Chemistry of ozone in water and wastewater treatment: from basic principles to applications
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
London
IWA Publishing
2012
|
| Schlagworte: | |
| Online-Zugang: | Volltext Inhaltsverzeichnis |
| Beschreibung: | Hier auch später erschienene, unveränderte Nachdrucke |
| Beschreibung: | IX, 302 Seiten Diagramme |
| ISBN: | 9781843393139 |
| DOI: | 10.2166/9781780400839 |
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Datensatz im Suchindex
| _version_ | 1804149040222306304 |
|---|---|
| adam_text | Titel: Chemistry of ozone in water and wastewater treatment
Autor: Sonntag, Clemens von
Jahr: 2012
Contents
About the Authors .......................................................... xi
Chapter 1
Historical background and scope of the book................................ 1
Chapter 2
Physical and chemical properties of ozone .................................. 7
2.1 Introductory Remarks ........................................................ 7
2.2 Generation of Ozone ........................................................ 8
2.3 Ozone Solubility in Water .................................................... 9
2.4 UV-VIS Spectrum of Ozone ................................................. 10
2.5 Determination of the Ozone Concentration .......................... ......... 12
2.5.1 The /V,A/-diethyl-p-phenylenediamine (DPD) method ............ ......... 12
2.5.2 The indigo method.................................................. 13
2.6 Methods for Measuring Ozone Kinetics ....................................... 14
2.6.1 Ozone decay measurements ......................................... 15
2.6.2 Quenching of ozone with buten-3-ol .................................. 16
2.6.3 Reactive absorption................................................. 16
2.6.4 Competition kinetics ................................................ 17
2.7 Reduction Potentials of Ozone and Other Oxygen Species .................... 18
2.8 Stability of Ozone Solutions ................................................ 19
2.9 Reactivity of Ozone ........................................................ 19
2.9.1 pH dependence of ozone reactions and the reactivity pK .............. 20
2.9.2 Multiple reaction sites within one molecule ............................. 21
Chapter 3
Ozone kinetics in drinking water and wastewater .......................... 23
3.1 Stability of Ozone in Various Water Sources .......................... ....... 23
vi Chemistry of Ozone in Water and Wastewater Treatment
3.2 Molecular Weight Distribution of Dissolved Organic Matter ........................ 31
3.3 Mineralisation and Chemical Oxygen Demand .................................. 33
3.4 Formation of Assimilable Organic Carbon ...................................... 33
3.5 Formation and Mitigation of Disinfection By-products ............................. 35
3.6 UV Absorbance of Dissolved Organic Matter .................................... 36
3.7 Relevance of Ozone Kinetics for the Elimination of Micropollutants ................. 37
3.8 Hydroxyl Radical Yield and OH-Scavenging Rate of Dissolved
Organic Matter ............................................................. 39
3.9 Elimination of Ozone-Refractory Micropollutants by the OH Route ................ 40
3.10 Ozone-based Advanced Oxidation Processes .................................. 42
3.10.1 Peroxone process ................................................... 42
3.10.2 UV photolysis of ozone ............................................... 45
3.10.3 Reaction of ozone with activated carbon ................................ 46
Chapter 4
Inactivation of micro-organisms and toxicological assessment of
ozone-induced products of micropollutants ................................ 49
4.1 Disinfection Kinetics ......................................................... 49
4.2 Inactivation Mechanisms: Role of Membranes and DNA .......................... 52
4.3 Reactions with Nucleic Acid Components ...................................... 53
4.4 Reaction with DNA .......................................................... 54
4.5 Application of Ozone for Disinfection in Drinking Water and Wastewater ............ 55
4.6 Toxicological Assessment of Ozone Induced Transformation Products ............. 55
4.7 Endocrine Disrupting Compounds ............................................. 56
4.7.1 Laboratory studies .................................................... 58
4.7.2 Full-scale studies ..................................................... 59
4.8 Antimicrobial Compounds .................................................... 60
4.9 Toxicity .................................................................... 62
Chapter 5
Integration ofozonation in drinking water and wastewater
process trains ............................................................. 65
5.1 Historical Aspects ........................................................... 65
5.1.1 Drinking water ....................................................... 65
5.1.2 Municipal wastewater ................................................. 65
5.2 Drinking Water Treatment Schemes Including Ozonation ......................... 66
5.3 Micropollutants in Water Resources, Drinking Water and Wastewater .............. 70
5.4 Enhanced Wastewater Treatment with Ozone ................................... 72
5.5 Energy Requirements for Micropollutant Transformation in Drinking Water
and Wastewater ............................................................ 73
5.6 Source Control ............................................................. 74
5.7 Reclamation of Wastewater .................................................. 75
5.8 Comparison of the Application of Ozone in the Urban Water Cycle ................. 77
Contents v¡¡
Chapter 6
Olefins .................................................................... 81
