Charge and exciton transport through molecular wires:
Gespeichert in:
| Weitere Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH-Verl.
2011
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XIII, 319 S. Ill., graph. Darst. |
| ISBN: | 9783527325016 |
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IMAGE 1
CONTENTS
LIST OF CONTRIBUTORS XI
1 INTRODUCTION: MOLECULAR ELECTRONICS AND MOLECULAR WIRES 1 FERDINAND C.
GROZEMA AND LAURENS D. A. SIEBBELES 1.1 INTRODUCTION 1
1.2 SINGLE-MOLECULE DEVICES 2 1.2.1 MOLECULAR RECTIFIERS 2 1.2.2
MOLECULAR SWITCHES 3 1.2.3 MOLECULAR TRANSISTORS 5 1.2.4 MOLECULAR
WIRES: CONNECTING THE DEVICES 6
1.3 TRANSPORT OF CHARGES AND EXCITONS IN MOLECULAR WIRES S 1.3.1
DEVIATIONS FROM EXPONENTIAL DISTANCE DEPENDENCE: TRANSFER TO HOPPING 9
1.3.2 CHARGES LOCALIZED ON CONJUGATED CHAINS 10 1.3.3 MOTION OF EXCITED
STATES 11
REFERENCES 11
PARTI MOLECULES BETWEEN ELECTRODES 17
2 QUANTUM INTERFERENCE IN ACYCLIC MOLECULES 19 GEMMA C. SOLOMON, DAVID Q
ANDREWS, AND MARIE A. RATNER 2.1 INTRODUCTION 19
2.1.1 RULES OF THUMB 20
2.1.2 BARRIER TUNNELING 21 2.1.3 LIMITATIONS ON DEVICE PERFORMANCE 21
2.1.4 UNDERLYING ASSUMPTIONS 22 2.1.5 EXCEPTIONS SEEN IN PRIOR WORK 23
2.2 THEORETICAL METHODS 23
2.2.1 ELECTRONIC STRUCTURE AND GEOMETRY 23 2.2.2 TRANSPORT 24
2.2.3 MOLECULAR DYNAMICS 25 2.2.4 DEPHASING 25
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/998577952
DIGITALISIERT DURCH
IMAGE 2
VI I CONTENTS
2.3 INTERFERENCE IN ACYCLIC CROSS-CONJUGATED MOLECULES 26
2.3.1 THE CHEMICAL NATURE OF CROSS-CONJUGATED MOLECULES 26 2.3.2 THE
"RULES" BREAK DOWN 30 2.4 UNDERSTANDING INTERFERENCE IN MODEL SYSTEMS 33
2.5 USING INTERFERENCE FOR DEVICES 36
2.5.1 SCHEMATIC DESIGNS 36 2.5.2 TUNING INTERFERENCE 38 2.5.3 TRANSISTOR
41
2.5.4 RECTIFIER 43
2.5.5 NEGATIVE DIFFERENTIAL RESISTANCE 46 2.6 PROBING THE LIMITS OF
CALCULATIONS: IMPORTANT REAL-WORLD PHENOMENA 47 2.6.1 THEORETICAL METHOD
47
2.6.2 DEPHASING 47
2.6.3 CONFORMATIONAL FREEDOM 48 2.6.4 SHORT CIRCUITS 50
2.6.5 TRANSPORT THROUGH INELASTIC AND EXCITED STATE CHANNELS 51 2.7
CONCLUSIONS 51
ACKNOWLEDGMENTS 52 REFERENCES 52
3 HOPPING TRANSPORT IN LONG CONJUGATED MOLECULAR WIRES CONNECTED TO
METALS 61 SEONG HO CHOI AND C. DANIEL FRISBIE 3.1 INTRODUCTION 61
3.2 CHARGE TRANSPORT MECHANISMS 63 3.2.1 TUNNELING (DIRECT TUNNELING AND
FIELD EMISSION) 63 3.2.2 HOPPING 67
3.2.3 RECENT RESULTS ON MOLECULAR WIRES CONNECTED TO METALS 69 3.3
OLIGOPHENYLENE IMINE MOLECULAR WIRES: A FLEXIBLE SYSTEM FOR EXAMINING
THE PHYSICAL ORGANIC CHEMISTRY OF HOPPING CONDUCTION IN MOLECULES 71
