Chemical energy storage:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
de Gruyter
2013
|
| Schriftenreihe: | de Gruyter graduate
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XX, 479 S. Ill., graph. Darst. |
| ISBN: | 3110264072 9783110264074 |
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| 245 | 1 | 0 | |a Chemical energy storage |c ed. by Robert Schlögl |
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IMAGE 1
CONTENTS
AUTHOR INDEX XV
1.1 THE SOLAR REFINERY 1
ROBERT SCHLIIGL
1.1.1 INTRODUCTION 1
1.1.2 THE ROLE O F CHEMISTRY IN THE ENERGY CHALLENGE 5
1.1.3 CHEMICAL REACTIONS AND CATALYSIS 7
1.1.4 THE DESIGN O F CATALYSTS AND PROCESSES 16
1.1.5 THE BIOLOGICAL ORIGIN O F OUR PRESENT ENERGY SYSTEM 17
1.1.6 CHEMICAL ENERGY STORAGE: ONE LONG-TERM SOLUTION 20
1.1.7 REFERENCES 30
1.2 ENERGY STORAGE STRATEGIES 35
FERDI SCHIITH
1.2.1 INTRODUCTION 35
1.2.2 GENERAL CONSIDERATIONS 35
1.2.3 HEAT (COLD) STORAGE 37
1.2.4 GRID-SCALE STORAGE O F ELECTRICAL ENERGY 39
1.2.4.1 STORAGE ON THE TRANSMISSION GRID SCALE 40
1.2.4.2 STORAGE ON DISTRIBUTION AND MEDIUM-VOLTAGE GRID SCALE 43
1.2.5 ENERGY STORAGE FOR MOBILE APPLICATIONS 44
1.2.5.1 CHEMICAL COMPOUNDS 45
1.2.5.2 TRACTION BATTERIES 46
1.2.6 SYSTEMS CONSIDERATIONS 47
1.3 ENERGY AND SOCIETY: A PRACTICAL GUIDE 49
GERHARD HOFMANN
1.3.1 NOTES 57
1.3.2 REFERENCES 57
2.1 BIOFUELS DERIVED FROM RENEWABLE FEEDSTOCKS 59
REGINA PALKOVITS AND WILLIAM R. H. WRIGHT
2.1.1 INTRODUCTION 59
HTTP://D-NB.INFO/1018469745
IMAGE 2
VI | C O N T E N T S
2.1.2 SOURCES O F BIOMASS 59
2.1.3 LIGNOCELLULOSE AS FEEDSTOCK 62
2.1.4 BIOETHANOL AS SUSTAINABLE BIOFUEL 63
2.1.5 BIODIESEL AS POTENTIAL BIOFUEL 66
2.1.6 PRODUCTION O F BIOFUEL VIA CHEMICAL TRANSFORMATIONS O F
LIGNOCELLULOSE 68
2.1.7 CONTROLLED TRANSFORMATIONS O F CARBOHYDRATES INTO HYDROCARBON
FUELS 72
2.1.8 CONTROLLED TRANSFORMATIONS O F CARBOHYDRATES INTO NOVEL BIOFUELS
76
2.1.8.1 TRANSFORMATIONS BASED ON LA 77
2.1.8.2 BIOFUEL COMPOUNDS BASED ON 5 - H M F 79
2.1.9 CONTROLLED TRANSFORMATIONS O F LIGNIN INTO POTENTIAL FUEL
COMPOUNDS 81
2.1.10 SUMMARY 82
2.1.11 ACKNOWLEDGMENT 82
2.1.12 REFERENCES 82
2.2 BIOMASS CONVERSION TO CHEMICALS 87
ARMIN BRANDNER AND PETER CLAUS
2.2.1 INTRODUCTION 87
2.2.2 CLASSIFICATION O F BIOMASS 88
2.2.2.1 LIGNOCELLULOSE 89
2.2.2.2 LIPIDS 94
2.2.2.3 PROTEINS 98
2.2.3 SELECTED KEY CHEMICALS 98
2.2.3.1 CELLULOSE 98
2.2.3.2 GLYCEROL 99
2.2.4 TECHNOLOGIES AND REQUIREMENTS FOR CHEMICAL PRODUCTION FROM BIOMASS
103
2.2.5 ECONOMIC CONSIDERATIONS 104
2.2.6 OUTLOOK 105
2.2.7 REFERENCES 105
2.3 THERMAL CONVERSION OF BIOMASS 109
NIKOLAI DEMARTINI, ATTE AHO, MIKKO HUPA, AND DMITRY YU. MURZIN
2.3.1 TORREFACTION 112
