Verfügbarkeit: Modern spectroscopy

Modern spectroscopy:

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1. Verfasser:	Hollas, John Michael (VerfasserIn)
Format:	Buch
Sprache:	English
Veröffentlicht:	Chichester [u.a.] Wiley 2010
Ausgabe:	4. ed., reprint.
Schlagworte:	Theorie Molekülspektroskopie Spektroskopie Atomspektroskopie Lehrbuch
Online-Zugang:	Inhaltsverzeichnis Klappentext
Beschreibung:	XXVII, 452 S. Ill., graph. Darst.
ISBN:	9780470844168 9780470844151

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Datensatz im Suchindex

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adam_text	Contents Preface to first edition xiii Preface to second edition xv Preface to third edition xvii Preface to fourth edition xix Units, dimensions and conventions xxi Fundamental constants xxiii Useful conversion factors xxv 1 Some important results in quantum mechanics 1 1.1 Spectroscopy and quantum mechanics 1 1.2 The evolution of quantum theory 2 1.3 The Schrödinger equation and some of its solutions 8 1.3.1 The Schrödinger equation 9 1.3.2 The hydrogen atom 11 1.3.3 Electron spin and nuclear spin angular momentum 17 1.3.4 The Born-Oppenheimer approximation 19 1.3.5 The rigid rotor 21 1.3.6 The harmonic oscillator 23 Exercises 25 Bibliography 26 2 Electromagnetic radiation and its interaction with atoms and molecules 27 2.1 Electromagnetic radiation 27 2.2 Absorption and emission of radiation 27 2.3 Line width 34 2.3.1 Natural line broadening 34 2.3.2 Doppler broadening 35 2.3.3 Pressure broadening 36 2.3.4 Power, or saturation, broadening 36 2.3.5 Removal of hne broadening 37 2.3.5.1 Effusive atomic or molecular beams 37 2.3.5.2 Lamb dip spectroscopy 37 CONTENTS Exercises 38 Bibliography 39 3 Generai features of experimental methods 41 3.1 The electromagnetic spectrum 41 3.2 General components of an absorption experiment 42 3.3 Dispersing elements 43 3.3.1 Prisms 43 3.3.2 Diffraction gratings 45 3.3.3 Fourier transformation and interferometers 48 3.3.3.1 Radiofrequency radiation 49 3.3.3.2 Infrared, visible and ultraviolet radiation 55 3.4 Components of absorption experiments in various regions of the spectrum 59 3.4.1 Microwave and millimetre wave 59 3.4.2 Far-infrared 61 3.4.3 Near-infrared and mid-infrared 62 3.4.4 Visible and near-ultraviolet 62 3.4.5 Vacuum- or far-ultraviolet 63 3.5 Other experimental techniques 64 3.5.1 Attenuated total reflectance spectroseopy and reflection-absorption infrared spectroseopy 64 3.5.2 Atomic absorption spectroseopy 64 3.5.3 Inductively coupled plasma atomic emission spectroseopy 66 3.5.4 Flash photolysis 67 3.6 Typical recording spectrophotometers for the near-infrared, mid-infrared, visible and near-ultraviolet regions 68 Exercise 70 Bibliography 70 4 Molecular symmetry 73 4.1 Elements of symmetry 73 4.1.1 л -Fold axis of symmetry, Cn 74 4.1.2 Plane of symmetry, σ 75 4.1.3 Centre of inversion, і 76 4.1.4 л -Fold rotation-reflection axis of symmetry, S„ 76 4.1.5 The identity element of symmetry, I (or E) 77 4.1.6 Generation of elements 77 4.1.7 Symmetry conditions for molecular chirality 78 4.2 Point groups 81 4.2.1 Cn point groups 82 4.2.2 S„ point groups 83 4.2.3 Cm point groups 83 4.2.4 £>„ point groups 83 4.2.5 С„ћ point groups 84 4.2.6 D^j point groups 84 4.2.7 D„h point groups 84 CONTENTS vii 4.2.8 Tđ point group 85 4.2.9 Оћ point group 85 4.2.10 Kh point group 86 4.2.11 4 point group 86 4.2.12 Other point groups 87 4.3 Point group character tables 87 4.3.1 C2v character table 87 4.3.2 C3„ character table 92 4.3.3 Cm character table 96 4.3.4 Ih character table 97 4.4 Symmetry and dipole moments 97 