6.1 Reactivity of Olefins ......................................................... 81
6.2 The Criegee Mechanism ..................................................... 84
6.3 Partial Oxidation ............................................................ 87
6.4 Decay of the Ozonide via Free Radicals ........................................ 88
6.5 Detection of a-Hydroxyalkylhydroperoxides ..................................... 88
6.6 Ozone Reactions of Olefins - Products and Reactions of Reactive Intermediates ___ 89
6.6.1 Methyl- and halogen-substituted olefins .................................. 89
6.6.2 Acrylonitrile, vinyl acetate, diethyl vinylphosphonate, vinyl phenyl sulfonate,
vinylsulfonic acid and vinylene carbonate ................................ 91
6.6.3 Acrylic, methacrylic, fumaric, maleic and muconic acids .................... 92
6.6.4 Muconic acids ....................................................... 96
6.6.5 Cinnamic acids ....................................................... 98
6.6.6 Dichloromaleic acid ................................................... 99
6.6.7 Pyrimidine nucleobases ............................................... 99
6.7 Micropollutants with Olefinic Functions ........................................ 102
Chapter 7
Aromatic compounds ..................................................... 109
7.1 Reactivity of Aromatic Compounds ........................................... 109
7.2 Decay of Ozone Adducts.................................................... 116
7.3 Ozone Reactions of Aromatic Compounds - Products and Reactions of Reactive
Intermediates .............................................................. 118
7.3.1 Methoxylated benzenes .............................................. 118
7.3.2 Phenols ............................................................ 121
7.4 Micropollutants with Aromatic Functions ....................................... 124
Chapter 8
Nitrogen-containing compounds .......................................... 131
8.1 Reactivity of Nitrogen-containing Compounds .................................. 131
8.2 General Mechanistic Considerations .......................................... 138
8.2.1 Aliphatic amines ..................................................... 138
8.2.2 Aromatic amines (anilines) ............................................ 143
8.2.3 Nitrogen-containing heterocyclic compounds ............................ 145
8.3 Micropollutants with Nitrogen-containing Functions ............................. 146
8.3.1 The /V-nitrosodimethylamine (NDMA) puzzle ............................ 156
Chapter 9
Reactions of sulfur-containing compounds ................................ 161
9.1 Reactivity of Sulfur-containing Compounds .................................... 161
9.2 Thiols .................................................................... 162
viii Chemistry of Ozone in Water and Wastewater Treatment
9.3 Sulfides, Disulfides and Sulfinic Acids......................................... 163
9.4 Sulfoxides ................................................................ 165
9.5 Micropollutants Containing an Ozone-reactive Sulfur ............................ 166
Chapter 10
Compounds with C-H functions as ozone-reactive sites.................... 169
10.1 Reactivity of Compounds with C-H Functions as Ozone-reactive Sites ........... 169
10.2 General Mechanistic Considerations......................................... 171
10.3 Formate Ion .............................................................. 173
10.4 2-Methyl-2-Propanol (Tertiary Butanol) ....................................... 175
10.5 2-Propanol ............................................................... 176
10.6 Carbohydrates ........................................................... 180
10.7 Dihydrogen Trioxide - Properties of a Short-lived Intermediate .................. 182
10.8 Saturated Micropollutants Lacking Ozone-reactive Heteroatoms ................. 184
Chapter 11
Inorganic anions and the peroxone process ............................... 185
11.1 Introductory Remarks ...................................................... 185
11.2 Hydroxide Ion ............................................................ 187
11.3 Hydroperoxide Ion - Peroxone Process ...................................... 188
11.4 Fluoride ................................................................. 189
11.5 Chloride ................................................................. 190
11.6 Hypochlorite .............................................................. 191
11.7 Chlorite .................................................................. 192
11.8 Bromide ................................................................. 192
11.9 Hypobromite ............................................................. 193
11.10 Bromite .................................................................. 194
11.11 Iodide ................................................................... 194
11.12 Nitrite ................................................................... 195
11.13 Azide .................................................................... 196
11.14 Hydrogen Sulfide ......................................................... 197
11.15 Hydrogen Sulfite .......................................................... 198
11.16 Brómate Formation and Mitigation in Water Treatment ......................... 198
11.17 Bromide-catalysed Reactions ............................................... 201
11.18 Mitigation of Iodide-related Problems ........................................ 202
Chapter 12
Reactions with metal ions................................................. 205
12.1 Reactivity of Metal Ions .................................................... 205
12.2 Arsenic .................................................................. 206
12.3 Cobalt ................................................................... 207