2.3.2 PYROLYSIS 112
2.3.2.1 INTRODUCTION 112
2.3.2.2 PYROLYSIS REACTORS 113
2.3.2.3 BIOMASS 114
2.3.2.4 COMPOSITION O F BIO-OIL 114
IMAGE 3
C O N T E N T S [ VII
2.3.2.5 UTILIZATION O F BIO-OIL 115
2.3.2.6 UPGRADING OF BIO-OIL 115
2.3.3 GASIFICATION 116
2.3.3.1 INTRODUCTION 116
2.3.3.2 GASIFICATION REACTORS 117
2.3.3.3 ENERGY IN GASIFICATION 118
2.3.4 COMBUSTION 118
2.3.4.1 INTRODUCTION 118
2.3.4.2 ENERGY IN COMBUSTION 119
2.3.4.3 CO-COMBUSTION 119
2.3.5 SUMMARY 120
2.3.6 REFERENCES 121
2.4 BIOMASS TO MINERALIZED CARBON: ENERGY GENERATION AND/OR CARBON
SEQUESTRATION 125
MARKUS ANTONIETTI
2.4.1 INTRODUCTION 125
2.4.2 H T C 126
2.4.2.1 H T C O F BIOMASS WASTE FOR ENVIRONMENTALLY FRIENDLY CARBON
SEQUESTRATION 126
2.4.2.2 H T C FOR "CARBON-NEGATIVE MATERIALS" 127
2.4.3 MINERALIZED BIOMASS AS ENERGY CARRIER 129
2.4.3.1 "BIOCOAL" AND ITS COMPARISON TO OTHER BIOFUELS, BIOGAS AND B I O
E T H A N O L . . . . 129 2.4.3.2 CARBON FUEL CELLS 132
2.4.4 DISCUSSION AND CONCLUSION 133
2.4.5 REFERENCES 133
3.1 ELECTROCHEMICAL CONCEPTS: A PRACTICAL GUIDE 135
KARL DOBLHOFER
3.1.1 INTRODUCTION 135
3.1.2 ELECTRODES IN ELECTROLYTES 137
3.1.3 ENERGETICS O F ELECTRODE REACTIONS 138
3.1.4 THE ELECTROCHEMICAL CELL 140
3.1.4.1 THE CONCEPT 140
3.1.4.2 CHEMICAL AND ELECTRIC ENERGY 142
3.1.4.3 THE MAXIMUM ELECTRIC ENERGY PRODUCED AND THE EQUILIBRIUM CELL
VOLTAGE 144
3.1.5 CONCENTRATION DEPENDENCE O F E: THE NERNST EQUATION 145
3.1.5.1 THE NERNST EQUATION 145
3.1.5.2 CONCENTRATION CELLS 147
IMAGE 4
VIII | C O N T E N T S
3.1.6 THE TEMPERATURE DEPENDENCE OF THE EQUILIBRIUM CELL VOLTAGE, E 148
3.1.7 CONCLUSION 148
3.1.8 ACKNOWLEDGMENT 149
3.1.9 REFERENCES 150
3.2 WATER-SPLITTING CONCEPTUAL APPROACH 151
JAN ROSSMEISL
3.2.1 INTRODUCTION 151
3.2.2 FUNDAMENTALS 151
3.2.3 STANDARD (REVERSIBLE) HYDROGEN ELECTRODE 152
3.2.4 THE CATHODE HALF-CELL REACTION 153
3.2.5 THE ANODE HALF-CELL REACTION 154
3.2.5.1 FREE ENERGY DIAGRAM 155
3.2.5.2 TAFEL EQUATION AND A ( J O E R 156
3.2.5.3 SCALING RELATIONS 158
3.2.5.4 UNIVERSAL SCALING AND TRENDS IN ACTIVITY 159
3.2.6 CONCLUSION 161
3.2.7 REFERENCES 161
3.3 FUEL CELLS 163
PETER STRASSER
3.3.1 WHAT IS A FUEL CELL? 164
3.3.2 COMPONENTS O F A FUEL CELL 165
3.3.3 PERFORMANCE CHARACTERISTICS O F A FUEL CELL 170
3.3.4 THE ELECTROCATALYSIS O F OXYGEN REDUCTION AT FUEL CELL CATHODES
173
3.3.4.1 UNDERSTANDING THE ELECTRODE POTENTIAL DEPENDENCE O F THE O R R
173
3.3.4.2 UNDERSTANDING AND PREDICTING TRENDS IN O R R ACTIVITY ON
TRANSITION-METAL CATALYSTS 174
3.3.4.3 NANOSTRUCTURED PT CORE-SHELL ELECTROCATALYSTS FOR THE O R R 177
3.3.4.4 NOBLE-METAL-FREE O R R P E M F C ELECTROCATALYSTS 182
3.3.5 CONCLUSIONS . 182
3.3.6 ACKNOWLEDGMENTS 183
