The molecule-metal interface:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH
2013
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XIV, 255 S. graph. Darst. |
| ISBN: | 9783527410606 9783527653171 |
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Datensatz im Suchindex
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| adam_text | IMAGE 1
CONTENTS
PREFACE X I
LIST O F CONTRIBUTORS XIII
1 INTRODUCTION TO THE MOLECULE-METAL INTERFACE 1 NOBUO UENO, NORBERT
KOCH, AND ANDREW T.S. WEE 1.1 FROM ORGANIC SEMICONDUCTORS TO ORGANIC
ELECTRONIC DEVICES 1 1.2 ROLE A N D FUNCTION O F INTERFACES IN ORGANIC
ELECTRONIC DEVICES 3 1.3 WHAT WILL WE LEARN ABOUT THE INTERFACES? 4
1.4 THE FERMI LEVEL A N D RELATED FUNDAMENTALS 6
1.4.1 DEFINITION O F THE FERMI LEVEL I N THIS BOOK 6 1.4.2 MEASURING THE
FERMI LEVEL O F ORGANIC SEMICONDUCTORS 8 1.4.3 THE WORK FUNCTION A N D
THE VACUUM LEVEL O F A SOLID WITH FINITE SIZE REFERENCES 13
PART O N E THEORY 15
2 BASIC THEORY O F T H E MOLECULE-METAL INTERFACE 17 FERNANDO FLORES AND
JOSE ORTEGA 2.1 INTRODUCTION 17
2.2 THE MOLECULE ENERGY GAP PROBLEM: IMAGE POTENTIAL EFFECTS 20 2.2.1
MOLECULE SELF-INTERACTION ENERGY 20 2.2.2 IMAGE POTENTIAL EFFECTS 25
2.3 THE UNIFIED IDIS MODEL: CHARGE TRANSFER, PAULI EXCLUSION PRINCIPLE
( PILLOW ) EFFECT A N D MOLECULAR DIPOLES 28 2.3.1 THE IDIS MODEL 28
2.3.2 PAULI REPULSION ( PILLOW ) EFFECT A N D THE UNIFIED IDIS-MODEL 31
2.3.3 MOLECULAR DIPOLE CORRECTIONS A N D THE UNIFIED IDIS MODEL 34 2.4
DFT CALCULATIONS FOR A SINGLE MOLECULE O N A SURFACE 35 2.4.1 C60 O N A
U ( L L L ) 35
2.4.2 T C N Q / A U ( L L L ) 38
2.4.3 TTF O N A U ( L L L ) 39
2.5 FROM A SINGLE MOLECULE TO A MONOLAYER 42
2.5.1 THE UNIFIED IDIS MODEL FOR A N ORGANIC AD-LAYER O N A METAL 42
2.5.2 C 6 0 / A U ( L L L ) 43
HTTP://D-NB.INFO/1027115861
IMAGE 2
V I | CONTENTS
2.5.3 T T F / A U ( L L L ) 4 5
2.5.4 MORE O N THE UNIFIED IDIS MODEL 46
REFERENCES 4 8
3 UNDERSTANDING T H E METAL-MOLECULE INTERFACE FROM FIRST PRINCIPLES 51
LEEOR KRONIK AND YOSHITADA MORIKAWA 3.1 INTRODUCTION 51
3.2 A BRIEF OVERVIEW O F DENSITY FUNCTIONAL THEORY 53 3.3 ELECTRONIC
STRUCTURE O F METAL-MOLECULE INTERFACES FROM DENSITY FUNCTIONAL THEORY:
CHALLENGES A N D PROGRESS 59
3.4 UNDERSTANDING METAL-MOLECULE INTERFACE DIPOLES F R O M FIRST
PRINCIPLES 64 3.4.1 N-ALKANE/METAL INTERFACES 6 7 3.4.2 BENZENE/METAL
INTERFACES 68
3.4.3 PENTACENE/METAL INTERFACES 72 3.4.4 PTCDA/METAL INTERFACES 75 3.5
TWO EXAMPLES O F COLLECTIVE EFFECTS AT METAL-MOLECULE INTERFACES 7 7
3.5.1 QUANTUM-CONFINED STARK EFFECT I N MONOLAYERS O F MOLECULES
CONSISTING
O F POLAR REPEATING UNITS 77 3.5.2 MAGNETIC MOLECULE/MAGNETIC METAL
INTERFACES 79 3.6 CONCLUDING REMARKS 81
REFERENCES 81
PART TWO ATOMIC STRUCTURE 91
4 STM STUDIES O F MOLECULE-METAL INTERFACES 93 SWEE LIANG WONG, HAN
HUANG, ANDREW T.S. WEE, AND WEI CHEN 4.1 INTRODUCTION TO SCANNING
TUNNELING MICROSCOPY 94 4.1.1 BASIC STM OPERATION 94
4.1.2 THEORY O F STM 96
4.1.3 SCANNING TUNNELING SPECTROSCOPY 98 4.2 FACTORS AFFECTING MOLECULAR
PACKING O N PERFECT SURFACES 100 4.2.1 MOLECULE-SUBSTRATE VS.
