Anion coordination chemistry:
Gespeichert in:
| Weitere Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH
2012
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XIV, 559 S. Ill., graph. Darst. 240 mm x 170 mm |
| ISBN: | 9783527323708 3527323708 |
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IMAGE 1
CONTENTS
PREFECE XI
LIST OF CONTRIBUTORS XIII
1 ASPECTS OF ANION COORDINATION FROM HISTORICAL PERSPECTIVES 1
ANTONIO BIANCHI, KRISTIN BOWMAN-JAMES, AND ENRIQUE GARCIA-ESPANA
1.1 INTRODUCTION 1
1.2 HALIDE AND PSEUDOHALIDE ANIONS 9 1.3 OXOANIONS 23
1.4 PHOSPHATE AND POLYPHOSPHATE ANIONS 29 1.5 CARBOXYLATE ANIONS AND
AMINO ACIDS 36 1.6 ANIONIC COMPLEXES: SUPERCOMPLEX FORMATION 42 1.7
NUCLEOTIDES 51
1.8 FINAL NOTES 60
REFERENCES 60
2 THERMODYNAMIC ASPECTS OF ANION COORDINATION 75 ANTONIO BIANCHI AND
ENRIQUE GARAA-ESPAIIA 2.1 INTRODUCTION 75
2.2 PARAMETERS DETERMINING THE STABILITY OF ANION COMPLEXES 76 2.2.1
TYPE OF BINDING GROUP: NONCOVALENT FORCES IN ANION COORDINATION 76 2.2.2
CHARGE OF ANIONS AND RECEPTORS 84 2.2.3 NUMBER OF BINDING GROUPS 85
2.2.3.1 ADDITIVITY OF NONCOVALENT FORCES 86 2.2.4 PREORGANIZATION 87
2.2.4.1 MACROCYDIC EFFECT 91 2.2.5 SOLVENT EFFECTS 93
2.3 MOLECULAR RECOGNITION AND SELECTIVITY 102 2.4 ENTHALPIE AND ENTROPIE
CONTRIBUTIONS IN ANION COORDINATION 130 REFERENCES 132
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/101209376X
DIGITALISIERT DURCH
IMAGE 2
V II CONTENTS
3 STRUCTURAL ASPECTS OF ANION COORDINATION CHEMISTRY 141
ROWSHAN ARA BEGUM, SUNG OK KANG, VICTOR W. DAY, AND KRISTIN BOWMAN-JAMES
3.1 INTRODUCTION 141
3.2 BASIC CONCEPTS OF ANION COORDINATION CHEMISTRY 142 3.3 CLASSES OF
ANION HOSTS 143
3.4 ACYCLES 144
3.4.1 BIDENTATE 144
3.4.2 TRIDENTATE 149
3.4.3 TETRADENTATE 155
3.4.4 PENTADENTATE 161
3.4.5 HEXADENTATE 162
3.5 MONOCYCLES 164
3.5.1 BIDENTATE 164
3.5.2 TRIDENTATE 165
3.5.3 TETRADENTATE 366
3.5.4 PENTADENTATE 174
3.5.5 HEXADENTATE 375
3.5.6 OCTADENTATE 177
3.5.7 DODECADENTATE 179 3.6 CRYPTANDS 181
3.6.1 BIDENTATE 383
3.6.2 TRIDENTATE 183
3.6.3 TETRADENTATE 184
3.6.4 PENTADENTATE 186
3.6.5 HEXADENTATE 188
3.6.6 SEPTADENTATE 192
3.6.7 OCTADENTATE 193
3.6.8 NONADENTATE 197
3.6.9 DECADENTATE 398
3.6.10 DODECADENTATE 399 3.7 TRANSITION-METAL-ASSISTED LIGANDS 201 3.7.1
BIDENTATE 201
3.7.2 TRIDENTATE 203
3.7.3 TETRADENTATE 204
3.7.4 HEXADENTATE 204
3.7.5 SEPTADENTATE 206 3.7.6 DODECADENTATE 208 3.8 LEWIS ACID LIGANDS