3.3.1 FORMING JUNCTIONS USING A SOFT, SPRING-LOADED CONTACT 75
3.3.2 ELECTRICAL TRANSPORT IN OPI WIRES 76 3.3.2.1 LENGTH DEPENDENCE OF
RESISTANCE 76 3.3.2.2 TEMPERATURE DEPENDENCE OF RESISTANCE 76 3.3.2.3
ELECTRIC FIELD DEPENDENCE OF CHARGE TRANSPORT 78 3.3.3 SUMMARY OF OPI
WIRE EXPERIMENTS TO DATE 83 3.4 OUTLOOK: PROBING THE PHYSICAL ORGANIC
CHEMISTRY OF HOPPING
CONDUCTION 83 REFERENCES 86
IMAGE 3
CONTENTS | VII
PART II DONOR-BRIDGE-ACCEPTOR SYSTEMS 93
4 TUNNELING THROUGH CONJUGATED BRIDGES IN DESIGNED DONOR-BRIDGE-ACCEPTOR
MOLECULES 95 BO ALBINSSON, MATTIAS P. ENG, AND JERKER MARTENSSON 4.1
INTRODUCTION 95
4.1.1 THEORETICAL BACKGROUND 95 4.1.1.1 MOLECULAR WIRES 96 4.1.1.2
ELECTRON AND ENERGY TRANSFER - THE FUNDAMENTALS 96 4.1.1.3 MECHANISMS
FOR ELECTRON AND ENERGY TRANSFER 97 4.1.1.4 THE DISTANCE DEPENDENCE OF
ELECTRON AND ENERGY TRANSFER
REACTIONS 98
4.1.1.5 SUPEREXCHANGE 99 4.2 THROUGH-BOND ELECTRONIC COUPLING IN N
-CONJUGATED BRIDGES 100 4.2.1 DISTANCE AND ENERGY GAP DEPENDENCE 200
4.2.1.1 SINGLET ENERGY TRANSFER MEDIATED BY N -BRIDGES 100 4.2.1.2
TRIPLET ENERGY TRANSFER 104 4.2.1.3 ELECTRON TRANSFER 106 4.2.1.4
INDUCED/ENHANCED INTERSYSTEM CROSSING 111
4.2.2 CONFORMATIONAL AND TEMPERATURE EFFECTS ON ELECTRON EXCHANGE 114
4.2.2.1 MODULATING THE TRANSFER RATE BY PREPARING DIFFERENT STATES USING
CONFORMATIONAL TRAPPING 116 4.2.2.2 CONFORMATIONAL CONTROL OF TUNNELING
THROUGH MOLECULAR BRIDGES 117 4.3 CONCLUSIONS 227
REFERENCES 227
5 BASE PAIR SEQUENCE AND HOLE TRANSFER THROUGH DNA: RATIONAL DESIGN OF
MOLECULAR WIRES 133 JOSH VURA-WEIS, FREDERICK D. LEWIS, MARK A. RATNER,
AND MICHAEL R.
WASIELEWSKI
5.1 INTRODUCTION 233
5.2 SPECTRAL SIGNATURES OF CHARGE TRANSFER 134 5.3 CHARGE INJECTION INTO
A-TRACTS 236 5.4 CROSSOVER FROM SUPEREXCHANGE TO HOPPING IN SA-A M -SD
239 5.5 SYMMETRY BREAKING IN SA-A N -SA 141 5.6 INFLUENCE OF A SINGLE G
ON CHARGE TRANSPORT 143 5.7 MOLECULAR WIRE BEHAVIOR IN S A - A 2 - 3 G W
- SD 147 5.8 CHARGE TRANSFER THROUGH ALTERNATING SEQUENCES 249
5.9 THEORETICAL DESCRIPTIONS OF CHARGE TRANSFER THROUGH DNA 152 5.9.1
GENERAL MODELS OF DNA CHARGE TRANSFER 252 5.9.2 SA-SD HAIRPINS 152
5.10 CONCLUSION 253
ACKNOWLEDGMENTS 253 REFERENCES 253
IMAGE 4
VIII CONTENTS
6 CHARGE TRANSPORT THROUGH MOLECULES: ORGANIC NANOCABLES FOR
MOLECULAR ELECTRONICS 257 MATEUSZ WIELOPOLSKI, DIRK M. GULDI, TIMOTHY
CLARK, AND NAZARIO MARTIN 6.1 INTRODUCTION 257
6.2 THEORETICAL CONCEPTS 259
6.2.1 DEFINITION OF THE "MOLECULAR WIRE" TERM 259 6.2.2 MECHANISMS OF
CHARGE TRANSFER THROUGH MOLECULAR WIRES 260 6.2.2.1 SUPEREXCHANGE
CHARGE-TRANSFER MECHANISM IN MOLECULAR WIRES 262 6.2.2.2 SEQUENTIAL
