The photophysics behind photovoltaics and photonics:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH
2012
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | VII, 212 S. Ill., graph. Darst. |
| ISBN: | 3527410546 9783527410545 9783527645138 |
Internformat
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Datensatz im Suchindex
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IMAGE 1
V
CONTENTS
1 INTRODUCTION 1
2 R A D I A T I O N - M A T T E R INTERACTION IN T H E TWO-LEVEL SYSTEM
7
2.1 INTRODUCTION 7
2.2 GENERALITY O N R A D I A T I O N - M A T T E R INTERACTION 7
2.3 SYNOPSIS O N T H E TWO-LEVEL MODEL 12
2.4 ABSORPTION J 6
2.5 N O N L I N E A R ABSORPTION 17
2.6 ADIABATIC APPROXIMATION 21
2.7 F R A N C K - C O N D O N PRINCIPLE 23
2.8 BEYOND C O N D O N APPROXIMATION 2 9
APPENDIX 2.A: T W O LEVEL DENSITY MATRIX 3 2
APPENDIX 2.B: PERTURBATION THEORY Q U I C K G U I D E 3 4
REFERENCES 3 4
3 MOLECULAR EXCITON 3 5
3.1 T H E MOLECULAR EXCITON I N AGGREGATES 3 5
3.1.1 PARALLEL DIPOLES (H-AGGREGATE) 3 7
3.1.2 IN-LINE DIPOLES (J-AGGREGATE) 3 8
3.1.3 OBLIQUE DIPOLES 3 9
3.1.4 COPLANAR DIPOLES 3 9
3.1.5 3D DIPOLE G E O M E T R Y (6 = 90) 4 0
3.2 VECTOR MODEL FOR T H E LARGE AGGREGATE 4 5
3.3 INTERACTION REGIMES A N D VIBRATIONAL DYNAMICS 4 7
3.4 QUICK VIEW O N AGGREGATE MULTIEXCITON STATES 4 9
3.5 T H E ROLE O F DISORDER 5 0
4 EXCITED STATES IN SOLIDS 53
4.1 O N T H E ORIGIN O F BANDS I N SOLIDS 5 3
4.2 EXCITONS 58
4.2.1 FRENKEL EXCITON 5 9
HTTP://D-NB.INFO/1015578381
IMAGE 2
VI C O N T E N T S
4.2.2 T H E W A N N I E R - M O T T EXCITON 63
4.2.3 I D EXCITONS 6 7
5 PHOTOEXCITATION DYNAMICS 71
5.1 PHOTOEXCITATION A N D RELAXATION SCENARIO I N INORGANIC
SEMICONDUCTORS 71
5.1.1 LINK TO PHOTOVOLTAIC 73
5.2 CONFINED STATES I N S E M I C O N D U C T I N G NANOCRYSTALS 73
5.3 CARRIER MULTIPLICATION I N NANOCRYSTALS 78
5.4 T H E EXCITATION Z O O I N MOLECULAR SEMICONDUCTORS 79
5.4.1 FREE CARRIERS 79
5.4.2 T R A P P E D CARRIERS 8 0
5.4.3 POLARONS 80
5.4.4 BIPOLARON 81
5.4.5 POLARON PAIR 81
5.4.6 C H A R G E T R A N S F E R STATE 8 2
5.4.7 C T EXCITON 8 2
5.4.8 W A N N I E R - M O T T EXCITON 8 2
5.4.9 T R I O N (CHARGED EXCITON) 83
5.4.10 FRENKEL EXCITONS 83
5.4.11 EXCITED MOLECULAR STATE 83
5.5 CONJUGATED POLYMERS 83
REFERENCES 8 7
6 PHOTOPHYSICS TOOL BOX 89
6.1 JABLONSKI D I A G R A M 8 9
6.2 STRICKLER-BERG RELATIONSHIP 91
6.3 ENERGY MIGRATION A N D T R A N S F E R 96
6.3.1 RADIATIVE MIGRATION 9 8
6.3.2 NONRADIATIVE ENERGY T R A N S F E R 99
6.4 T H E VAVILOV-KASHA RULE 103
6.5 T H E G A P LAW A N D RADIATIONLESS TRANSITIONS I N MOLECULES 105
6.6 RATE EQUATIONS 112
6.7 TRIPLET G E N E R A T I O N 114
6.7.1 SPIN FLIP 115
6.7.2 RADICAL PAIR R E C O M B I N A T I O N 118
6.7.3 SINGLET FISSION 120
APPENDIX 6. A: DERIVATION O F T H E STRICKLER-BERG RELATION 122
REFERENCES 123
7 VIBRATIONAL SPECTROSCOPY 125
7.1 T H E SEMICLASSICAL PICTURE O F T H E INTERACTION O F LIGHT W I T H
MOLECULES 125
7.2 DERIVATION O F T H E CORRELATION F U N C T I O N 129
7.3 T H E FULL VIBRONIC CORRELATOR I N T I M E 130
IMAGE 3
CONTENTS | V I I
7.4 R A M A N SCATTERING 131
7.5 C O H E R E N T P H O N O N S 136
REFERENCES 143