3.3.7 REFERENCES 183
3.4 MOLECULAR CONCEPTS OF WATER SPLITTING: NATURE'S APPROACH 185
NICHOLAS COX AND WOLFGANG LUBITZ
3.4.1 INTRODUCTION 185
IMAGE 5
C O N T E N T S | IX
3.4.2 WATER OXIDATION 187
3.4.2.1 PSII 187
3.4.2.2 GEOMETRIC STRUCTURE O F THE W O C 190
3.4.2.3 ELECTRONIC STRUCTURE O F THE W O C 192
3.4.2.4 FUNCTION OF THE W O C 194
3.4.2.5 SUGGESTED MECHANISMS OF O O BOND FORMATION 195
3.4.2.6 SUMMARY: PRINCIPLES O F PHOTOSYNTHETIC WATER SPLITTING 197
3.4.2.7 CURRENT WATER-SPLITTING CATALYSTS 198
3.4.3 HYDROGEN PRODUCTION AND CONVERSION 199
3.4.3.1 CLASSIFICATION O F HYDROGENASES 200
3.4.3.2 STRUCTURE O F [NIFE] AND [FEFE] HYDROGENASES 200
3.4.3.3 INTERMEDIATE STATES AND REACTION MECHANISMS 203
3.4.3.4 OXYGEN SENSITIVITY AND TOLERANCE 209
3.4.3.5 DESIGN PRINCIPLES O F HYDROGENASES 210
3.4.3.6 MOLECULAR CATALYSTS FOR H2 CONVERSION AND PRODUCTION 211
3.4.4 CONCLUSIONS 213
3.4.5 ACKNOWLEDGMENTS 214
3.4.6 NOTES 214
3.4.7 REFERENCES 215
3.5 BATTERIES: CONCEPTS AND SYSTEMS 225
DOMINIK SAMUELIS AND JOACHIM MAIER
3.5.1 INTRODUCTION 225
3.5.2 SECONDARY BATTERY SYSTEMS 228
3.5.3 LITHIUM BATTERIES 232
3.5.4 THERMODYNAMICS O F ELECTROCHEMICAL ENERGY STORAGE 236
3.5.5 KINETICS OF ENERGY STORAGE 239
3.5.6 MATERIALS OPTIMIZATION: ADJUSTING SCREWS 240
3.5.7 OUTLOOK 244
3.5.8 ACKNOWLEDGMENTS 244
3.5.9 NOTE . , 245
3.5.10 REFERENCES 245
4.1 CHEMICAL KINETICS: A PRACTICAL GUIDE 249
SEBASTIAN ARNDT AND REINHARD SCHOMACKER
4.1.1 THEORY 249
4.1.1.1 INTRODUCTION 249
4.1.1.2 COURSE OF A CATALYTIC REACTION 249
4.1.1.3 REACTION KINETICS 251
IMAGE 6
X | C O N T E N T S
4.1.2 PRACTICAL ASPECTS 258
4.1.2.1 LABORATORY REACTORS 258
4.1.2.2 PRELIMINARY TESTS 258
4.1.2.3 COMPARATIVE STUDIES 259
4.1.2.4 DEVELOPMENT O F KINETIC MODELS 260
4.1.3 EXAMPLES 264
4.1.3.1 OXIDATIVE COUPLING O F METHANE 264
4.1.3.2 DECOMPOSITION O F AMMONIA 267
4.1.3.3 SLURRY REACTION 270
4.1.4 NOTES 273
4.1.5 ACKNOWLEDGMENT 274
4.1.6 ABBREVIATIONS 274
4.1.7 REFERENCES 275
4.2 SYNTHESIS OF SOLID CATALYSTS 277
ANNETTE TRUNSCHKE
4.2.1 MACROSCOPIC CATALYST BODIES 280
4.2.2 THE ACTIVE PHASE 285
4.2.3 DISPERSED SURFACE SPECIES 296
4.2.4 FINAL REMARKS 300
4.2.5 ACKNOWLEDGMENTS 301
4.2.6 REFERENCES 301
4.3 IN SITU ANALYSIS OF HETEROGENEOUS CATALYSTS IN CHEMICAL ENERGY
CONVERSION 311
JAN-DIERK GRUMVALDT
4.3.1 SETTING THE SCENE FOR CATALYST CHARACTERIZATION IN ENERGY-RELATED
CATALYSIS AND ENERGY STORAGE 311
4.3.2 THE BENCH O F COMPLEMENTARY CHARACTERIZATION METHODS 312
4.3.3 IMPORTANCE O F IN SITU STUDIES 314
4.3.4 IN SITU CELL DESIGN: A CHALLENGE BETWEEN ENGINEERING AND
SPECTROSCOPY FOR DYNAMIC EXPERIMENTS AND STRUCTURE PERFORMANCE
RELATIONSHIPS 316
