Environmental surfaces and interfaces from the nanoscale to the global scale:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Hoboken, NJ
Wiley
2009
|
| Schlagworte: | |
| Online-Zugang: | Cover Inhaltsverzeichnis |
| Beschreibung: | XVII, 441 S. Ill., graph. Darst. |
| ISBN: | 9780470400364 |
Internformat
MARC
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| 100 | 1 | |a Maurice, Patricia A. |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Environmental surfaces and interfaces from the nanoscale to the global scale |c Patricia A. Maurice |
| 264 | 1 | |a Hoboken, NJ |b Wiley |c 2009 | |
| 300 | |a XVII, 441 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 650 | 4 | |a Surface chemistry | |
| 650 | 4 | |a Environmental chemistry | |
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Datensatz im Suchindex
| _version_ | 1804140019933249536 |
|---|---|
| adam_text | CONTENTS
Preface
xv
Constants and Units
xvii
Periodic Table of the Elements
1
Some Fundamental Chemical Thermodynamic and Kinetic Concepts
1
Concentration Units,
1
Thermodyamic Versus Kinetic Approaches,
2
Introductory Thermodynamics,
3
Gibbs Energy,
4
Chemical Potential and Activity,
4
Equilibrium Constants,
5
Calculating the Equilibrium Constant from Gibbs Energy Changes,
6
Temperature Effects on
К«,,
8
Calculating Activities,
9
Saturation Indices (Sis),
12
Carbonate Equilibria in Open or Closed Systems,
13
Calcite
Equilibria in a System Open to Atmospheric Carbon Dioxide,
14
Redox
Reactions,
17
Metal Speciation Diagrams,
19
A Brief Introduction to Kinetics,
20
Overall Versus Elementary Reactions,
20
Molecularity and Reaction Order,
21
Transition State Theory and
thé Arrhenius
Equation,
24
Michaelis-Menten Kinetics,
25
The Elovich Equation for Chemisorption Kinetics,
26
Simultaneous Versus Sequential Reaction Sequences,
27
Transport Versus Surface Control of Mineral Growth and Dissolution
Rates,
28
vii
viii CONTENTS
Rate Laws for Surface-Controlled Mineral Growth and Dissolution,
30
Equilibration Time in Porous Media,
31
Questions for Further Thought,
31
Further Reading,
34
2
The
Hydrologie
Cycle as Context for Environmental Surfaces and Interfaces
35
The Structure and Fundamental Properties of Water,
35
The Chemical Composition of the Earth,
37
The Critical Zone,
38
The
Hydrologie
Cycle,
38
Oceans,
39
Atmosphere,
40
Underground water,
43
Soils and Soil Water,
44
Groundwater,
45
Surface Waters: Focus on Rivers,
52
Stream Load,
52
Gibbs Plots,
54
The Hyporheic Zone,
56
The OTIS Model and Solute Transport in Streams,
56
Particle Transport and Sedimentation,
57
Water Budgets and Chemical Fluxes in Terrestrial Ecosystems,
59
Questions for Further Thought,
62
Further Reading,
66
3
Some Minerals of Special Interest to Environmental Surface Chemistry
67
Gibbsite,
67
Quartz,
68
Kaolinite,
69
Smectite: Example Montmorillonite,
71
Fe(hydr)oxides,
73
Hematite,
73
Goethite,
73
Lepidocrocite,
76
Magherniţe,
77
Ferrihydrite,
77
Magnetite,
77
Manganese Oxides,
77
Calcite,
78
Feldspars,
79
Zeolites,
79
Questions for Further Thought,
81
Further Reading,
81
4
Some Key Techniques for Investigating Surfaces and Interfaces
82
A Brief Overview of Some Commonly Used Techniques,
82
In-Depth Descriptions of Some Key Techniques,
86
Scanning Electron Microscopy
(SEM),
86
CONTENTS ix
Transmission Electron
Microscopy
(ТЕМ),
87
Scanning Tunneling Microscopy (STM),
90
Case Study: Imaging Parameters and High-Resolution Imaging of
Hematite,
91
AFM and
Interfacial
Forces,
92
Х
-Ray Photoelectron Spectroscopy (XPS),
99
BET Surface Area Measurements,
100
Some Synchrotron-Based Techniques,
103
Microscopies for
Biofilm
Imaging,
108
Questions for Further Thought,
108
Further Reading, 111
5
Surfaces and Interfaces
112
What is a Surface? What is an Interface?,
112
