Verfügbarkeit: Molecules at work

Molecules at work: selfassembly, nanomaterials, molecular machinery

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Bibliographische Detailangaben
Weitere Verfasser:	Pignataro, Bruno 1972- (HerausgeberIn)
Format:	Buch
Sprache:	English
Veröffentlicht:	Weinheim Wiley-VCH 2012
Schlagworte:	Katalyse Chemische Synthese Aufsatzsammlung
Online-Zugang:	Inhaltsverzeichnis Inhaltstext Inhaltsverzeichnis
Beschreibung:	Literaturangaben
Beschreibung:	XXIV, 391 S. Ill., graph. Darst. 25 cm
ISBN:	3527330933 9783527645817 9783527330935

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Datensatz im Suchindex

_version_	1805146799927721984
adam_text	IMAGE 1 V CONTENTS PREFACE X I I I LIST O F CONTRIBUTORS XXI PART I SELF ASSEMBLY 1 1 YOCTOLITER-SIZED VESSELS A S POTENTIAL BIOLOGICAL MODELS 3 SHESHANATH V. BHOSALE, BRADLEY E. WILMAN, A N D STEVEN J. LANGFORD 1.1 INTRODUCTION 3 1.2 CAVITIES O N GLASS PLATES A N D GOLD SURFACES 5 1.3 PREPARATION A N D CONFIRMATION O F RIGID YOCTOWELL CAVITY 6 1.3.1 CONFIRMATION O F RIGID G A P S 7 1.4 MOLECULAR SORTING 7 1.5 YOCTOWELL-BASED MOLECULAR RECOGNITION EVENTS 9 1.6 CONCLUSION 11 A C K N O W L E D G M E N T S 12 REFERENCES 12 2 SWITCHABLE H O S T - G U E S T INTERACTIONS O F SUPRAMOLECULAR RINGS A N D CAGES 13 GUIDO H. CLEVER 2.1 INTRODUCTION 13 2.2 H O S T - G U E S T C H E M I S T R Y 15 2.3 SWITCHING IN S U P R A M O L E C U L A R SYSTEMS 17 2.4 NATURAL PARAGONS 19 2.5 TYPES O F EXTERNAL I N P U T A N D M E T H O D S FOR ANALYSIS 20 2.5.1 SWITCHABLE H O S T C O M P O U N D S 21 2.5.2 SWITCHABLE G U E S T C O M P O U N D S 26 2.6 CONCLUSION 33 REFERENCES 3 4 HTTP://D-NB.INFO/1016558589 IMAGE 2 V I I CONTENTS PART II NANOMATERIALS 3 9 3 TAILORED GRAPHENE-TYPE MOLECULES BY CHEMICAL SYNTHESIS 41 MILAN KIVALA A N D XINLIANG FENG 3.1 INTRODUCTION 41 3.2 SYNTHETIC CONCEPTS TOWARD EXPANDED P A H S - N A N O G R A P H E N E S 43 3.2.1 H E X A B E N Z O C O R O N E N E S (HBCS) A N D RELATED SYSTEMS 4 3 3.2.2 LARGE P A H S 48 3.2.3 G R A P H E N E N A N O R I B B O N S 5 5 3.2.4 HETEROATOM-CONTAINING P A H S 6 0 3.3 CONCLUSION A N D OUTLOOK 64 REFERENCES 6 6 4 ANALYZING T H E SURFACE AREA PROPERTIES O F MICROPOROUS MATERIALS 71 ABBIE TREWIN 4.1 INTRODUCTION 71 4.1.1 ENERGY 71 4.1.2 H2 STORAGE 71 4.1.3 CO2 C A P T U R E A N D SEQUESTRATION 72 4.1.4 G A S SEPARATION 73 4.2 MICROPOROUS MATERIALS 74 4.2.1 F R A M E W O R K MATERIALS 74 4.2.2 NETWORK MATERIALS 74 4.2.3 MOLECULAR MATERIALS 76 4.2.4 STRUCTURAL FLEXIBILITY 7 9 4.3 POROSITY 81 4.3.1 W H A T IS POROSITY? 