Resonance radiation and excited atoms:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Cambridge [u.a.]
Cambridge Univ. Press
1971 [erschienen] 2009
|
| Ausgabe: | Digitally printed version, [Nachdr. der Ausg. Cambridge, 1934] |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XVI, 338 S. graph. Darst. |
| ISBN: | 9780521114820 9780521084338 |
Internformat
MARC
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| 100 | 1 | |a Mitchell, Allan C. G. |d 1902-1963 |e Verfasser |0 (DE-588)134043987 |4 aut | |
| 245 | 1 | 0 | |a Resonance radiation and excited atoms |c by Allan C. G. Mitchell and Mark W. Zemansky |
| 250 | |a Digitally printed version, [Nachdr. der Ausg. Cambridge, 1934] | ||
| 264 | 1 | |a Cambridge [u.a.] |b Cambridge Univ. Press |c 1971 [erschienen] 2009 | |
| 300 | |a XVI, 338 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 650 | 4 | |a Radiation | |
| 650 | 4 | |a Fluorescence | |
| 650 | 4 | |a Atoms | |
| 650 | 4 | |a Atoms | |
| 650 | 4 | |a Fluorescence | |
| 650 | 4 | |a Radiation | |
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| 700 | 1 | |a Zemansky, Mark W. |e Verfasser |4 aut | |
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Datensatz im Suchindex
| _version_ | 1804139334573490176 |
|---|---|
| adam_text | CONTENTS
Chapter I
INTRODUCTION
1.
Genebal
Remarks page I
2.
Introduction to Line Spectra
2
a. Characteristics of Line Spectra
2
b. Energy Level Diagrams
8
с
Metastable States
10
d. Notion of Mean Life of an Excited State
10
3.
Remarks on Fluorescence
11
4.
Qualitative Investigations of Resonance
Radiation and
Lene Fluorescence
14
а. Resonance Radiation
14
б.
Resonance Radiation and Line Fluorescence
16
5.
Sources for Exciting Resonance Radiation
20
а. Arcs without Foreign Gas
21
б.
Arcs with Stationary Foreign Gas
22
e. Arcs with Circulating Foreign Gas
25
β.
Resonance Lamps
28
7.
Resonance Radiation and Specular Reflec¬
tion in Mercury Vapour
31
8.
Hyperftne Structure of Line Spectra
34
9.
Investigations on the Hyperfine Structure
of Resonance Radiation
39
CONTENTS
Chapter
Π
PHYSICAL AND CHEMICAL EFFECTS CON¬
NECTED WITH RESONANCE RADIATION
Stbpwisb Radiation
а. Mercury 4*
б.
Effect of Admixture of Foreign Gases
47
с ТЪе
Appearance of the Forbidden Line
2656
(б^-б*?,)
52
â.
The Hyperfine Structure of Stepwise Radiation
52
e. Cadmium and Zinc
54
2.
Production of Spbctba by Collision with
Excited Atoms: Sensitized
Fluorescence
56
α.
The Principle of Microscopic Reversibility
56
6.
Efficiency of
Collisione
of the Second Kind between Atoms
and Electrons
57
e. Collisions of the Second Kind between Two Atoms
59
d. Sensitized Fluorescence
59
e. Effect of MetaeUble Atoms
65
ƒ.
Efficiency of Collisions of the Second Kind between Atoms
ββ
д.
Conservation of Spin Angular Momentum in Collisions of
the Second Kind
69
3.
Interaction of Excited Atoms with Mole¬
cules. Chemical Reactions taking place in
the Presence of Optically Excited Atoms;
Sensitized Band Fluorescence
71
a. Introduction
71
b. Reactions taking place in the Presence of Excited
Mercury Atoms
71
е. The Mechanism of the Activation of Hydrogen by Excited
Mercury Atoms
76
d. Reactions involving Hydrogen
81
t. The Sensitized Formation of Ozone
82
ƒ.
The Sensitized Decomposition of Ammonia
83
g. Other Decompositions sensitized by Excited Mercury
Atoms
85
λ.
Reactions sensitized by other Metallic Vapours activated
by the Absorption of Resonance Radiation
86
4.
Bands Connected with Resonance Lines
87
a. Mercury-Rare Gas Bands
87
b.
Continua
apparently associated with Resonance
Lines 88
CONTENTS
ХІ
Chapter
III
ABSORPTION
LINES
AND MEASURE¬
MENTS OF THE LIFETIME OF THE
RESONANCE STATE
1.
