Quantum control of molecular processes:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH
2012
|
| Ausgabe: | 2., revised and enlarged ed. |
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XVII, 544 S. Ill., graph. Darst. |
| ISBN: | 9783527409044 3527409041 9783527639724 9783527639717 |
Internformat
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| 100 | 1 | |a Shapiro, Moshe |d 1944-2013 |e Verfasser |0 (DE-588)1018150749 |4 aut | |
| 245 | 1 | 0 | |a Quantum control of molecular processes |c Moshe Shapiro and Paul Brumer |
| 250 | |a 2., revised and enlarged ed. | ||
| 264 | 1 | |a Weinheim |b Wiley-VCH |c 2012 | |
| 300 | |a XVII, 544 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
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Datensatz im Suchindex
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IMAGE 1
VIL
CONTENTS
PREFACE TO THE SECOND EDITION XIII
PREFACE TO THE FIRST EDITION XV
1 PRELIMINARIES OF THE INTERACTION OF LIGHT WITH MATTER 1
2 WEAK-FIELD PHOTODISSOCIATION 5 2.1 PHOTOEXCITATION OF A MOLECULE WITH
A PULSE OF LIGHT 6 2.2 STATE PREPARATION DURING THE PULSE S 2.3
PHOTODISSOCIATION 13
2.3.1 GENERAL FORMALISM 13 2.3.2 ELECTRONIC STATES 20 2.3.3
ENERGY-RESOLVED QUANTITIES 21 2.A APPENDIX: MOLECULAR STATE LIFETIME IN
PHOTODISSOCIATION 22
3 WEAK-FIELD COHERENT CONTROL 25 3.1 TRADITIONAL EXCITATION 25 3.2
PHOTODISSOCIATION FROM A SUPERPOSITION STATE 26 3.2.1 BICHROMATIC
CONTROL 28
'S.2.2 ENERGY AVERAGING AND SATELLITE CONTRIBUTIONS 31 3.3 THE PRINCIPLE
OF COHERENT CONTROL 33 3.4 INTERFERENCE BETWEEN N-PHOTON AND M-PHOTON
ROUTES 35 3 A.I MULTIPHOTON ABSORPTION 35
3.4.2 ONE- VS. THREE-PHOTON INTERFERENCE 39 3.4.2.1 ONE- VS.
THREE-PHOTON INTERFERENCE: THREE-DIMENSIONAL FORMALISM 41 3.4.3 ONE- VS.
TWO-PHOTON INTERFERENCE: SYMMETRY BREAKING 50 3.5 POLARIZATION CONTROL
OF DIFFERENTIAL CROSS SECTIONS 56
3.6 PUMP-DUMP CONTROL: FEW LEVEL EXCITATION 57 3.A APPENDIX:
MODE-SELECTIVE CHEMISTRY 68
4 CONTROL OF INTRAMOLECULAR DYNAMICS 71 4.1 INTRAMOLECULAR DYNAMICS 71
4.1.1 TIME EVOLUTION AND THE ZERO-ORDER BASIS 72 4.1.2 PARTITIONING OF
THE HUBERT SPACE 73
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1013143930
DIGITALISIERT DURCH
IMAGE 2
VIII CONTENTS
4.1.3 INITIAL STATE CONTROL AND OVERLAPPING RESONANCES 75
4.1.3.1 INTERNAL CONVERSION IN PYRAZINE 77 4.1.3.2 INTRAMOLECULAR
VIBRATIONAL REDISTRIBUTION: OCS 78
5 OPTIMAL CONTROL THEORY 83 5.1 PUMP-DUMP EXCITATION WITH MANY LEVELS:
THE TANNOR-RICE SCHEME 83 5.2 OPTIMAL CONTROL THEORY 89
5.2.1 GENERAL PRINCIPLES OF OPTIMAL CONTROL THEORY 89
