Nonlinear dynamics with polymers: fundamentals, methods and applications
Gespeichert in:
| Weitere Verfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
Wiley-VCH
2010
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XIII, 254 S. Ill., graph. Darst. |
| ISBN: | 9783527325290 |
Internformat
MARC
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Datensatz im Suchindex
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| adam_text |
Contents
List of Contributors X/
1
Introduction
)
John A. Pojman and
Qui
Tran-Cong-Miyata
1.1
Overview
1
1.2
What Follows
2
1.3
The Future
4
References
4
2
What Is Nonlinear Dynamics and How Does It Relate to Polymers?
5
Irving R. Epstein, John A. Pojman, and
Qui Tran-Cong-Miyata
2.1
Introduction
5
2.2
Nonlinear Dynamics
5
2.3
Some Key Ideas of Nonlinear Chemical Dynamics
6
2.3.1
Chemical Oscillations
7
2.3.2
Waves and Patterns
7
2.3.3
More Complex Phenomena
8
2.4
Polymeric Systems
9
2.4.1
What Is Special about Polymers?
10
2
A.I Challenges
10
2.4.3
Sources of Feedback
10
2.4.4
Nonlinear Dynamics and Phase Separation of Reacting Systems
12
2.4.5
Spatial Structures in Polymeric Systems
13
2.4.6
Approaches to Nonlinear Dynamics in Polymeric Systems
13
2.4.6.1
Oscillations in
a C STR
16
2.5
Conclusions
16
References
16
3
Evolution of Nonlinear Rheology and Network Formation during
Thermoplastic
Polyurethane
Polymerization and Its Relationship to
Reaction Kinetics, Phase Separation, and Mixing
21
I. Sedat
Gums, Changdo Jung, and Sadhan C.
Jana
3.1
Introduction
21
Nonlinear Dynamics with Polymers: Fundamentals, Methods and Applications.
Edited by John A. Pojman and
Qui Tran-Cong-Miyata
Copyright
Є
2010
WILEY-VCH
Verlag
GmbH
&
Co. KGaA,
Weinheim
ISBN:
978-3-527-32529-0
VI
Contents
3.2
Brief Overview of
Evolution
of Nonlinear Rheological Properties
during Polymerization
22
3.2.1
The Relationship between Nonlinear Rheology and the Extent of
Polymerization during the Growth of Linear Chains
22
3.2.2
Relationship between Nonlinear Rheology and the Extent of
Polymerization during the Growth of Nonlinear Chains
24
3.2.3
Chemical Structure of the Monomers and Polymerization Mechanism
in
Polyurethane
Polymerization
25
3.2.4
Evolution of Nonlinear Rheology during
Polyurethane
Polymerization
26
3.2.5
Basic Reactions and Phase Separation Kinetics in Synthesis of
Polyurethanes and Their Relationship to the Evolution of Nonlinear
Rheology
27
3.3
Evolution of Nonlinear Rheology and Network Formation during
Thermoplastic
Polyurethane
Polymerization: Effects of Mixer Design,
Mixing Protocol, Catalyst Concentration, and Timescales
27
3.3.1
Effects of Mixing
29
3.3.1.1
Mechanism of Mixing
29
3.3.1.2
Laminar Mixing under Shear and Extensional Flow with Constant
Shear and Elongation Rates
30
3.3.1.3
Dispersive and Distributive Mixing
30
3.3.1.4
Chaotic Mixing
31
3.3.1.5
Effect of Mixing on Systems Undergoing Chemical Reactions
32
3.3.2
Analysis of Timescale of Mixing and Chemical Reactions during TPU
Polymerization
32
3.3.3
Simultaneous Effects of Mixing, Chemical Reaction, and Molecular
Diffusion on the Evolution of Nonlinear Rheological Properties
36
3.4
Conclusions
38
References
40
4
Frontal Polymerization
45
John A. Pojman
4.1
Introduction
45
4.1.1
Requirements for Frontal Polymerizations
45
4.1.2
Types of Systems
46
4.1.3
Characteristics of Frontal Polymerization
47
4.2
Applications
49
4.2.1
Cure-On-Demand Putty
49
4.2.2
Adhesive
50
4.2.3
Coatings
51
4.3
Motivation for Studying Nonlinear Dynamics with Frontal
Polymerization
5Î
4.4
Convective Instabilities
52
4.4.1
Buoyancy-Driven Convection
52
4.4.2
Effect of Surface-Tension-Driven Convection
55
Contents
VII
4.5
Thermal
Instabilities
56
4.5.1
Effect of Complex Kinetics
57
4.5.2
Effect of Bubbles
58
4.5.3
Effect of Buoyancy
59
4.5.4
Other Factors
59
4.6
Snell's Law
59
4.7
Three-Dimensional Frontal Polymerization
60
4.8
Impact on Applications
61
4.9
Conclusions
62
References
62
5
Isothermal Frontal Polymerization
69
Lydia
L.