230
3.8.1 TRANSITION METAL CASCADE COMPLEXES 230 3.8.2 OTHER LEWIS ACID
DONOR LIGANDS 233 3.8.2.1 BORON-BASED LIGANDS 233 3.8.2.2 TIN-BASED
LIGANDS 214
3.8.2.3 HG-BASED LIGANDS 236 3.9 CONCLUSION 218
IMAGE 3
CONTENTS VII
ACKNOWLEDGMENTS 218
REFERENCES 218
4 SYNTHETIC STRATEGIES 227 ANDREA BENCINI AND JOSE M. LLINARES 4.1
INTRODUCTION 227
4.2 DESIGN AND SYNTHESIS OF POLYAMINE-BASED RECEPTORS FOR ANIONS 227
4.2.1 ACYCLIC POLYAMINE RECEPTORS 229 4.2.2 TRIPODAL POLYAMINE RECEPTORS
234 4.2.3 MACROCYDIC POLYAMINE RECEPTORS WITH ALIPHATIC SKELETONS 236
4.2.4 MACROCYDIC RECEPTORS INCORPORATING A SINGLE AROMATIC UNIT 241
4.2.5 MACROCYDIC RECEPTORS INCORPORATING TWO AROMATIC UNITS 243 4.2.6
ANION RECEPTORS CONTAINING SEPARATED MACROCYDIC BINDING
UNITS 249
4.2.7 CRYPTANDS 252
4.3 DESIGN AND SYNTHESIS OF AMIDE RECEPTORS 258 4.3.1 ACID HALIDES AS
STARTING MATERIALS 259 4.3.1.1 ACYCLIC AMIDE RECEPTORS 259 4.3.1.2
MACROCYDIC AMIDE RECEPTORS 267 4.3.2 ESTERS AS STARTING MATERIALS 270
4.3.3 USING COUPLING REAGENTS 276
REFERENCES 279
5 TEMPLATE SYNTHESIS 289
JACK K. CLEGG AND LEONARD F. LINDOY 5.1 INTRODUCTORY REMARKS 289
5.2 MACROCYDIC SYSTEMS 290
5.3 BOWL-SHAPED SYSTEMS 297
5.4 CAPSULE, CAGE, AND TUBE-SHAPED SYSTEMS 300 5.5 CIRCULAR HELICATES
AND MESO-HELICATES 306 5.6 MECHANICALLY LINKED SYSTEMS 308
5.7 CONCLUDING REMARKS 334
REFERENCES 335
6 ANION-7R INTERACTIONS IN MOLECULAR RECOGNITION 321 DAVID QUINONERO,
ANTONIO FRONTERA, AND PERE M. DEYA 6.1 INTRODUCTION 323
6.2 PHYSICAL NATURE OF THE INTERACTION 322 6.3 ENERGETIC AND GEOMETRIC
FEATURES OF THE INTERACTION DEPENDING ON THE HOST (AROMATIC MOIETIES)
AND THE GUEST (ANIONS) 323
6.4 INFLUENCE OF OTHER NONCOVALENT INTERACTIONS ON THE ANION-7R
INTERACTION 330 6.4.1 INTERPLAY BETWEEN CATION-^ AND ANION-JR
INTERACTIONS 330 6.4.2 INTERPLAY BETWEEN 7R-7R AND ANION-7R INTERACTIONS
332 6.4.3 INTERPLAY BETWEEN ANION-;R AND HYDROGEN-BONDING INTERACTIONS
334
IMAGE 4
VIII CONTENTS
6.4.4 INFLUENCE OF METAL COORDINATION ON THE ANION-JR INTERACTION 337
6.5 EXPERIMENTAL EXAMPLES OF ANION-JR INTERACTIONS IN THE SOLID STATE
AND IN SOLUTION 338 6.6 CONCLUDING REMARKS 353 REFERENCES 354
7 RECEPTORS FOR BIOLOGICALLY RELEVANT ANIONS 363 STEFAN KUBIK 7.1
INTRODUCTION 363
7.2 PHOSPHATE RECEPTORS 364 7.2.1 INTRODUCTION 364 7.2.2 PHOSPHATE,
PYROPHOSPHATE, TRIPHOSPHATE 366 7.2.3 NUDEOTIDES 387 7.2.4 PHOSPHATE
