Supramolecular polymer chemistry:
Gespeichert in:
| Weitere Verfasser: | |
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| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH-Verl.
2012
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| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | Literaturangaben |
| Beschreibung: | XVIII, 372 S. Ill., graph. Darst. |
| ISBN: | 352732321X 9783527323210 9783527639786 |
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| 245 | 1 | 0 | |a Supramolecular polymer chemistry |c ed. by Akira Harada |
| 264 | 1 | |a Weinheim |b Wiley-VCH-Verl. |c 2012 | |
| 300 | |a XVIII, 372 S. |b Ill., graph. Darst. | ||
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Datensatz im Suchindex
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IMAGE 1
CONTENTS
PREFACE XIII LIST OF CONTRIBUTORS XV
PART ONE FORMATION OF SUPRAMOLECULAR POLYMERS 1
1 MULTIPLE HYDROGEN-BONDED SUPRAMOLECULAR POLYMERS 3 WILCO P.J. APPEL,
MARKO M.L NIEUWENHUIZEN, AND E.W. MEIJER 1.1 INTRODUCTION 3
1.1.1 HISTORICAL BACKGROUND 3 1.1.2 SUPRAMOLECULAR CHEMISTRY 4 1.1.3
SUPRAMOLECULAR POLYMERIZATION MECHANISMS 4 1.2 GENERAL CONCEPTS OF
HYDROGEN-BONDING MOTIFS 6 1.2.1 ARRAYS OF MULTIPLE HYDROGEN BONDS 6
1.2.2 PREORGANIZATION THROUGH INTRAMOLECULAR HYDROGEN BONDING 8 1.2.3
TAUTOMERIC EQUILIBRIA 9 1.3 HYDROGEN-BONDED MAIN-CHAIN SUPRAMOLECULAR
POLYMERS 10 1.3.1 THE ESTABLISHMENT OF SUPRAMOLECULAR POLYMERS 10 1.3.2
SUPRAMOLECULAR POLYMERIZATIONS 13 1.3.3 HYDROPHOBIE COMPARTMENTALIZATION
14 1.4 FROM SUPRAMOLECULAR POLYMERS TO SUPRAMOLECULAR MATERIALS 16 1.4.1
THERMOPLASTIC ELASTOMERS 16 1.4.2 PHASE SEPARATION AND ADDITIONAL
LATERAL INTERACTIONS IN
SUPRAMOLECULAR POLYMERS IN THE SOLID STATE 18 1.4.3 SUPRAMOLECULAR
THERMOPLASTIC ELASTOMERS BASED ON ADDITIONAL LATERAL INTERACTIONS AND
PHASE SEPARATION 19 1.5 FUTURE PERSPECTIVES 23
REFERENCES 25
2 CYCLODEXTRIN-BASED SUPRAMOLECULAR POLYMERS 29 AKIRA HARADA AND
YOSHINORI TAKASHIMA 2.1 INTRODUCTION 29
2.2 SUPRAMOLECULAR POLYMERS IN THE SOLID STATE 29 2.2.1 CRYSTAL
STRUCTURES OF CD ALIPHATIC TETHERS 30 2.2.2 CRYSTAL STRUCTURES OF SS-CDS
AROMATIC TETHERS 31
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1012093751
DIGITALISIERT DURCH
IMAGE 2
VI CONTENTS
2.3 FORMATION OF HOMO-INTRAMOLECULAR AND INTERMOLECULAR COMPLEXES BY
CDS-GUEST CONJUGATES 33 2.3.1 SUPRAMOLECULAR STRUCTURES FORMED BY
6-MODIFIED CC-CDS 33 2.3.2 SUPRAMOLECULAR STRUCTURES FORMED BY
6-MODIFIED SS-CDS 39 2.3.3 SUPRAMOLECULAR STRUCTURES FORMED BY 3-MODIFIED