81 4.3.2 INTRINSIC VERSUS EXTRINSIC POROSITY 81 4.3.3 M E A S U R I N G POROSITY 8 2 4.3.4 CALCULATED SURFACE AREAS A N D SIMULATED G A S UPTAKES 83 4.3.5 GAS-DIFFUSION M E C H A N I S M S 84 4.4 POROUS MATERIALS A N D CALCULATING SURFACE AREAS 8 5 4.4.1 F R A M E W O R K MATERIALS 8 5 4.4.2 NETWORK MATERIALS 86 4.4.3 MOLECULAR MATERIALS 88 4.4.4 MOLECULAR SOLIDS WITH S O M E EXTRINSIC POROSITY 8 9 4.4.5 MOLECULAR SOLIDS WITH INTRINSIC POROSITY 9 0 4.5 S U M M A R Y 92 ACKNOWLEDGMENTS 92 REFERENCES 93 5 NANOSTRUCTURED MATERIALS BASED O N CORE-SUBSTITUTED N A P H T H A L E N E DIIMIDES 9 7 SHESHANATH V. BHOSALE, BRADLEY E. WILMAN, A N D STEVEN J. LANGFORD 5.1 INTRODUCTION 9 7 IMAGE 3 CONTENTS \| V I I 5.2 SYNTHESIS O F NOVEL CNDI DERIVATIVES 99 5.3 ELECTRON T R A N S F E R 102 5.4 S U P R A M O L E C U L A R SELF-ASSEMBLY O F CNDI 105 5.5 CONCLUSION 110 A C K N O W L E D G M E N T S 110 REFERENCES 110 6 METAL PHOSPHIDES: FROM C H E M I S T ' S ODDITIES T O DESIGNED FUNCTIONAL MATERIALS 113 SOPHIE CARENCO, MATTHIEU DEMANGE, CEDRIC BOISSIERE, CLEMENT SANCHEZ, A N D NICOLAS MEZAILLES 6.1 INTRODUCTION 113 6.2 BULK METAL PHOSPHIDES: A LONG HISTORY 113 6.2.1 A NEW FAMILY O F SYNTHETIC INORGANIC MATERIALS 113 6.2.2 FIRST SET O F APPLICATIONS 114 6.2.3 BULK METAL P H O S P H I D E S A N D TODAY'S APPLICATIONS 114 6.3 W H I T E P H O S P H O R U S FOR T H E LOW-TEMPERATURE SYNTHESIS O F METAL P H O S P H I D E NANOPARTICLES 115 6.3.1 W H I T E P H O S P H O R U S AS A LOW-TEMPERATURE REAGENT 115 6.3.2 ARYL- A N D ALKYL-PHOSPHINES AS " P " A T O M D O N O R IN H A R S H C O N D I T I O N S FOR T H E SYNTHESIS O F METAL P H O S P H I D E NANOPARTICLES 115 6.3.3 NICKEL P H O S P H I D E NANOPARTICLES F R O M P 4 I N STOICHIOMETRIC A N D MILD CONDITIONS 116 6.3.4 GENERALIZATION O F T H E W H I T E P H O S P H O R U S NANOSCALE ROUTE 118 REFERENCES 119 7 "ARTIFICIAL SUPERMOLECULE": PROGRESS IN T H E STUDY O F II-V COLLOIDAL SEMICONDUCTOR NANOCRYSTALS 121 SHIDING MIAO, ALEXANDER EYCHMULLER, A N D STEPHEN G. HICKEY 7.1 INTRODUCTION 121 7.2 OPTICAL PROPERTIES O F I I - V NANOCRYSTALS 124 7.2.1 ABSORPTION 124 7.2.2 P H O T O L U M I N E S C E N C E 127 7.2.3 LIFETIME M E A S U R E M E N T 131 7.3 SYNTHESIS O F II-V NANOCRYSTALS 133 7.3.1 SYNTHESIS M E T H O D S 133 7.3.2 SYNTHESIS O F CD3P2 NANOCRYSTALS 134 7.3.2.1 "HOT-INJECTION" SYNTHESIS 134 7.3.2.2 H I G H - T E M P E R A T U R E , GAS-BUBBLING SYNTHESIS WITH EX SITU-PRODUCED P H 3 139 7.3.3 SYNTHESIS O F Z N J P 2 NANOCRYSTALS 140 7.3.4 SYNTHESIS O F CDJAS2 NANOCRYSTALS 142 7.3.5 S U M M A R Y O F T H E SYNTHESIS O F II-V NANOCRYSTALS 143 1 A CONCLUSIONS A N D OUTLOOK 143 REFERENCES 146 IMAGE 4 V I I I 1 CONTENTS 8 LUMINESCENT DENDRIMERS 155 GIACOMO BERGAMINI 8.1 INTRODUCTION 155 8.2 INTRINSIC PHOTOCHEMICAL A N D PHOTOPHYSICAL PROPERTIES O F O R G A N I C DENDRIMERS 