Condensed-phase molecular spectroscopy and photophysics:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Hoboken, NJ
Wiley
2013
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis Klappentext |
| Beschreibung: | Includes index. |
| Beschreibung: | XIII, 330 S. Ill., graph. Darst. |
| ISBN: | 9780470946701 |
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| 245 | 1 | 0 | |a Condensed-phase molecular spectroscopy and photophysics |c Anne Myers Kelley |
| 264 | 1 | |a Hoboken, NJ |b Wiley |c 2013 | |
| 300 | |a XIII, 330 S. |b Ill., graph. Darst. | ||
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| 500 | |a Includes index. | ||
| 650 | 4 | |a Quantentheorie | |
| 650 | 4 | |a Condensed matter |x Spectra | |
| 650 | 4 | |a Molecular spectroscopy | |
| 650 | 4 | |a Quantum theory | |
| 650 | 4 | |a Semiconductors |x Spectra | |
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Datensatz im Suchindex
| _version_ | 1804150133661630464 |
|---|---|
| adam_text | CONTENTS
PREFACE
xi
1 REVIEW
OF TIME-INDEPENDENT QUANTUM MECHANICS
1
1.1
States, Operators, and Representations
/ 1
1.2
Eigenvalue Problems and the
Schrödinger
Equation
/ 4
1.3
Expectation Values, Uncertainty Relations
/ 6
1.4
The Particle in a Box
/ 7
1.5
Harmonic Oscillator
/ 9
1.6
The Hydrogen Atom and Angular Momentum
/ 12
1.7
Approximation Methods
/15
1.8
Electron Spin
/ 18
1.9
The Born-Oppenheimer Approximation
/ 22
1.10
Molecular
Orbitals / 22
1.11
Energies and Time Scales; Separation of Motions
/ 25
Further Reading
/ 26
Problems
/ 27
2
ELECTROMAGNETIC RADIATION
31
2.1
Classical Description of Light
/ 31
2.2
Quantum Mechanical Description of Light
/ 35
2.3
Fourier Transform Relationships Between Time and
Frequency
/ 38
VÍ
CONTENTS
2.4
Blackbody
Radiation / 40
2.5 Light
Sources
for Spectroscopy
/ 42
References and Further Reading
/ 44
Problems
/ 44
3
RADIATION-MATTER INTERACTIONS
47
3.1
The Time-Dependent
Schrödinger
Equation
/ 47
3.2
Time-Dependent Perturbation Theory
/ 50
3.3
Interaction of Matter with the Classical Radiation Field
/ 54
3.4
Interaction of Matter with the Quantized Radiation Field
/ 59
References and Further Reading
/ 63
Problems
/ 64
4
ABSORPTION AND EMISSION OF LIGHT
67
4.1
Einstein Coefficients for Absorption and Emission
/ 67
4.2
Other Measures of Absorption Strength
/ 69
4.3
Radiative Lifetimes
/ 72
4.4
Oscillator Strengths
/ 73
4.5
Local Fields
/ 73
Further Reading
/ 74
Problems
/ 75
5
SYSTEM-BATH INTERACTIONS
79
5.1
Phenomenological Treatment of Relaxation and Lineshapes
/ 79
5.2
The Density Matrix
/ 86
5.3
Density Matrix Methods in Spectroscopy
/ 90
5.4
Exact Density Matrix Solution for a Two-Level System
/ 95
References and Further Reading
/ 98
Problems
/ 98
6
SYMMETRY CONSIDERATIONS
103
6.1
Qualitative Aspects of Molecular Symmetry
/ 103
6.2
Introductory Group Theory
/ 104
6.3
Finding the Symmetries of Vibrational Modes of a Certain
Type
/ 109
6.4
Finding the Symmetries of All Vibrational Modes
/
111
Further Reading
/113
Problems
/ 113
CONTENTS
VÌI
7
MOLECULAR
VIBRATIONS
AND INFRARED
SPECTROSCOPY
115
7.1
Vibrational Transitions
/115
7.2
Diatomic Vibrations
/117
7.3
Anharmonicity
/118
7.4
Polyatomic Molecular Vibrations: Normal Modes
/ 121
7.5
Symmetry Considerations
/ 127
7.6
Isotopie
Shifts
/ 130
7.7
Solvent Effects on Vibrational Spectra
/ 130
References and Further Reading
/135
Problems
/ 135
8
ELECTRONIC SPECTROSCOPY
139
8.1
Electronic Transitions
/ 139
8.2
Spin and Orbital Selection Rules
/ 141
8.3
Spin-Orbit Coupling
/ 143
8.4
Vibronic Structure
/ 143
8.5
Vibronic Coupling
/ 148
8.6
The Jahn-Teller Effect
/ 151
8.7
Considerations in Large Molecules
/ 152
8.8
Solvent Effects on Electronic Spectra
/ 154
Further Reading
/ 159
Problems
/ 160
9
PHOTOPHYSICAL PROCESSES
163
9.1
Jabłoński
Diagrams
/163
9.2
Quantum Yields and Lifetimes
/166
9.3
Fermi s Golden Rule for Radiationless Transitions
/ 167
9.4
Internal Conversion and Intersystem Crossing
/167
9.5
Intramolecular Vibrational Redistribution
/ 173
9.6
Energy Transfer
/179
9.7