A-CDS 40 2.3.4 HETERO-SUPRAMOLECULAR STRUCTURES FORMED BY MODIFIED CDS
42 2.4 FORMATION OF INTERMOLECULAR COMPLEXES BY CD AND GUEST DIMERS 44
2.5 ARTIFICIAL MOLECULAR MUSCLE BASED ON C2-DAISY CHAIN 45 2.6
CONCLUSION AND OUTLOOK 48
REFERENCES 48
3 SUPRA-MACROMOLECULAR CHEMISTRY: TOWARD DESIGN OF NEW ORGANIC MATERIALS
FROM SUPRAMOLECULAR STANDPOINTS 52 KAZUNORI SUGIYASU AND SEIJI SHINKAI
3.1 INTRODUCTION 51
3.2 SMALL MOLECULES, MACROMOLECULES, AND SUPRAMOLECULES: DESIGN OF THEIR
COMPOSITE MATERIALS 53 3.2.1 INTERACTIONS BETWEEN SMALL MOLECULES AND
MACROMOLECULES 53 3.2.2 INTERACTIONS BETWEEN SMALL MOLECULES AND
MOLECULAR ASSEMBLIES 56 3.2.3 INTERACTIONS BETWEEN MOLECULAR ASSEMBLIES
58 3.2.4 INTERACTIONS BETWEEN MACROMOLECULES 60 3.2.5 INTERACTIONS
BETWEEN MACROMOLECULAR ASSEMBLIES 63 3.2.6 INTERACTIONS BETWEEN
MACROMOLECULES AND MOLECULAR ASSEMBLIES 65 3.3 CONCLUSION AND OUTLOOK 67
REFERENCES 68
4 POLYMERIZATION WITH DITOPIC CAVITAND MONOMERS 71 FRANCESCO TANCINI AND
ENRICO DALCANALE 4.1 INTRODUCTION 71
4.2 CAVITANDS 72
4.3 SELF-ASSEMBLY OF DITOPIC CAVITAND MONOMERS 75 4.3.1 STRUCTURAL
MONOMER CLASSIFICATION OF SUPRAMOLECULAR POLYMERIZATION 75 4.3.2
HOMODITOPIC CAVITANDS SELF-ASSEMBLED VIA SOLVOPHOBIC N-N STACKING
INTERACTIONS 77
4.3.3 HETERODITOPIC CAVITANDS COMBINING SOLVOPHOBIC INTERACTIONS AND
METAL-IIGAND COORDINATION 78 4.3.4 HETERODITOPIC CAVITANDS COMBINING
SOLVOPHOBIC INTERACTIONS AND HYDROGEN BONDING 82 4.3.5 HETERODITOPIC
CAVITANDS SELF-ASSEMBLED VIA HOST-GUEST
INTERACTIONS 84
4.3.6 HOMODITOPIC CAVITANDS SELF-ASSEMBLED VIA HOST-GUEST INTERACTIONS
88 4.4 CONCLUSIONS AND OUTLOOK 91
REFERENCES 92
IMAGE 3
CONTENTS VII
PART TWO SUPRAMOLECULAR POLYMERS WITH UNIQUE STRUCTURES 95
5 POLYMERS CONTAINING COVALENTLY BONDED AND SUPRAMOLECULARLY ATTACHED
CYCLODEXTRINS AS SIDE CROUPS 97 HELMUT RITTER, MONIR TABATABAI, AND
BERND-KRISTOF MUELLER
5.1 POLYMERS WITH COVALENTLY BONDED CYCLODEXTRINS AS SIDE GROUPS 97
5.1.1 SYNTHESIS AND POLYMERIZATION OF MONOFUNCTIONAL CYDODEXTRIN
MONOMERS 98 5.1.2 POLYMER-ANALOGOUS REACTION WITH MONOFUNCTIONAL
CYDODEXTRIN 100
5.1.3 STRUCTURE-PROPERTY RELATIONSHIP OF POLYMERS CONTAINING
CYDODEXTRINS AS SIDE GROUP 102 5.2 SIDE CHAIN POLYROTAXANES AND
POLYPSEUDOROTAXANES 105 5.2.1 SIDE CHAIN POLYROTAXANES 106 5.2.2 SIDE
CHAIN POLYPSEUDOROTAXANE (POLYMER (POLYAXIS)/
CYDODEXTRIN (ROTOR)) 111 REFERENCES 120
6 ANTIBODY DENDRIMERS AND DNA CATENANES 127 HIROYASU YAMAGUCHI AND AKIRA