4.3.5 CASE STUDIES IN GAS PHASE, LIQUID PHASE, HIGH PRESSURE, AND OTHER
DEMANDING REACTION CONDITIONS 318
4.3.6 WATCHING ENSEMBLES AND REACTORS AT WORK: SPATIALLY RESOLVED
STUDIES 321
IMAGE 7
C O N T E N T S | XI
4.3.7 CONCLUSIONS AND OUTLOOK 323
4.3.8 ACKNOWLEDGMENT 324
4.3.9 REFERENCES 324
4.4 MODEL SYSTEMS IN CATALYSIS FOR ENERGY ECONOMY 329
NIKLAS NILIUS, MARTIN STERRER, SHAMIL SHAIKHUTDINOV, DIETRICH MENZEL,
AND HANS-JOACHIM FREUND
4.4.1 INTRODUCTION 329
4.4.2 FIRST CASE STUDY: CONTROLLING NANOPARTICLE SHAPES ON NONDOPED AND
DOPED OXIDE SUPPORTS 331
4.4.3 SECOND CASE STUDY: PREPARATION O F OXIDE-SUPPORTED PALLADIUM MODEL
CATALYSTS BY PD DEPOSITION FROM SOLUTION 336
4.4.4 THIRD CASE STUDY: STRONG METAL/SUPPORT INTERACTION EFFECTS 340
4.4.5 FOURTH CASE STUDY: PHOTOCHEMISTRY AT NANOPARTICLES 344
4.4.6 SYNOPSIS 348
4.4.7 REFERENCES 348
4.5 CHALLENGES IN MOLECULAR ENERGY RESEARCH 353
SERENA DEBEER, MAURICE VAN GASTEL, ECKHARD BILL, SHENGFA YE, TARAS
PETRENKO, DIMITRIOS A. PANTAZIS, FRANK NEESE
4.5.1 INTRODUCTION 353
4.5.2 MODERN SPECTROSCOPY AND QUANTUM CHEMISTRY AS A MEANS T O DECIPHER
REACTION MECHANISMS 355
4.5.3 FUNDAMENTAL CHEMISTRY O F ENERGY CONVERSION 357
4.5.3.1 HYDROGEN PRODUCTION 357
4.5.3.2 WATER OXIDATION 360
4.5.3.3 OXYGEN ACTIVATION 364
4.5.3.4 METHANE OXIDATION 368
4.5.3.5 CONVERSION O F DINITROGEN TO AMMONIA 370
4.5.4 SUMMARY AND OUTLOOK 372
4.5.5 ACKNOWLEDGMENTS 373
4.5.6 REFERENCES 373
5.1 PHOTOELECTROCHEMICAL CO2 ACTIVATION TOWARD ARTIFICIAL LEAVES 379
GABRIELE CENTI AND SIGLINDA PERATHONER
5.1.1 INTRODUCTION 379
5.1.2 ARTIFICIAL LEAVES AND PEC CO2 ACTIVATION 380
IMAGE 8
XII | C O N T E N T S
5.1.3 FUNDAMENTALS O F WATER AND CO2 ELECTROLYSIS 382
5.1.4 DESIGNING THE ELECTROCATALYTIC CATHODE FOR CO2 REDUCTION 388
5.1.5 DESIGNING THE PHOTOANODE 391
5.1.6 PEC CELLS FOR CO2 CONVERSION 395
5.1.7 CONCLUSIONS 397
5.1.8 REFERENCES 398
5.2 THERMOCHEMICAL CO2 ACTIVATION 401
KEVIN KAHLER, THOMAS FRANZKE, AND MARTIN MUHLER
5.2.1 INTRODUCTION 401
5.2.2 GENERAL KINETIC AND THERMODYNAMIC CONSIDERATIONS 402
5.2.3 SOLARTHERMAL CYCLES 403
5.2.3.1 GENERAL PRINCIPLES 403
5.2.3.2 EXAMPLES 408
5.2.4 DRY REFORMING OF METHANE 411
5.2.5 SUMMARY 411
5.2.6 REFERENCES 411
5.3 METHANOL CHEMISTRY 413
EDWARD KUNKES AND MALTE BEHRENS
5.3.1 WHY METHANOL? 413
5.3.2 INTRODUCTION TO METHANOL SYNTHESIS AND STEAM REFORMING 415
5.3.3 TODAY'S INDUSTRIAL METHANOL SYNTHESIS 417
5.3.4 THE REACTION MECHANISM OF METHANOL SYNTHESIS 419
5.3.5 METHANOL SYNTHESIS FROM CO2: THERMODYNAMIC AND KINETIC
CONSIDERATIONS 422
5.3.6 CU/ZNO-BASED METHANOL SYNTHESIS CATALYSTS 426
5.3.7 METHANOL STEAM REFORMING (MSR) 430
5.3.8 CHALLENGES AND PERSPECTIVES IN CATALYST AND PROCESS DEVELOPMENT
