Mechanisms in homogeneous and heterogeneous epoxidation catalysis:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Amsterdam [u.a.]
Elsevier
2008
|
| Ausgabe: | 1. ed. |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis Inhaltsverzeichnis |
| Beschreibung: | Includes bibliographical references and index |
| Beschreibung: | XXI, 501 S. Ill., graph. Darst. 25cm |
| ISBN: | 0444531882 9780444531889 |
Internformat
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| 245 | 1 | 0 | |a Mechanisms in homogeneous and heterogeneous epoxidation catalysis |c ed. by S. Ted Oyama |
| 250 | |a 1. ed. | ||
| 264 | 1 | |a Amsterdam [u.a.] |b Elsevier |c 2008 | |
| 300 | |a XXI, 501 S. |b Ill., graph. Darst. |c 25cm | ||
| 336 | |b txt |2 rdacontent | ||
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| 500 | |a Includes bibliographical references and index | ||
| 650 | 0 | 7 | |a Heterogene Katalyse |0 (DE-588)4123377-3 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Homogene Katalyse |0 (DE-588)4160579-2 |2 gnd |9 rswk-swf |
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Datensatz im Suchindex
| _version_ | 1804143189017231362 |
|---|---|
| adam_text | IMAGE 1
CONTRIBUTORS
P. XIII
PREFACE
P. XIX
INTRODUCTION
P. 1
RATES, KINETICS, AND MECHANISMS OF EPOXIDATION: HOMOGENEOUS,
HETEROGENEOUS, AND BIOLOGICAL ROUTES
P. 3
INTRODUCTION
P. 4
EPOXIDE USES AND MARKETS
P. 5
CATALYSTS AND RATES IN COMMODITY AND HETEROGENEOUS EPOXIDATION PROCESSES
P. 12
CATALYSTS AND RATES IN HOMOGENEOUS EPOXIDATION REACTIONS P. 16
CATALYSTS AND RATES IN BIOMIMETIC EPOXIDATION REACTIONS
P. 25
CATALYSTS AND RATES IN BIOLOGICAL EPOXIDATION REACTIONS
P. 28
SUMMARY AND PERSPECTIVE ON THE REACTIVITY RESULTS
P. 30
OXIDANTS FOR EPOXIDATION
P. 35
MECHANISMS
P. 37
HOMOGENEOUS EPOXIDATION BY EARLY TRANSITION METALS (LEWIS ACID
MECHANISM) P. 47
MAIN GROUP ELEMENTS
P. 57
HOMOGENEOUS EPOXIDATION BY LATE TRANSITION METALS (REDOX MECHANISM) P.
59
BIOLOGICAL SYSTEMS
P. 70
PERSPECTIVE AND CONCLUSIONS
P. 71
ACKNOWLEDGMENTS
P. 72
REFERENCES
P. 72
HOMOGENEOUS CATALYSIS
P. 101
UNPRECEDENTED SELECTIVITY IN THE H[SUBSCRIPT 2]O[SUBSCRIPT 2]
EPOXIDATION OF SIMPLE ALKENES IMPARTED BY SOFT PT(II) LEWIS ACID
CATALYSTS
P. 103
INTRODUCTION
P. 104
CATALYST SYNTHESIS AND LEWIS ACID PROPERTIES
P. 105
GENERAL EPOXIDATION ACTIVITY
P. 106
REGIOSELECTIVITY
P. 107
DIASTEREOSELECTIVITY
P. 108
ENANTIOSELECTIVITY
P. 109
REACTIONS IN MICELLAR MEDIA
P. 110
REACTION MECHANISM
P. 113
CONCLUSIONS
P. 113
REFERENCES
P. 115
LEWIS ACID CATALYZED EPOXIDATION OF OLEFINS USING HYDROGEN PEROXIDE:
PROWING PROMINENCE AND EXPANDING RANGE
P. 119
INTRODUCTION
P. 120
INDUSTRIAL PROCESSES FOR PROPYLENE OXIDE MANUFACTURE: PRESENT AND FUTURE
P. 123
A NEW PRESSURE INTENSIFIED EPOXIDATION PROCESS FOR LIGHT OLEFINS P. 126
EXPANDING RANGE OF LEWIS ACID CATALYSIS CHEMISTRY
P. 130
MID- TO LATE TRANSITION METAL CATALYSTS ALSO PERFORM EPOXIDATION
REACTIONS BY THE LEWIS ACID MECHANISM
