Gold chemistry: highlights and future directions in the life sciences
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| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim
WILEY-VCH
2009
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| Ausgabe: | 1. Aufl. |
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XVI, 408 S. Ill., graph. Darst. |
| ISBN: | 9783527320868 |
Internformat
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| 245 | 1 | 0 | |a Gold chemistry |b highlights and future directions in the life sciences |c ed. by Fabian Mohr |
| 250 | |a 1. Aufl. | ||
| 264 | 1 | |a Weinheim |b WILEY-VCH |c 2009 | |
| 300 | |a XVI, 408 S. |b Ill., graph. Darst. | ||
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Datensatz im Suchindex
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IMAGE 1
CONTENTS
PREFACE XI FOREWORD XII I LIST OF CONTRIBUTORS XV
GOLD(L) NITROGEN CHEMISTRY 1 HANAN E. ABDOU, AHMED A. MOHAMED, ANDJOHN
P. FACKLERJR 1.1 INTRODUCTION 1
1.2 TETRA-, TRI-. AND DINUCLEAR GOLD(I) AMIDINATE COMPLEXES 3 1.3
OXIDATIVE-ADDITION REACTIONS TO THE DINUCLEAR GOLD(I) AMIDINATE COMPLEX
9 1.4 MERCURY(II) CYANIDE COORDINATION POLYMER 13 1.5 FORMATION OF
MIXED-LIGAND TETRANUCLEAR GOLD(I) NITROGEN CLUSTERS 15 1.6 SOLVENT
INFLUENCES ON OXIDATION AND NUCLEARITY OF GOLD
GUANIDINATE DERIVATIVES 21 1.7 CYCLIC TRINUCLEAR GOLD(I) NITROGEN
COMPOUNDS 24 1.8 OXIDATIVE-ADDITION REACTIONS TO THE CYCLIC TRINUCLEAR
GOLD(I)-NITROGEN COMPOUNDS 28 1.9 SUPRAMOLECULAR ENTITIES OF TRINUCLEAR
GOLD(I) COMPLEXES
SANDWICHING SMALL ORGANIC ACIDS 30 1.10 GOLD(I) AND SILVER(I)
MIXED-METAL TRINUCLEAR COMPLEXES 33 1.11 CO OXIDATION OVER AU/TIOZ
PREPARED FROM GOLD NITROGEN COMPLEXES 36 1.12 MISCE]]ANEOUS OBSERVATIONS
37
REFERENCES 37
2 CHEMISTRY OFGOLD(LLI) COMPLEXES WITH NITROGEN AND OXYGEN LIGANDS 47
MARIA AGOSTINA CINELLU 2.1 INTRODUCTION 47
2.2 NITROGEN DONOR LIGANDS 47
2.2.1 COMPLEXES WITH NEUTRAL MONODENTATE LIGANDS 47 2.2.2 COMPLEXES WITH
ANIONIC MONODENTATE LIGANDS 51
GOLD CHEMISTL}': /\.PPHCATLOLTS AND !-,'UTU.RL' DRRECTLOM IN THE 1 FIE
SCIENCES" EDITED BY FABIAN MOHR COPYNGHT 2009 WILEYVCH VERLAG GMBH &
CO. KGAA. WEINHCIM ISBN: 97~L527120~G~
IV
IMAGE 2
VII CONTENTS
2.2.3 2.2.4
2.2.5 2.3 2.3.1 2.3.2 2.3.3 2.3.4 2.3.5
3
3.1 3.2 3.2.1 3.2.1.1 3.2.1.2
3.2.1.3
3.2.1.4
3.2.2 3.2.2.1
3.2.3 3.2.4 3.2.5 3.2.5.1
3.2.5.2 3.2.5.3
3.2.5.4 3.2.5.5 3.2.5.6
3.2.5.7 3.2.5.8 3.2.5.9 3.2.5.10
3.3
COMPLEXES WITH MULTIDENTATE LIGANDS 53 COMPLEXES WITH MULTIDENTATE
LIGANDS CONTAINING ANIONIC N-DONORS 59 COMPLEXES WITH POLYAZAMACROCYCLIC
LIGANDS 63
OXYGEN DONOR LIGANDS 65 HYDROXO COMPLEXES 65 OXO COMPLEXES 69 ALKOXO
COMPLEXES 72
COMPLEXES WITH OTHER O-DONOR LIGANDS 76 COMPLEXES WITH MIXED N/O LIGANDS
78 REFERENCES 80
PENTAFLUOROPHENYL GOLD COMPLEXES 93
A. LUQUIN, E. CERRADA, AND M. LAGUNA
INTRODUCTION 93 PENTAFLUOROPHENYLGOLD(I) DERIVATIVES 94 NEUTRAL
PENTAFLUOROPHENYLGOLD(I) DERIVATIVES 95 NEUTRAL PENTAFLUOROPHENYLGOLD(I)
DERIVATIVES WITH C-DONOR LIGANDS 97 NEUTRAL PENTAFLUOROPHENYLGOLD(I)
DERIVATIVES WITH N-DONOR LIGANDS 100
NEUTRAL PENTAFLUOROPHENYLGOLD(I) DERIVATIVES WITH P-DONOR LIGANDS 101
NEUTRAL PENTAFLUOROPHENYLGOLD(I) DERIVATIVES WITH S-DONOR LIGANDS 102
ANIONIC PENTAFLUOROPHENYLGOLD(I) DERIVATIVES 103
REACTIVITY OF THE ANIONIC PENTAFLUOROPHENYLGOLD(I) COMPLEXES
Q[AU(CC,FS)X] 105 CATIONIC PENTAFLUOROPHENYLGOLD(I) DERIVATIVES 107 DI
AND POLYNUCLEAR PENTAFLUOROPHENYLGOLD(I) DERIVATIVES 108
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) COMPLEXES 117 HETERONUCLEAR
