Holdings: Mechanisms in homogeneous and heterogeneous epoxidation catalysis

Mechanisms in homogeneous and heterogeneous epoxidation catalysis:

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Bibliographic Details
Format:	Book
Language:	English
Published:	Amsterdam [u.a.] Elsevier 2008
Edition:	1. ed.
Subjects:	Heterogene Katalyse Homogene Katalyse Epoxidation
Online Access:	Inhaltsverzeichnis Inhaltsverzeichnis
Item Description:	Includes bibliographical references and index
Physical Description:	XXI, 501 S. Ill., graph. Darst. 25cm
ISBN:	0444531882 9780444531889

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MARC


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adam_text	IMAGE 1 CONTRIBUTORS P. XIII PREFACE P. XIX INTRODUCTION P. 1 RATES, KINETICS, AND MECHANISMS OF EPOXIDATION: HOMOGENEOUS, HETEROGENEOUS, AND BIOLOGICAL ROUTES P. 3 INTRODUCTION P. 4 EPOXIDE USES AND MARKETS P. 5 CATALYSTS AND RATES IN COMMODITY AND HETEROGENEOUS EPOXIDATION PROCESSES P. 12 CATALYSTS AND RATES IN HOMOGENEOUS EPOXIDATION REACTIONS P. 16 CATALYSTS AND RATES IN BIOMIMETIC EPOXIDATION REACTIONS P. 25 CATALYSTS AND RATES IN BIOLOGICAL EPOXIDATION REACTIONS P. 28 SUMMARY AND PERSPECTIVE ON THE REACTIVITY RESULTS P. 30 OXIDANTS FOR EPOXIDATION P. 35 MECHANISMS P. 37 HOMOGENEOUS EPOXIDATION BY EARLY TRANSITION METALS (LEWIS ACID MECHANISM) P. 47 MAIN GROUP ELEMENTS P. 57 HOMOGENEOUS EPOXIDATION BY LATE TRANSITION METALS (REDOX MECHANISM) P. 59 BIOLOGICAL SYSTEMS P. 70 PERSPECTIVE AND CONCLUSIONS P. 71 ACKNOWLEDGMENTS P. 72 REFERENCES P. 72 HOMOGENEOUS CATALYSIS P. 101 UNPRECEDENTED SELECTIVITY IN THE H[SUBSCRIPT 2]O[SUBSCRIPT 2] EPOXIDATION OF SIMPLE ALKENES IMPARTED BY SOFT PT(II) LEWIS ACID CATALYSTS P. 103 INTRODUCTION P. 104 CATALYST SYNTHESIS AND LEWIS ACID PROPERTIES P. 105 GENERAL EPOXIDATION ACTIVITY P. 106 REGIOSELECTIVITY P. 107 DIASTEREOSELECTIVITY P. 108 ENANTIOSELECTIVITY P. 109 REACTIONS IN MICELLAR MEDIA P. 110 REACTION MECHANISM P. 113 CONCLUSIONS P. 113 REFERENCES P. 115 LEWIS ACID CATALYZED EPOXIDATION OF OLEFINS USING HYDROGEN PEROXIDE: PROWING PROMINENCE AND EXPANDING RANGE P. 119 INTRODUCTION P. 120 INDUSTRIAL PROCESSES FOR PROPYLENE OXIDE MANUFACTURE: PRESENT AND FUTURE P. 123 A NEW PRESSURE INTENSIFIED EPOXIDATION PROCESS FOR LIGHT OLEFINS P. 126 EXPANDING RANGE OF LEWIS ACID CATALYSIS CHEMISTRY P. 130 MID- TO LATE TRANSITION METAL CATALYSTS ALSO PERFORM EPOXIDATION REACTIONS BY THE LEWIS ACID MECHANISM P. 131 ACKNOWLEDGMENTS P. 148 IMAGE 2 REFERENCES P. 149 ACTIVATION OF HYDROGEN PEROXIDE BY POLYOXOMETALATES P. 155 INTRODUCTION P. 156 ACTIVATION OF HYDROGEN PEROXIDE BY