P. 131
ACKNOWLEDGMENTS
P. 148
IMAGE 2
REFERENCES
P. 149
ACTIVATION OF HYDROGEN PEROXIDE BY POLYOXOMETALATES
P. 155
INTRODUCTION
P. 156
ACTIVATION OF HYDROGEN PEROXIDE BY POLYOXOMETALATES
P. 157
CATALYTIC OXIDATION BY POLYOXOMETALATES
P. 166
CONCLUSIONS
P. 170
FUTURE VIEW
P. 170
ACKNOWLEDGMENTS
P. 171
REFERENCES
P. 171
OXAZIRIDINIUM SALT-MEDIATED CATALYTIC ASYMMETRIC EPOXIDATION P. 177
INTRODUCTION
P. 178
PAGE GROUP FINDINGS
P. 184
ACKNOWLEDGMENTS
P. 214
REFERENCES
P. 214
SELECTIVE AEROBIC RADICAL EPOXIDATION OF [ALPHA]-OLEFINS CATALYZED BY
N-HYDROXYPHTHALIMIDE
P. 217
INTRODUCTION
P. 218
EXPERIMENTAL
P. 219
RESULTS AND DISCUSSION
P. 220
CONCLUSIONS
P. 227
ACKNOWLEDGMENTS
P. 227
REFERENCES
P. 227
HETEROGENEOUS CATALYSIS
P. 231
INVESTIGATION OF THE ORIGINS OF SELECTIVITY IN ETHYLENE EPOXIDATION ON
PROMOTED AND UNPROMOTED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3]
CATALYSTS: A DETAILED KINETIC, MECHANISTIC AND ADSORPTIVE STUDY
P. 233
INTRODUCTION
P. 234
THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF OXYGEN ON
SILVER AND THE STRUCTURE OF THE OXIDE OVERLAYER AND REACTION CONDITIONS
P. 235
THE ADSORPTION OF ETHYLENE AND ETHYLENE OXIDE ON CLEAN AND OXIDISED
AG(111) AND AG(110) P. 240
THE REACTION MECHANISM
P. 242
SUBSURFACE OXYGEN
P. 247
PROMOTION
P. 249
THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON AN
UNOXIDISED AND OXIDISED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3]
CATALYST
P. 254
THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON AN
OXIDISED AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST SUBTENDING
THE [ALPHA SUBSCRIPT 1]-O STATE ONLY
P. 255
THE DETAILED KINETICS OF THE ADSORPTION AND DESORPTION OF ETHYLENE ON
THE [ALPHA SUBSCRIPT 2]-O STATE PRINCIPALLY
P. 257
ETHYLENE DESORPTION FROM AN UNOXIDISED AND OXIDISED CS-PROMOTED
AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST
P. 257
THE DESORPTION OF ETHYLENE FROM AN OXIDISED CL-PROMOTED
CS/AG/[ALPHA]-AL[SUBSCRIPT 2]O[SUBSCRIPT 3] CATALYST
P. 258
IMAGE 3
OVERALL CONCLUSIONS
P. 259
ACKNOWLEDGEMENT
P. 261
REFERENCES
P. 261
COMPUTATIONAL STRATEGIES FOR IDENTIFICATION OF BIMETALLIC ETHYLENE
EPOXIDATION CATALYSTS
P. 265
INTRODUCTION
P. 266
COMPUTATIONAL DETAILS
P. 267
ACTIVATION ENERGIES ON AG
P. 270
EXTENSION TO AG-BASED BIMETALLIC CATALYSTS
P. 272
PREDICTIONS USING MICROKINETIC MODELING
P. 276
CONCLUSIONS
P. 279
ACKNOWLEDGMENTS
P. 279
REFERENCES
P. 279
EFFECT OF SUPPORT ON ETHYLENE EPOXIDATION ON AG, AU, AND AU-AG CATALYSTS
P. 283
INTRODUCTION
P. 284
EXPERIMENTAL
P. 285
RESULTS AND DISCUSSION
P. 287
CONCLUSIONS
P. 295
ACKNOWLEDGMENTS
P. 295
REFERENCES
P. 295
EPOXIDATION OF PROPYLENE WITH OXYGEN-HYDROGEN MIXTURES
P. 297
INTRODUCTION
P. 298
LIQUID-PHASE EPOXIDATION OF PROPYLENE
P. 300
GAS-PHASE EPOXIDATION OF PROPYLENE
P. 301
CONCLUSIONS
P. 310
REFERENCES
P. 311
PROPYLENE EPOXIDATION BY O[SUBSCRIPT 2] + H[SUBSCRIPT 2] OVER AU
NANOPARTICLES ON TI-NANOPOROUS SUPPORTS
