INHOMOGENEOUS MATERIALS 183
7.4 CALCULATIONS OF TEMPERATURE DEPENDENCE OF THE CHARGE-CARRIER
MOBILITY: INFLUENCE OF CARRIER CONCENTRATION AND ELECTRIC FIELD . . 185
7.4.1 THE INFLUENCE OF THE CARRIER CONCENTRATION ON I I ( T ) IN ZERO
ELECTRIC-FIELD LIMIT (MEYER-NELDEL COMPENSATION
RULE) 185
7.4.2 THE INFLUENCE OF THE ELECTRIC FIELD ON /X ( T ) 189
7.5 THE INFLUENCE OF ELECTRIC FIELD ON MEYER-NELDEL TEMPERATURE AND THE
INFLUENCE OF CHARGE CARRIER CONCENTRATION ON GILL TEMPERATURE 193
7.6 CONCLUDING REMARKS ON THE COMPARISON OF DIFFERENT MODELS FOR THE MNR
IN OFETS 196
REFERENCES 199
8 CHARGE TRANSPORT IN ORGANIC DIODES AND OFETS: A COMPARISON . . 203
MUJEEB ULLAH, A. PIVRIKAS, N.S. SARICIFTCI, AND H. SITTER 8.1
INTRODUCTION 204
8.2 EXPERIMENTAL DETAILS AND SAMPLE CONFIGURATION 205
8.3 EVALUATION OF CHARGE CARRIER MOBILITY 206
8.3.1 CHARGE CARRIER MOBILITY MEASUREMENTS BY CHARGE EXTRACTION BY
LINEARLY INCREASING VOLTAGE 207
8.3.2 CHARGE CARRIER MOBILITY MEASUREMENTS BY ORGANIC FIELD-EFFECT
TRANSISTOR 208
8.4 TYPE OF MOBILE CHARGE CARRIERS IN C6O FILMS 209
8.5 CHARGE CARRIER CONCENTRATION DEPENDENCE OF ELECTRON MOBILITY . . 210
8.6 ELECTRIC FIELD DEPENDENCE OF ELECTRON MOBILITY 214
8.7 TEMPERATURE DEPENDENCE OF CHARGE CARRIER MOBILITY 216
8.7.1 MEYER-NELDEL RULE 216
8.7.2 GILL'S LAW 218
8.7.3 ELECTRIC FIELD AND CARRIER CONCENTRATION DEPENDENCE OF
MEYER-NELDEL ENERGY AND GILL ENERGY, RESPECTIVELY . 220 8.8 GRAIN
SIZE DEPENDENCE OF CHARGE CARRIER MOBILITY AND MEYER-NELDEL ENERGY 221
8.9 CONCLUSION 225
REFERENCES 227
IMAGE 5
CONTENTS XI
PART IV OPTICAL PROPERTIES
9 EXCITED-STATE DYNAMICS AND LASER ACTION IN EPITAXIAL ORGANIC
NANOFIBERS 231
FRANCESCO QUOCHI, MICHELE SABA, ANDREA MURA, AND GIOVANNI BONGIOVANNI
9.1 INTRODUCTION 231
9.2 EXCITED-STATE DYNAMICS AND RANDOM LASING OF ORGANIC MEDIA . . 232
9.3 GROWTH AND CHARACTERIZATION OF P- 6P EPITAXIAL NANOFIBERS 233 9.3.1
FLUORESCENCE MICROSCOPY 234
9.3.2 ATOMIC-FORCE MICROSCOPY 235
9.4 EXCITED-STATE DYNAMICS OF P- 6P EPITAXIAL NANOFIBERS 236
9.4.1 TRANSIENT FLUORESCENCE SPECTROSCOPY 237
9.4.2 TRANSIENT ABSORPTION SPECTROSCOPY 238
9.5 OPTICAL AMPLIFICATION AND LASER ACTION IN P- 6P EPITAXIAL NANOFIBERS
239
9.5.1 COHERENT RANDOM LASING VS. AMPLIFIED SPONTANEOUS EMISSION 239
9.5.2 MONOMOLECULAR LASING 241
9.5.3 MICROSCOPIC ORIGIN OF RANDOM LASING 242
9.5.4 GUIDED AMPLIFICATION OF SPONTANEOUS EMISSION 243
9.6 PHOTONIC SENSING USING P- 6P EPITAXIAL NANOFIBERS 244
9.7 SEXIPHENYL-SEXITHIOPHENE HETEROEPITAXIAL NANOFIBERS 244
9.8 CONCLUSION 247
REFERENCES 248
10 IN-SITU, REAL-TIME INVESTIGATION OF ORGANIC THIN FILM GROWTH USING
REFLECTANCE DIFFERENCE SPECTROSCOPY 251
LIDONG SUN AND PETER ZEPPENFELD 10.1 INTRODUCTION 251
10.2 REFLECTANCE DIFFERENCE SPECTROSCOPY (RDS)/REFLECTANCE ANISOTROPY
SPECTROSCOPY (RAS) 252
10.3 RESULTS AND DISCUSSION 255
10.3.1 ORGANIC-INORGANIC HETEROEPITAXY 256
10.3.2 ORGANIC-ORGANIC HETEROEPITAXY ON METAL SURFACE 263 10.4
CONCLUSIONS AND FUTURE PERSPECTIVES 267
REFERENCES 268
PART V DEVICES
11 DIPOLE-CONTROLLED ENERGY LEVEL ALIGNMENT AT DIELECTRIC INTERFACES IN
ORGANIC FIELD-EFFECT TRANSISTORS 273
PHILIPP STADLER, ANNA M. TRACK, GEORG KOLLER, N. SERDAR SARICIFTCI, AND
MICHAEL G. RAMSEY 11.1 INTRODUCTION 273
11.2 MATERIAL AND STRUCTURAL ASPECTS IN OFETS 275