INTERMOLECULAR INTERACTIONS 100 4.2.2 COMMENSURABILITY WITH SUBSTRATE
103 4.2.3 MOLECULAR DENSITY DEPENDENT PHASE TRANSITIONS 104 4.3
INFLUENCE O F INHOMOGENEITY AT METAL SURFACES 106 4.3.1 PHYSICAL
INHOMOGENEITY AT CRYSTALLINE INTERFACES 106
4.3.2 SURFACE ELECTRONIC STATES 108 4.3.3 MOLECULE-INDUCED MODIFICATION
O F SURFACE TOPOGRAPHY 109 4.4 MANIPULATION O F MOLECULES USING STM 112
4.5 SUMMARY 11 6
REFERENCES 116
5 NEXAFS STUDIES O F MOLECULAR ORIENTATIONS AT MOLECULE-SUBSTRATE
INTERFACES 119 DONG-CHEN QI, WEI CHEN, AND ANDREW T.S. WEE 5.1
PRINCIPLES O F NEXAFS 120
IMAGE 3
CONTENTS | V I I
5.1.1 THE X-RAY ABSORPTION PROCESS 120
5.1.2 MOLECULAR ORBITALS A N D CHARACTERISTIC RESONANCES I N /(-SHELL
NEXAFS SPECTRA 123 5.1.3 MOLECULAR ORIENTATION A N D POLARIZATION
DEPENDENCE O F THE RESONANCE INTENSITIES 125 5.1.4 TECHNIQUES A N D
INSTRUMENTATION O F NEXAFS 127 5.1.5 RADIATION DAMAGE O F NEXAFS 129 5.2
MOLECULAR ORIENTATIONS AT INTERFACES: THE EFFECT O F MOLECULE-SUBSTRATE
INTERACTIONS 129
5.2.1 ORGANIC/METAL INTERFACES 130 5.2.2 ORGANIC/SEMICONDUCTOR
INTERFACES 132 5.2.3 ORGANIC/ORGANIC HETEROJUNCTION INTERFACES 136 5.2.4
CUPC O N OTHER TECHNOLOGICALLY IMPORTANT SUBSTRATES 139 5.3 MOLECULAR
ORIENTATIONS AT INTERFACES: THE EFFECT O F STRONG INTERMOLECULAR
INTERACTIONS 140
5.4 MOLECULAR ORIENTATIONS O F SELF-ASSEMBLED MONOLAYERS 143 5.5 SUMMARY
A N D OUTLOOK 147
REFERENCES 148
6 X-RAY STANDING WAVES AND SURFACES X-RAY SCATTERING STUDIES O F
MOLECULE-METAL INTERLACES 153 ALEXANDER GERLACH, CHRISTOPH BURKER,
TAKUYA HOSOKAI, AND FRANK SCHREIBER 6.1 INTRODUCTION 153
6.2 X-RAY STANDING WAVE THEORY 154
6.2.1 GENERAL CONSIDERATIONS O N WAVE FIELDS IN CRYSTALS 154 6.2.2 T H E
TWO-BEAM APPROXIMATION 155 6.2.3 T H E DARWIN CURVE 156
6.2.4 X-RAY ABSORPTION A N D DIPOLE APPROXIMATION 159 6.2.5 THE COHERENT
POSITION A N D THE COHERENT FRACTION 161 6.3 X-RAY STANDING WAVE
EXPERIMENTS 162
6.3.1 BEAMLINE SETUP AT ID32 162
6.3.2 EXPERIMENTAL DETAILS 163
6.4 EXAMPLES: ORGANIC MONOLAYERS O N METALS 164 REFERENCES 170
PART THREE ELECTRONIC STRUCTURE 173
7 FUNDAMENTAL ELECTRONIC STRUCTURE O F ORGANIC SOLIDS AND THEIR
INTERFACES BY PHOTOEMISSION SPECTROSCOPY AND RELATED METHODS 175 NOBUO
UENO, SATOSHI KERA, AND KANAME KANAI 7.1 INTRODUCTION 175
7.2 GENERAL VIEW O F ELECTRONIC STRUCTURE O F ORGANIC SOLIDS 176 7.2.1
FROM SINGLE MOLECULE TO MOLECULAR SOLID 176 7.2.2 CONTRIBUTION O F
POLARON 17 9
7.2.3 REQUIREMENT FROM THERMODYNAMIC EQUILIBRIUM 179 7.3 ELECTRONIC