The Challenges of Defining Surfaces and Interfaces,
113
Surfaces are Complex,
114
Relaxation and Reconstruction,
114
Surface Sites,
115
Surface Microtopography,
116
Surface Free Energy,
117
Water Near Surfaces,
119
Dynamic Surfaces,
120
Bacterial Substrates,
120
Fractal Properties of Surfaces and Environmental Particles,
120
Interdisciplinary Topic of Study,
123
Surface Free Energy and Surface Excess,
124
Surface Tension and Related Phenomena,
126
Surfactants and Micelles,
126
Contact Angle,
127
The Young-Laplace Equation,
128
Meniscus and Capillarity,
128
The Gibbs Equation,
130
Some Approaches to Surface and Interface Modeling,
130
Case Study: Bacteria-Mineral-Gas Interactions in the
Vadose Zone,
132
Questions for Further Thought,
133
Further Reading,
135
6
The Charged Interface and Surface Complexation
136
Some Evidence for Surface Charge,
136
Sources of Mineral Surface Charge,
137
Points of Zero Charge,
139
Case Study: The Surface Charge Properties of Kaolinitic Soils,
140
Sorption
Terminology,
141
Cation Exchange Capacity,
145
Sorption
Isotherms,
148
Adsorption Isotherm Equations,
151
The Langmuir Isotherm Equation,
151
The
Freundlich
Isotherm Equation,
152
The Frumkin Isotherm Equation,
153
χ
CONTENTS
The Double Layer, Gouy-Chapman Theory,
153
Beyond Gouy-Chapman: Surface Complexation Models,
155
Constant Capacitance Model (CCM),
161
The Diffuse Double Layer (DDL) Model,
161
Triple Layer Model (TLM),
161
Charge Distribution CD/MUSIC Model,
162
Model Verification and Validation,
163
Case Study: Incorporating the Work Associated with Removal of Water
During Adsorption into the TLM,
164
DĽVO
Theory and Colloid Attachment in Porous Media,
165
Questions for Further Thought,
168
Further Reading,
172
7 Sorption:
Inorganic Cations and Anions
173
A Typical
Sorption
Experiment Design,
174
Metal Cation
Sorption, 176
The Complexity of Cation Adsorption,
179
Inorganic
Anion
Adsorption,
183
Phosphate Adsorption,
184
Nitrate Adsorption,
186
Sulfate
Adsorption,
186
Carbonate
Sorption, 186
Importance of
Redox
State and Valence to Inorganic Ion Adsorption,
187
Chromium,
187
Neptunium,
188
Uranium,
188
Selenium,
188
Case Study: Arsenic Speciation and Mobility,
189
Questions for Further Thought,
192
Further Reading,
193
8 Sorption:
Organic Compounds
194
A Brief Introduction to Organic Chemistry,
195
Some Organic Compounds of Interest in Environmental Surface
Chemistry,
200
Polymers,
200
Organic Surfactants, Including Fatty Acids,
200
Humic Substances,
201
Polycyclic Aromatic Hydrocarbons (PAHs),
202
Substituted Nitrobenzenes (SNBs),
204
Volatile Organic Compounds (VOCs),
205
Sorption
of Simple Organic Ligands, Surfactants, and Natural Organic
Matter,
205
Adsorption of Simple Organic Ligands,
205
Adsorption of
Anionie
Surfactants, Fatty Acids,
207
Sorption
of Cationic Surfactants,
208
Sorption
of Phospholipid Surfactants:
Biomedical
Implications,
209
Adsorption of Humic And Fulvic Acids
(NOM),
210
CONTENTS xi
Metal-Ligand Coadsorption:
Ternary Surface Complexes,
214
Sorption
of Some Organic Pollutants,
215
Vapor Pressure, Solubility, and Density,
215
The
Octanol-
Water Partition Constant, Kow,
218
Organic Fuel and Solvent Leaks: Volatilization, Solubility, Density,
and K0VI,
219
The Hammett Constant
σ
for Substituted Aromatic Acids Based on
the Benzene Ring,
220
Case Study:
Sorption
of SNBs,
221
Molecular Dynamics (MD) Modeling of Atrazine Absorption,
223
The
K¿
Approach to
Hydrophobie
Organic Compound Transport in
Porous Media,
224
Activated Carbon and
Sorption
of VOCs,
226
Questions for Further Thought,
227
Further Reading,
230
9
Mineral Nucleation and Growth
231
Saturation State and Mineral Nucleation: An Example of the
Confluence of Thermodynamics and Kinetics,
231
Hydroxypyromorphite Nucleation,
233
Heterogeneous Nucleation and Epitaxial Growth,