Exercises 102 Bibliography 102 5 Rotational spectroscopy 103 5.1 Linear, symmetric rotor, spherical rotor and asymmetric rotor molecules 103 5.2 Rotational infrared, millimetre wave and microwave spectra 105 5.2.1 Diatomic and linear polyatomic molecules 105 5.2.1.1 Transition frequencies or wavenumbers 105 5.2.1.2 Intensities 110 5.2.1.3 Centrifugal distortion 111 5.2.1.4 Diatomic molecules in excited vibrational states 112 5.2.2 Symmetric rotor molecules 113 5.2.3 Stark effect in diatomic, linear and symmetric rotor molecules 115 5.2.4 Asymmetric rotor molecules 116 5.2.5 Spherical rotor molecules 117 5.2.6 Interstellar molecules detected by their radiofŕequency, microwave or millimetre wave spectra 119 5.3 Rotational Raman spectroscopy 122 5.3.1 Experimental methods 122 5.3.2 Theory of rotational Raman scattering 124 5.3.3 Rotational Raman spectra of diatomic and linear polyatomic molecules 126 5.3.4 Nuclear spin statistical weights 128 5.3.5 Rotational Raman spectra of symmetric and asymmetric rotor molecules 131 5.4 Structure determination from rotational constants 131 Exercises 134 Bibliography 135 6 Vibrational spectroscopy 137 6.1 Diatomic molecules 137 6.1.1 Infrared spectra 138 6.1.2 Raman spectra 140 6.1.3 Anharmonicity 142 6.1.3.1 Electrical anharmonicity 142 6.1.3.2 Mechanical anharmonicity 142 CONTENTS 6.1.4 Vibration-rotation spectroscopy 4 6.1.4.1 Infrared spectra 147 6.1.4.2 Raman spectra * 6.2 Polyatomic molecules $4 6.2.1 Group vibrations 54 6.2.2 Number of normal vibrations of each symmetry species 162 6.2.2.1 Non-degenerate vibrations 63 6.2.2.2 Degenerate vibrations 65 6.2.3 Vibrational selection rules 66 6.2.3.1 Infrared spectra 166 170 6.2.3.2 Raman spectra XIŁ 6.2A Vibration-rotation spectroscopy 173 6.2.4.1 Infrared spectra of linear molecules 174 6.2.4.2 Infrared spectra of symmetric rotors 17° 6.2.4.3 Infrared spectra of spherical rotors 180 6.2.4.4 Infrared spectra of asymmetric rotors 181 6.2.5 Anharmonicity 184 6.2.5.1 Potential energy surfaces 184 6.2.5.2 Vibrational term values 186 6.2.5.3 Local mode treatment of vibrations 187 6.2.5.4 Vibrational potential functions with more than one minimum 188 6.2.5.4(a) Inversion vibrations 189 6.2.5.4(b) Ring-puckering vibrations 191 6.2.5.4^) Torsionai vibrations 192 Exercises 195 Bibliography 196 7 Electronic spectroscopy 199 7.1 Atomic spectroscopy 199 7.1.1 The periodic table 199 7.1.2 Vector representation of momenta and vector coupling approximations 201 7.1.2.1 Angular momenta and magnetic moments 201 7.1.2.2 Coupling of angular momenta 205 7.1.2.3 Russell-Saunders coupling approximation 206 7.1.2.3(a) Non-equivalent electrons 206 7 Л .2.3(0) Equivalent electrons 210 7.1.3 Spectra of alkali metal atoms 213 7.1.4 Spectrum of the hydrogen atom 216 7.1.5 Spectra of helium and the alkaline earth metal atoms 219 7.1.6 Spectra of other polyelectronic atoms 222 7.2 Electronic spectroscopy of diatomic molecules 225 7.2.1 Molecular orbitais 225 7.2.1.1 Homonuclear diatomic molecules 225 7.2.1.2 Heteronuclear diatomic molecules 232 7.2.2 Classification of electronic states 233 7.2.3 Electronic selection rules 236 7.2.4 Derivation of states arising from configurations 237 7.2.5 Vibrational coarse structure 240 7.2.5.1 Potential energy curves in excited electronic states 240 7.2.5.2 Progressions and sequences 242 CONTENTS ix 7.2.5.3 The Franck-Condon principie 246 7.2.5.4 Deslandres tables 250 7.2.5.5 Dissociation energies 250 7.2.5.6 Repulsive states and continuous spectra 253 7.2.6 Rotational fine structure 254 7.2.6.1 Σ — Σ electronic and vibronic transitions 254 7.2.6.2 Я — žľ electronic and vibronic transitions 257 7.3 Electronic spectroscopy of polyatomic molecules 260 7.3.1 Molecular orbitais and electronic states 260 7.3.1.1 AH2 molecules 261 7.3.1. l(a) Z HAH =180° 261 7.3.1.1(0) L HAH = 90° 263 7.3.1.2 Formaldehyde (H2CO) 265 7.3.1.3 Benzene 267 7.3.1.4 Crystal field and ligand field molecular orbitais 270 7.3.1 .4(a) Crystal field theory 271 7.3. 