Spatially resolved impedance of nonlinear inhomogeneous devices: [using the example of lead-acid batteries]
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Aachen
Shaker
2010
|
| Schriftenreihe: | Aachener Beiträge des ISEA
53 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | VII, 203 S. graph. Darst. |
| ISBN: | 9783832294830 |
Internformat
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| 100 | 1 | |a Kowal, Julia |d 1979- |e Verfasser |0 (DE-588)143306804 |4 aut | |
| 245 | 1 | 0 | |a Spatially resolved impedance of nonlinear inhomogeneous devices |b [using the example of lead-acid batteries] |c Julia Kowal |
| 264 | 1 | |a Aachen |b Shaker |c 2010 | |
| 300 | |a VII, 203 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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| 490 | 1 | |a Aachener Beiträge des ISEA |v 53 | |
| 502 | |a Zugl.: Aachen, Techn. Hochsch., Diss., 2010 | ||
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Datensatz im Suchindex
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| adam_text | IMAGE 1
CONTENT
1 INTRODUCTION AND MOTIVATION 1
2 ELAECTROCHEMICAL IMPEDANCE SPECTROSCOPY 5
2.1 IDENTIFICATION OF PROCESSES 6
2.2 IMPEDANCE SPECTROSCOPY ON BATTENES 7
3 ELECTRODE KINETICS 9
3.1 EQUILIBRIUM POTENTIAL 10
3.2 OVERPOTENTIAL 11
3.3 ELECTRICAL DOUBLE LAYER 11
3.4 OHMIC POLARISATION 13
3.5 CHARGE AND MASS FLUX 14
3.6 CHARGE TRANSFER 15
3.7 MASS TRANSPORT 17
3.8 CHEMICAL REACTIONS 20
3.9 ADSORPTION 22
3.9.1 ADSORPTION ISOTHERMS 23
3.9.2 INFLUENCE OF ADSORPTION ON ELECTRODE KINETICS 24
3.9.3 ADSORPTION IMPEDANCE 25
3.9.4 ORIGIN OF NEGATIVE SMALL-SIGNAL IMPEDANCE 28
3.10 CRYSTALLISATION 31
3.11 POROUS SURFACES 32
4 DEVICES WITH INHOMOGENEOUS IMPEDANCE 35
4.1 LEAD-ACID BATTERIES 36
4.1.1 DESIGN AND APPLICATIONS 37
4.1.2 COURSE OF REACTION 39
4.1.3 INHOMOGENEITIES 44
4.1.4 IMPEDANCE SPECTRA 49
4.2 OTHER INHOMOGENEOUS DEVICES 56
4.2.1 LITHIUM-ION BATTERIES 56
4.2.2 FUELCELLS 57
4.2.3 ORGANIC LIGHT-EMITTING DIODES (OLEDS) 58
5 IMPEDANCE-BASED MODELLING APPROACH 60
5.1 MODELS FOR ELECTROCHEMICAL STORAGE SYSTEMS 60
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1008814148
DIGITALISIERT DURCH
IMAGE 2
VI CONTENT
5.1.1 IMPLEMENTATIONS OF BATTERY MODELS 62
5.1.2 ELECTRICAL, THERMAL AND AGEING MODELS 64
5.1.3 SUMMARY AND COMPARISON OF BATTERY MODELS 67
5.2 IMPEDANCE-BASED MODELLING OF BATTENES 68
5.2.1 MEASUREMENT SETUP 68
5.2.2 EQUIVALENT CIRCUIT OF THE POSITIVE AND NEGATIVE ELECTRODE OF A
LEAD-ACID BATTERY 71 5.2.3 LIMITATIONS OF ELECTROCHEMICAL IMPEDANCE
SPECTROSCOPY 72
5.2.4 PARAMETER-IDENTIFICATION METHODS 74
5.2.5 MODEL PARAMETERISATION 77
6 LARGE-SIGNAL IMPEDANCE OF NONLINEAR DEVICES FROM SMALL-SIGNAL
IMPEDANCE 79
6.1 METHOD FOR CALCULATION OF LARGE-SIGNAL IMPEDANCE FROM SMALL-SIGNAL
IMPEDANCE 82 6.2 SIMULATED IMPEDANCE SPECTROSCOPY 83
6.3 VOLTAGE DEPENDENCY 85
6.3.1 R(U) PARALLEL C(U) 85
6.3.2 R(U) PARALLEL C(K) WITH A CONSTANT SERIES RESISTANCE 86
6.3.3 VERIFICATION BY SIMULATIONS 88
6.3.4 EXPERIMENTAL VERIFICATION 89
6.4 APPLICATION TO CURRENT DEPENDENCY AND MIXED CURRENT AND VOLTAGE