233
From Nucleation to Growth,
236
Ostwald Ripening,
236
Transport and Surface Controlled Growth,
236
The Special Importance of Kink Sites,
237
BCF Theory,
238
Growth Mode and Driving Force,
240
Case Study:
Calcite
Birth and Spread versus Spiral Growth: BCF
Theory,
241
Rates of Step Advancement,
242
Impurities and Growth at Steps,
245
Monte Carlo Simulations of Crystal Growth,
246
Biomineralization,
247
Carbonate Precipitation in the Marine Environment,
249
Questions for Further Thought,
251
Further Reading,
252
10
Mineral Weathering and Dissolution
253
Chemical, Physical, and Biological Weathering,
253
Thermodynamics of Mineral Weathering,
256
Kinetics of Mineral Dissolution,
260
Etch Pit Formation,
261
Oxalate Promoted Dissolution of Hematite,
263
Comparison of Laboratory-and Field-Based Dissolution Rates,
264
Reactive Surface Area and Feldspar Dissolution,
266
Rainfall and Weathering: An Example from the Hawaiian Islands,
269
Case Study: Weathering in die Antarctic Dry Valleys,
270
ні
CONTENTS
Reactors for Dissolution Experiments,
273
The Use of Radiogenic Isotopes in Weathering Studies,
276
Questions for Further Thought,
276
Further Reading,
279
11
Plants as Environmental Surfaces
280
Ecohydrology and Soil Moisture Balance,
280
Some Notes on Angiosperm Physiology,
282
The Nutrient Needs of Plants,
282
Effects of Plants on Mineral Dissolution and Weathering,
284
Modes of Plant Elemental Cycling,
287
Plants and Biomineralization: Phytoliths,
287
Plants and Formations in Limestone Caves,
289
Phytoremediation as an Example of Plant-Mineral-Contaminant
Interactions,
291
Case Study: Phytoremediation of Atrazine,
293
Questions for Further Thought,
294
Further Reading,
295
12
Microorganisms As Environmental Surfaces
296
How Microorganisms make a Living ,
298
Metabolic Pathways,
298
Microbial
Redox
Reactions and Michaelis-Menten Kinetics,
303
Microbial Temperature Ranges and Extremophiles,
305
Microbial Growth Curves,
306
Bacterial Groups,
307
Bacterial Cell Walls,
307
Bacterial Adhesion and
Biofilms,
309
Bacterial-Metal Interactions,
312
Bacterial-Promoted Mineral Dissolution,
313
Dissolution of Fe(in)(hydr)oxides by DIRB,
313
Dissimilatory Metal-Reducing Bacteria,
315
Microbial Effects on Carbonate Dissolution,
315
The Importance of Field-Based Studies,
317
Case Study: The In Situ Microcosm Approach,
318
Coupling In Situ Microcosms with Community Analysis,
318
Siderophores,
320
Microbial Biomineralization,
322
Carbonate Precipitation,
322
Fe(III)(hydr)oxide Precipitaton: BIOS,
323
Banded Iron Formations (BIF),
324
(Alumino)silicate Precipitation,
326
Case Study:
Bioremediatìon
of
U
at the Oak Ridge National Laboratory
Site,
327
Microbial Fuel Cells,
329
Questions for Further Thought,
332
Further Reading,
333
CONTENTS xlii
13
Environmental Nanoscience and Nanotechnology
335
What is a Nanoparticle?,
335
Nanoparticle Occurrence and Distribution,
337
What Makes a Nanoparticle Different?,
339
Nanoparticle Surface Area, Stability, and Reactivity,
340
Nanoparticles Have a Different Electronic Structure,
340
How Electronic Structure Influences Nanoparticle Behavior,
342
Nanoparticle Disorder and Defect Structures,
343
Ferrihydrite Size, Structure, and Stability,
343
Effects of
pH
and Adsorbed Ions on Nanoparticle Stabilities,
344
Case Study: Fe(hydr)oxide Size and Stability,
345
Secondary Growth of Nanoparticles,
346
Self-Assembly and Templating,
348
Nanoparticle Transport in Porous Media,
348
The Emergence of Nanotechnology,
350
Potential Environmental Effects of Engineered Nanoparticles,
351
Questions for Further Thought,
353
Further Reading,
354
14
The Big Picture: Interface Processes and the Environment
356
Reactive Transport Models for Metals and Radionuclides in Porous
Media,
356
The K<j Approach Encounters Difficulties for Metals and