Polarization and Molecular Reonentation in Solution
/182
References and Further Reading
/ 186
Problems
/ 186
10
LIGHT SCATTERING
191
10.1
Rayleigh Scattering from Particles
/191
10.2
Classical Treatment of Molecular Raman and Rayleigh
Scattering
/ 193
VIU
CONTENTS
10.3
Quantum
Mechanical Treatment of Molecular Raman and
Rayleigh Scattering
/ 195
10.4
Nonresonant
Raman Scattering
/ 204
10.5
Symmetry Considerations and Depolarization Ratios in Raman
Scattering
/ 206
10.6
Resonance Raman Spectroscopy
/ 207
References and Further Reading
/211
Problems
/ 211
11
NONLINEAR AND PUMP-PROBE SPECTROSCOPIES
215
11.1
Linear and Nonlinear Susceptibilities
/ 215
11.2
Multiphoton Absorption
/ 216
11.3
Pump-Probe Spectroscopy: Transient Absorption and Stimulated
Emission
/ 219
11.4
Vibrational Oscillations and Impulsive Stimulated
Scattering
/ 225
11.5
Second Harmonic and Sum Frequency Generation
/ 227
11.6
Four-Wave Mixing
/ 232
11.7
Photon Echoes
/ 232
References and Further Reading
/ 234
Problems
/ 234
12
ELECTRON TRANSFER PROCESSES
239
12.1
Charge-Transfer Transitions
/ 239
12.2
Marcus Theory
/ 243
12.3
Spectroscopy of Anions and Cations
/ 247
References and Further Reading
/ 248
Problems
/ 248
13
COLLECTIONS OF MOLECULES
251
13.1
Van
der Waals
Molecules
/ 251
13.2
Dimers and Aggregates
/ 252
13.3
Localized and Delocalized Excited States
/ 253
13.4
Conjugated Polymers
/ 256
References
/ 259
Problems
/ 259
14
METALS AND PLASMONS
263
14.1
Dielectric Function of a Metal
/ 263
14.2
Plasmons
/ 266
CONTENTS
ІХ
14.3
Spectroscopy of Metal Nanoparticles
/ 268
14.4
Surface-Enhanced Raman and Fluorescence
/ 270
References and Further Reading
/ 274
Problems
/ 275
15
CRYSTALS
277
15.1
Crystal Lattices
/ 277
15.2
Phonons in Crystals
/ 281
15.3
Infrared and Raman Spectra
/ 284
15.4
Phonons in Nanocrystals
/ 286
References and Further Reading
/ 287
Problems
/ 287
16
ELECTRONIC SPECTROSCOPY OF SEMICONDUCTORS
291
16.1
Band Structure
/ 291
16.2
Direct and Indirect Transitions
/ 296
16.3
Excitons
/ 296
16.4
Defects
/ 298
16.5
Semiconductor Nanocrystals
/ 298
Further Reading
/ 302
Problems
/ 302
APPENDICES
A PHYSICAL CONSTANTS, UNIT SYSTEMS,
AND CONVERSION FACTORS
305
В
MISCELLANEOUS MATHEMATICS REVIEW
309
С
MATRICES AND DETERMINANTS
313
D
CHARACTER TABLES FOR SOME COMMON
POINT GROUPS
317
E
FOURIER TRANSFORMS
321
INDEX
323
An
introduction to one of the fundamental tools
in chemical research- -spectroscopy and photophysics
in condensed-phase and extended systems
grcal
deal ot modern research in chemistry and materials science involves the interaction
ot radiation with condensed-phase systems such as molecules in liquids and solids as well
as molecule* in more complex media, molecular aggregates, metals, semiconductors, and
composites. Condensed Phase Molecular Spectroscopy and Photophysics was developed to
till the need tor a textbook that introduces the basics ot traditional molecular spectroscopy
v it
h
a strong emphasis on condensed-phase >vstetns. It also examines optical processes in
extended s steins
stidi
as metals, semiconductor--, And conducting polymers, and atldresses
(he unique optical properties
Ы
Banoscaie systems
Condensed Phase Molecular Spectroscopy and Photophysics begins with an introduction to
quantum
mechanic-, thai -its a solid foundation for understanding the text s
subséquent
topics, including:
•
Electromagnetic radiation and radiation matter interactions
•
Molecular vibrations and infrared spectroscopy
•
Electronic spectroscopy
•
Photoplu
^н
al
processes
anti
light
scattering
Nonlinear
anti
pump-probe ^pectroseopies
•
Electron transfer processes
Each chapter contains problems ranging From simple to complex, enabling reatlers to
gradually build then skills And problem-solving abilities. Written tor upper-level under
gt aduate and graduate courses in physical and materials ehembtiv. this text is uniquely
designed to
equi})
readers to solve a broad array ot current problems and challenge
-
in ehemtsUA-
ΛΝΝΕ
MYERS KELLEY earned a BS in chemistrv
ťrom
the Umversitv ot California, Riverside.