General Properties of Absorption Lines page
92
a. The Notion of an Absorption Line
92
b. The Einstein Theory of Radiation
93
с
The Relation between /-value and Lifetime
96
2.
The Absorption Coefficient of a Gas
97
a. Expression for the Absorption Coefficient
97
b. Characteristics of an Absorption Line with a Small
Natural Damping Ratio
101
с
The Central Region of the Line
102
d. The Edges of the Line
103
3.
Emission and Diffusion of Resonance Radia¬
tion
106
а. Emission Characteristics of a Resonance Lamp
106
б.
Methods of Measuring Lifetime
110
e. Resonance Lamp with Electrical Cut-Off
110
d. Resonance Lamp with Optical Cut-Off 111
e. Atomic Ray Optically Excited
114
ƒ.
Canal Ray
116
g. Absolute Intensity of a Resonance Line
115
4.
Absorption within and at the Edges of a
Resonance Line
116
a. Area under the Absorption Coefficient
116
b. Absorption Coefficient at the Centre of a Resonance Line
117
c. Method of
Ladenburg
and
Reiche 118
d.
Method in which E,
-
С
exp
-
(^
t.
Measurements on Simple Lines
123
ƒ.
Absorption of a Number of Separate Simple Lines of
Different Intensities
124
g. Absorption of a Line with Overlapping Components
126
A. Absorption of a Gas in a Magnetic Field
127
i. Absorption Coefficient at the Edges of a Resonance Line
128
j. Total Energy Absorbed from a Continuous Spectrum by a
Resonance Line that is not Completely Resolved
130
xu contents
5. Magneto-Rotation
at the Edges of a Reso¬
nance Line
1Ще
133
а. Magneto-Rotation at the Edges of a Resolved Resonance
Line
133
б.
Magneto-Rotation and Absorption of a Resonance Line
that is not Completely Resolved
135
6.
Dispersion at the Edges of a Resonance Line
139
а. General Dispersion Formula
139
б.
Normal Dispersion of an Unexcited Gas very far from the
Absorption Lines
14°
с
Anomalous Dispersion of an Unexcited Gas at the Edges of
a Resonance Line
141
d. Anomalous Dispersion of a Strongly Excited Gas at the
Edges of the Absorption Lines A^
144
7.
Tables of Lifetimes and Discussion
145
а. Summary of Methods of Measuring Lifetime and Tables
of Lifetimes
145
б.
Discussion of Tables
146
e. Electron Excitation Functions
149
d. The
Pauli-Houston
Formula
160
e. Higher Series Members of the Alkalies
151
Chapter IV
COLLISION PROCESSES INVOLVING
EXCITED ATOMS
1.
Types of Collision Processes
154
a. The Meaning of Collision
154
b. The Meaning of
Effective
Cross-Section
165
с
Collisions of the Second Kind
156
d. Perturbing Collisions
156
2.
Classical Theory of
Lorentz
Broadening of
an Absorption Line
158
а. The Phenomenon of
Lorentz
Broadening
158
б.
The Simple
Lorentz
Theory
169
e. Combination of Lorentz,Natural, and Doppkx Broadening
160
CONTENTS Xiii
3.
Experiments on
Lorentz
Broadening page
162
α.
Photographic Measurements
162
б.-
Measurements involving Magneto-Rotation
164
с
Experimente
on the Absorption of Resonance Radiation
165
d. Evaluation of Effective Cross-Sections for
Lorentz
Broadening
170
e.
Lorentz
Broadening in a Sodium Flame
170
ƒ.
The Shift of the Absorption Line
174
g. The Asymmetry in Broadening
174
4.
Quantum Theory of
Lorentz
Broadening
175
а. Preliminary Theories
175
б.
Weisskopf s Theory
177
c. Lenz s Theory
179
5.
Holtsmark
Broadening
183
6.
Early Measurements of the Quenching of
Resonance Radiation
187
а. Quenching of Resonance Radiation by Foreign Gases
187
б.
Experiments of Stuart with Mercury
188
c. Experiments with Sodium and Cadmium
189
Ί.
Difficulty of interpreting Early Experiments
190
7.
Theory of the Quenching Curve from an
Ideal Resonance Lamp
191
а. The Stern-
Volmer
Formula
191
б.