DEPENDENCY 93 6.4.1 CURRENT DEPENDENCY 93
6.4.2 MIXED CURRENT AND VOLTAGE DEPENDENCY 94
6.4.3 SIMULATIONS OF CURRENT AND VOLTAGE-DEPENDENT EQUIVALENT CIRCUITS
95 6.5 FITTING PROCEDURE FOR NONLINEAR EQUIVALENT CIRCUITS 98
6.6 APPLICATION TO ELECTRODE KINETICS 99
6.6.1 CHARGE TRANSFER 99
6.6.2 SIGN CONVENTION FOR POSITIVE AND NEGATIVE ELECTRODES 102
6.6.3 CHARGE TRANSFER IN COMBINATION WITH ADSORPTION/DESORPTION 102
6.6.4 NEGATIVE ELECTRODE OF A LEAD-ACID BATTERY 108
6.6.5 CONCENTRATION LIMITATION IN LEAD-ACID BATTERIES 112
6.7 CONCLUSION 117
7 SPATIALLY-RESOLVED IMPEDANCE OF INHOMOGENEOUS NONLINEAR
DEVICES. . ... .. ...... 118
7.1 INTRODUCTION 118
7.1.1 NOMENCLATURE 119
7.1.2 ASSUMPTIONS AND LIMITATIONS OF THE PROCEDURES 120
7.1.3 PARAMETER IDENTIFICATION FOR NONLINEAR INHOMOGENEOUS EQUIVALENT
CIRCUITS 121 7.2 NONLINEAR EQUIVALENT CIRCUITS WITH MORE THAN ONE LAYER
121
7.2.1 CURRENT-DEPENDENT RESISTANCES 121
7.2.2 VOLTAGE-DEPENDENT RESISTANCES 123
7.2.3 EXAMPLE SIMULATION 123
7.3 DIFFERENT EQUILIBRIUM VOLTAGE IN THE DIFFERENT LAYERS 125
IMAGE 3
CONTENT VUE
7.3.1 TWOLAYERS 125
7.3.2 HIGHER NUMBER OF LAYERS 127
7.3.3 EXAMPLE SIMULATION 128
7.4 2D VS. 1D FITTING 130
7.4.1 LARGE DIFFERENCE BETWEEN RT,* AND 2 AE VERT 132
7.4.2 LARGE DIFFERENCE BETWEEN EQUILIBRIUM POTENTIALS UO, AND I/ 0,2
135 7.5 POROSITY 138
7.5.1 PARAMETER VARIATION 139
7.5.2 COMPARISON WITH ID FIT 141
7.6 CONCLUSION 143
8 S U M M A RY 144
9 BLBLIOGRAPHY 148
A A P P E N D IX 178
A.1 CONSTANTS 178
A.2 GLOSSARY 178
A.3 ABBREVIATIONS 179
A.4 GRAPHICAL USER INTERFACES (GUI) FOR AUTOMATED FITTING (SEE CHAPTER
5.2.5) 181 A.5 EQUATIONS FOR ACTFOC), B(T}DC) AND D(T}DC) IN CHAPTER
6.6.3 182
A.6 FIT VALUES FOR AI/O = 10 MV AND 50 MV IN CHAPTER 7.3.3 183
A.7 SIMULATION RESULTS FROM CHAPTER 7.4 184
A.7.1 REFERENCE SIMULATION 184
A.7.2 LARGE DIFFERENCE BETWEEN EQUILIBRIUM POTENTIALS UO, AND C/0,2
(CHAPTER 7.4.2) 185 A.8 DELTA-STAR TRANSFORMATION FOR THREE AND FIVE
PORE ELEMENTS CORRESPONDING TO CHAPTER 7.5 186 A.9 SIMULATION RESULTS
FROM CHAPTER 7.5 189
A.9.1 PARAMETER VARIATION 189
A.9.2 COMPARISON WITH ID FIT 190
B DEUTSCHE ZUSAMMENFASSUNG 192
KAPITEL 1: EINLEITUNG 192
KAPITEL 2: ELEKTROCHEMISCHE IMPEDANZSPEKTROSKOPIE 193
KAPITEL 3: ELEKTRODENKINETIK 194
KAPITEL 4: BAUTEILE MIT INHOMOGENER IMPEDANZ 195
KAPITEL 5: IMPEDANZBASIERTER MODELLIERUNGSANSATZ 197
KAPITEL 6: BERECHNUNG DER GROSSSIGNALIMPEDANZ VON NICHTLINEAREN BAUTEILEN
AUS DER KLEINSIGNALIMPEDANZ 198
KAPITEL 7: ORTSAUFGELOESTE IMPEDANZ VON NICHTLINEAREN INHOMOGENEN
BAUTEILEN 199 KAPITEL 8: ZUSAMMENFASSUNG UND AUSBLICK 200
C LEBENSLAUF 202
|
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| dewey-search | 621.31242 |
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| dewey-tens | 620 - Engineering and allied operations |
| discipline | Elektrotechnik / Elektronik / Nachrichtentechnik |
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| id | DE-604.BV037420217 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T23:23:57Z |
| institution | BVB |
| isbn | 9783832294830 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-022572481 |