P. 315
INTRODUCTION
P. 316
PROPYLENE EPOXIDATION OVER AU/TS-1 CATALYSTS
P. 317
AU ON TI-CONTAINING MESOPOROUS SUPPORTS
P. 322
PROMOTERS AND POSTSYNTHESIS SUPPORT TREATMENTS
P. 324
REACTION KINETICS
P. 327
CONCLUSIONS AND FUTURE OUTLOOK
P. 331
ACKNOWLEDGMENTS
P. 333
REFERENCES
P. 333
THE EPOXIDATION OF PROPENE OVER GOLD NANOPARTICLE CATALYSTS P. 339
INTRODUCTION
P. 340
EXPERIMENTAL
P. 341
RESULTS AND DISCUSSION
P. 343
CONCLUSIONS
P. 352
ACKNOWLEDGMENTS
P. 353
IMAGE 4
REFERENCES
P. 353
PROPYLENE EPOXIDATION VIA SHELL S SMPO PROCESS: 30 YEARS OF RESEARCH AND
OPERATION P. 355
INTRODUCTION
P. 356
CATALYTIC EPOXIDATION
P. 358
SMPO PROCESS IMPROVEMENT
P. 363
CONCLUSIONS
P. 369
ACKNOWLEDGMENT
P. 369
REFERENCES
P. 369
PROPYLENE EPOXIDATION WITH ETHYLBENZENE HYDROPEROXIDE OVER TI-CONTAINING
CATALYSTS PREPARED BY CHEMICAL VAPOR DEPOSITION
P. 373
INTRODUCTION
P. 374
EXPERIMENTAL
P. 375
RESULTS AND DISCUSSION
P. 376
CONCLUSIONS
P. 385
ACKNOWLEDGMENT
P. 385
REFERENCES
P. 385
METAL SPECIES SUPPORTED ON ORGANIC POLYMERS AS CATALYSTS FOR THE
EPOXIDATION OF ALKENES
P. 387
INTRODUCTION
P. 388
SUPPORTED MANGANESE CATALYSTS
P. 389
SUPPORTED MOLYBDENUM CATALYSTS
P. 396
SUPPORTED RUTHENIUM AND IRON CATALYSTS
P. 398
SUPPORTED TITANIUM CATALYSTS
P. 399
SUPPORTED TUNGSTEN CATALYSTS
P. 400
SUPPORTED RHENIUM CATALYSTS
P. 401
SUPPORTED COBALT, NICKEL, AND PLATINUM CATALYSTS
P. 402
SUPPORTED BINOL-COMPLEXES OF LANTHANOIDS AND CALCIUM
P. 402
CONCLUSION
P. 403
ACKNOWLEDGMENT
P. 407
REFERENCES
P. 407
PHASE-TRANSFER CATALYSIS
P. 413
FINE-TUNING AND RECYCLING OF HOMOGENEOUS TUNGSTATE AND POLYTUNGSTATE
EPOXIDATION CATALYSTS
P. 415
INTRODUCTION
P. 416
CHARACTERISTICS AND PREPARATION OF SANDWICH POMS
P. 417
BENCHMARKING SANDWICH POM-CATALYZED EPOXIDATIONS
P. 418
EFFECT OF CARBOXYLIC ACIDS AS COCATALYSTS IN TUNGSTATE-CATALYZED
EPOXIDATIONS P. 420
EPOXIDATIONS THAT AFFORD ACID-SENSITIVE PRODUCTS
P. 421
SANDWICH POM CATALYST RECYCLING
P. 425
CONCLUSIONS
P. 426
ACKNOWLEDGMENTS
P. 427
REFERENCES
P. 427
IMAGE 5
REACTION-CONTROLLED PHASE-TRANSFER CATALYSIS FOR EPOXIDATION OF OLEFINS
P. 429
INTRODUCTION
P. 430
REACTION-CONTROLLED PHASE-TRANSFER CATALYST BASED ON QUATERNARY AMMONIUM
PHOSPHOTUNGSTATES
P. 431
INFLUENCE OF THE COMPOSITION OF THE HETEROPOLYPHOSPHOTUNGSTATE ANION
[40] P. 432
INFLUENCE OF DIFFERENT QUATERNARY AMMONIUM CATIONS [43]
P. 433
EPOXIDATION OF PROPYLENE WITH IN SITU GENERATED H[SUBSCRIPT
2]O[SUBSCRIPT 2] AS THE OXIDANT
P. 435
EPOXIDATION OF PROPYLENE WITH AQUEOUS H[SUBSCRIPT 2]O[SUBSCRIPT 2] [45]
AS THE OXIDANT
P. 438
EPOXIDATION OF CYCLOHEXENE AND OTHERS OLEFINS
P. 439
EPOXIDATION OF ALLYL CHLORIDE
P. 440
CONCLUSION
P. 444
ACKNOWLEDGMENTS
P. 444
REFERENCES
P. 444
BIOMIMETIC CATALYSIS
P. 449
BIO-INSPIRED IRON-CATALYZED OLEFIN OXIDATIONS: EPOXIDATION VERSUS
CIS-DIHYDROXYLATION
P. 451
INTRODUCTION
P. 452
STRUCTURE-REACTIVITY CORRELATION OF CATALYSTS
P. 453
TOWARD SYNTHETICALLY USEFUL APPLICATIONS
P. 457
MECHANISTIC LANDSCAPE