Effect of
Lorentz
Broadening on Quenching
193
8.
Radiation Diffusion and Quenching
196
a. Milne s Theory
196
ft. Use of Mime s Theory to study Quenching
197
c. Equivalent Opacity at Low Pressure
200
d. Derivation of a Theoretical Quenching Curve
201
e. Experimental Determinations of Quenching Cross-Sections
202
9.
Collisions of Excited Atoms produced by
Optical Dissociation
204
a. The Optical Dissociation of
Nal
204
ft. Experimental Results
205
e. Evaluation of Effective Cross-Sections
206
10.
Other Collision Processes
213
«.
Collisions involving the Sodium Transition 2Pj, |
-*
2P|,
j
213
b. Collisions connected with Photo-ionization
215
<·.
Collisions involving the Enhancement of Spark Lines
217
xiv
contents
11.
Theoretical Interpretation of Quenching
Collisions page
218
a. General Principles
218
b. Enhancement of Copper and Aluminium Ionic Levels
220
c. Energy Interchange with Molecules
221
d. Collisions with Excited Mercury Atoms
223
e. Collisions with Excited Cadmium Atoms
225
ƒ.
Collisions with Excited Sodium Atoms
226
g.
Collisione
with Excited Thallium Atoms
228
12.
Rapidity of Escape of Diffused Resonance
Radiation from a Gas
228
а. Experiments with Mercury Vapour at Low Pressures
228
б.
Mime s Theory
230
c. Experiments with Mercury Vapour at Higher Pressures
232
d. Equivalent Opacity at High Pressure
233
13.
Diffusion and Collisions of Metastable
Atoms
236
o. Early Work
236
6.
Theory of Measurement with Inert Gases
237
с
Experimental Results with Neon, Argon, and Helium
240
d. Theoretical Interpretation of Results with Inert Gases
245
«.
Methods of studying Metastable Mercury Atoms in
Nitrogen
250
ƒ.
Results and their Interpretation with Metastable Mercury
Atoms in Nitrogen
252
g. Metaetable Mercury Atoms in Mercury Vapour
253
λ.
The Simultaneous Production and Destruction of Meta¬
stable Atoms
254
Chapter V
THE POLARIZATION OF RESONANCE
RADIATION
1.
Introduction
258
2.
General Description of Apparatus for
Polarization Work
258
3.
Hanle s Experiments on Mercury Vapour
262
CONTENTS
XV
4.
Theory of Hanle s Experiments page
264
а. Classical Theory
264
б.
Quantum Theory of Polarization and the
Zeeman
Effect 2C7
5.
Experimental Verification of Magnetic
Depolarization and Angle of Maximum
Polarization in the Case of Mercury
270
6.
Polarization of Sodium Resonance Radia¬
tion
:
Breakdown of Classical Theory
272
a. Experimental Results on the Polarization of Sodium
Resonance Radiation
272
The
Zeeman
Levels for Sodium; Van Vleck s Formulas for
Polarization
272
e. Further Comparison of Experiment with Theory
276
7.
Polarization of Lines of other Elements:
Mean Lives of Several Excited States
278
а. Resonance Lines
278
б.
Line Fluorescence
280
8.
Effect of Hyperfine Structure on the
Polarization of Resonance Radiation
283
а. Detailed Experimental Investigation of the Polarization
of Mercury Resonance Radiation
283
б.
Theory of the Effect of Hyperfine Structure on the
Polarization of Resonance Radiation
285
c. Theory of the Effect of Hyperfine Structure on the
Polarization of Line Fluorescence
290
d. Comparison of Experiment with Present Theory of
Polarization
291
e. Effect of Hyperfine Structure on Magnetic Depolarization
and the Angle of Maximum Polarization
296
ƒ.
Effect of Large Magnetic Fields; Paschen-Back Effect of
Hyperfine Structure
301
9.
Stepwise Radiation
304
a. Polarization of Stepwise Radiation
304
b. Mean Life of the 73S1 State of Mercury
307
10.
Depolarization by Collision
308
11.
Effect of Electric Fields on Resonance
Radiation
312
а. Measurements on Frequency (Stark Effect)
312
б.
Measurements on Polarization
314
XVI
CONTENTS
APPENDIX
I. Absorption Coefficient of a Gas page
319
П.
Value of
-
Ѓ
.
Є~?ІУ
>.
for small values of a
321
III. Line Absorption
Л,.