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| physical | VII, 203 S. graph. Darst. |
| publishDate | 2010 |
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| series | Aachener Beiträge des ISEA |
| series2 | Aachener Beiträge des ISEA |
| spelling | Kowal, Julia 1979- Verfasser (DE-588)143306804 aut Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] Julia Kowal Aachen Shaker 2010 VII, 203 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Aachener Beiträge des ISEA 53 Zugl.: Aachen, Techn. Hochsch., Diss., 2010 Raumauflösung (DE-588)4320079-5 gnd rswk-swf Impedanzspektroskopie (DE-588)4161400-8 gnd rswk-swf Simulation (DE-588)4055072-2 gnd rswk-swf Ersatzschaltbild (DE-588)4152878-5 gnd rswk-swf Stromverteilung (DE-588)4183760-5 gnd rswk-swf Batterie (DE-588)4004687-4 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Batterie (DE-588)4004687-4 s Impedanzspektroskopie (DE-588)4161400-8 s Raumauflösung (DE-588)4320079-5 s Stromverteilung (DE-588)4183760-5 s Ersatzschaltbild (DE-588)4152878-5 s Simulation (DE-588)4055072-2 s DE-604 Aachener Beiträge des ISEA 53 (DE-604)BV005721577 53 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022572481&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Kowal, Julia 1979- Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] Aachener Beiträge des ISEA Raumauflösung (DE-588)4320079-5 gnd Impedanzspektroskopie (DE-588)4161400-8 gnd Simulation (DE-588)4055072-2 gnd Ersatzschaltbild (DE-588)4152878-5 gnd Stromverteilung (DE-588)4183760-5 gnd Batterie (DE-588)4004687-4 gnd |
| subject_GND | (DE-588)4320079-5 (DE-588)4161400-8 (DE-588)4055072-2 (DE-588)4152878-5 (DE-588)4183760-5 (DE-588)4004687-4 (DE-588)4113937-9 |
| title | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] |
| title_auth | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] |
| title_exact_search | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] |
| title_full | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] Julia Kowal |
| title_fullStr | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] Julia Kowal |
| title_full_unstemmed | Spatially resolved impedance of nonlinear inhomogeneous devices [using the example of lead-acid batteries] Julia Kowal |
| title_short | Spatially resolved impedance of nonlinear inhomogeneous devices |
| title_sort | spatially resolved impedance of nonlinear inhomogeneous devices using the example of lead acid batteries |
| title_sub | [using the example of lead-acid batteries] |
| topic | Raumauflösung (DE-588)4320079-5 gnd Impedanzspektroskopie (DE-588)4161400-8 gnd Simulation (DE-588)4055072-2 gnd Ersatzschaltbild (DE-588)4152878-5 gnd Stromverteilung (DE-588)4183760-5 gnd Batterie (DE-588)4004687-4 gnd |
| topic_facet | Raumauflösung Impedanzspektroskopie Simulation Ersatzschaltbild Stromverteilung Batterie Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022572481&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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| work_keys_str_mv | AT kowaljulia spatiallyresolvedimpedanceofnonlinearinhomogeneousdevicesusingtheexampleofleadacidbatteries |