11.3 ORGANIC INTERLAYERS IN OFETS 276
IMAGE 6
XII CONTENTS
11.4 THRESHOLD VOLTAGE AS INTERFACE PARAMETER 278
11.5 THE ROLE OF THE DIELECTRIC INTERLAYER IN OFETS 281
11.6 PHOTOEMISSION SPECTROSCOPY ON TRANSISTOR-RELATED STRUCTURE . . .
283 11.7 DISCUSSION 287
11.8 CONCLUSION AND OUTLOOK 287
11.9 SUMMARY 288
REFERENCES 289
12 NATURAL MATERIALS FOR ORGANIC ELECTRONICS 295
MIHAI IRIMIA-VLADU, ERIC D. GLOWACKI, NIYAZI SERDAR SARICIFTCI, AND
SIEGFRIED BAUER 12.1 INTRODUCTION 295
12.2 NATURAL SUBSTRATES & SMOOTHENING LAYERS 296
12.2.1 NATURAL SUBSTRATES 296
12.2.2 NATURAL SMOOTHENING LAYERS 305
12.3 NATURAL DIELECTRICS & SEMICONDUCTORS 306
12.3.1 NATURAL DIELECTRICS 306
12.3.2 UNIPOLAR AND AMBIPOLAR NATURAL SEMICONDUCTORS 308 12.4
BIOCOMPATIBLE & BIODEGRADABLE ELECTRODES 311
12.5 CONCLUSION 315
REFERENCES 315
INDEX 319 |
| any_adam_object | 1 |
| author2 | Sitter, Helmut 1951- |
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| author_GND | (DE-588)140879765 |
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| building | Verbundindex |
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| ctrlnum | (OCoLC)846891676 (DE-599)DNB1025651529 |
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| dewey-ones | 621 - Applied physics |
| dewey-raw | 621.381045 |
| dewey-search | 621.381045 |
| dewey-sort | 3621.381045 |
| dewey-tens | 620 - Engineering and allied operations |
| discipline | Chemie / Pharmazie Maschinenbau / Maschinenwesen Physik Elektrotechnik / Elektronik / Nachrichtentechnik |
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| genre | (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV040948493 |
| illustrated | Illustrated |
| indexdate | 2024-08-21T00:41:28Z |
| institution | BVB |
| isbn | 9783642338472 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-025927079 |
| oclc_num | 846891676 |
| open_access_boolean | |
| owner | DE-29T DE-11 DE-20 |
| owner_facet | DE-29T DE-11 DE-20 |
| physical | XV, 323 S. Ill., graph. Darst. |
| publishDate | 2013 |
| publishDateSearch | 2013 |
| publishDateSort | 2013 |
| publisher | Springer |
| record_format | marc |
| series | Springer Series in Materials Science |
| series2 | Springer Series in Materials Science |
| spelling | Small organic molecules on surfaces fundamentals and applications Helmut Sitter ... ed. Berlin [u.a.] Springer 2013 XV, 323 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer Series in Materials Science 173 Festkörperoberfläche (DE-588)4127823-9 gnd rswk-swf Wechselwirkung (DE-588)4064937-4 gnd rswk-swf Oberflächenphysik (DE-588)4134881-3 gnd rswk-swf Oberflächenreaktion (DE-588)4140095-1 gnd rswk-swf Optoelektronik (DE-588)4043687-1 gnd rswk-swf Organisches Molekül (DE-588)4133471-1 gnd rswk-swf Molekül (DE-588)4039972-2 gnd rswk-swf Polymerelektronik (DE-588)7735306-7 gnd rswk-swf Oberfläche (DE-588)4042907-6 gnd rswk-swf Grenzfläche (DE-588)4021991-4 gnd rswk-swf Organisches Halbleiterbauelement (DE-588)7737294-3 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Polymerelektronik (DE-588)7735306-7 s Optoelektronik (DE-588)4043687-1 s Organisches Halbleiterbauelement (DE-588)7737294-3 s Organisches Molekül (DE-588)4133471-1 s DE-604 Festkörperoberfläche (DE-588)4127823-9 s Molekül (DE-588)4039972-2 s Wechselwirkung (DE-588)4064937-4 s 1\p DE-604 Grenzfläche (DE-588)4021991-4 s 2\p DE-604 Oberfläche (DE-588)4042907-6 s 3\p DE-604 Oberflächenreaktion (DE-588)4140095-1 s 4\p DE-604 Oberflächenphysik (DE-588)4134881-3 s 5\p DE-604 Sitter, Helmut 1951- (DE-588)140879765 edt Erscheint auch als Online-Ausgabe 978-3-642-33848-9 Springer Series in Materials Science 173 (DE-604)BV000683335 173 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=4116209&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025927079&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 2\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 3\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 4\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 5\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Small organic molecules on surfaces fundamentals and applications Springer Series in Materials Science Festkörperoberfläche (DE-588)4127823-9 gnd Wechselwirkung (DE-588)4064937-4 gnd Oberflächenphysik (DE-588)4134881-3 gnd Oberflächenreaktion (DE-588)4140095-1 gnd Optoelektronik (DE-588)4043687-1 gnd Organisches Molekül (DE-588)4133471-1 gnd Molekül (DE-588)4039972-2 gnd Polymerelektronik (DE-588)7735306-7 gnd Oberfläche (DE-588)4042907-6 gnd Grenzfläche (DE-588)4021991-4 gnd Organisches Halbleiterbauelement (DE-588)7737294-3 gnd |
| subject_GND | (DE-588)4127823-9 (DE-588)4064937-4 (DE-588)4134881-3 (DE-588)4140095-1 (DE-588)4043687-1 (DE-588)4133471-1 (DE-588)4039972-2 (DE-588)7735306-7 (DE-588)4042907-6 (DE-588)4021991-4 (DE-588)7737294-3 (DE-588)4143413-4 |
| title | Small organic molecules on surfaces fundamentals and applications |
| title_auth | Small organic molecules on surfaces fundamentals and applications |
| title_exact_search | Small organic molecules on surfaces fundamentals and applications |
| title_full | Small organic molecules on surfaces fundamentals and applications Helmut Sitter ... ed. |
| title_fullStr | Small organic molecules on surfaces fundamentals and applications Helmut Sitter ... ed. |
| title_full_unstemmed | Small organic molecules on surfaces fundamentals and applications Helmut Sitter ... ed. |
| title_short | Small organic molecules on surfaces |
| title_sort | small organic molecules on surfaces fundamentals and applications |
| title_sub | fundamentals and applications |
| topic | Festkörperoberfläche (DE-588)4127823-9 gnd Wechselwirkung (DE-588)4064937-4 gnd Oberflächenphysik (DE-588)4134881-3 gnd Oberflächenreaktion (DE-588)4140095-1 gnd Optoelektronik (DE-588)4043687-1 gnd Organisches Molekül (DE-588)4133471-1 gnd Molekül (DE-588)4039972-2 gnd Polymerelektronik (DE-588)7735306-7 gnd Oberfläche (DE-588)4042907-6 gnd Grenzfläche (DE-588)4021991-4 gnd Organisches Halbleiterbauelement (DE-588)7737294-3 gnd |
| topic_facet | Festkörperoberfläche Wechselwirkung Oberflächenphysik Oberflächenreaktion Optoelektronik Organisches Molekül Molekül Polymerelektronik Oberfläche Grenzfläche Organisches Halbleiterbauelement Aufsatzsammlung |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=4116209&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025927079&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000683335 |
| work_keys_str_mv | AT sitterhelmut smallorganicmoleculesonsurfacesfundamentalsandapplications |