156 8.3 ENERGY TRANSFER A N D ENERGY UPCONVERSION I N M U L T I C H R O M O P H O R I C DENDRIMERS 161 8.4 DENDRIMERS AS LIGANDS FOR METAL I O N S 164 8.5 SELF-ASSEMBLY 168 8.6 D E N D R I M E R S AS PHOTOSWITCHABLE H O S T S 170 8.7 CONCLUSION A N D PERSPECTIVES 172 REFERENCES 173 9 FABRICATION O F ULTRAMICROPOROUS SILICA M E M B R A N E S FOR PERVAPORATION A N D G A S SEPARATION 177 VITTORIO BOFFA 9.1 ULTRAMICROPOROUS SILICA M E M B R A N E S 177 9.1.1 CONTEXT 177 9.1.2 G A S SEPARATION A N D PERVAPORATION 177 9.1.3 FABRICATION 180 9.1.4 MICROPOROSITY A S S E S S M E N T I N SILICA M E M B R A N E S 182 9.1.5 H Y D R O T H E R M A L STABILITY-INSTABILITY O F MICROPOROUS SILICA 184 9.2 M X O Y - S I L I C A M E M B R A N E 185 9.2.1 FABRICATION 185 9.2.2 STABILITY, SELECTIVITY, A N D REACTIVITY 187 9.2.3 M E M B R A N E OPTIMIZATION 193 9.3 HYBRID ORGANIC-SILICA M E M B R A N E S 193 9.3.1 FABRICATION 193 9.3.2 " H Y D R O P H O B I C " SILICA M E M B R A N E S 196 9.3.3 M E M B R A N E S F R O M BRIDGED ORGANOSILANES 197 9.3.4 ORGANIC-SILICA M E M B R A N E S FOR CO2 SEPARATION 199 9.4 PERSPECTIVES IN T H E FABRICATION A N D APPLICATION O F SILICA M E M B R A N E S 2 0 0 REFERENCES 200 10 N E W DIRECTIONS IN T H E FIGHT A G A I N S T CANCER: FROM METAL COMPLEXES T O NANOSTRUCTURED MATERIALS 207 SANTIAGO GOMEZ-RUIZ 10.1 INTRODUCTION 207 10.2 METAL COMPLEXES IN C A N C E R T R E A T M E N T 208 10.2.1 P L A T I N U M COMPLEXES 2 0 8 10.2.2 N O N - P L A T I N U M TRANSITION-METAL COMPLEXES 2 1 0 10.2.2.1 G R O U P 4 METAL COMPLEXES 211 10.2.2.2 G R O U P 8 METAL COMPLEXES 213 IMAGE 5 CONTENTS I I X 10.2.2.3 G R O U P 11 METAL COMPLEXES 216 10.2.3 M A I N GROUP-METAL COMPLEXES 229 10.2.3.1 G A L L I U M COMPLEXES 219 10.2.3.2 T I N COMPLEXES 220 10.3 NANOSTRUCTURED MATERIALS IN C A N C E R T R E A T M E N T S 221 10.3.1 MACROMOLECULAR SYSTEMS 2 2 2 10.3.1.1 CUCURBIT[N]URILS A N D CYCLODEXTRINS 2 2 2 10.3.1.2 LIPOSOMES A N D LIPID NANOCAPSULES 223 10.3.1.3 O T H E R MACROMOLECULAR SYSTEMS 224 10.3.2 C E R A M I C MATERIALS 224 10.3.2.1 N A N O S T R U C T U R E D CALCIUM-PHOSPHATE-BASED MATERIALS FUNCTIONALIZED WITH METAL COMPLEXES 2 2 6 10.3.2.2 MESOPOROUS SILICAS FUNCTIONALIZED WITH METAL COMPLEXES 2 2 7 10.3.2.3 C A R B O N N A N O T U B E S FUNCTIONALIZED WITH METAL COMPLEXES 228 10.3.3 NANOPARTICLES 230 REFERENCES 2 3 0 PART III MOLECULAR MACHINERY 243 11 MOLECULAR ROTORS: IMAGING INTRACELLULAR VISCOSITY 2 4 5 MARINA K. KUIMOVA 11.1 INTRODUCTION 2 4 5 11.2 THEORETICAL BACKGROUND 246 11.3 BIOLOGICAL APPLICATIONS O F MOLECULAR ROTORS 2 4 7 11.3.1 FLUORESCENCE-LIFETIME-BASED MOLECULAR ROTORS 249 11.3.2 TIME-RESOLVED FLUORESCENCE ANISOTROPY M E A S U R E M E