HARADA 6.1 MOLECULAR RECOGNITION IN BIOLOGICAL SYSTEMS 127 6.1.1
SUPRAMOLECULAR COMPLEX FORMATION OF ANTIBODIES 127
6.1.2 SUPRAMOLECULAR COMPLEXES PREPARED BY DNAS 129 6.1.3 OBSERVATION OF
TOPOLOGICAL STRUCTURES OF SUPRAMOLECULAR COMPLEXES BY ATOMIC FORCE
MICROSCOPY (AFM) 129 6.2 ANTIBODY SUPRAMOLECULES 130 6.2.1 STRUCTURAL
PROPERTIES OF INDIVIDUAL ANTIBODY MOLECULES 130 6.2.2 SUPRAMOLECULAR
FORMATION OF ANTIBODIES WITH MULTIVALENT
ANTIGENS 130
6.2.2.1 SUPRAMOLECULAR FORMATION OF ANTIBODIES WITH DIVALENT ANTIGENS
131 6.2.2.2 DIRECT OBSERVATION OF SUPRAMOLECULAR COMPLEXES OF ANTIBODIES
WITH PORPHYRIN DIMERS 133 6.2.2.3 APPLICATIONS FOR THE HIGHLY SENSITIVE
DETECTION METHOD OF SMALL
MOLECULES BY THE SUPRAMOLECULAR COMPLEXES BETWEEN ANTIBODIES AND
MULTIVALENT ANTIGENS 134 6.2.3 SUPRAMOLECULAR DENDRIMERS CONSTRUCTED BY
IGM AND CHEMICALLY MODIFIED IGG 336
6.2.3.1 PREPARATION OF ANTIBODY DENDRIMERS AND THEIR TOPOLOGICAL
STRUCTURES 136 6.2.3.2 BINDING PROPERTIES OF ANTIBODY DENDRIMERS FOR
ANTIGENS 136 6.3 DNA SUPRAMOLECULES 139
6.3.1 IMAGING OF INDIVIDUAL PLASMID DNA MOLECULES 139 6.3.2 PREPARATION
OF NICKED DNA BY THE ADDITION OF DNASE I TO PLASMID DNA 240 6.3.3
CATENATION REACTION WITH TOPOISOMERASE I 241
IMAGE 4
VIII CONTENTS
6.3.4 AFM IMAGES OF DNA CATENANES 143
6.3.5 DNA [N]CATENANES PREPARED BY IRREVERSIBLE REACTION WITH DNA IIGASE
144 6.4 CONDUSIONS 145
REFERENCES 246
7 CROWN ETHER-BASED POLYMERIC ROTAXANES 252 TERRY L PRICE JR. AND HARRY
W. GIBSON 7.1 INTRODUCTION 252
7.2 DAISY CHAINS 253
7.3 SUPRAMOLECULAR POLYMERS 256 7.4 DENDRITIC ROTAXANES 257
7.5 DENDRONIZED POLYMERS 258
7.6 MAIN CHAIN ROTAXANES BASED ON POLYMERIC CROWNS (INDUDING CROSSLINKED
SYSTEMS) 262 7.7 SIDE CHAIN ROTAXANES BASED ON PENDENT CROWNS 166 7.8
POLY[2]ROTAXANES 170
7.9 POLY[3]ROTAXANES 173
7.10 POLYMERIC END GROUP PSEUDOROTAXANES 176 7.11 CHAIN EXTENSION AND
BLOCK COPOLYMERS FROM END GROUPS 176 7.12 STAR POLYMERS FROM CROWN
FUNCTIONALIZED POLYMERS 179
REFERENCES 281
PART THREE PROPERTIES AND FUNCTIONS 283
8 PROCESSIVE ROTAXANE CATALYSTS 285 JOHANNES A.A.W. ELEMANS, ALAN E.
ROWAN, AND ROELANDJ.M. NOLTE 8.1 INTRODUCTION 285
8.2 RESULTS AND DISCUSSION 185
8.2.1 CATALYSIS 185
8.2.2 THREADING 187
8.3 CONCLUSION 192
REFERENCES 192
9 EMERGING BIOMEDICAL FUNCTIONS THROUGH'MOBILE'POLYROTAXANES 295
NOBUHIKO YUI 9.1 INTRODUCTION 195
9.2 MULTIVALENT INTERACTION USING IIGAND-CONJUGATED POLYROTAXANES 196
9.3 THE FORMATION OF POLYROTAXANE LOOPS AS A DYNAMIC INTERFACE 197 9.4