12.4 Copper .................................................................. 207
Contents ix
12.5 Iron ..................................................................... 207
12.6 Lead .................................................................... 208
12.7 Manganese .............................................................. 208
12.8 Selenium ................................................................ 209
12.9 Silver ................................................................... 209
12.10 Tin ...................................................................... 211
12.11 Metal Ions as Micropollutants ............................................... 211
Chapter 13
Reactions with free radicals ............................................... 213
13.1 Reactivity of Radicals ..................................................... 213
13.2 Ozone Reactions with Reducing Radicals .................................... 214
13.3 Ozone Reactions with Carbon-centered Radicals .............................. 215
13.4 Ozone Reactions with Oxygen-centered Radicals ............................. 217
13.5 Ozone Reactions with Nitrogen- and Sulfur-centred Radicals ................... 219
13.6 Ozone Reactions with Halogen-centred Radicals .............................. 220
Chapter 14
Reactions of hydroxyl and peroxyl radicals ................................ 225
14.1 Introductory Remarks ..................................................... 225
14.2 Hydroxyl Radical Reactions ................................................ 225
14.2.1 Addition reactions ................................................. 225
14.2.2 H-abstraction reactions ............................................. 227
14.2.3 Electron transfer reactions .......................................... 228
14.3 Determination of OH Rate Constants ........................................ 229
14.4 Detection of OH in Ozone Reactions ........................................ 230
14.5 Determination of OH Yields in Ozone Reactions .............................. 232
14.6 Formation of Peroxyl Radicals .............................................. 233
14.7 Redox Properties of Peroxyl Radicals and Reaction with Ozone ................. 233
14.8 Unimolecular Decay of Peroxyl Radicals ..................................... 234
14.9 Bimolecular Decay of Peroxyl Radicals ...................................... 235
14.10 Reactions of Oxyl Radicals................................................. 236
14.11 Involvement of OH Radicals in Chlorate and Brómate Formation ................ 237
14.11.1 Chlorate formation ................................................ 237
14.11.2 Brómate formation ................................................ 238
14.12 Degradation of Ozone-refractory Micropollutants by OH/Peroxyl Radicals ........ 241
14.12.1 Saturated aliphatic compounds ..................................... 241
14.12.2 Aromatic compounds ............................................. 243
14.12.3 Chlorinated olefins ............................................... 245
14.12.4 Perfluorinated compounds ......................................... 248
References ............................................................... 249
Index..................................................................... 287
|
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| spelling | Sonntag, Clemens von 1936-2013 Verfasser (DE-588)105963348 aut Chemistry of ozone in water and wastewater treatment from basic principles to applications Clemens von Sonntag and Urs von Gunten London IWA Publishing 2012 IX, 302 Seiten Diagramme txt rdacontent n rdamedia nc rdacarrier Hier auch später erschienene, unveränderte Nachdrucke Abwasserreinigung (DE-588)4000313-9 gnd rswk-swf Ozonisierung (DE-588)4173040-9 gnd rswk-swf Wasseraufbereitung (DE-588)4064698-1 gnd rswk-swf Wasseraufbereitung (DE-588)4064698-1 s Abwasserreinigung (DE-588)4000313-9 s Ozonisierung (DE-588)4173040-9 s DE-604 Gunten, Urs von 1959- Verfasser (DE-588)1089185286 aut Erscheint auch als Online-Ausgabe 10.2166/9781780400839 978-1-7804-0083-9 https://doi.org/10.2166/9781780400839 Verlag kostenfrei Volltext HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024896371&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Sonntag, Clemens von 1936-2013 Gunten, Urs von 1959- Chemistry of ozone in water and wastewater treatment from basic principles to applications Abwasserreinigung (DE-588)4000313-9 gnd Ozonisierung (DE-588)4173040-9 gnd Wasseraufbereitung (DE-588)4064698-1 gnd |
| subject_GND | (DE-588)4000313-9 (DE-588)4173040-9 (DE-588)4064698-1 |
| title | Chemistry of ozone in water and wastewater treatment from basic principles to applications |
| title_auth | Chemistry of ozone in water and wastewater treatment from basic principles to applications |
| title_exact_search | Chemistry of ozone in water and wastewater treatment from basic principles to applications |
| title_full | Chemistry of ozone in water and wastewater treatment from basic principles to applications Clemens von Sonntag and Urs von Gunten |
| title_fullStr | Chemistry of ozone in water and wastewater treatment from basic principles to applications Clemens von Sonntag and Urs von Gunten |
| title_full_unstemmed | Chemistry of ozone in water and wastewater treatment from basic principles to applications Clemens von Sonntag and Urs von Gunten |
| title_short | Chemistry of ozone in water and wastewater treatment |
| title_sort | chemistry of ozone in water and wastewater treatment from basic principles to applications |
| title_sub | from basic principles to applications |
| topic | Abwasserreinigung (DE-588)4000313-9 gnd Ozonisierung (DE-588)4173040-9 gnd Wasseraufbereitung (DE-588)4064698-1 gnd |
| topic_facet | Abwasserreinigung Ozonisierung Wasseraufbereitung |
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