Lewis and Vladimir A. Volpert
5.1
Introduction
69
5.1.1
A Comparison between TFP and IFP: Their Mechanisms and Front
Properties
69
5.1.2
Background
71
5.2
Mathematical Models
74
5.3
Experimental IFP
79
5.4
Comparison of Experimental and Mathematical IFP
85
5.5
Conclusions
87
Acknowledgments
88
References
88
6
Reaction-Induced Phase Separation of Polymeric Systems under
Stationary Nonequilibrium Conditions
9]
Hideyuki Nakanishi, Daisuke Fujiki, Dan-Thuy Van-Pham,
and
Qui Tran-Cong-Miyata
6.1
Introduction
91
6.2
Overview of Theoretical Studies on Phase Separation Kinetics of
Nonreactive and Reactive Binary Mixtures
92
6.2.1
Phase Separation of Nonreacting Mixtures
92
6.2.2
Phase Separation of Reacting Mixtures
94
6.3
Chemical Reactions in Polymeric Systems: the Non-Mean-Field
Kinetics
97
6.3.1
Reaction Kinetics in the Bulk State of Polymer
97
6.3.2
Reaction Kinetics in the Liquid State of Polymer Mixtures
98
6.4
Reaction-Induced Elastic Strain and Its Relaxation Behavior
99
6.5
Phase Separation under
Nonuniform
Conditions in Polymeric
Systems
101
6.5.1
Polymers with Spatially Graded Continuous Structures
303
6.5.2
Morphology with Arbitrary Symmetry and Distribution of Length
Scales
105
6.5.2.1
The Computer-Assisted Irradiation Method
105
VIII Contents
6.5.2.2 Polymers
with an Arbitrary
Distribution
of Characteristic Length
Scales
106
6.6
Conclusions
109
Acknowledgments
110
References
110
7
Gels Coupled to Oscillatory Reactions
115
Ryo Yoshida
7.1
Introduction
115
7.2
Design of Self-Oscillating Gel
116
7.3
Self-Oscillating Behaviors of the Gel
117
7.3.1
Self-Oscillation of the Miniature Bulk Gel
117
7.3.2
Control of Oscillating Behaviors
119
7.3.3
Peristaltic Motion of Gels with Propagation of Chemical Wave
119
7.3.4
Self-Oscillation with Structural Color Changes
121
7.4
Design of Biomimetic Micro-ZNanoactuator Using Self-Oscillating
Polymer and Gel
122
7.4.1
Self-Walking Gel
122
7.4.2
Mass Transport Surface Utilizing Peristaltic Motion of Gel
124
7.4.3
Microfabrication
of Self-Oscillating Gel for
Microdevices 124
7
ЛА
Control of Chemical Wave Propagation in Self-Oscillating Gel
Array
126
7.4.5
Self-Oscillating Polymer Chains as "Nano-Oscillators"
127
7.4.6
Self-Flocculating/Dispersing Oscillation of
Microgels
128
7'.4.7
Fabrication of
Microgel
Beads Monolayer
129
7.4.8
Attempts of Self-Oscillation under Physiological
Conditions
131
7.5
Conclusion
132
References
132
8
Self-Oscillating Gels as Biomimetic Soft Materials
135
Olga
Kuksenok, Victor V. Yashin, Pratyush Dayal, and Anna
С
Balázs
8.1
Introduction
135
8.2
Methodology
137
8.2.1
Continuum Equations
137
8.2.2
Formulation of the Gel Lattice Spring Model (gLSM)
140
8.3
Sensitivity to Mechanical Deformation
143
8.3.1
Capturing Effects of Local Mechanical Impact on Homogeneous BZ
Gels
143
8.3.2
Straining Heterogeneous BZ Gels
147
8.4
Sensitivity to Light
154
8.5
Conclusions
160
Acknowledgments
160
References
161
Contents
IX
9 Chemoelastodynamics
of Responsive Gels
163
Jacques Boissonade, Pierre Borckmans, Patrick De Kepper,
and
Stéphane
Metern
9.1
I
ntroduction 163
9.2 Elastodynamics
of Responsive
Gels:
a
Brief
Survey 1
64
9.3
Oscillatory
Gel Dynamics
Using an Oscillating Chemical
Reaction
166
9.3.1
The Approach
166
9.3.2
Coupling to the Oscillating Belousov-Zhabotinsky Reaction
169
9.3.3
Numerical Integration Results
171
9.4
Chemodynamic Oscillations Induced by Geometric Feedback
174
9.4.1
Spatial Bistability and Related Chemomechanical Instabilities
174
9.4.2
Simple Models
175
9.4.3
A More Realistic Model: The Polyelectrolyte Model
177
9.5
Experimental Observations
181
9.5.1
Experimental Results
182
9.5.1.1
Case of the Chlorite-Tetrathionate Reaction
182
9.5.1.2
Case of the Bromate-Sulfite Reaction
184
9.6
Conclusions and Perspectives
285
References
186
10
Oscillatory Systems Created with Polymer Membranes
189
Ronald A.