6 DECOHERENCE AND ITS EFFECTS ON CONTROL 95 6.1 DECOHERENCE 95 6.1.1
MASTER EQUATIONS 98 6.2 SAMPLE COMPUTATIONAL RESULTS ON DECOHERENCE 100
6.2.1 ELECTRONIC DECOHERENCE 100 6.2.2 VIBRATIONAL DECOHERENCE IN
CONDENSED PHASES 102 6.2.3 DECOHERENCE: TOWARDS THE CLASSICAL LIMIT 106
6.3 ENVIRONMENTAL EFFECTS ON CONTROL: SOME THEOREMS 109
6.3.1 ENVIRONMENT CAN LIMIT CONTROL 109 6.3.2 ENVIRONMENT CAN ENHANCE
CONTROL 112 6.3.2.1 ENVIRONMENTALLY ASSISTED TRANSPORT 112 6.3.3
ENVIRONMENTALLY ASSISTED ONE-PHOTON PHASE CONTROL 114
6.3.4 ISOLATED MOLECULES 116 6.3.5 NONISOLATED SYSTEMS 117 6.4
DECOHERENCE AND CONTROL 119 6.4.1 THE OPTICAL BLOCH EQUATION 120
6.4.1.1 DECOHERENCE EFFECTS IN ONE-PHOTON VS. THREE-PHOTON ABSORPTION
121 6.4.2 COUNTERING COLLISIONAL EFFECTS 126 6.4.3 ADDITIONAL CONTROL
STUDIES 129 6.4.4 STATE STABILITY AGAINST DECOHERENCE 133 6.4.5
OVERLAPPING RESONANCES AND DECOHERENCE CONTROL: QUALITATIVE
MOTIVATION 135 6.4.6 CONTROL OF DEPHASING 139 6.5 COUNTERING PARTIALLY
COHERENT LASER EFFECTS IN PUMP-DUMP CONTROL 142 6.6 COUNTERING CW LASER
JITTER 149
6.6.1 LASER PHASE ADDITIVITY 150 6.6.2 INCOHERENT INTERFERENCE CONTROL
151
7 CASE STUDIES IN COHERENT CONTROL 153 7.1 TWO-PHOTON VS. TWO-PHOTON
CONTROL 153 7.1.1 EXPERIMENTAL IMPLEMENTATION 160 7.2 CONTROL OVER THE
REFRACTIVE INDEX 169
7.2.1 BICHROMATIC CONTROL 171 7.3 THE MOLECULAR PHASE IN THE PRESENCE OF
RESONANCES 176
IMAGE 3
CONTENTS IX
7.3.1 THEORY OF SCATTERING RESONANCES 178
7.3.2 THREE-PHOTON VS. ONE-PHOTON COHERENT CONTROL IN THE PRESENCE OF
RESONANCES 182 7.3.2.1 CASE (A): AN INDIRECT TRANSITION TO AN ISOLATED
RESONANCE 184 7.3.2.2 CASE (B): A PURELY DIRECT TRANSITION TO THE
CONTINUUM 184 7.3.2.3 CASE (C): AN INDIRECT TRANSITION TO A SET OF
OVERLAPPING RESONANCES 185 7.3.2 A CASE (D): A SUM OF DIRECT AND
INDIRECT TRANSITION TO AN ISOLATED RESONANCE 185 7.4 CONTROL OF CHAOTIC
DYNAMICS 186
8 COHERENT CONTROL OF BIMOLECULAR PROCESSES 191 8.1 FIXED ENERGY
SCATTERING: ENTANGLED INITIAL STATES 191 8.1.1 ISSUES IN THE PREPARATION
OF THE SCATTERING SUPERPOSITION 193 8.1.2 IDENTICAL PARTICLE COLLISIONS
195
8.1.3 SAMPLE CONTROL RESULTS 198 8.1.3.1 M SUPERPOSITIONS 198 8.1.3.2
CONTROL IN COLD ATOMS: PENNING VS. DISSOCIATIVE IONIZATION 201 8.1.3.3
CONTROL IN ELECTRON IMPACT DISSOCIATION 207 8.1.4 EXPERIMENTAL
IMPLEMENTATION: FIXED TOTAL ENERGY 211 8.1.5 OPTIMAL CONTROL OF
BIMOLECULAR SCATTERING 212
8.1.5.1 OPTIMIZED BIMOLECULAR SCATTERING: THE TOTAL SUPPRESSION OF A
REACTIVE EVENT 214 8.1.6 SCULPTED IMPLODING WAVES 216 8.2 TIME DOMAIN:
FAST TIMED COLLISIONS 217
8.2.1 NONENTANGLED WAVE PACKET SUPERPOSITIONS: TIME-DEPENDENT SCATTERING
217 8.2.2 ENTANGLED OR WAVE PACKETS? 220
9 THE INTERACTION OF LIGHT WITH MATTER: A CLOSER LOOK 223 9.1 CLASSICAL
ELECTRODYNAMICS OF A PULSE OF LIGHT 223 9.1.1 THE CLASSICAL HAMILTONIAN
223 9.1.2 THE FREE LIGHT FIELD 226 9.2 THE DYNAMICS OF QUANTIZED
PARTICLES AND CLASSICAL LIGHT FIELDS 228
10 COHERENT CONTROL WITH QUANTUM LIGHT 233 10.1 THE QUANTIZATION OF THE
ELECTROMAGNETIC FIELD 233 10.1.1 LIGHT-MATTER INTERACTIONS 235 10.2
QUANTUM LIGHT AND QUANTUM INTERFERENCE 236
10.2.1 ONE-PHOTON VS. TWO-PHOTON QUANTUM FIELD CONTROL 238 10.2.1.1 USE
OF NUMBER STATES 238 10.2.1.2 USE OF COHERENT STATES 239
10.2.2 PUMP-DUMP COHERENT CONTROL 240
IMAGE 4
X CONTENTS
10.2.2.1 RESULTS WITH QUANTIZED LIGHT 240
10.2.2.2 RESULTS WITH CLASSICAL FIELDS 242 10.2.3 PHASE-INDEPENDENT
CONTROL 243 10.3 QUANTUM FIELD CONTROL OF ENTANGLEMENT 245 10.3.1
LIGHT-MATTER ENTANGLEMENT 245
10.3.2 CREATING ENTANGLEMENT BETWEEN A CHAIN OF MOLECULES AND A
RADIATION FIELD 247 10.4 CONTROL OF ENTANGLEMENT IN QUANTUM FIELD CHIRAL
SEPARATION 250
11 COHERENT CONTROL BEYOND THE WEAK-FIELD REGIME: BOUND STATES AND
RESONANCES 253 11.1 ADIABATIC POPULATION TRANSFER 253 11.1.1 ADIABATIC
STATES, TRAPPING, AND ADIABATIC FOLLOWING 254
11.1.2 THE MULTISTATE EXTENSION OF STI RAP 260 11.2 AN ANALYTIC SOLUTION
OF THE NONDEGENERATE QUANTUM CONTROL PROBLEM 261 11.3 THE DEGENERATE
QUANTUM CONTROL PROBLEM 266
11.4 ADIABATIC ENCODING AND DECODING OF QUANTUM INFORMATION 271 11.5
MULTISTATE PIECEWISE ADIABATIC PASSAGE 275 11.5.1 MULTISTATE PIECEWISE
ADIABATIC PASSAGE - EXPERIMENTS 280 11.5.1.1 CHIRPED ADIABATIC PASSAGE
281
11.5.1.2 RABI FLOPPING 283 11.6 ELECTROMAGNETICALLY INDUCED TRANSPARENCY
290 11.6.1 EIT: A RESONANCE PERSPECTIVE 291 11.6.2 EIT AS EMERGING FROM
THE INTERFERENCE BETWEEN
RESONANCES 293 11.6.2.1 UNSTRUCTURED CONTINUA 300 11.6.2.2 STRUCTURED
CONTINUA 300 11.6.3 PHOTOABSORPTION 301 11.6.4 THE RESONANCE DESCRIPTION
OF SLOWING DOWN OF LIGHT BY
EIT 306
12 PHOTODISSOCIATION BEYOND THE WEAK-FIELD REGIME 315 12.1 ONE-PHOTON
DISSOCIATION WITH LASER PULSES 315 12.1.1 SLOWLY VARYING CONTINUUM 318
12.1.2 BICHROMATIC CONTROL 319
12.1.3 RESONANCE 319 12.2 COMPUTATIONAL EXAMPLES 325
13 COHERENT CONTROL BEYOND THE WEAK-FIELD REGIME: THE CONTINUUM 329 13.1
CONTROL OVER POPULATION TRANSFER TO THE CONTINUUM BY TWO-PHOTON
PROCESSES 329 13.1.1 THE ADIABATIC APPROXIMATION FOR A FINAL CONTINUUM
MANIFOLD 330
13.2 PULSED INCOHERENT INTERFERENCE CONTROL 335 13.3 RESONANTLY ENHANCED
PHOTOASSOCIATION 345
IMAGE 5
CONTENTS XI
13.3.1 THEORY OF PHOTOASSOCIATION OF A COHERENT WAVE PACKET 346
13.3.2 PHOTOASSOCIATION BY THE CONSECUTIVE APPLICATION OF APC AND STI
RAP 353 13.3.3 INTERFERENCE BETWEEN DIFFERENT PATHWAYS 357 13.3.4
EXPERIMENTAL REALIZATIONS 359 13.4 LASER CATALYSIS 363
13.4.1 THE COUPLING OF A BOUND STATE TO TWO CONTINUA BY A LASER PULSE
364
14 COHERENT CONTROL OF THE SYNTHESIS AND PURIFICATION OF CHIRAL
MOLECULES 373 14.1 PRINCIPLES OF ELECTRIC DIPOLE ALLOWED ENANTIOMERIC
CONTROL 374 14.2 SYMMETRY BREAKING IN THE TWO-PHOTON DISSOCIATION OF