CYTOCLEAVABLE POLYROTAXANES FOR GENE DELIVERY 1 99 9.5 CONDUSION 202
9.6 APPENDIX 203
REFERENCES 204
IMAGE 5
CONTENTS IX
10 SLIDE-RING MATERIALS USING POLYROTAXANE 205
KAZUAKI KALO AND KOHZO ITO 10.1 INTRODUCTION 205
10.2 PULLEY EFFECT OF SLIDE-RING MATERIALS 208 10.3 SYNTHESIS OF
SLIDE-RING MATERIALS 209 10.4 SCATTERING STUDIES OF SLIDE-RING GELS 222
10.5 MECHANICAL PROPERTIES OF SLIDE-RING GELS 213 10.6 SLIDING GRAFT
COPOLYMERS 215 10.7 RECENT TRENDS OF SLIDE-RING MATERIALS 226 10.7.1
INTRODUCTION: DIVERSIFICATION OF THE MAIN CHAIN POLYMER 226 10.7.2
ORGANIC-INORGANIC HYBRID SLIDE-RING MATERIALS 229 10.7.3 DESIGN OF
MATERIALS FROM INTRAMOLECULAR DYNAMICS OF
POLYROTAXANES 224
10.8 CONCLUDING REMARKS 226 REFERENCES 227
11 STIMULI-RESPONSIVE SYSTEMS 232 AKIHITO HASHIDZUME AND AKIRA HARADA
11.1 INTRODUCTION 231
11.2 STIMULI AND RESPONSES 232 11.2.1 STIMULI 232
11.2.1.1 TEMPERATURE 231 11.2.1.2 PRESSURE, FORCE, STRESS, AND
ULTRASOUND 232 11.2.1.3 PH 233 11.2.1.4 CHEMICALS 233 11.2.1.5
ELECTROMAGNETIC WAVES OR LIGHT 233 11.2.1.6 REDOX 234 11.2.2 RESPONSES
234 11.2.2.1 MOVEMENT 235 11.2.2.2 CAPTURE AND RELEASE OF CHEMICALS 235
11.2.2.3 CHEMICAL REACTIONS 235 11.2.2.4 CHANGE IN VISCOELASTIC
PROPERTIES, OR GEL-TO-SOL AND SOL-TO-GEL
TRANSITIONS 236
11.2.2.5 CHANGE IN COLOR 236 11.3 EXAMPLES OF STIMULI-RESPONSIVE
SUPRAMOLECULAR POLYMER SYSTEMS 236 11.3.1 TEMPERATURE-RESPONSIVE SYSTEMS
236 11.3.2 PRESSURE-, FORCE-, AND SONICATION-RESPONSIVE SYSTEMS 239
11.3.3 PH-RESPONSIVE SYSTEMS 241 11.3.4 CHEMICAL-RESPONSIVE SYSTEMS 246
11.3.5 PHOTO-RESPONSIVE SYSTEMS 249 11.3.6 REDOX-RESPONSIVE SYSTEMS 255
11.3.7 MULTI-STIMULI-RESPONSIVE SYSTEMS 259
11.4 CONDUDING REMARKS 262 REFERENCES 262
IMAGE 6
X CONTENTS
12 PHYSICAL ORGANIC CHEMISTRY OF SUPRAMOLECULAR POLYMERS 269
STEPHEN L CRAIG AND DONGHUA XU 12.1 INTRODUCTION AND BACKGROUND 269 12.2
LINEAR SUPRAMOLECULAR POLYMERS 270 12.2.1 N,C,N-PINCER METAL COMPLEXES
270 12.2.2 LINEAR SPS 272
12.2.3 THEORY RELATED TO THE PROPERTIES OF LINEAR SPS 274 12.2.4 LINEAR
SPS IN THE SOLID STATE 275 12.3 CROSS-LINKED SPS NETWORKS 276
12.3.1 REVERSIBILITY IN SEMIDILUTE UNENTANGLED SPS NETWORKS 276 12.3.2
PROPERTIES OF SEMIDILUTE ENTANGLED SPS NETWORKS 283 12.3.3 THE STICKY
REPTATION MODEL 285
12.4 HYBRID POLYMER GELS 286
12.5 CONCLUSION 288
REFERENCES 288
13 TOPOLOGICAL POLYMER CHEMISTRY: A QUEST FOR STRANGE POLYMER RINGS 293
YASUYUKI TEZUKA 13.1 INTRODUCTION 293
13.2 SYSTEMATIC CLASSIFICATION OF NONLINEAR POLYMER TOPOLOGIES 293 13.3