Siegel
10.1
Introduction
189
10.2
Survey of Synthetic Membrane Oscillators
191
10.2.1
Teorell Oscillator
191
10.2.2
Polyelectrolyte Membrane-Based Oscillators
193
10.2.3
Thermofluidic Oscillator
194
10.2.4
Lipid/Organic Membrane Analogs
296
10.2.5
Membrane/Enzyme Oscillators
296
10.2.6
General Discussion
198
10.3
Hydrogel-Enyzme Oscillator for Rhythmic Hormone
Delivery
299
10.3.1
General Scheme
200
10.3.2
Bistability of Hydrogel Membrane Permeability
202
10.3.3
Oscillator Operation
204
10.3.4
Oscillator Prototype
205
10.3.5
Analysis of Factors Affecting Oscillations Over Time
207
10.3.6
Tuning
pH
Range of Oscillations
208
10.3.7
Discussion and Conclusion
211
Acknowledgments
222
References
222
Further Reading
227
X Contents
11
Structure Formation in Inorganic Precipitation Systems
219
Oliver
Steinbock
and Jason
Pagano
11.1
Introduction
219
11.2
Permanent Patterns from Inorganic Precipitation and Deposition
Processes
220
11.3
Tube Formation in Precipitation Systems and Silica Gardens
221
11.4
Historic and Cultural Links
222
11.5
Some Recent Developments
223
11.6
Experimental Methods
224
11.7
Growth Regimes
225
11.8
Wall Composition and Morphology
228
11.9
Relaxation Oscillations
230
11.10
Radius Selection
233
11.11
Bubbles as Templates
235
11.12
Toward Applications
237
11.13
Outlook and Conclusions
238
Acknowledgments
239
References
239
Index
243 |
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| spellingShingle | Nonlinear dynamics with polymers fundamentals, methods and applications Phasenumwandlung (DE-588)4132140-6 gnd Nichtlineare Dynamik (DE-588)4126141-0 gnd Polymere (DE-588)4046699-1 gnd |
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| title | Nonlinear dynamics with polymers fundamentals, methods and applications |
| title_auth | Nonlinear dynamics with polymers fundamentals, methods and applications |
| title_exact_search | Nonlinear dynamics with polymers fundamentals, methods and applications |
| title_full | Nonlinear dynamics with polymers fundamentals, methods and applications ed. by John A. Pojman and Qui Tran-Cong-Miyata |
| title_fullStr | Nonlinear dynamics with polymers fundamentals, methods and applications ed. by John A. Pojman and Qui Tran-Cong-Miyata |
| title_full_unstemmed | Nonlinear dynamics with polymers fundamentals, methods and applications ed. by John A. Pojman and Qui Tran-Cong-Miyata |
| title_short | Nonlinear dynamics with polymers |
| title_sort | nonlinear dynamics with polymers fundamentals methods and applications |
| title_sub | fundamentals, methods and applications |
| topic | Phasenumwandlung (DE-588)4132140-6 gnd Nichtlineare Dynamik (DE-588)4126141-0 gnd Polymere (DE-588)4046699-1 gnd |
| topic_facet | Phasenumwandlung Nichtlineare Dynamik Polymere Aufsatzsammlung |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3474332&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=020464227&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT pojmanjohna nonlineardynamicswithpolymersfundamentalsmethodsandapplications AT trancongmiyataqui nonlineardynamicswithpolymersfundamentalsmethodsandapplications |