ESTERS 395 7.2.5 POLYNUCLEOTIDES 407 7.3 CARBOXYLATE RECEPTORS 410 7.3.1
INTRODUCTION 410 7.3.2 ACETATE 412
7.3.3 DI- AND TRICARBOXYLATES 425 7.3.4 AMINO ACIDS 433 7.3.5 PEPTIDE
C-TERMINAL CARBOXYLATES 444 7.3.6 PEPTIDE SIDE-CHAIN CARBOXYLATES 450
7.3.7 SIALIC ACIDS 453 7.4 CONCLUSION 453
REFERENCES 453
8 SYNTHETIC AMPHIPHILIC PEPTIDES THAT SELF-ASSEMBLE TO MEMBRANE-ACTIVE
ANION TRANSPORTERS 465 GEORGE W. GOKEL AND MEGAN M. DASCHBACH
8.1 INTRODUCTION AND BACKGROUND 465 8.2 BIOMEDICAL IMPORTANCE OF
CHLORIDE CHANNELS 466 8.2.1 A NATURAL CHLORIDE COMPLEXING AGENT 468 8.3
THE DEVELOPMENT OF SYNTHETIC CHLORIDE CHANNELS 468 8.3.1 CATIONS,
ANIONS, COMPLEXATION, AND TRANSPORT 468 8.3.2 ANION COMPLEXATION STUDIES
470
8.3.3 TRANSPORT OF IONS 470 8.3.4 SYNTHETIC CHLORIDE TRANSPORTERS 470
8.4 APPROACHES TO SYNTHETIC CHLORIDE CHANNELS 473 8.4.1 TOMICH'S
SEMISYNTHETIC PEPTIDES 472
8.4.2 CYDODEXTRIN AS A SYNTHETIC CHANNEL DESIGN ELEMENT 473 8.4.3
AZOBENZENE AS A PHOTO-SWITCHABLE GATE 474 8.4.4 CALIXARENE-DERIVED
CHLORIDE TRANSPORTERS 474 8.4.5 OLIGOPHENYLENES AND 7R-SLIDES 477
8.4.6 CHOLAPODS AS ION TRANSPORTERS 479 8.4.7 TRANSPORT MEDIATED BY
ISOPHTHALAMIDES AND DIPICOLINAMIDES 481
IMAGE 5
CONTENTS IX
8.5 THE DEVELOPMENT OF AMPHIPHILIC PEPTIDES AS ANION CHANNELS 481
8.5.1 THE BILAYER MEMBRANE 482 8.5.2 INITIAL DESIGN CRITERIA FOR
SYNTHETIC ANION TRANSPORTERS (SATS) 482 8.5.3 SYNTHESIS OF THE
N-TERMINAL ANCHOR MODULE 483
8.5.4 PREPARATION OF THE HEPTAPEPTIDE 484 8.5.5 INITIAL ASSESSMENT OF
ION TRANSPORT 485 8.6 STRUCTURAL VARIATIONS IN THE SAT MODULAR ELEMENTS
488 8.6.1 VARIATIONS IN THE N-TERMINAL ANCHOR CHAINS 488 8.6.2 ANCHORING
EFFECT OF THE C-TERMINAL RESIDUE 489 8.6.3 STUDIES OF VARIATIONS IN THE
PEPTIDE MODULE 493 8.6.3.1 STRUCTURAL VARIATIONS IN THE HEPTAPEPTIDE 492
8.6.3.2 VARIATIONS IN THE GLY-PRO PEPTIDE LENGTH AND SEQUENCE 493
8.6.4 VARIATIONS IN THE ANCHOR CHAIN TO PEPTIDE LINKER MODULE 494 8.6.5
COVALENT LINKAGE OF SATS: PSEUIO-DIMERS 496 8.6.6 CHLORIDE BINDING BY
THE AMPHIPHILIC HEPTAPEPTIDES 498 8.6.7 THE EFFECT ON TRANSPORT OF
CHARGED SIDECHAINS 499 8.6.8 FLUORESCENT PROBES OF SAT STRUCTURE AND
FUNCTION 500
8.6.8.1 AGGREGATION IN AQUEOUS SUSPENSION AND IN THE BILAYER 501 8.6.8.2
FLUORESCENCE RESONANCE ENERGY TRANSFER STUDIES 503 8.6.8.3 INSERTION OF
SATS INTO THE BILAYER 504 8.6.8.4 POSITION OF SATS IN THE BILAYER 505