322
IV. The Absorption A*
323
V. The Function
8 324
VI. The Absorption
Α ^γ
324
VII.
Kuhn
β
Theory of Magneto-Rotation
325
VIII.
Effect of Hyperfine Structure on the Value of
χ,
327
-
f°
-
IX. Value of
-
f°
-
T^*
Ч
ÍOT • «e
value8 of a 328
j
О**
+
(
)*
T
+
(ω
-
у)
X. Diffused Transmitted Resonance Radiation
330
XI. Samson s Equivalent Opacity
330
XII.
Kenty s Equivalent Opacity
331
ΧΙΠ.
Polarization of Resonance Radiation excited by Unpolarized
Light
331
Index
335
|
| any_adam_object | 1 |
| author | Mitchell, Allan C. G. 1902-1963 Zemansky, Mark W. |
| author_GND | (DE-588)134043987 |
| author_facet | Mitchell, Allan C. G. 1902-1963 Zemansky, Mark W. |
| author_role | aut aut |
| author_sort | Mitchell, Allan C. G. 1902-1963 |
| author_variant | a c g m acg acgm m w z mw mwz |
| building | Verbundindex |
| bvnumber | BV035649421 |
| classification_rvk | UM 2200 |
| ctrlnum | (OCoLC)316824278 (DE-599)BVBBV035649421 |
| dewey-full | 535.3 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 535 - Light and related radiation |
| dewey-raw | 535.3 |
| dewey-search | 535.3 |
| dewey-sort | 3535.3 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| edition | Digitally printed version, [Nachdr. der Ausg. Cambridge, 1934] |
| format | Book |
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| id | DE-604.BV035649421 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T21:42:26Z |
| institution | BVB |
| isbn | 9780521114820 9780521084338 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-017704050 |
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| owner_facet | DE-703 |
| physical | XVI, 338 S. graph. Darst. |
| publishDate | 1971 |
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| publisher | Cambridge Univ. Press |
| record_format | marc |
| spelling | Mitchell, Allan C. G. 1902-1963 Verfasser (DE-588)134043987 aut Resonance radiation and excited atoms by Allan C. G. Mitchell and Mark W. Zemansky Digitally printed version, [Nachdr. der Ausg. Cambridge, 1934] Cambridge [u.a.] Cambridge Univ. Press 1971 [erschienen] 2009 XVI, 338 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Radiation Fluorescence Atoms Resonanzstrahlung (DE-588)4177860-1 gnd rswk-swf Atom (DE-588)4003412-4 gnd rswk-swf Spektroskopie (DE-588)4056138-0 gnd rswk-swf Resonanzstrahlung (DE-588)4177860-1 s Atom (DE-588)4003412-4 s Spektroskopie (DE-588)4056138-0 s 1\p DE-604 Zemansky, Mark W. Verfasser aut Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017704050&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Mitchell, Allan C. G. 1902-1963 Zemansky, Mark W. Resonance radiation and excited atoms Radiation Fluorescence Atoms Resonanzstrahlung (DE-588)4177860-1 gnd Atom (DE-588)4003412-4 gnd Spektroskopie (DE-588)4056138-0 gnd |
| subject_GND | (DE-588)4177860-1 (DE-588)4003412-4 (DE-588)4056138-0 |
| title | Resonance radiation and excited atoms |
| title_auth | Resonance radiation and excited atoms |
| title_exact_search | Resonance radiation and excited atoms |
| title_full | Resonance radiation and excited atoms by Allan C. G. Mitchell and Mark W. Zemansky |
| title_fullStr | Resonance radiation and excited atoms by Allan C. G. Mitchell and Mark W. Zemansky |
| title_full_unstemmed | Resonance radiation and excited atoms by Allan C. G. Mitchell and Mark W. Zemansky |
| title_short | Resonance radiation and excited atoms |
| title_sort | resonance radiation and excited atoms |
| topic | Radiation Fluorescence Atoms Resonanzstrahlung (DE-588)4177860-1 gnd Atom (DE-588)4003412-4 gnd Spektroskopie (DE-588)4056138-0 gnd |
| topic_facet | Radiation Fluorescence Atoms Resonanzstrahlung Atom Spektroskopie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017704050&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT mitchellallancg resonanceradiationandexcitedatoms AT zemanskymarkw resonanceradiationandexcitedatoms |