1.4(b) Ligand field theory 273 7.3. 1.4(c) Electronic transitions 275 7.3.2 Electronic and vibróme selection rules 275 7.3.3 Chromophores 278 7.3.4 Vibrational coarse structure 278 7.3.4.1 Sequences 278 7.3.4.2 Progressions 279 7.3.4.2(a) Totally symmetric vibrations 279 7.3.4.2(b) Non-totally symmetric vibrations 279 7.3.5 Rotational fine structure 283 7.3.6 Diffuse spectra 284 Exercises 287 Bibliography 288 8 Photoelectron and related spectroscopies 289 8.1 Photoelectron spectroscopy 289 8.1.1 Experimental methods 291 8.1.1.1 Sources of monochromatic ionizing radiation 291 8.1.1.2 Electron velocity analysers 294 8.1.1.3 Electron detectors 294 8.1.1.4 Resolution 294 8.1.2 Ionization processes and Koopmans theorem 295 8.1.3 Photoelectron spectra and their interpretation 297 8.1.3.1 Ultraviolet photoelectron spectra of atoms 297 8.1.3.2 Ultraviolet photoelectron spectra of molecules 298 8.1.3.2(a) Hydrogen 298 8.1.3.2(b) Nitrogen 300 8. 1.3.2(c) Hydrogen bromide 302 8.1.3.2(d) Water 305 8.1.3.2(e) Benzene 305 8.1.3.3 X-ray photoelectron spectra of gases 307 8.1.3.4 X-ray photoelectron spectra of solids 313 8.2 Auger electron and X-ray fluorescence spectroscopy 315 8.2.1 Auger electron spectroscopy 317 8.2.1.1 Experimental method 317 CONTENTS 8.2.1.2 Processes in Auger electron ejection 318 8.2.1.3 Examples of Auger electron spectra 319 8.2.2 X-ray fluorescence spectroscopy 322 8.2.2.1 Experimental method 322 8.2.2.2 Processes in X-ray fluorescence 324 8.2.2.3 Examples of X-ray fluorescence spectra 325 8.3 Extended X-ray absorption fine structure 327 Exercises 334 Bibliography 335 9 Lasers and laser spectroscopy 337 9.1 General discussion of lasers 337 9.1.1 General features and properties 337 9.1.2 Methods of obtaining population inversion 340 9.1.3 Laser cavity modes 341 9.1.4 g-switching 342 9.1.5 Mode locking 344 9.1.6 Harmonic generation 345 9.2 Examples of lasers 346 9.2.1 The ruby and alexandrite lasers 346 9.2.2 The titanium-sapphire laser 348 9.2.3 The neodymium-YAG laser 349 9.2.4 The diode or semiconductor laser 350 9.2.5 The helium-neon laser 352 9.2.6 The argon ion and krypton ion lasers 354 9.2.7 The nitrogen (N2) laser 355 9.2.8 The excimer and exciplex lasers 356 9.2.9 The carbon dioxide laser 358 9.2.10 The dye lasers 359 9.2.11 Laser materials in general 362 9.3 Uses of lasers in spectroscopy 362 9.3.1 Hyper Raman spectroscopy 363 9.3.2 Stimulated Raman spectroscopy 365 9.3.3 Coherent anti-Stokes Raman scattering spectroscopy 367 9.3.4 Laser Stark (or laser electron resonance) spectroscopy 368 9.3.5 Two-photon and multiphoton absorption 371 9.3.6 Multiphoton dissociation and laser separation of isotopes 374 9.3.7 Single vibronic level, or dispersed, fluorescence 377 9.3.8 Light detection and ranging (LIDAR) 379 9.3.9 Cavity ring-down spectroscopy 382 9.3.10 Femtosecond spectroscopy 387 9.3.11 Spectroscopy of molecules in supersonic jets 393 9.3.11.1 Properties of a supersonic jet 3 93 9.3.11.2 Fluorescence excitation spectroscopy 396 9.3.11.3 Single vibronic level, or dispersed, fluorescence spectroscopy 400 9.3.11.4 Zero kinetic energy photoelectron spectroscopy 402 Exercises 404 Bibliography 405 CONTENTS xi Appendix A Character tables 407 В Symmetry species of