8.6.9 SELF-ASSEMBLY STUDIES OF THE AMPHIPHILES 505 8.6.10 THE BIOLOGICAL
ACTIVITY OF AMPHIPHILIC PEPTIDES 508 8.6.11 NONTRANSPORTER,
MEMBRANE-ACTIVE COMPOUNDS 509 8.7 CONCLUSIONS 509
ACKNOWLEDGMENTS 509 REFERENCES 530
9 ANION SENSING BY FLUORESCENCE QUENCHING OR REVIVAL 523 VALERIA
AMENDOLA, LUIGI FABBRIZZI, MAURIZIO LICCHELLI, AND ANGELO TAGLIETTI 9.1
INTRODUCTION 521
9.2 ANION RECOGNITION BY DYNAMIC AND STATIC QUENCHING OF FLUORESCENCE
522 9.3 FLUORESCENT SENSORS BASED ON ANTHRACENE AND ON A POLYAMINE
FRAMEWORK 529 9.4 TURNING ON FLUORESCENCE WITH THE INDICATOR
DISPLACEMENT
APPROACH 538
9.4.1 EPILOG 550
REFERENCES 551
INDEX 553 |
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| indexdate | 2024-07-21T00:18:35Z |
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| isbn | 9783527323708 3527323708 |
| language | English |
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| physical | XIV, 559 S. Ill., graph. Darst. 240 mm x 170 mm |
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| spelling | Anion coordination chemistry ed. by Kristin Bowman-James ... Weinheim Wiley-VCH 2012 XIV, 559 S. Ill., graph. Darst. 240 mm x 170 mm txt rdacontent n rdamedia nc rdacarrier Koordinationslehre (DE-588)4133952-6 gnd rswk-swf Anion (DE-588)4130938-8 gnd rswk-swf Anion (DE-588)4130938-8 s Koordinationslehre (DE-588)4133952-6 s DE-604 Bowman-James, Kristin (DE-588)1017520372 edt X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3830283&prov=M&dok%5Fvar=1&dok%5Fext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024618915&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Anion coordination chemistry Koordinationslehre (DE-588)4133952-6 gnd Anion (DE-588)4130938-8 gnd |
| subject_GND | (DE-588)4133952-6 (DE-588)4130938-8 |
| title | Anion coordination chemistry |
| title_auth | Anion coordination chemistry |
| title_exact_search | Anion coordination chemistry |
| title_full | Anion coordination chemistry ed. by Kristin Bowman-James ... |
| title_fullStr | Anion coordination chemistry ed. by Kristin Bowman-James ... |
| title_full_unstemmed | Anion coordination chemistry ed. by Kristin Bowman-James ... |
| title_short | Anion coordination chemistry |
| title_sort | anion coordination chemistry |
| topic | Koordinationslehre (DE-588)4133952-6 gnd Anion (DE-588)4130938-8 gnd |
| topic_facet | Koordinationslehre Anion |
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