Verfügbarkeit: Landmarks in organo-transition metal chemistry

Landmarks in organo-transition metal chemistry: a personal view

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Bibliographische Detailangaben
1. Verfasser:	Werner, Helmut (VerfasserIn)
Format:	Buch
Sprache:	English
Veröffentlicht:	New York [u.a.] Springer 2009
Schriftenreihe:	Profiles in inorganic chemistry
Schlagworte:	Werner, Helmut > 1934- Geschichte 1800-2000 Organometallic chemistry Organometallic chemistry / History Organometallic compounds Organometallic compounds / History Geschichte Organometallic chemistry > History Organometallic compounds > History Carbene Metallcarbonyle Metallorganische Chemie Autobiografie
Online-Zugang:	Inhaltsverzeichnis
Beschreibung:	XXI, 348 S. Ill., graph. Darst.
ISBN:	9780387098470 9780387098487

Internformat

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Datensatz im Suchindex

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adam_text	CONTENTS 1 PROLOGUE ............................................... 1 REFERENCES ............................................. 7 2 BIOGRAPHICAL SKETCH ...................................... 9 2.1 THE YEARS AT HOME ................................. 9 2.2 THE FIRST MOVE: FROM MIIHLHAUSEN TO JENA .............. 19 2.3 THE SECOND MOVE: FROM JENA TO MUNICH ................ 24 2.4 THE FIRST YEARS AT MUNCHEN .......................... 26 2.5 FROM MUNCHEN TO PASADENA AND BACK .................. 31 2.6 CROSSING THE BORDER: THE YEARS AT ZURICH ................ 41 2.7 BACK TO GERMANY ................................... 50 BIOGRAPHIES ...................................... 64 3 THE NINETEENTH CENTURY: A SEQUENCE OF ACCIDENTAL DISCOVERIES..... 69 3.1 THE BEGINNINGS OF ORGANOMETALLIC CHEMISTRY ............. 69 3.2 WILHELM CHRISTOPH ZEISE AND THE FIRST TRANSITION METAL IR-COMPLEX ........................................ 70 3.3 EDWARD FRANKLAND S PIONEERING STUDIES ................. 71 3.4 VICTOR GRIGNARD: THE FATHER OF ORGANOMETALLICS FOR ORGANIC SYNTHESIS .......................................... 74 3.5 PAUL SCHIITZENBERGER AND LUDWIG MOND: THE FIRST METAL CARBONYLS ......................................... 75 BIOGRAPHIES ...................................... 78 REFERENCES ......................................... 83 4 TRANSITION METAL CARBONYLS: FROM SMALL MOLECULES TO GIANT CLUSTERS ........................................ 85 4.1 A CLASS OF PECULIAR COMPOUNDS ...................... 85 4.2 THE GIANT WORK OF WALTER HIEBER ...................... 89 4.3 HIEBER AND HIS FOLLOWERS ............................. 93 4.4 SURPRISINGLY STABLE: MULTIPLY CHARGED CARBONYL METALLATC ANIONS ........................................... 98 4.5 METAL CARBONYL CATIONS: NOT INCAPABLE OF EXISTENCE ....... 100 XV XVI CONTENTS 4.6 HIGHLY LABILE METAL CARBONYLS ....................... 102 4.7 THE EXITING CHEMISTRY OF METAL CARBONYL CLUSTERS........ 105 4.8 OTTO ROELEN AND WALTER REPPE: INDUSTRIAL APPLICATIONS OF METAL CARBONYLS ................................. 110 4.9 BIOGRAPHIES ..................................... 114 REFERENCES ........................................ 119 5A SCIENTIFIC REVOLUTION: THE DISCOVERY OF THE SANDWICH COMPLEXES ............................................. 129 5.1 THE EARLY DAYS: FERROCENE ........................... 129 5.2 THE RIVALRY OF FISCHER AND WILKINSON .................. 135 5.3 FISCHER S STAR: BIS(BENZENE)CHROMIUM .................. 136 5.4 HEIN S POLYPHENYLCHROMIUM COMPOUNDS ............. 138 5.5 ZEISS AND TSUTSUI: HEIN S WORK REVISITED ............... 140 5.6 WILKINSON S NEXT STEPS .............................. 145 5.7 FROM SANDWICH COMPLEXES TO ORGANOMETALLIC DENDRIMERS ....................................... 146 5.8 THE TAMING OF CYCLOBUTADIENE: A CASE OF THEORY BEFORE EXPERIMENT ....................................... 150 5.9 THE SMALLER AND LARGER RING BROTHERS OF FERROCENE....... 