TOPOLOGICAL ISOMERISM 296 13.4 DESIGNING UNUSUAL POLYMER RINGS BY
ELECTROSTATIC
SELF-ASSEMBLY AND COVALENT FIXATION 298 13.5 CONCLUSION AND FUTURE
PERSPECTIVES 302 REFERENCES 303
14 STRUCTURE AND DYNAMIC BEHAVIOR OF ORGANOMETALLIC ROTAXANES 305 YUJI
SUZAKI, TOMOKO ABE, ERIKO CHIHARA, SHINTARO MURATA, MASAKI HORIE, AND
KOHTARO OSAKADA 14.1 INTRODUCTION 305
14.1.1 CRYSTALS OF PSEUDOROTAXANES 307 14.1.2 SYNTHESIS OF
FERROCENE-CONTAINING [2]ROTAXANES BY THE
THREADING-FOLLOWED-BY-END-CAPPING STRATEGY 312 14.1.3 DETHREACTING
REACTION OF ROTAXANE-IIKE COMPLEX 326 14.1.4 PHOTOCHEMICAL PROPERTIES OF
FERROCENE-CONTAINING
ROTAXANES 328
14.1.5 FERROCENE-CONTAINING [3]ROTAXANE AND SIDE-CHAIN POLYROTAXANE 320
14.1.5.1 STRATEGIES AND SYNTHESIS OF [3]ROTAXANES 320 14.1.5.2
STRATEGIES AND SYNTHESIS OF SIDE-CHAIN
TYPE POLYROTAXANE 322
IMAGE 7
CONTENTS XI
14.2 CONCLUSION 324
14.3 APPENDIX: EXPERIMENTAL SECTION 324 REFERENCES 326
15 POLYROTAXANE NETWORK AS A TOPOLOGICALLY CROSS-LINKED POLYMER:
SYNTHESIS AND PROPERTIES 332 TOSHIKAZU TAKATA, TAKAYUKI ARAL, YASUHIRO
KOHSAKA, MASAHIRO SHIOYA, AND YASUHITO KOYAMA 15.1 INTRODUCTION 332
15.2 LINKING OF WHEELS OF MAIN-CHAIN-TYPE POLYROTAXANE - STRUCTURALLY
DEFINED POLYROTAXANE NETWORK 332 15.3 LINKING OF MACROCYCLIC UNITS OF
POLYMACROCYDE WITH AXLE UNIT TO DIRECTLY YIELD A POLYROTAXANE NETWORK
336 15.3.1 POLYROTAXANE NETWORKS HAVING CROWN ETHERS AS THE WHEEL AT THE
CROSS-LINK POINTS (I) 336 15.3.2 POLYROTAXANE NETWORK HAVING CROWN
ETHERS AS THE WHEEL AT THE CROSS-LINK POINTS (II) 337 15.3.3
POLYROTAXANE NETWORK HAVING CYCLODEXTRINS AS CROSS-LINK POINTS:
EFFECTIVE USE OF OLIGOCYDODEXTRIN 339 15.4 LINKING OF WHEELS OF
POLYROTAXANE CROSS-LINKER TO AFFORD POLYROTAXANE NETWORK: DESIGN OF THE
CROSS-LINKER 342 15.5 CONCLUSION 344
REFERENCES 345
16 FROM CHEMICAL TOPOLOGY TO MOLECULAR MACHINES 347 JEAN-PIERRE SAUVAGE
16.1 INTRODUCTION 347
16.2 COPPER(I)-TEMPLATED SYNTHESIS OF CATENANES: THE 'ENTWINING'
APPROACH AND THE 'GATHERING AND THREADING' STRATEGY 347 16.3 MOLECULAR
KNOTS 349
16.4 MOLECULAR MACHINES BASED ON CATENANES AND ROTAXANES 353 16.5
TWO-DIMENSIONAL INTERLOCKING ARRAYS 354 16.6 A [3]ROTAXANE ACTING AS AN
ADJUSTABLE RECEPTOR TOWARD A MOLECULAR 'PRESS' 355
16.7 CONDUSION 356
REFERENCES 356
INDEX 362 |
| any_adam_object | 1 |
| author2 | Harada, Akira |
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| author_GND | (DE-588)1018150617 |
| author_facet | Harada, Akira |