FOR ENERGY-RELATED APPLICATION O F METHANOL 433
5.3.9 NOTES 435
5.3.10 REFERENCES 435
IMAGE 9
C O N T E N T S | XIII
5.4 SYNTHESIS GAS TO HYDROGEN, METHANOL, AND SYNTHETIC FUELS 443
JAN VAN DE LOOSDRECHT AND J. W. (HANS) NIEMANTSVERDRIET
5.4.1 INTRODUCTION 443
5.4.2 PRODUCTION O F SYNTHESIS GAS 443
5.4.3 APPLICATIONS O F SYNTHESIS GAS: H2 AND METHANOL 445
5.4.3.1 SYNGAS TO HYDROGEN: THE W G S REACTION 445
5.4.3.2 SYNGAS TO METHANOL 446
5.4.4 SYNGAS TO SYNTHETIC FUELS: THE FISCHER-TROPSCH SYNTHESIS 446
5.4.4.1 CHEMISTRY AND CATALYSTS 447
5.4.5 REFERENCES 455
INDEX 459 |
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| genre | 1\p (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV039845456 |
| illustrated | Illustrated |
| indexdate | 2025-02-20T07:06:22Z |
| institution | BVB |
| isbn | 3110264072 9783110264074 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-024705287 |
| oclc_num | 761193764 |
| open_access_boolean | |
| owner | DE-91G DE-BY-TUM DE-1028 DE-703 DE-862 DE-BY-FWS DE-11 DE-1046 DE-634 DE-188 DE-20 DE-1050 DE-19 DE-BY-UBM DE-29T DE-1102 DE-92 DE-573 DE-526 DE-M347 |
| owner_facet | DE-91G DE-BY-TUM DE-1028 DE-703 DE-862 DE-BY-FWS DE-11 DE-1046 DE-634 DE-188 DE-20 DE-1050 DE-19 DE-BY-UBM DE-29T DE-1102 DE-92 DE-573 DE-526 DE-M347 |
| physical | XX, 479 S. Ill., graph. Darst. |
| publishDate | 2013 |
| publishDateSearch | 2013 |
| publishDateSort | 2013 |
| publisher | de Gruyter |
| record_format | marc |
| series2 | de Gruyter graduate |
| spellingShingle | Chemical energy storage Energiespeicherung (DE-588)4014722-8 gnd Energieumwandlung (DE-588)4014730-7 gnd Chemische Energie (DE-588)4204749-3 gnd |
| subject_GND | (DE-588)4014722-8 (DE-588)4014730-7 (DE-588)4204749-3 (DE-588)4143413-4 |
| title | Chemical energy storage |
| title_auth | Chemical energy storage |
| title_exact_search | Chemical energy storage |
| title_full | Chemical energy storage ed. by Robert Schlögl |
| title_fullStr | Chemical energy storage ed. by Robert Schlögl |
| title_full_unstemmed | Chemical energy storage ed. by Robert Schlögl |
| title_short | Chemical energy storage |
| title_sort | chemical energy storage |
| topic | Energiespeicherung (DE-588)4014722-8 gnd Energieumwandlung (DE-588)4014730-7 gnd Chemische Energie (DE-588)4204749-3 gnd |
| topic_facet | Energiespeicherung Energieumwandlung Chemische Energie Aufsatzsammlung |
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| work_keys_str_mv | AT schloglrobert chemicalenergystorage |
Beschreibung
THWS Schweinfurt Zentralbibliothek Lesesaal
| Signatur: |
2000 ZP 4100 S345 |
|---|---|
| Exemplar 1 | ausleihbar Verfügbar Bestellen |