STRUCTURE I N RELATION TO CHARGE TRANSPORT 180
IMAGE 4
V I I I | CONTENTS
7.3.1 ULTRAVIOLET PHOTOEMISSION SPECTROSCOPY 180
7.3.1.1 ENERGY A N D M O M E N T U M CONSERVATION 180 7.3.1.2 ENERGY
BAND DISPERSION A N D ESTIMATION O F BAND TRANSPORT MOBILITY 183 7.3.1.3
DENSITY O F STATES EFFECTS I N POLYCRYSTALLINE FILMS 184 7.3.2 ELECTRON
SPECTROSCOPY USING METASTABLE ATOM BEAM: CHARACTERIZATION
O F THE MOLECULAR ORIENTATION VIA WAVEFUNCTION SPREAD 186 7.3.2.1
PRINCIPLE A N D CHARACTERISTICS 188 7.3.2.2 CHARACTERIZATION O F THE
MOLECULAR ORIENTATION 189 7.3.2.3 SPATIAL WAVEFUNCTION DISTRIBUTION O F
BAND GAP STATES 190
7.3.3 INVERSE PHOTOEMISSION SPECTROSCOPY (IPES) 191 7.3.3.1
CHARACTERISTICS O F IPES 191 7.3.3.2 COMPARISON BETWEEN UPS-IPES A N D
TUNNELING SPECTROSCOPY 195 7.3.3.3 COMPARISON WITH NEAR-EDGE X-RAY
ABSORPTION FINE STRUCTURE
SPECTROSCOPY (NEXAFS) 198 7.3.4 PROBING ELECTRON-PHONON COUPLING,
HOPPING MOBILITY A N D POLARON BY UPS 200
7.3.4.1 BASIC BACKGROUND 200 7.3.4.2 EXPERIMENTAL REORGANIZATION ENERGY
A N D POLARON BINDING ENERGY 202 7.4 ELECTRONIC STRUCTURE AT WEAKLY
INTERACTING INTERFACES 206 7.4.1 EFFECTS O F INHOMOGENEITY O F THE
SUBSTRATE SURFACE ON THE ENERGY LEVEL
ALIGNMENT 206
7.4.2 STRANGE BAND BENDING 207
7.4.3 RADIATION EFFECTS O N THE ENERGY LEVEL ALIGNMENT 208 7.4.4
MYSTERIOUS PHENOMENA: FERMI LEVEL ALIGNMENT ISSUE 209 7.4.4.1 IMPACTS O
F INTERFACE DIPOLE LAYER ON THE ENERGY LEVEL ALIGNMENT 209 7.4.4.2
IMPACTS O F DISORDER O N THE ENERGY LEVEL ALIGNMENT A N D BAND
BENDING . 211
7.5 SUMMARY 213
REFERENCES 214
8 ENERGY LEVELS A T MOLECULE-METAL INTERFACES 219 ANTOINE KAHN AND
NORBERT KOCH 8.1 INTRODUCTION 219
8.2 THE ORGANIC-ELECTRODE INTERFACE 221
8.3 GAP STATES 223
8.4 METAL ELECTRODES 228
8.5 TUNING O F CHARGE INJECTION BARRIERS 232
8.5.1 STRONG ELECTRON ACCEPTOR A N D DONOR MOLECULES 234 8.5.2
SELF-ASSEMBLED MONOLAYERS WITH DIPOLES 236 8.6 CONDUCTIVE POLYMER
ELECTRODES 237
REFERENCES 238
9 VIBRATIONAL SPECTROSCOPIES FOR FUTURE STUDIES O F MOLECULE-METAL
INTERFACE 243 WEI-YANG CHOU 9.1 INTRODUCTION 243
IMAGE 5
CONTENTS | I X
9.2 SELECTION RULES FOR INFRARED A N D RAMAN SPECTRA 244
9.3 RAMAN/IR APPLICATION IN ORGANIC FILMS 245
REFERENCES 249
10 GENERAL OUTLOOK 251 NORBERT KOCH, NOBUO UENO, AND ANDREW T.S. WEE
INDEX 253
|
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| indexdate | 2024-07-10T00:34:32Z |
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| language | English |