N T S O F MOLECULAR ROTORS 252 11.3.3 RATIOMETRIC FLUORESCENT MOLECULAR ROTORS 2 5 5 11.3.4 RATIOMETRIC MOLECULAR ROTOR M E A S U R E M E N T S O F VISCOSITY D U R I N G P D T 2 5 7 11.4 CONCLUSIONS A N D OUTLOOK 2 5 8 A C K N O W L E D G M E N T S 259 REFERENCES 259 12 SURFACE-FUNCTIONALIZED INORGANIC COLLOIDAL NANOCRYSTALS IN FUNCTIONAL N A N O C O M P O S I T E MATERIALS FOR MICROFABRICATION 2 6 3 CHIARA INGROSSO, MARINELLA STRICCOLI, ANGELA AGOSTIANO, A N D MARIA LUCIA CURRI 12.1 INTRODUCTION 263 12.2 COLLOIDAL NANOCRYSTALS: PROPERTIES, SYNTHESIS, A N D SURFACE FUNCTIONALIZATION 2 6 4 12.2.1 PROPERTIES O F NANOCRYSTALS 264 12.2.2 COLLOIDAL SYNTHESIS O F NANOCRYSTALS 2 6 5 12.2.3 SURFACE FUNCTIONALIZATION O F NANOCRYSTALS 266 12.3 NC-BASED NANOCOMPOSITES FOR MICROFABRICATION 269 IMAGE 6 X \| CONTENTS 12.4 CONCLUSIONS A N D F U T U R E PERSPECTIVES 2 7 9 REFERENCES 280 13 FLUORESCENCE SENSING O F TEMPERATURE A N D OXYGEN WITH FULLERENES 285 MARIO N. BERBERAN-SANTOS A N D CARLOS BALEIZAO 13.1 INTRODUCTION 285 13.2 THERMALLY ACTIVATED DELAYED FLUORESCENCE: F U N D A M E N T A L ASPECTS 287 13.3 SENSING APPLICATIONS 2 9 2 13.3.1 OXYGEN S E N S I N G 293 13.3.1.1 S U B - P P M OXYGEN S E N S O R BASED O N C70 294 13.3.1.2 C70 I N A DUAL S E N S O R SYSTEM 297 13.3.2 T E M P E R A T U R E S E N S I N G 3 0 0 13.3.2.1 C70 DISPERSED IN POLYMER FILMS 3 0 2 13.3.2.2 C70 ENCAPSULATED I N POLYMER NANOPARTICLES 304 13.4 CONCLUSIONS A N D F U T U R E PERSPECTIVES 307 A C K N O W L E D G M E N T S 308 REFERENCES 308 14 G O I N G BEYOND GLUCOSE S E N S I N G WITH BORONIC ACID RECEPTORS 3 1 5 ALEXANDER SCHILLER 14.1 INTRODUCTION 3 1 5 14.2 INDICATOR DISPLACEMENT ASSAYS FOR T H E DETECTION O F SUGARS 316 14.3 GLUCOSE S E N S I N G WITH BORONIC ACID RECEPTORS 3 1 7 14.3.1 ALLOSTERIC INDICATOR DISPLACEMENT ASSAY FOR T H E DETECTION O F CARBOHYDRATES 318 14.3.2 A1DA SACCHARIDE S E N S I N G SYSTEM - B O R O N I C - A C I D - A P P E N D E D BENZYL BIPYRIDINUM SALTS A N D A FLUORESCENT REPORTER DYE 3 1 9 14.3.3 AIDA GLUCOSE S E N S O R FOR C O N T I N U O U S MONITORING 3 2 0 14.4 SOLUTION-PHASE S E N S O R ARRAYS WITH BORONIC-ACID-APPENDED BIPYRIDINIUM SALTS 321 14.4.1 RECOGNITION O F NEUTRAL SACCHARIDES 3 2 2 14.4.2 RECOGNITION O F P H O S P H O S U G A R S A N D NUCLEOTIDES 324 14.5 CARBOHYDRATE-ACTIVE E N Z Y M E ASSAYS 3 2 7 14.6 BORONIC-ACID-APPENDED BIPYRIDINIUM SALTS A T W O R K - NOVOSIDES 3 3 0 14.7 CONCLUSIONS A N D PERSPECTIVES 333 A C K N O W L E D G M E N T S 334 REFERENCES 3 3 4 15 DESIGN O F NOVEL IRIDIUM COMPLEXES T O OBTAIN STABLE A N D EFFICIENT LIGHT-EMITTING ELECTROCHEMICAL CELLS 339 RUBEN D. COSTA 15.1 BRIEF HISTORY O F ELECTROLUMINESCENCE A N D OPTOELECTRONIC