Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions:
Gespeichert in:
| 1. Verfasser: | |
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| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
2012
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| Schlagworte: | |
| Online-Zugang: | kostenfrei Inhaltsverzeichnis |
| Beschreibung: | Nebentitel: Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen |
| Beschreibung: | 127 Bl. Ill., graph. Darst. |
Internformat
MARC
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| 245 | 1 | 0 | |a Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |c Yan Zhang |
| 246 | 1 | 3 | |a Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen |
| 264 | 1 | |c 2012 | |
| 300 | |a 127 Bl. |b Ill., graph. Darst. | ||
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| 500 | |a Nebentitel: Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen | ||
| 502 | |a Berlin, Freie Univ., Diss., 2012 | ||
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Datensatz im Suchindex
| _version_ | 1804149412825399296 |
|---|---|
| adam_text | IMAGE 1
CONTENTS
CHAPTER 1 INTRODUCTION
1.1 HOMOGENEOUS NUCLEATION IN SINGLE LEVITATED DROPLETS 2
1.2 CHARGE EFFECTS ON HOMOGENEOUS NUCLEATION 7
1.3 ORGANIZATION O F THIS THESIS 8
10
12
16
20
23
26
29
29
31
33
33
33
CHAPTER 3 EXPERIMENTAL DETAILS
3.1 OPTICAL LEVITATION O F SINGLE DROPLET 35
3.2 XANES SPECTROSCOPY ON SINGLE LEVITATED DROPLETS 37
3.2.1 EXPERIMENTAL DETAILS O F OPTICAL LEVITATION IN COMBINATION WITH
HARD X-RAYS 37
3.2.2 PRELIMINARY ADJUSTMENT 40
3.3 EXPERIMENTAL SETUP FOR XANES STUDIES USING SOFT X-RAYS 42
3.4 ELECTRODYNAMIC LEVITATION TRAP 44
3.5 DETERMINATION O F THE MICROPARTICLE CHARGE 46
CHAPTER 2 THEORETICAL BACKGROUND
2.1 OPTICAL LEVITATION
2.2 THERMODYNAMIC EQUILIBRIUM O F AQUEOUS SOLUTION DROPLET
2.3 HOMOGENEOUS NUCLEATION THEORY
2.4 THEORY O F SUPERSATURATED ELECTROLYTE SOLUTIONS
2.5 DISCRETE DIPOLE APPROXIMATION
2.6 X-RAY ABSORPTION
2.7 DENSITY FUNCTIONAL THEORY
2.7.1 BASICS O F QUANTUM CHEMISTRY
2.7.2 THE KOHN-SHAM THEORY
2.8 CORE-LEVEL ELECTRON ENERGY LOSS SPECTRA CALCULATIONS
2.8.1 CASTEP
2.8.2 CPMD
HTTP://D-NB.INFO/1026905710
IMAGE 2
3.6 EXPERIMENTAL PROCEDURE O F EFFLORESCENCE DETERMINATION
3.7 COMBINATION O F OPTICAL LEVITATION AND ELECTRODYNAMIC LEVITATION
3.8 AQUEOUS SALT SOLUTIONS AND SOLID SAMPLES
48
49
50
CHAPTER 4 RESULTS AND DISCUSSION
4.1 PHASE DIAGRAMS O F ELECTROLYTE SOLUTIONS 52
4.1.1 PHASE DIAGRAM O F NABR 52
4.1.2 PHASE DIAGRAMS O F CABR2 AND ZNBR2 58
4.2 XANES STUDIES O F CLUSTER FORMATION IN HOMOGENEOUS NUCLEATION OF
SINGLE LEVITATED MICRODROPLETS 61
4.2.1 XANES STUDIES O F AQUEOUS NABR SOLUTIONS AND SOLID NABR 63
4.2.2 THEORETICAL SIMULATION O F THE BR K-EDGE IN NABR NANOCLUSTERS 67
4.2.3 XANES STUDIES O F CABR 2 AND ITS DILUTE SOLUTION AND SOLIDS 72
4.2.4 SIMULATIONS O F DILUTED AND SUPERSATURATED CABR2 SOLUTIONS 75
4.2.5 XANES STUDIES O F ZNBR2 DROPLETS AND ITS E ILUTE SOLUTION AND THE
SOLID 80
4.3 NEAR-EDGE STRUCTURE O F SUPERSATURATED KBR DROPLETS 82
4.4 CHARGE EFFECTS ON THE NUCLEATION PROCESS O F SINGLE LEVITATED
DROPLETS 86
4.4.1 EFFLORESCENCE MEASUREMENTS O F SINGLE NEUTRAL / CHARGED DROPLETS
86
4.4.2 CHARGE EFFECTS ON THE EFFLORESCENCE O F SINGLE LEVITATED DROPLETS
90
4.5 SIMULATIONS O F SCATTERING PATTERNS IN CRYSTALLIZING DROPLETS 99
CHAPTER 5 CONCLUSIONS AND OUTLOOK
5.1 CONCLUSIONS 107
5.2 OUTLOOK 110
SUMMARY (ENGLISH) 111
ZUSAMMENFASSUNG (DEUTSCH) 113
REFERENCES 115
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| any_adam_object | 1 |
| author | Zhang, Yan |
| author_facet | Zhang, Yan |
| author_role | aut |
| author_sort | Zhang, Yan |
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| building | Verbundindex |
| bvnumber | BV040367526 |
| collection | ebook |
| ctrlnum | (OCoLC)839927846 (DE-599)BVBBV040367526 |
| dewey-full | 541 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541 |
| dewey-search | 541 |
| dewey-sort | 3541 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| format | Thesis Book |
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| indexdate | 2024-07-10T00:22:37Z |
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| language | English |
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| physical | 127 Bl. Ill., graph. Darst. |
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| spelling | Zhang, Yan Verfasser aut Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions Yan Zhang Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen 2012 127 Bl. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Nebentitel: Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen Berlin, Freie Univ., Diss., 2012 (DE-588)4113937-9 Hochschulschrift gnd-content Erscheint auch als Online-Ausgabe urn:nbn:de:kobv:188-fudissthesis000000038654-2 http://www.diss.fu-berlin.de/diss/receive/FUDISS_thesis_000000038654 kostenfrei Volltext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025221211&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Zhang, Yan Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |
| subject_GND | (DE-588)4113937-9 |
| title | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |
| title_alt | Untersuchungen von flüssigem und festem Phasenübergang der solvatisierten Ionen in Übersättigt-Lösungen |
| title_auth | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |
| title_exact_search | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |
| title_full | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions Yan Zhang |
| title_fullStr | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions Yan Zhang |
| title_full_unstemmed | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions Yan Zhang |
| title_short | Investigations of liquid-solid phase transition of solvated ions in supersaturated solutions |
| title_sort | investigations of liquid solid phase transition of solvated ions in supersaturated solutions |
| topic_facet | Hochschulschrift |
| url | http://www.diss.fu-berlin.de/diss/receive/FUDISS_thesis_000000038654 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025221211&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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