152 5.10 SANDWICHES WITH P5 AND HETEROCYCLES AS RING LIGANDS ..... 154 5.11 TWO HIGHLIGHTS FROM THE 21ST CENTURY .................. 157 5.12 BRINTZINGER S SANDWICH-TYPE CATALYSTS ................. 159 5.13 WOODWARD AND THE NOBEL PRIZE ....................... 161 BIOGRAPHIES .................................... 163 REFERENCES ........................................ 169 6 ONE DECK MORE: THE CHEMICAL BIG MAC .................... 177 6.1 THE BREAKTHROUGH: [NI2(C5H5)3]+ ..................... 177 6.2 THE IRON AND RUTHENIUM COUNTERPARTS ................. 182 6.3 ARENE-BRIDGED TRIPLE-DECKER SANDWICHES ............... 185 6.4 BIG MACS WITH BRIDGING P5, P6 AND HETEROCYCLES AS LIGANDS ........................................ 186 6.5 TETRA-, PENTA- AND HEXA-DECKER SANDWICH COMPLEXES ..... 189 NOTES ............................................ 191 REFERENCES ........................................ 191 7 THE BINDING OF ETHENE AND ITS CONGENERS: PROTOTYPICAL METAL 7T-COMPLEXES ........................................... 195 7.1 FROM 1827 TO THE 1930S: IN THE FOOTSTEPS OF ZEISE ........ 195 7.2 REIHLEN S STRANGE BUTADIENE IRON TRICARBONYL............ 199 7.3 MICHAEL DEWAR S LANDMARK CONTRIBUTION ............. 200 7.4 THE DEWAR-CHATT-DUNCANSON MODEL .................. 202 7.5 AN EXCITING BRANCH: MONO- AND OLIGOOLEFIN METAL CARBONYLS ................................... 204 CONTENTS XVII 7.6 SCHRAUZER S EARLY STUDIES ON HOMOLEPTIC OLEFIN NICKEL(0) COMPLEXES ................................ 208 7.7 WILKE S MASTERPIECES AND THE NAKED NICKEL ............ 209 7.8 STONE AND THE FAMILY OF OLEFIN PALLADIUM(0) AND PLATINUM(0) COMPOUNDS ...................................... 214 7.9 TIMMS , FISCHER S AND GREEN S DISTINCTIVE SHARES ......... 216 7.10 A RECENT MILESTONE: JONAS OLEFIN ANALOGUES OF HIEBER S METAL CARBONYLATES ................................ 219 BIOGRAPHIES ..................................... 221 REFERENCES ........................................ 228 8 METAL CARBENES AND CARBYNES: THE TAMING OF NON-EXISTING MOLECULES .............................................. 235 8.1 THE SEARCH FOR DIVALENT CARBON COMPOUNDS ............ 235 8.2 FROM WANZLICK S AND OFELE S WORK TO ARDUENGO S CARBENES ......................................... 237 8.3 THE BREAKTHROUGH: FISCHER S METAL CARBENES ............ 238 8.4 THE NEXT HIGHLIGHT: FISCHER S METAL CARBYNES ........... 241 8.5 OFELE S, CASEY S AND CHATT S ROUTES TO METAL CARBENES .... 242 8.6 LAPPERT S SEMINAL WORK ON BIS(AMINO)CARBENE COMPLEXES . 244 8.7 A BIG STEP: SCHROCK S METAL CARBENES AND CARBYNES ...... 247 8.8 FISCHER AND HIS FOLLOWERS ........................... 253 8.9 USING THE ISOLOBAL ANALOGY: METAL COMPLEXES WITH BRIDGING CARBENES AND CARBYNES ............................. 256 8.10 THE SEEMINGLY EXISTING CCL2 AND ITS GENERATION AT TRANSITION METAL CENTERS ............................ 259 8.11 THE CONGENERS OF METAL CARBYNES WITH M=E TRIPLE BONDS ...................................... 263 8.12 THE FIRST AND SECOND GENERATION OF GRUBBS RUTHENIUM CARBENES ......................................... 263 8.13 FROM METAL CARBENES TO OPEN-SHELL METAL CARBYNE AND CARBIDO COMPLEXES ................................ 268 8.14 THE DOTZ REACTION AND THE USE OF METAL CARBENES FOR ORGANIC SYNTHESIS .................................. 271 8.15 OLEFIN METATHESIS: A LANDMARK IN APPLIED ORGANOMETALLIC CHEMISTRY ........................................ 272 8.16 AN EXTENSION: METAL COMPLEXES WITH UNSATURATED CARBENES 274 BIOGRAPHIES .................................... 276 REFERENCES ........................................ 284 9 METAL ALKYLS AND METAL ARYLS: THE TRUE TRANSITION ORGANOMETALLICS ......................................... 297 9.1 THE EXTENSIONS OF FRANKLAND S PIONEERING WORK ......... 297 9.2 HETEROLEPTIC COMPLEXES WITH METAL-ALKYL AND METAL-ARYL BONDS ........................................... 299 XVIII CONTENTS 9.3 CHATT AND HIS CONTEMPORARIES ........................ 