Radionuclides,
356
Comparison of the Kd versus Surface Complexation Modeling
Approaches,
357
Acid Rain Effects on Chemical Weathering,
358
What Makes Rainfall Acidic?,
359
Effects of Acid Rain,
360
Acid Rain and Chemical Weathering,
360
The Small Watershed Approach,
362
NETPATHandPHREEQC,
362
The Clean Air Act and Acid Rain Over Time,
363
Acid Mine Drainage,
364
The Environmental Problem,
365
Nanoparticles and AMD,
365
Hydrobiogeochemical and Photoreductive Processes,
365
Biofilms
and AMD,
367
Potential Remediation Strategies,
369
Environmental Particles and Climate Change,
369
Climate Forcing and Feedbacks,
370
Volcanoes and Climate,
373
CO2 and Weathering,
374
Modeling the
С
Cycle Over Geologic Tune,
376
Scaling Phenomena: Integrating Observations from the Atomic to the
Watershed to the Global Scale,
378
The Concept of the
Macroscope,
378
xiv CONTENTS
Embedded
Sensor Network Systems, 379
Sensors
for Surface and
Interface
Phenomena,
380
New
Opportunities: New Challenges,
380
Questions for Further Thought,
381
Further Readings,
383
Glossary of Terms
385
References
405
Index
437
|
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| id | DE-604.BV035736583 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T21:53:20Z |
| institution | BVB |
| isbn | 9780470400364 |
| language | English |
| lccn | 2008045483 |
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| spelling | Maurice, Patricia A. Verfasser aut Environmental surfaces and interfaces from the nanoscale to the global scale Patricia A. Maurice Hoboken, NJ Wiley 2009 XVII, 441 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Surface chemistry Environmental chemistry Oberflächenchemie (DE-588)4126166-5 gnd rswk-swf Natur (DE-588)4041358-5 gnd rswk-swf Grenzflächenchemie (DE-588)4246080-3 gnd rswk-swf Natur (DE-588)4041358-5 s Grenzflächenchemie (DE-588)4246080-3 s DE-604 Oberflächenchemie (DE-588)4126166-5 s DE-576;wiley image/jpeg http://swbplus.bsz-bw.de/bsz309092639cov.htm 20090729213000 Cover Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=018013074&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Maurice, Patricia A. Environmental surfaces and interfaces from the nanoscale to the global scale Surface chemistry Environmental chemistry Oberflächenchemie (DE-588)4126166-5 gnd Natur (DE-588)4041358-5 gnd Grenzflächenchemie (DE-588)4246080-3 gnd |
| subject_GND | (DE-588)4126166-5 (DE-588)4041358-5 (DE-588)4246080-3 |
| title | Environmental surfaces and interfaces from the nanoscale to the global scale |
| title_auth | Environmental surfaces and interfaces from the nanoscale to the global scale |
| title_exact_search | Environmental surfaces and interfaces from the nanoscale to the global scale |
| title_full | Environmental surfaces and interfaces from the nanoscale to the global scale Patricia A. Maurice |
| title_fullStr | Environmental surfaces and interfaces from the nanoscale to the global scale Patricia A. Maurice |
| title_full_unstemmed | Environmental surfaces and interfaces from the nanoscale to the global scale Patricia A. Maurice |
| title_short | Environmental surfaces and interfaces from the nanoscale to the global scale |
| title_sort | environmental surfaces and interfaces from the nanoscale to the global scale |
| topic | Surface chemistry Environmental chemistry Oberflächenchemie (DE-588)4126166-5 gnd Natur (DE-588)4041358-5 gnd Grenzflächenchemie (DE-588)4246080-3 gnd |
| topic_facet | Surface chemistry Environmental chemistry Oberflächenchemie Natur Grenzflächenchemie |
| url | http://swbplus.bsz-bw.de/bsz309092639cov.htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=018013074&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT mauricepatriciaa environmentalsurfacesandinterfacesfromthenanoscaletotheglobalscale |