PENTAFLUOROPHENYLGOLD(I) BISMUTH COMPLEXES 117 HETERONUCLEAR
PENTAFLUOROPHENYLGOLD(I) TIN COMPLEXES 117
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) THALLIUM COMPLEXES 117
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) SILVER COMPLEXES 119
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) COPPER COMPLEXES 122
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) PALLADIUM COMPLEXES 122
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) RHODIUM COMPLEXES 123
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) IRON COMPLEXES 123
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) MANGANESE COMPLEXES 126
HETERONUCLEAR PENTAFLUOROPHENYLGOLD(I) CHROMIUM, GOLD MOLYBDENUM AND
GOLD TUNSTEN COMPLEXES 126 PENTAFLUOROPHENYLGOLD(III) DERIVATIVES 127
IMAGE 3
3.3.1 3.3.2 3.3.2.1 3.3.2.2 3.3.2.3 3.3.2.4 3.3.3
3.3.4 3.3.5 3.4 3.5 3.5.1 3.5.2 3.6
CONTENTS I VII
MONONUCLEAR PENTAFLUOROPHENYLGOLD (III) DERIVATIVES 130 DI AND
POLYNUCLEAR PENTAFLUOROPHENYLGOLD(III) DERIVATIVES 138 C-DONOR LIGANDS
138 DIAMINE AND CARBENE BRIDGES 143
N-, P- AND AS-DONOR LIGANDS 143 S- AND SE-DONOR LIGANDS 147
POLYNUCLEAR PENTAFLUOROPHENYLGOLD DERIVATIVES WITH AU(I)-AU(III) BOND
148 HETEROPOLYNUCLEAR PENTAFLUOROPHENYLGOLD(III) DERIVATIVES 149
PENTAFLUOROPHENYLGOLD(III) DERIVATIVES AS CATALYST 150
GOLD CLUSTERS 155 PENTAFLUOROPHENYLGOLD(II) DERIVATIVES 156 DINUCLEAR
PENTAFLUOROPHENYLGOLD(LL) COMPLEXES 156 POLYNUCLEAR
PENTAFLUOROPHENYLGOLD(IJ) COMPLEXES 159 OUTLOOK AND FUTURE TRENDS 162
REFERENCES 163
4 THEORETICAL CHEMISTRY OF GOLD - FROM ATOMS TO MOLECULES,
CLUSTERS, SURFACES AND THE SOLID STATE 183
PETER SCHWERDTFEGER AND MATTHIAS LEIN 4.1 INTRODUCTION 183
4.2 THE ORIGIN OF THE RELATIVISTIC MAXIMUM AT GOLD ALONG THE 6TH PERIOD
OF ELEMENTS IN THE PERIODIC TABLE 186 4.3 CALCULATIONS ON ATOMIC GOLD
189
4.4 RELATIVISTIC METHODS FOR MOLECULAR CALCULATIONS AND DIATOMIC GOLD
COMPOUNDS 194 4.5 CALCULATIONS ON INORGANIC AND ORGANOMETALLIC GOLD
COMPOUNDS 203 4.6 CALCULATIONS ON GOLD CLUSTERS 212
4.7 CALCULATIONS ON INFINITE SYSTEMS: FROM SURFACES TO THE SOLID STATE
OF GOLD 216 4.8 SUMMARY 220
REFERENCES 221
5 LUMINESCENCE AND PHOTOPHYSICS OF GOLD COMPLEXES 249
CHI-MING CHE AND SIU-WAI LAI 5.1 INTRODUCTION 249
5.2 SPECTROSCOPIC PROPERTIES OF GOLD(I) COMPLEXES 250 5.2.1 MONONUCLEAR
GOLD(I) COMPLEXES 250 5.2.2 DI- AND POLYNUCLEAR GOLD(L) COMPLEXES WITH
METAL-METAL INTERACTIONS 252 5.2.3 HIGH-ENERGY L[5DCR', GPCR] EXCITED
STATE VERSUS VISIBLE
METAL-ANION/SOLVENT EXCIPLEX EMISSION 262 5.2.4 CHEMOSENSORY
APPLICATIONS 267 5.3 SPECTROSCOPIC PROPERTIES OF GOLD(III) COMPLEXES 270
5.4 PHOTOINDUCED ELECTRON TRANSFER REACTIONS OF GOLD COMPLEXES 273
IMAGE 4
VIII I CONTENTS
5.5 CONCLUDING REMARKS 274