300 9.4 LAPPERT, WILKINSON AND THE ISOLATION OF STABLE METAL ALKYLS AND ARYLS ......................................... 304 9.5 AN APPARENT CONFLICT: METAL ALKYLS AND ARYLS CONTAINING A- ANDRR-DONOR LIGANDS ................................ 310 9.6 BINARY METAL ALKYLS WITH M-M MULTIPLE BONDS .......... 314 9.7 THE RECENT HIGHLIGHT: POWER S RCRCRR AND THE FIVEFOLD CR- CR BONDING ................................. 315 9.8 NOVEL PERSPECTIVES: METAL ALKYLS AND ARYLS FORMED BY C-H AND C-C ACTIVATION ................................ 317 9.9 METAL ALKYLS AND ARYLS IN CATALYSIS ..................... 324 REFERENCES ......................................... 325 10 EPILOGUE ............................................... 337 INDEX ..................................................... 341
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spelling	Werner, Helmut Verfasser aut Landmarks in organo-transition metal chemistry a personal view Helmut Werner New York [u.a.] Springer 2009 XXI, 348 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Profiles in inorganic chemistry Werner, Helmut 1934- (DE-588)129826715 gnd rswk-swf Geschichte 1800-2000 gnd rswk-swf Organometallic chemistry Organometallic chemistry / History Organometallic compounds Organometallic compounds / History Geschichte Organometallic chemistry History Organometallic compounds History Carbene (DE-588)4147281-0 gnd rswk-swf Metallcarbonyle (DE-588)4137337-6 gnd rswk-swf Metallorganische Chemie (DE-588)4602390-2 gnd rswk-swf (DE-588)4003939-0 Autobiografie gnd-content Metallorganische Chemie (DE-588)4602390-2 s Geschichte 1800-2000 z DE-604 Werner, Helmut 1934- (DE-588)129826715 p Metallcarbonyle (DE-588)4137337-6 s Carbene (DE-588)4147281-0 s Digitalisierung Deutsches Museum application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017085994&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Werner, Helmut Landmarks in organo-transition metal chemistry a personal view Werner, Helmut 1934- (DE-588)129826715 gnd Organometallic chemistry Organometallic chemistry / History Organometallic compounds Organometallic compounds / History Geschichte Organometallic chemistry History Organometallic compounds History Carbene (DE-588)4147281-0 gnd Metallcarbonyle (DE-588)4137337-6 gnd Metallorganische Chemie (DE-588)4602390-2 gnd
subject_GND	(DE-588)129826715 (DE-588)4147281-0 (DE-588)4137337-6 (DE-588)4602390-2 (DE-588)4003939-0
title	Landmarks in organo-transition metal chemistry a personal view
title_auth	Landmarks in organo-transition metal chemistry a personal view
title_exact_search	Landmarks in organo-transition metal chemistry a personal view
title_full	Landmarks in organo-transition metal chemistry a personal view Helmut Werner
title_fullStr	Landmarks in organo-transition metal chemistry a personal view Helmut Werner
title_full_unstemmed	Landmarks in organo-transition metal chemistry a personal view Helmut Werner
title_short	Landmarks in organo-transition metal chemistry
title_sort	landmarks in organo transition metal chemistry a personal view
title_sub	a personal view
topic	Werner, Helmut 1934- (DE-588)129826715 gnd Organometallic chemistry Organometallic chemistry / History Organometallic compounds Organometallic compounds / History Geschichte Organometallic chemistry History Organometallic compounds History Carbene (DE-588)4147281-0 gnd Metallcarbonyle (DE-588)4137337-6 gnd Metallorganische Chemie (DE-588)4602390-2 gnd
topic_facet	Werner, Helmut 1934- Organometallic chemistry Organometallic chemistry / History Organometallic compounds Organometallic compounds / History Geschichte Organometallic chemistry History Organometallic compounds History Carbene Metallcarbonyle Metallorganische Chemie Autobiografie
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work_keys_str_mv	AT wernerhelmut landmarksinorganotransitionmetalchemistryapersonalview

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