POLYOXOMETALATES P. 157 CATALYTIC OXIDATION BY POLYOXOMETALATES P. 166 CONCLUSIONS P. 170 FUTURE VIEW P. 170 ACKNOWLEDGMENTS P. 171 REFERENCES P. 171 OXAZIRIDINIUM SALT-MEDIATED CATALYTIC ASYMMETRIC EPOXIDATION P. 177 INTRODUCTION P. 178 PAGE GROUP FINDINGS P. 184 ACKNOWLEDGMENTS P. 214 REFERENCES P. 214 SELECTIVE AEROBIC RADICAL EPOXIDATION OF [ALPHA]-OLEFINS CATALYZED BY N-HYDROXYPHTHALIMIDE P. 217 INTRODUCTION P. 218 EXPERIMENTAL P. 219 RESULTS AND DISCUSSION P. 220 CONCLUSIONS P. 227 ACKNOWLEDGMENTS P. 227 REFERENCES P. 227 HETEROGENEOUS CATALYSIS P. 231 INVESTIGATION OF THE ORIGINS OF SELECTIVITY IN ETHYLENE EPOXIDATION ON PROMOTED AND UNPROMOTED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYSTS: A DETAILED KINETIC, MECHANISTIC AND ADSORPTIVE STUDY P. 233 INTRODUCTION P. 234 THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF OXYGEN ON SILVER AND THE STRUCTURE OF THE OXIDE OVERLAYER AND REACTION CONDITIONS P. 235 THE ADSORPTION OF ETHYLENE AND ETHYLENE OXIDE ON CLEAN AND OXIDISED AG(111) AND AG(110) P. 240 THE REACTION MECHANISM P. 242 SUBSURFACE OXYGEN P. 247 PROMOTION P. 249 THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON AN UNOXIDISED AND OXIDISED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST P. 254 THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON AN OXIDISED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST SUBTENDING THE [ALPHA SUBSCRIPT 1]-O STATE ONLY P. 255 THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON THE [ALPHA SUBSCRIPT 2]-O STATE PRINCIPALLY P. 257 ETHYLENE DESORPTION FROM AN UNOXIDISED AND OXIDISED CS-PROMOTED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST P. 257 THE DESORPTION OF ETHYLENE FROM AN OXIDISED CL-PROMOTED CS/AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST P. 258 IMAGE 3 OVERALL CONCLUSIONS P. 259 ACKNOWLEDGEMENT P. 261 REFERENCES P. 261 COMPUTATIONAL STRATEGIES FOR IDENTIFICATION OF BIMETALLIC ETHYLENE EPOXIDATION CATALYSTS P. 265 INTRODUCTION P. 266 COMPUTATIONAL DETAILS P. 267 ACTIVATION ENERGIES ON AG P. 270 EXTENSION TO AG-BASED BIMETALLIC CATALYSTS P. 272 PREDICTIONS USING MICROKINETIC MODELING P. 276 CONCLUSIONS P. 279 ACKNOWLEDGMENTS P. 279 REFERENCES P. 279 EFFECT OF SUPPORT ON ETHYLENE EPOXIDATION ON AG, AU, AND AU-AG CATALYSTS P. 283 INTRODUCTION P. 284 EXPERIMENTAL P. 285 RESULTS AND DISCUSSION P. 287 CONCLUSIONS P. 295 ACKNOWLEDGMENTS P. 295 REFERENCES P. 295 EPOXIDATION OF PROPYLENE WITH OXYGEN-HYDROGEN MIXTURES P. 297 INTRODUCTION P. 298 LIQUID-PHASE EPOXIDATION OF PROPYLENE P. 300 GAS-PHASE EPOXIDATION OF PROPYLENE P. 301 CONCLUSIONS P. 310 REFERENCES P. 311 PROPYLENE EPOXIDATION