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| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 547 - Organic chemistry |
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| id | DE-604.BV039858541 |
| illustrated | Illustrated |
| indexdate | 2024-07-21T00:22:55Z |
| institution | BVB |
| isbn | 352732321X 9783527323210 9783527639786 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-024718147 |
| oclc_num | 769467700 |
| open_access_boolean | |
| owner | DE-703 DE-92 DE-20 DE-91G DE-BY-TUM DE-19 DE-BY-UBM |
| owner_facet | DE-703 DE-92 DE-20 DE-91G DE-BY-TUM DE-19 DE-BY-UBM |
| physical | XVIII, 372 S. Ill., graph. Darst. |
| publishDate | 2012 |
| publishDateSearch | 2012 |
| publishDateSort | 2012 |
| publisher | Wiley-VCH-Verl. |
| record_format | marc |
| spelling | Supramolecular polymer chemistry ed. by Akira Harada Weinheim Wiley-VCH-Verl. 2012 XVIII, 372 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Literaturangaben Polymere (DE-588)4046699-1 gnd rswk-swf Supramolekulare Chemie (DE-588)4306141-2 gnd rswk-swf Polymere (DE-588)4046699-1 s Supramolekulare Chemie (DE-588)4306141-2 s DE-604 Harada, Akira (DE-588)1018150617 edt Erscheint auch als Online-Ausgabe, EPUB 978-3-527-63979-3 Erscheint auch als Online-Ausgabe, MOBI 978-3-527-63981-6 Erscheint auch als Online-Ausgabe, PDF 978-3-527-63980-9 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3830282&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024718147&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Supramolecular polymer chemistry Polymere (DE-588)4046699-1 gnd Supramolekulare Chemie (DE-588)4306141-2 gnd |
| subject_GND | (DE-588)4046699-1 (DE-588)4306141-2 |
| title | Supramolecular polymer chemistry |
| title_auth | Supramolecular polymer chemistry |
| title_exact_search | Supramolecular polymer chemistry |
| title_full | Supramolecular polymer chemistry ed. by Akira Harada |
| title_fullStr | Supramolecular polymer chemistry ed. by Akira Harada |
| title_full_unstemmed | Supramolecular polymer chemistry ed. by Akira Harada |
| title_short | Supramolecular polymer chemistry |
| title_sort | supramolecular polymer chemistry |
| topic | Polymere (DE-588)4046699-1 gnd Supramolekulare Chemie (DE-588)4306141-2 gnd |
| topic_facet | Polymere Supramolekulare Chemie |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3830282&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024718147&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT haradaakira supramolecularpolymerchemistry |