CHARGE-TRANSFER MECHANISM IN MOLECULAR WIRES 262
6.2.3 PARAMETERS FOR CONTROLLING THE CHARGE-TRANSFER MECHANISM 163
6.2.3.1 ENERGY MATCHING 263 6.2.3.2 ELECTRONIC COUPLING 265 6.2.3.3
TEMPERATURE 267
6.2.3.4 SPECIFIC ASPECTS OF PHOTOINDUCED ELECTRON TRANSFER IN ORGANIC
TT-CONJUGATED SYSTEMS 267 6.3 CHARGE TRANSPORT ALONG TR-CONJUGATED
BRIDGES IN COO-CONTAINING DONOR-BRIDGE-ACCEPTOR CONJUGATES 268 6.3.1 C 6
O-WIRE-EXTTF 270
6.3.1.1 C 50 -OPPV-EXTTF 170 6.3.1.2 QO-OPPE-EXTTF 272 6.3.1.3 C 60
-OFL-EXTTF 275 6.3.2 C S0 -WIRE-ZNP/H 2 P 276
6.3.2.1 C 60 -OPPV-ZNP/H 2 P 276 6.3.2.2 C S0 -OPPE-ZNP/H 2 P 278 6.3.3
QO-WIRE-FC 282
6.3.3.1 C 6 O-ZNP-FC 282 6.3.3.2 CCO-OT-FC 282 6.4 CONCLUSIONS 283
REFERENCES 284
PART 111 CHARGE TRANSPORT THROUGH WIRES IN SOLUTION 2 89
7 ELECTRON AND EXCITON TRANSPORT TO APPENDED TRAPS 292 JOHN R. MILLER,
ANDREW R. COOK, KIRK S. SCHANZE, AND PAIBOON SREEARUNOTHAI
7.1 INTRODUCTION 292
7.1.1 APPENDED TRAP AND MICROWAVE CONDUCTIVITY COMPARISON 292 7.1.2
TRANSPORT MECHANISMS 293 7.2 EXPERIMENTAL METHODS TO INVESTIGATE
TRANSPORT TO APPENDED TRAPS 294
7.2.1 INJECTION OF ELECTRONS AND HOLES 294 7.2.2 EXCITON CREATION IN
WIRES 294 7.3 RESULTS ON TRANSPORT TO TRAPS 196
7.3.1 ELECTRON AND HOLE TRANSPORT TO TRAPS 296 7.3.1.1 A NONCONJUGATED
CHAINS 296
IMAGE 5
CONTENTS IX
7.3.1.2 CHARGE TRANSPORT IN JR-CONJUGA TED CHAINS 296
7.3.2 ONE-DIMENSIONAL DIFFUSION OF POLARONS ALONG POLYMER CHAINS 298
7.3.3 OBSERVED TRANSPORT OF TRIPLET EXCITONS ALONG CONJUGATED CHAINS 199
7.3.4 OBSERVED TRANSPORT OF SINGLET EXCITONS ALONG CONJUGATED CHAINS 200
7.3.5 THE IMPACT OF POLYDISPERSITY: DIFFUSION TO TRAPS IN A POLYMER
HAVING A
DISTRIBUTION OF LENGTHS 202 7.4 COMPARISONS AND PERSPECTIVES 203
REFERENCES 203
8 ELECTRON LATTICE DYNAMICS AS A METHOD TO STUDY CHARGE TRANSPORT IN
CONJUGATED POLYMERS 207 SVEN STAFSTROEM AND MAGNUS HULTELL
8.1 INTRODUCTION 207
8.1.1 IDEAL CONJUGATED POLYMERS 209 8.1.2 DISORDERED CONJUGATED POLYMERS
222 8.1.3 MOBILITY 222
8.1.4 ELECTRON-LATTICE DYNAMICS I 214 8.2 METHODOLOGY 215
8.2.1 HAMILTONIAN 225
8.2.2 ELECTRON-LATTICE DYNAMICS II 226 8.2.3 ELECTRONIC HAMILTONIAN 228
8.2.4 LATTICE ENERGY 229 8.2.5 ELECTRON-LATTICE DYNAMICS III 220 8.3
RESULTS 222
8.3.1 INTRACHAIN POLARON DYNAMICS 222 8.3.2 INTERCHAIN POLARON DYNAMICS
224 8.3.3 TORSIONAL DYNAMICS 225 8.3.4 DYNAMICS IN THE PHOTOEXCITED
STATE 231 8.4 SUMMARY 235
ACKNOWLEDGMENTS 236 REFERENCES 236
9 CHARGE TRANSPORT ALONG ISOLATED CONJUGATED MOLECULAR WIRES MEASURED BY
PULSE RADIOLYSIS TIME-RESOLVED MICROWAVE CONDUCTIVITY 239 FERDINAND C.