PURE STATES 376 14.3 PURIFICATION OF RACEMIC MIXTURES BY "LASER
DISTILLATION" 381 14.4 ENANTIOMER CONTROL: ORIENTED MOLECULES 395 14.5
ADIABATIC PURIFICATION OF MIXTURES OF RIGHT-HANDED AND LEFT-HANDED
CHIRAL MOLECULES 397 14.5.1 VIBRATIONAL STATE DISCRIMINATION OF CHIRAL
MOLECULES 399 14.5.2 SPATIAL SEPARATION OF ENANTIOMERS 404 14.5.3
INTERNAL HAMILTONIAN AND DRESSED STATES 405 14.5.4 LASER CONFIGURATION
408 14.5.5 SPATIAL SEPARATION USING A COLD MOLECULAR TRAP 409 14.A
APPENDIX: COMPUTATION OF B- A- B' ENANTIOMER SELECTIVITY 413
15 STRONG-FIELD COHERENT CONTROL 415 15.1 STRONG-FIELD PHOTODISSOCIATION
WITH CONTINUOUS WAVE QUANTIZED FIELDS 415 15.1.1 THE COUPLED-CHANNELS
EXPANSION 419
15.1.2 NUMBER STATES VS. CLASSICAL LIGHT 423 15.2 STRONG-FIELD
PHOTODISSOCIATION WITH PULSED QUANTIZED FIELDS 425 15.2.1 LIGHT-INDUCED
POTENTIALS 426 15.3 CONTROLLED FOCUSING, DEPOSITION, AND ALIGNMENT OF
MOLECULES 429
15.3.1 FOCUSING AND DEPOSITION 429 15.3.2 STRONG-FIELD MOLECULAR
ALIGNMENT 435
16 COHERENT CONTROL WITH FEW-CYCLE PULSES 443 16.1 THE CARRIER ENVELOPE
PHASE 443 16.2 COHERENT CONTROL AND THE CEO FREQUENCY MEASUREMENT 445
16.3 THE RECOLLISION MODEL 446
16.3.1 STEP 1: TUNNEL IONIZATION 447 16.3.2 STEP 2: CLASSICAL "SWING"
MOTION 448 16.3.3 STEP 3: RECOLLISION 448 16.3.4 STEP 4: EMISSION OF A
PHOTON 450 16.4 CEP STABILIZATION AND CONTROL 451
16.4.1 THE ATTOSECOND STREAK CAMERA 452 16.5 COHERENT CONTROL OF SAMPLE
MOLECULAR SYSTEMS 453
IMAGE 6
XII CONTENTS
16.5.1 ONE-PHOTON VS. TWO-PHOTON CONTROL WITH FEW-CYCLE PULSES 453
16.5.1.1 BACKWARD-FORWARD ASYMMETRY IN THE DISSOCIATIVE
PHOTOIONIZATIONOF D2. 453 16.5.2 CONTROL OF THE GENERATION OF
HIGH-HARMONICS 455 16.5.3 CONTROL OF ELECTRON TRANSFER PROCESSES 456
16.5.4 ELECTRON TRANSFER IN ALKALI HALIDES 457
17 CASE STUDIES IN OPTIMAL CONTROL 463 17.1 CREATING EXCITED STATES 463
17.1.1 USING PREPARED STATES 467 17.2 OPTIMAL CONTROL IN THE
PERTURBATIVE DOMAIN 468 17.3 ADAPTIVE FEEDBACK CONTROL 472 17.4 ANALYSIS
OF ADAPTIVE FEEDBACK EXPERIMENTS 480
17.4.1 TRANS-CIS ISOMERIZATION IN 3,3'-DIETHYL-2,2'-THIACYANINE IODIDE
480 17.4.2 CONTROLLED STOKES EMISSION VS. VIBRATIONAL EXCITATION IN
METHANOL 486 17.5 INTERFERENCE AND OPTIMAL CONTROL 487
18 COHERENT CONTROL IN THE CLASSICAL LIMIT 491 18.1 THE ONE-PHOTON VS.
TWO-PHOTON SCENARIO REVISITED 491 18.1.1 RESONANT REGIME 491 18.1.2
OFF-RESONANT EXTENSION 492
18.1.3 A THREE-STATE EXAMPLE 494 18.1.4 QUANTUM FEATURES 495 18.2 THE
QUARTIC OSCILLATOR 496 18.3 CONTROL IN AN OPTICAL LATTICE 499 18.3.1
EQUIVALENCE WITH DIPOLE DRIVING 501
18.3.2 COMPUTATIONAL RESULTS 502
APPENDIX COMMON NOTATION USED IN THE BOOK (IN ORDER OF APPEARANCE) 507
REFERENCES 513
SUBJECT INDEX 537 |
| any_adam_object | 1 |
| author | Shapiro, Moshe 1944-2013 Brumer, Paul |
| author_GND | (DE-588)1018150749 (DE-588)1018150781 |
| author_facet | Shapiro, Moshe 1944-2013 Brumer, Paul |
| author_role | aut aut |
| author_sort | Shapiro, Moshe 1944-2013 |
| author_variant | m s ms p b pb |
| building | Verbundindex |
| bvnumber | BV039764126 |
| classification_rvk | UH 5680 UM 3200 VE 5650 |
| ctrlnum | (OCoLC)751755101 (DE-599)DNB1013143930 |