REFERENCES 276
6 GOLD COMPOUNDS AND THEIR APPLICATIONS IN MEDICINE 283 ELIZABETH A.
PACHECO, EDWARD R. T. TIEKINK, AND MICHAEL W. WHITEHOUSE 6.1
INTRODUCTION 283
6.2 THE AQUEOUS CHEMISTRY OF GOLD COMPOUNDS 283 6.2.1 STRUCTURES OF
GOLD(I) AND GOLD(III) COMPLEXES 284 6.2.2 OXIDATION-REDUCTION REACTIONS
284 6.2.3 LIGAND EXCHANGE MECHANISMS 285 6.3 MEDICINALLY [MPORTANT GOLD
COMPLEXES. THEIR ANALOGS
AND REACTIONS 287
6.3.1 OLIGOMERIC GOLD(I) THIOLATES AND ANALOGS 287 6.3.2
BIS(THIOLATO)GOLD(I) SPECIES 290 6.3.3 DITHIOCARBAMATES 291
6.3.4 AURANOFIN AND OTHER PHOSPHINE(THIOLATO)GOLD(I) SPECIES 291 6.3.5
AU-S BOND LENGTH COMPARISONS 292 6.3.6 COMPLEXES OF DIPHOSPHINE LIGANDS
293 6.3.7 GOLD(I) CYANIDE COMPLEXES 294 6.3.8 HETEROCYCLIC CARBENES 295
6.4 GOLD-PROTEIN REACTIONS AND COMPLEXES 295 6.4.1 SERUM ALBUMIN 295
6.4.2 METALLOTHIONEINS 297
6.4.3 SELENIUM-DEPENDENT GLUTATHIONE PEROXIDASE 300 6.4.4 GOLD(III)
OXIDATION OF INSULIN AND RIBONUCLEASE 301 6.4.5 ENZYME INHIBITION 301
6.4.6 ZINC FINGER PROTEINS 302
6.4.7 HEMOGLOBIN AND INTERPROTEIN GOLD TRANSFER ("TRANSAURATION") 303
6.4.8 MITOCHONDRIAL THIOREDOXIN REDUCTASE 303 6.5 PHYSIOLOGICAL AND
CELLULAR BIOCHEMISTRY 304 6.5.1 BIOLOGICAL LIGAND EXCHANGE 304
6.5.2 THE SULFHYDRYL-SHUTTLE MODEL 305 6.5.3 EQUILIBRATION OF INTRA- AND
EXTRACELLULAR GOLD 305 6.5.4 CYTOTOXICITY AND ANTITUMOR ACTIVITY OF GOLD
COMPLEXES 306 6.5.5 OXIDATION STATES IN VIVO 307
6.5.6 LMMUNOCHEMICAL CONSEQUENCES OF GOLD(II I) 308 6.5.7 ANTI-HIV
ACTIVITY 308
6.5.8 GOLD NANOPARTICLES 309
6.6 CONCLUSIONS 309
REFERENCES 310
7 NANOSCIENCE OF GOLD AND GOLD SURFACES 321
M. B CORTIE AND A. MCDONAGH 7.1 INTRODUCTION 321
7.2 FORMS OF GOLD AT THE NANOSCALE 323
IMAGE 5
7.2.1 7.2.2 7.2.3 7.2.4 7.2.5 7.2.6
7.2.7 7.2.8 7.2.8.1 7.2.8.2 7.3 7.3.1 7.3.1.1 7.3.1.2 7.3.1.3 7.3.2
7.3.2.1 7.3.3 7.3.3.1 7.4 7.4.1 7.4.2 7.4.3 7.4.4 7.4.4.1 7.4.5 7.4.6
7.4.7 7.4.8 7.5
CLUSTERS AND NANOPARTICJES OF LESS THAN 5 NM DIAMETER 323 NANOSPHERES
325 NANOSHELLS 325 NANORODS 327 OTHER NANOPARTICLE SHAPES 327
MESOPOROUS SPONGES 327 THIN FILMS 329 ASSEMBLAGES OF NANOPARTICLES 330
DISORDERED AGGREGATES 330
COLLOIDAL CRYSTALS 330 ONSET OF NEW PHENOMENA 331 OPTICAL 331 THE
PLASMON RESONANCE 331
MANIPULATION OF THE PLASMON RESONANCE 332 FLUORESCENCE AND LUMINESCENCE
333 PHYSICAL 334 DEPRESSION OF THE MELTING POINT 334 CHEMICAL 334
HETEROGENEOUS CATALYSIS 334 SURFACE CHEMISTRY OF GOLD 335 HYDROGEN 335
HALOGENS 336 OXYGEN 337
SULFUR 338 ISOTHIOCYANATES 339 SELENIUM AND TELLURIUM 339 NITROGEN 340
PHOSPHORUS, ARSENIC, ANTIMONY 341 CARBON 342 CONCLUSIONS 342 REFERENCES
343
CONTENTS IIX
8 LIQUID CRYSTALS BASED ON GOLD COMPOUNDS 357 SILVERIO COCO AND PABLO
ESPINET 8.1 INTRODUCTION 357