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| publisher | Wiley-VCH |
| record_format | marc |
| spelling | The molecule-metal interface ed. by Norbert Koch ... Weinheim Wiley-VCH 2013 XIV, 255 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Physics Surface chemistry Surfaces (Physics) Oberflächenphysik (DE-588)4134881-3 gnd rswk-swf Molekülverbindungen (DE-588)4170388-1 gnd rswk-swf Grenzflächenphysik (DE-588)4452968-5 gnd rswk-swf Grenzflächenchemie (DE-588)4246080-3 gnd rswk-swf Metallverbindungen (DE-588)4169640-2 gnd rswk-swf Grenzflächenphysik (DE-588)4452968-5 s Grenzflächenchemie (DE-588)4246080-3 s DE-604 Oberflächenphysik (DE-588)4134881-3 s Metallverbindungen (DE-588)4169640-2 s Molekülverbindungen (DE-588)4170388-1 s Koch, Norbert 1971- Sonstige (DE-588)1035399520 oth Erscheint auch als Online-Ausgabe, EPUB 978-3-527-65319-5 Erscheint auch als Online-Ausgabe, MOBI 978-3-527-65318-8 Erscheint auch als Online-Ausgabe, PDF 978-3-527-65320-1 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025859660&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | The molecule-metal interface Physics Surface chemistry Surfaces (Physics) Oberflächenphysik (DE-588)4134881-3 gnd Molekülverbindungen (DE-588)4170388-1 gnd Grenzflächenphysik (DE-588)4452968-5 gnd Grenzflächenchemie (DE-588)4246080-3 gnd Metallverbindungen (DE-588)4169640-2 gnd |
| subject_GND | (DE-588)4134881-3 (DE-588)4170388-1 (DE-588)4452968-5 (DE-588)4246080-3 (DE-588)4169640-2 |
| title | The molecule-metal interface |
| title_auth | The molecule-metal interface |
| title_exact_search | The molecule-metal interface |
| title_full | The molecule-metal interface ed. by Norbert Koch ... |
| title_fullStr | The molecule-metal interface ed. by Norbert Koch ... |
| title_full_unstemmed | The molecule-metal interface ed. by Norbert Koch ... |
| title_short | The molecule-metal interface |
| title_sort | the molecule metal interface |
| topic | Physics Surface chemistry Surfaces (Physics) Oberflächenphysik (DE-588)4134881-3 gnd Molekülverbindungen (DE-588)4170388-1 gnd Grenzflächenphysik (DE-588)4452968-5 gnd Grenzflächenchemie (DE-588)4246080-3 gnd Metallverbindungen (DE-588)4169640-2 gnd |
| topic_facet | Physics Surface chemistry Surfaces (Physics) Oberflächenphysik Molekülverbindungen Grenzflächenphysik Grenzflächenchemie Metallverbindungen |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025859660&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT kochnorbert themoleculemetalinterface |