BY O[SUBSCRIPT 2] + H[SUBSCRIPT 2] OVER AU NANOPARTICLES ON TI-NANOPOROUS SUPPORTS P. 315 INTRODUCTION P. 316 PROPYLENE EPOXIDATION OVER AU/TS-1 CATALYSTS P. 317 AU ON TI-CONTAINING MESOPOROUS SUPPORTS P. 322 PROMOTERS AND POSTSYNTHESIS SUPPORT TREATMENTS P. 324 REACTION KINETICS P. 327 CONCLUSIONS AND FUTURE OUTLOOK P. 331 ACKNOWLEDGMENTS P. 333 REFERENCES P. 333 THE EPOXIDATION OF PROPENE OVER GOLD NANOPARTICLE CATALYSTS P. 339 INTRODUCTION P. 340 EXPERIMENTAL P. 341 RESULTS AND DISCUSSION P. 343 CONCLUSIONS P. 352 ACKNOWLEDGMENTS P. 353 IMAGE 4 REFERENCES P. 353 PROPYLENE EPOXIDATION VIA SHELL S SMPO PROCESS: 30 YEARS OF RESEARCH AND OPERATION P. 355 INTRODUCTION P. 356 CATALYTIC EPOXIDATION P. 358 SMPO PROCESS IMPROVEMENT P. 363 CONCLUSIONS P. 369 ACKNOWLEDGMENT P. 369 REFERENCES P. 369 PROPYLENE EPOXIDATION WITH ETHYLBENZENE HYDROPEROXIDE OVER TI-CONTAINING CATALYSTS PREPARED BY CHEMICAL VAPOR DEPOSITION P. 373 INTRODUCTION P. 374 EXPERIMENTAL P. 375 RESULTS AND DISCUSSION P. 376 CONCLUSIONS P. 385 ACKNOWLEDGMENT P. 385 REFERENCES P. 385 METAL SPECIES SUPPORTED ON ORGANIC POLYMERS AS CATALYSTS FOR THE EPOXIDATION OF ALKENES P. 387 INTRODUCTION P. 388 SUPPORTED MANGANESE CATALYSTS P. 389 SUPPORTED MOLYBDENUM CATALYSTS P. 396 SUPPORTED RUTHENIUM AND IRON CATALYSTS P. 398 SUPPORTED TITANIUM CATALYSTS P. 399 SUPPORTED TUNGSTEN CATALYSTS P. 400 SUPPORTED RHENIUM CATALYSTS P. 401 SUPPORTED COBALT, NICKEL, AND PLATINUM CATALYSTS P. 402 SUPPORTED BINOL-COMPLEXES OF LANTHANOIDS AND CALCIUM P. 402 CONCLUSION P. 403 ACKNOWLEDGMENT P. 407 REFERENCES P. 407 PHASE-TRANSFER CATALYSIS P. 413 FINE-TUNING AND RECYCLING OF HOMOGENEOUS TUNGSTATE AND POLYTUNGSTATE EPOXIDATION CATALYSTS P. 415 INTRODUCTION P. 416 CHARACTERISTICS AND PREPARATION OF SANDWICH POMS P. 417 BENCHMARKING SANDWICH POM-CATALYZED EPOXIDATIONS P. 418 EFFECT OF CARBOXYLIC ACIDS AS COCATALYSTS IN TUNGSTATE-CATALYZED EPOXIDATIONS P. 420 EPOXIDATIONS THAT AFFORD ACID-SENSITIVE PRODUCTS P. 421 SANDWICH POM CATALYST RECYCLING P. 425 CONCLUSIONS P. 426 ACKNOWLEDGMENTS P. 427 REFERENCES P. 427 IMAGE 5 REACTION-CONTROLLED PHASE-TRANSFER CATALYSIS FOR EPOXIDATION OF OLEFINS P. 429 INTRODUCTION P. 430 REACTION-CONTROLLED PHASE-TRANSFER CATALYST BASED ON QUATERNARY AMMONIUM PHOSPHOTUNGSTATES P. 431 INFLUENCE OF THE COMPOSITION OF THE HETEROPOLYPHOSPHOTUNGSTATE ANION [40] P. 432 INFLUENCE OF DIFFERENT QUATERNARY AMMONIUM CATIONS [43] P. 433 EPOXIDATION OF PROPYLENE WITH IN SITU GENERATED H[SUBSCRIPT 2]O[SUBSCRIPT 2] AS THE OXIDANT P. 435 EPOXIDATION OF PROPYLENE WITH AQUEOUS H[SUBSCRIPT 2]O[SUBSCRIPT 2] [45] AS THE OXIDANT P. 438 EPOXIDATION OF