8.1.1 A FEW GENERAL CONCEPTS IN LIQUID CRYSTALS 357 8.1.2 GOLD, AN IDEAL
METAL FOR LC STUDIES 360
8.2 PYRIDINE COMPLEXES 361
8.3 DITHIOBENZOATE COMPLEXES 361
8.4 ISOCYANIDE COMPLEXES 362
8.4.1 ISOCYANIDE-HALIDE COMPLEXES 362 8.4.2 [SOCYANIDE-ALKYNYL COMPLEXES
370 8.4.3 ISOCYANIDE-FLUOROPHENYL DERIVATIVES 372 8.4.4 IONIC
BIS(ISOCYANIDE) DERIVATIVES 379 8.4.5 MIXTURES: LIQUID CRYSTALLINE
"MOLECULAR ALLOYS" 383
IMAGE 6
X I CONTENTS
8.5 CARBENE COMPLEXES 384
8.6 COMPLEXES CONTAINING PYRAZOLE-TYPE LIGANDS 387 8.6.1 TRINUCLEAR GOLD
PYRAZOLATE RINGS: METALLACROWNS 387 8.6.2 "MONONUCLEAR" COMPLEXES 388
8.7 IONIC IMIDAZOLIUM DERIVATIVES 388
8.8 LIQUID CRYSTALLINE GOLD NANOPARTICLES 388 8.9 CONCLUSIONS 390
REFERENCES 392
INDEX 397 |
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| indexdate | 2024-07-20T10:06:40Z |
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| publisher | WILEY-VCH |
| record_format | marc |
| spelling | Gold chemistry highlights and future directions in the life sciences ed. by Fabian Mohr 1. Aufl. Weinheim WILEY-VCH 2009 XVI, 408 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Goldverbindungen (DE-588)4157895-8 gnd rswk-swf Goldverbindungen (DE-588)4157895-8 s DE-604 Mohr, Fabian 1975- (DE-588)137759819 edt text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3113107&prov=M&dok_var=1&dok_ext=htm Inhaltstext OEBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017322558&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Gold chemistry highlights and future directions in the life sciences Goldverbindungen (DE-588)4157895-8 gnd |
| subject_GND | (DE-588)4157895-8 |
| title | Gold chemistry highlights and future directions in the life sciences |
| title_auth | Gold chemistry highlights and future directions in the life sciences |
| title_exact_search | Gold chemistry highlights and future directions in the life sciences |
| title_full | Gold chemistry highlights and future directions in the life sciences ed. by Fabian Mohr |
| title_fullStr | Gold chemistry highlights and future directions in the life sciences ed. by Fabian Mohr |
| title_full_unstemmed | Gold chemistry highlights and future directions in the life sciences ed. by Fabian Mohr |
| title_short | Gold chemistry |
| title_sort | gold chemistry highlights and future directions in the life sciences |
| title_sub | highlights and future directions in the life sciences |
| topic | Goldverbindungen (DE-588)4157895-8 gnd |
| topic_facet | Goldverbindungen |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3113107&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017322558&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT mohrfabian goldchemistryhighlightsandfuturedirectionsinthelifesciences |