vibrations 423 Index of Atoms and Molecules 429 Subject Index 439 MODERN SPECTROSCOPY Fourth Edition J. Michael Hollas, University of Reading, UK The fourth edition of Modern Spectroscopy introduces the reader to a wide range of spectroscopies and includes both the background theory and applications to structure determination and chemical analysis. It covers rotational, vibrational, electronic, photoelectron and Auger spectroscopy, as well as EXAFS, and the theory of lasers and laser spectroscopy. New material includes laser detection and ranging (LIDAR), cavity ring- down spectroscopy, femtosecond lasers, femtosecond spectroscopy and very high resolution fluorescence of large molecules. In addition the clarity of figures has been greatly improved with some new infrared spectra run by Professor Ben van der Veken at the University of Antwerp especially for this new edition. A revised and updated edition of a successful, clearly written textbook Modern Spectroscopy, Fourth Edition: Includes the latest developments in modern laser techniques. Contains a discussion of molecular symmetry. > Provides numerous worked examples, calculations and questions at the end of chapters. > Has improved the clarity of many of the figures. Written by an author with many years teaching and research experience, Modern Spectroscopy, Fourth Edition will prove invaluable for students of chemistry» physics, and chemical physics studying atomic and molecular spectroscopy, lasers and laser spectroscopy, and molecular symmetry.
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spelling	Hollas, John Michael Verfasser aut Modern spectroscopy J. Michael Hollas 4. ed., reprint. Chichester [u.a.] Wiley 2010 XXVII, 452 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Theorie (DE-588)4059787-8 gnd rswk-swf Molekülspektroskopie (DE-588)4128850-6 gnd rswk-swf Spektroskopie (DE-588)4056138-0 gnd rswk-swf Atomspektroskopie (DE-588)4143333-6 gnd rswk-swf (DE-588)4123623-3 Lehrbuch gnd-content Molekülspektroskopie (DE-588)4128850-6 s DE-604 Atomspektroskopie (DE-588)4143333-6 s Spektroskopie (DE-588)4056138-0 s Theorie (DE-588)4059787-8 s 1\p DE-604 Digitalisierung UB Regensburg application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020495566&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Regensburg application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020495566&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk
spellingShingle	Hollas, John Michael Modern spectroscopy Theorie (DE-588)4059787-8 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Spektroskopie (DE-588)4056138-0 gnd Atomspektroskopie (DE-588)4143333-6 gnd
subject_GND	(DE-588)4059787-8 (DE-588)4128850-6 (DE-588)4056138-0 (DE-588)4143333-6 (DE-588)4123623-3
title	Modern spectroscopy
title_auth	Modern spectroscopy
title_exact_search	Modern spectroscopy
title_full	Modern spectroscopy J. Michael Hollas
title_fullStr	Modern spectroscopy J. Michael Hollas
title_full_unstemmed	Modern spectroscopy J. Michael Hollas
title_short	Modern spectroscopy
title_sort	modern spectroscopy
topic	Theorie (DE-588)4059787-8 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Spektroskopie (DE-588)4056138-0 gnd Atomspektroskopie (DE-588)4143333-6 gnd
topic_facet	Theorie Molekülspektroskopie Spektroskopie Atomspektroskopie Lehrbuch
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020495566&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020495566&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA
work_keys_str_mv	AT hollasjohnmichael modernspectroscopy

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