CYCLOHEXENE AND OTHERS OLEFINS P. 439 EPOXIDATION OF ALLYL CHLORIDE P. 440 CONCLUSION P. 444 ACKNOWLEDGMENTS P. 444 REFERENCES P. 444 BIOMIMETIC CATALYSIS P. 449 BIO-INSPIRED IRON-CATALYZED OLEFIN OXIDATIONS: EPOXIDATION VERSUS CIS-DIHYDROXYLATION P. 451 INTRODUCTION P. 452 STRUCTURE-REACTIVITY CORRELATION OF CATALYSTS P. 453 TOWARD SYNTHETICALLY USEFUL APPLICATIONS P. 457 MECHANISTIC LANDSCAPE P. 459 ACKNOWLEDGMENT P. 466 REFERENCES P. 466 QUANTUM CHEMICAL ANALYSIS OF THE REACTION PATHWAY FOR STYRENE EPOXIDATION CATALYZED BY MN-PORPHYRINS P. 471 INTRODUCTION P. 472 METHODOLOGY P. 473 RESULTS P. 475 CONCLUSIONS P. 483 ACKNOWLEDGMENTS P. 483 REFERENCES P. 484 INDEX P. 487 TABLE OF CONTENTS PROVIDED BY BLACKWELL S BOOK SERVICES AND R.R. BOWKER. USED WITH PERMISSION.
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spelling	Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama 1. ed. Amsterdam [u.a.] Elsevier 2008 XXI, 501 S. Ill., graph. Darst. 25cm txt rdacontent n rdamedia nc rdacarrier Includes bibliographical references and index Heterogene Katalyse (DE-588)4123377-3 gnd rswk-swf Homogene Katalyse (DE-588)4160579-2 gnd rswk-swf Epoxidation (DE-588)4152560-7 gnd rswk-swf Epoxidation (DE-588)4152560-7 s Homogene Katalyse (DE-588)4160579-2 s Heterogene Katalyse (DE-588)4123377-3 s DE-604 Oyama, S. Ted Sonstige oth DE-601 pdf/application http://www.gbv.de/dms/bowker/toc/9780444531889.pdf Inhaltsverzeichnis GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020510724&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Mechanisms in homogeneous and heterogeneous epoxidation catalysis Heterogene Katalyse (DE-588)4123377-3 gnd Homogene Katalyse (DE-588)4160579-2 gnd Epoxidation (DE-588)4152560-7 gnd
subject_GND	(DE-588)4123377-3 (DE-588)4160579-2 (DE-588)4152560-7
title	Mechanisms in homogeneous and heterogeneous epoxidation catalysis
title_auth	Mechanisms in homogeneous and heterogeneous epoxidation catalysis
title_exact_search	Mechanisms in homogeneous and heterogeneous epoxidation catalysis
title_full	Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama
title_fullStr	Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama
title_full_unstemmed	Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama
title_short	Mechanisms in homogeneous and heterogeneous epoxidation catalysis
title_sort	mechanisms in homogeneous and heterogeneous epoxidation catalysis
topic	Heterogene Katalyse (DE-588)4123377-3 gnd Homogene Katalyse (DE-588)4160579-2 gnd Epoxidation (DE-588)4152560-7 gnd
topic_facet	Heterogene Katalyse Homogene Katalyse Epoxidation
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