GROZEMA AND LAURENS D. A. SIEBBELES 9.1 INTRODUCTION 239
9.2 PULSE-RADIOLYSIS TIME-RESOLVED MICROWAVE CONDUCTIVITY 240 9.3
MECHANISMS FOR CHARGE TRANSPORT ALONG CONJUGATED CHAINS 244 9.4 THE
MEANING OF THE MOBILITY AT MICROWAVE FREQUENCIES 245 9.5 CHARGE
TRANSPORT ALONG LADDER-TYPE PPP 249 9.6 EFFECT OF TORSIONAL DISORDER ON
THE MOBILITY 251
9.6.1 SIMULATIONS OF CHARGE TRANSPORT ALONG PHENYLENE-VINYLENE CHAINS
253 9.6.2 MEAN SQUARED DISPLACEMENT OF A CHARGE ON PHENYLENE-VINYLENE
CHAINS 256
IMAGE 6
X| CONTENTS
9.6.3 MOBILITY OF CHARGES ALONG PHENYLENE-VINYLENE CHAINS 256
9.6.4 COMPARISON OF THE CALCULATED MOBILITY WITH EXPERIMENTAL DATA 257
9.7 EFFECT OF CHAIN COILING ON THE MOBILITY OF CHARGES 258 9.7.1
COMPARISON OF EXPERIMENTAL AND CALCULATED DATA 263 9.8 SUPRAMOLECULAR
CONTROL OF CHARGE TRANSPORT ALONG MOLECULAR
WIRES 264
9.9 SUMMARY AND OUTLOOK 267
REFERENCES 268
PART IV EXCITON TRANSPORT THROUGH CONJUGATED MOLECULAR WIRES 272
10 STRUCTURE PROPERTY RELATIONSHIPS FOR EXCITON TRANSFER IN CONJUGATED
POLYMERS 273 TRISHA L. ANDREW AND TIMOTHY M. SWAGER 10.1 INTRODUCTION
273
10.2 SIGNAL GAIN IN AMPLIFYING FLUORESCENT POLYMERS 274 10.3 DIRECTING
ENERGY TRANSFER WITHIN CPS: DIMENSIONALITY AND MOLECULAR DESIGN 278
10.3.1 SOLUTIONS VS THIN FILMS 278 10.3.2 AGGREGATES 282 10.3.3 KINETICS
OF ENERGY MIGRATION IN THIN FILMS 289 10.4 LIFETIME MODULATION 292
10.4.1 TRIPHENYLENE-INCORPORATED PPES 293 10.4.2 CHRYSENE-INCORPORATED
PPES 297 10.4.3 THIOPHENE-BASED MODEL COMPOUNDS AND PPES 298 10.5
CONFORMATIONAL DEPENDENCE ON ENERGY MIGRATION: CONJUGATED
POLYMER - LIQUID CRYSTAL SOLUTIONS 302 10.6 CONCLUSIONS 307
REFERENCES 308
INDEX 322 |
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| illustrated | Illustrated |
| indexdate | 2024-07-21T00:07:21Z |
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| language | English |
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| publisher | Wiley-VCH-Verl. |
| record_format | marc |
| spelling | Charge and exciton transport through molecular wires ed. by Laurens D. A. Siebbeles ... Weinheim Wiley-VCH-Verl. 2011 XIII, 319 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Exzitonenbeweglichkeit (DE-588)4257328-2 gnd rswk-swf Ladungstransport (DE-588)4166400-0 gnd rswk-swf Nanodraht (DE-588)4707308-1 gnd rswk-swf Nanodraht (DE-588)4707308-1 s Ladungstransport (DE-588)4166400-0 s Exzitonenbeweglichkeit (DE-588)4257328-2 s DE-604 Siebbeles, Laurens D. A. (DE-588)143450182 edt X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3385138&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024386620&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Charge and exciton transport through molecular wires Exzitonenbeweglichkeit (DE-588)4257328-2 gnd Ladungstransport (DE-588)4166400-0 gnd Nanodraht (DE-588)4707308-1 gnd |
| subject_GND | (DE-588)4257328-2 (DE-588)4166400-0 (DE-588)4707308-1 |
| title | Charge and exciton transport through molecular wires |
| title_auth | Charge and exciton transport through molecular wires |
| title_exact_search | Charge and exciton transport through molecular wires |
| title_full | Charge and exciton transport through molecular wires ed. by Laurens D. A. Siebbeles ... |
| title_fullStr | Charge and exciton transport through molecular wires ed. by Laurens D. A. Siebbeles ... |
| title_full_unstemmed | Charge and exciton transport through molecular wires ed. by Laurens D. A. Siebbeles ... |
| title_short | Charge and exciton transport through molecular wires |
| title_sort | charge and exciton transport through molecular wires |
| topic | Exzitonenbeweglichkeit (DE-588)4257328-2 gnd Ladungstransport (DE-588)4166400-0 gnd Nanodraht (DE-588)4707308-1 gnd |
| topic_facet | Exzitonenbeweglichkeit Ladungstransport Nanodraht |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3385138&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024386620&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT siebbeleslaurensda chargeandexcitontransportthroughmolecularwires |