P. 459
ACKNOWLEDGMENT
P. 466
REFERENCES
P. 466
QUANTUM CHEMICAL ANALYSIS OF THE REACTION PATHWAY FOR STYRENE
EPOXIDATION CATALYZED BY MN-PORPHYRINS
P. 471
INTRODUCTION
P. 472
METHODOLOGY
P. 473
RESULTS
P. 475
CONCLUSIONS
P. 483
ACKNOWLEDGMENTS
P. 483
REFERENCES
P. 484
INDEX
P. 487
TABLE OF CONTENTS PROVIDED BY BLACKWELL S BOOK SERVICES AND R.R. BOWKER.
USED WITH PERMISSION.
|
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| illustrated | Illustrated |
| indexdate | 2024-07-09T22:43:35Z |
| institution | BVB |
| isbn | 0444531882 9780444531889 |
| language | English |
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| physical | XXI, 501 S. Ill., graph. Darst. 25cm |
| publishDate | 2008 |
| publishDateSearch | 2008 |
| publishDateSort | 2008 |
| publisher | Elsevier |
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| spelling | Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama 1. ed. Amsterdam [u.a.] Elsevier 2008 XXI, 501 S. Ill., graph. Darst. 25cm txt rdacontent n rdamedia nc rdacarrier Includes bibliographical references and index Heterogene Katalyse (DE-588)4123377-3 gnd rswk-swf Homogene Katalyse (DE-588)4160579-2 gnd rswk-swf Epoxidation (DE-588)4152560-7 gnd rswk-swf Epoxidation (DE-588)4152560-7 s Homogene Katalyse (DE-588)4160579-2 s Heterogene Katalyse (DE-588)4123377-3 s DE-604 Oyama, S. Ted Sonstige oth DE-601 pdf/application http://www.gbv.de/dms/bowker/toc/9780444531889.pdf Inhaltsverzeichnis GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020510724&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Mechanisms in homogeneous and heterogeneous epoxidation catalysis Heterogene Katalyse (DE-588)4123377-3 gnd Homogene Katalyse (DE-588)4160579-2 gnd Epoxidation (DE-588)4152560-7 gnd |
| subject_GND | (DE-588)4123377-3 (DE-588)4160579-2 (DE-588)4152560-7 |
| title | Mechanisms in homogeneous and heterogeneous epoxidation catalysis |
| title_auth | Mechanisms in homogeneous and heterogeneous epoxidation catalysis |
| title_exact_search | Mechanisms in homogeneous and heterogeneous epoxidation catalysis |
| title_full | Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama |
| title_fullStr | Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama |
| title_full_unstemmed | Mechanisms in homogeneous and heterogeneous epoxidation catalysis ed. by S. Ted Oyama |
| title_short | Mechanisms in homogeneous and heterogeneous epoxidation catalysis |
| title_sort | mechanisms in homogeneous and heterogeneous epoxidation catalysis |
| topic | Heterogene Katalyse (DE-588)4123377-3 gnd Homogene Katalyse (DE-588)4160579-2 gnd Epoxidation (DE-588)4152560-7 gnd |
| topic_facet | Heterogene Katalyse Homogene Katalyse Epoxidation |
| url | http://www.gbv.de/dms/bowker/toc/9780444531889.pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020510724&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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