m
1980
ňnd
a PhD in biophysical chemistrv
trom
the University or California, Berkeley,
m
19Я4-
Foilowing po^iloctoral work at the Univer^itv ot Pennsvlvania. she held faculty positions, at the
Universitv ot Rochester 1
1987-1999)
and Kansas State University
(1999-2003}
before becom¬
ing one of the founding tacultv at the Universitv of California. Merced,
m
2003.
Her primary
ni h
area has been resonance Raman sptxMveeapf, linear and nonlinear, but she has also
worked in several other areas of spectroscopv including single
rnolecuie
and line-narrowed
fluorescence,
tour wave
mixing, and time-resolved methods. She is a Fellow of the American
Physical SocietN and the American Ass<xidtion for the Advancement of Science.
ИГ
Design:
Míchati Rutkouski
.
гг
llíuítrjtioii:
&
Anne Savers fCefiev
ibscribe to our
frçe Cner-isîrv eNewsletter
at
Visit
w
¡ey.com/cremistry
wilev.com
Also available
as an e-book
170-0-4 70-4 41=70-1
90000
9 780470 946701
|
| any_adam_object | 1 |
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| author_facet | Myers Kelley, Anne |
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| classification_tum | CHE 160f |
| ctrlnum | (OCoLC)835334357 (DE-599)BVBBV040797466 |
| dewey-full | 543/.54 |
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| dewey-ones | 543 - Analytical chemistry |
| dewey-raw | 543/.54 |
| dewey-search | 543/.54 |
| dewey-sort | 3543 254 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik Chemie |
| format | Book |
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| id | DE-604.BV040797466 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T00:34:05Z |
| institution | BVB |
| isbn | 9780470946701 |
| language | English |
| lccn | 2012040299 |
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| physical | XIII, 330 S. Ill., graph. Darst. |
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| spelling | Myers Kelley, Anne Verfasser aut Condensed-phase molecular spectroscopy and photophysics Anne Myers Kelley Hoboken, NJ Wiley 2013 XIII, 330 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Includes index. Quantentheorie Condensed matter Spectra Molecular spectroscopy Quantum theory Semiconductors Spectra Fotophysik (DE-588)4193388-6 gnd rswk-swf Spektroskopie (DE-588)4056138-0 gnd rswk-swf Flüssigkeit (DE-588)4017621-6 gnd rswk-swf Spektroskopie (DE-588)4056138-0 s Flüssigkeit (DE-588)4017621-6 s Fotophysik (DE-588)4193388-6 s DE-604 Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025777635&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025777635&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext |
| spellingShingle | Myers Kelley, Anne Condensed-phase molecular spectroscopy and photophysics Quantentheorie Condensed matter Spectra Molecular spectroscopy Quantum theory Semiconductors Spectra Fotophysik (DE-588)4193388-6 gnd Spektroskopie (DE-588)4056138-0 gnd Flüssigkeit (DE-588)4017621-6 gnd |
| subject_GND | (DE-588)4193388-6 (DE-588)4056138-0 (DE-588)4017621-6 |
| title | Condensed-phase molecular spectroscopy and photophysics |
| title_auth | Condensed-phase molecular spectroscopy and photophysics |
| title_exact_search | Condensed-phase molecular spectroscopy and photophysics |
| title_full | Condensed-phase molecular spectroscopy and photophysics Anne Myers Kelley |
| title_fullStr | Condensed-phase molecular spectroscopy and photophysics Anne Myers Kelley |
| title_full_unstemmed | Condensed-phase molecular spectroscopy and photophysics Anne Myers Kelley |
| title_short | Condensed-phase molecular spectroscopy and photophysics |
| title_sort | condensed phase molecular spectroscopy and photophysics |
| topic | Quantentheorie Condensed matter Spectra Molecular spectroscopy Quantum theory Semiconductors Spectra Fotophysik (DE-588)4193388-6 gnd Spektroskopie (DE-588)4056138-0 gnd Flüssigkeit (DE-588)4017621-6 gnd |
| topic_facet | Quantentheorie Condensed matter Spectra Molecular spectroscopy Quantum theory Semiconductors Spectra Fotophysik Spektroskopie Flüssigkeit |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025777635&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025777635&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT myerskelleyanne condensedphasemolecularspectroscopyandphotophysics |