DEVICES 3 3 9 15.2 LIGHT-EMITTING ELECTROCHEMICAL CELLS: MOTIVATION A N D DEFINITION 3 4 0 IMAGE 7 CONTENTS \| X I 15.3 IONIC TRANSITION-METAL COMPLEXES BASED O N IR(LII) METAL C O R E FOR LECS 343 15.4 STRATEGIES TO DESIGN IRIDIUM(IIL) COMPLEXES FOR HIGHLY EFFICIENT LECS 346 15.5 STRATEGIES TO DESIGN IRIDIUM(III) COMPLEXES FOR HIGHLY STABLE LECS 3 5 0 15.6 OUTLOOK A N D CONCLUSIONS 356 ACKNOWLEDGMENTS 3 5 7 REFERENCES 357 16 PHOTOCHEMICALLY DRIVEN MOLECULAR DEVICES A N D MACHINES 361 SERENA SILVI 16.1 INTRODUCTION 363 16.1.1 FEATURES O F MOLECULAR DEVICES A N D MACHINES 36 J 16.2 SWITCHES A N D LOGIC GATES 3 6 3 16.3 MOLECULAR MACHINES 369 16.3.1 T H R E A D I N G - D E T H R E A D I N G MOTIONS 371 16.3.2 MOLECULAR SHUTTLES 3 7 5 16.4 CONCLUSIONS 3 8 0 A C K N O W L E D G M E N T S 381 REFERENCES 381 INDEX 3 8 5
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spelling	Molecules at work selfassembly, nanomaterials, molecular machinery ed. by Bruno Pignataro Weinheim Wiley-VCH 2012 XXIV, 391 S. Ill., graph. Darst. 25 cm txt rdacontent n rdamedia nc rdacarrier Literaturangaben Katalyse (DE-588)4029921-1 gnd rswk-swf Chemische Synthese (DE-588)4133806-6 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Chemische Synthese (DE-588)4133806-6 s Katalyse (DE-588)4029921-1 s DE-604 Pignataro, Bruno 1972- (DE-588)135576520 edt application/pdf http://d-nb.info/1016558589/04 Inhaltsverzeichnis text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3902530&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025108991&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Molecules at work selfassembly, nanomaterials, molecular machinery Katalyse (DE-588)4029921-1 gnd Chemische Synthese (DE-588)4133806-6 gnd
subject_GND	(DE-588)4029921-1 (DE-588)4133806-6 (DE-588)4143413-4
title	Molecules at work selfassembly, nanomaterials, molecular machinery
title_auth	Molecules at work selfassembly, nanomaterials, molecular machinery
title_exact_search	Molecules at work selfassembly, nanomaterials, molecular machinery
title_full	Molecules at work selfassembly, nanomaterials, molecular machinery ed. by Bruno Pignataro
title_fullStr	Molecules at work selfassembly, nanomaterials, molecular machinery ed. by Bruno Pignataro
title_full_unstemmed	Molecules at work selfassembly, nanomaterials, molecular machinery ed. by Bruno Pignataro
title_short	Molecules at work
title_sort	molecules at work selfassembly nanomaterials molecular machinery
title_sub	selfassembly, nanomaterials, molecular machinery
topic	Katalyse (DE-588)4029921-1 gnd Chemische Synthese (DE-588)4133806-6 gnd
topic_facet	Katalyse Chemische Synthese Aufsatzsammlung
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