Holdings: Late transition metal amido complexes

Late transition metal amido complexes: electronic structure and reactivity

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Bibliographic Details
Main Author:	Askevold, Björn Birger 1982- (Author)
Format:	Thesis Book
Language:	English
Published:	2012
Subjects:	Chemische Synthese Übergangsmetallkomplexe Hochschulschrift
Online Access:	Volltext https://nbn-resolving.org/urn:nbn:de:bvb:91-diss-20120515-1106483-1-5 Inhaltsverzeichnis
Physical Description:	177 S. graph. Darst.

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MARC


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adam_text	IMAGE 1 TABLE O F CONTENTS A INTRODUCTION 11 1 LATE TRANSITION METAL AMIDO COMPLEXES: METAL-LIGAND BONDING AND REACTIVITY 12 2 LATE TRANSITION METAL AMIDO COMPLEXES: RELEVANCE FOR CATALYSIS AND MLC 16 3 GOAL AND MOTIVATION 19 B RESULTS AND DISCUSSION 21 1 REACTIVITY O F IRIDIUM(I) PNP AMIDO COMPLEX TOWARDS PROTONATION AND OXIDATION 22 1.1 INTRODUCTION 23 1.2 RESULTS AND DISCUSSION 25 1.3 CONCLUSION 30 1.4 EXPERIMENTAL SECTION 30 1.5 CYCLIC VOLTAMMETRY 33 1.6 COMPUTATIONAL METHODS 34 2 A SQUARE-PLANAR RUTHENIUM(II) COMPLEX WITH LOW-SPIN CONFIGURATION 38 2.1 INTRODUCTION 39 2.2 RESULTS AND DISCUSSION 40 2.3 CONCLUSION 45 2.4 SYNTHETIC AND ANALYTICAL DETAILS 46 2.5 SINGLE CRYSTAL X-RAY DIFFRACTION 48 2.6 SPECTROSCOPIC RESULTS 49 2.7 COMPUTATIONAL RESULTS 56 3 SQUARE-PLANAR RUTHENIUM(II) PNP PINCER COMPLEXES: CONTROL OF ELECTRONIC STRUCTURE BY TUNING O F N-M T :-DONATION 64 3.1 INTRODUCTION 65 3.2 RESULTS AND DISCUSSION 69 3.3 CONCLUSIONS 78 3.4 SYNTHETIC AND ANALYTICAL DETAILS 79 3.5 SPECTROSCOPIC RESULTS 82 3.6 COMPUTATIONAL RESULTS 87 HTTP://D-NB.INFO/1026863589 IMAGE 2 4 AMMONIA FORMATION BY METAL-LIGAND COOPERATIVE HYDROGENOLYSIS O F A NITRIDO LIGAND 89 4.1 ABSTRACT 90 4.2 INTRODUCTION 90 4.3 RESULTS AND DISCUSSION 92 4.4 CONCLUSIONS 99 4.5 SYNTHETIC AND ANALYTICAL DETAILS 101 4.6 CRYSTALLOGRAPHIC DETAILS 107 4.7 COMPUTATIONAL EXAMINATIONS 109 5 LEARNING FROM THE NEIGHBOURS: IMPROVING HOMOGENEOUS CATALYSTS WITH FUNCTIONAL LIGANDS MOTIVATED BY HETEROGENEOUS AND BIO-CATALYSIS 124 5.1 INTRODUCTION 125 5.2 INSPIRATION FROM HETEROGENEOUS CATALYSIS: HOMOGENEOUS POLYMERIZATION CATALYSTS WITH LEWIS ACIDIC CO-LIGANDS 126 5.3 BIO-INSPIRED HOMOGENEOUS CATALYSIS: METAL-LIGAND COOPERATING (MLC) CATALYSIS 130 5.4 CONCLUDING REMARKS 15 5 C SUMMARY 157 D ZUSAMMENFASSUNG 165 E LIST O F PUBLICATION 173 1 JOURNAL PUBLICATIONS 174 1 PRESENTATIONS 174 F CURRICULUM VITAE 175
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discipline	Chemie / Pharmazie Chemie
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spelling	Askevold, Björn Birger 1982- Verfasser (DE-588)1026863449 aut Late transition metal amido complexes electronic structure and reactivity Björn Birger Askevold 2012 177 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier München, Techn. Univ., Diss., 2012 Chemische Synthese (DE-588)4133806-6 gnd rswk-swf Übergangsmetallkomplexe (DE-588)4131837-7 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Übergangsmetallkomplexe (DE-588)4131837-7 s Chemische Synthese (DE-588)4133806-6 s DE-604 Erscheint auch als Online-Ausgabe urn:nbn:de:bvb:91-diss-20120515-1106483-1-5 http://mediatum.ub.tum.de/node?id=1106483 Verlag kostenfrei Volltext https://nbn-resolving.org/urn:nbn:de:bvb:91-diss-20120515-1106483-1-5 Resolving-System DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025175301&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Askevold, Björn Birger 1982- Late transition metal amido complexes electronic structure and reactivity Chemische Synthese (DE-588)4133806-6 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd
subject_GND	(DE-588)4133806-6 (DE-588)4131837-7 (DE-588)4113937-9
title	Late transition metal amido complexes electronic structure and reactivity
title_auth	Late transition metal amido complexes electronic structure and reactivity
title_exact_search	Late transition metal amido complexes electronic structure and reactivity
title_full	Late transition metal amido complexes electronic structure and reactivity Björn Birger Askevold
title_fullStr	Late transition metal amido complexes electronic structure and reactivity Björn Birger Askevold
title_full_unstemmed	Late transition metal amido complexes electronic structure and reactivity Björn Birger Askevold
title_short	Late transition metal amido complexes
title_sort	late transition metal amido complexes electronic structure and reactivity
title_sub	electronic structure and reactivity
topic	Chemische Synthese (DE-588)4133806-6 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd
topic_facet	Chemische Synthese Übergangsmetallkomplexe Hochschulschrift
url	http://mediatum.ub.tum.de/node?id=1106483 https://nbn-resolving.org/urn:nbn:de:bvb:91-diss-20120515-1106483-1-5 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025175301&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
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