8 CHARGE TRANSFER A N D TRANSPORT 145
8.1 ADIABATIC ELECTRON TRANSFER: CLASSICAL M A R C U S THEORY 145
8.2 Q U A N T U M MECHANICAL EXPRESSIONS FOR ELECTRON TRANSFER:
NONADIABATIC
M U L T I P H O N O N REGIME 149 8.3 T H E D O N O R - A C C E P T O R
INTERFACE 151
8.4 C H A R G E PHOTOGENERATION I N EXCITONIC SEMICONDUCTORS 152
8.5 SYNOPSIS O N T R A N S P O R T 159
8.5.1 EXPERIMENTS TO M E A S U R E MOBILITY 163
8.5.1.1 T I M E O F FLIGHT (TOF) 163
8.5.1.2 PHOTOCONDUCTIVITY 164
8.5.1.3 FIELD EFFECT TRANSISTOR (FET) 166
8.5.1.4 P U M P PROBE 167
8.5.1.5 DIODE 170
8.5.1.6 OPTICAL T R A N S I T I O N S 171
8.5.2 EXTENDED VERSUS LOCALIZED STATES 173
REFERENCES 176
9 P U M P PROBE A N D O T H E R MODULATION TECHNIQUES 177
9.1 ELECTROABSORPTION 177
9.2 P U M P PROBE 181
9.3 C W P H O T O I N D U C E D ABSORPTION 193
A P P E N D I X 9.A: P U M P PROBE I N T H E TWO-LEVEL SYSTEM 198
APPENDIX 9.B: T H E C O H E R E N T COUPLING I N DEGENERATE P U M P
PROBE 2 0 0
10 CONCLUSION 205
BIBLIOGRAPHY 209
INDEX 211 |
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| author | Lanzani, Guglielmo |
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| dewey-ones | 530 - Physics |
| dewey-raw | 530.416 |
| dewey-search | 530.416 |
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| discipline | Physik Energietechnik |
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| language | English |
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| spelling | Lanzani, Guglielmo Verfasser (DE-588)130593117 aut The photophysics behind photovoltaics and photonics Guglielmo Lanzani Weinheim Wiley-VCH 2012 VII, 212 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Fotophysik (DE-588)4193388-6 gnd rswk-swf Fotovoltaik (DE-588)4121476-6 gnd rswk-swf Fotophysik (DE-588)4193388-6 s DE-604 Fotovoltaik (DE-588)4121476-6 s Erscheint auch als Online-Ausgabe, EPUB 978-3-527-64514-5 Erscheint auch als Online-Ausgabe, MOBI 978-3-527-64516-9 Erscheint auch als Online-Ausgabe, PDF 978-3-527-64515-2 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3887212&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024835552&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Lanzani, Guglielmo The photophysics behind photovoltaics and photonics Fotophysik (DE-588)4193388-6 gnd Fotovoltaik (DE-588)4121476-6 gnd |
| subject_GND | (DE-588)4193388-6 (DE-588)4121476-6 |
| title | The photophysics behind photovoltaics and photonics |
| title_auth | The photophysics behind photovoltaics and photonics |
| title_exact_search | The photophysics behind photovoltaics and photonics |
| title_full | The photophysics behind photovoltaics and photonics Guglielmo Lanzani |
| title_fullStr | The photophysics behind photovoltaics and photonics Guglielmo Lanzani |
| title_full_unstemmed | The photophysics behind photovoltaics and photonics Guglielmo Lanzani |
| title_short | The photophysics behind photovoltaics and photonics |
| title_sort | the photophysics behind photovoltaics and photonics |
| topic | Fotophysik (DE-588)4193388-6 gnd Fotovoltaik (DE-588)4121476-6 gnd |
| topic_facet | Fotophysik Fotovoltaik |
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