| dewey-full | 535.2 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 535 - Light and related radiation |
| dewey-raw | 535.2 |
| dewey-search | 535.2 |
| dewey-sort | 3535.2 |
| dewey-tens | 530 - Physics |
| discipline | Chemie / Pharmazie Physik |
| edition | 2., revised and enlarged ed. |
| format | Book |
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| id | DE-604.BV039764126 |
| illustrated | Illustrated |
| indexdate | 2024-07-21T00:18:57Z |
| institution | BVB |
| isbn | 9783527409044 3527409041 9783527639724 9783527639717 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-024625246 |
| oclc_num | 751755101 |
| open_access_boolean | |
| owner | DE-11 DE-19 DE-BY-UBM DE-703 DE-20 |
| owner_facet | DE-11 DE-19 DE-BY-UBM DE-703 DE-20 |
| physical | XVII, 544 S. Ill., graph. Darst. |
| publishDate | 2012 |
| publishDateSearch | 2012 |
| publishDateSort | 2012 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Shapiro, Moshe 1944-2013 Verfasser (DE-588)1018150749 aut Quantum control of molecular processes Moshe Shapiro and Paul Brumer 2., revised and enlarged ed. Weinheim Wiley-VCH 2012 XVII, 544 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Molekülphysik (DE-588)4039979-5 gnd rswk-swf Optische Kohärenz (DE-588)4519405-1 gnd rswk-swf Molekulardynamik (DE-588)4170370-4 gnd rswk-swf Quantenoptik (DE-588)4047990-0 gnd rswk-swf Molekülphysik (DE-588)4039979-5 s Quantenoptik (DE-588)4047990-0 s DE-604 Optische Kohärenz (DE-588)4519405-1 s Molekulardynamik (DE-588)4170370-4 s Brumer, Paul Verfasser (DE-588)1018150781 aut X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3847397&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024625246&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Shapiro, Moshe 1944-2013 Brumer, Paul Quantum control of molecular processes Molekülphysik (DE-588)4039979-5 gnd Optische Kohärenz (DE-588)4519405-1 gnd Molekulardynamik (DE-588)4170370-4 gnd Quantenoptik (DE-588)4047990-0 gnd |
| subject_GND | (DE-588)4039979-5 (DE-588)4519405-1 (DE-588)4170370-4 (DE-588)4047990-0 |
| title | Quantum control of molecular processes |
| title_auth | Quantum control of molecular processes |
| title_exact_search | Quantum control of molecular processes |
| title_full | Quantum control of molecular processes Moshe Shapiro and Paul Brumer |
| title_fullStr | Quantum control of molecular processes Moshe Shapiro and Paul Brumer |
| title_full_unstemmed | Quantum control of molecular processes Moshe Shapiro and Paul Brumer |
| title_short | Quantum control of molecular processes |
| title_sort | quantum control of molecular processes |
| topic | Molekülphysik (DE-588)4039979-5 gnd Optische Kohärenz (DE-588)4519405-1 gnd Molekulardynamik (DE-588)4170370-4 gnd Quantenoptik (DE-588)4047990-0 gnd |
| topic_facet | Molekülphysik Optische Kohärenz Molekulardynamik Quantenoptik |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3847397&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024625246&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT shapiromoshe quantumcontrolofmolecularprocesses AT brumerpaul quantumcontrolofmolecularprocesses |