Design of heterogeneous catalysts: new approaches based on synthesis, characterization and modeling
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Weinheim
WILEY-VCH
2009
|
| Schlagworte: | |
| Online-Zugang: | Inhaltstext Inhaltsverzeichnis |
| Beschreibung: | XVII, 322 S. Ill., graph. Darst. 240 mm x 170 mm |
| ISBN: | 9783527320790 |
Internformat
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| 245 | 1 | 0 | |a Design of heterogeneous catalysts |b new approaches based on synthesis, characterization and modeling |c ed. by Umit S. Ozkan |
| 264 | 1 | |a Weinheim |b WILEY-VCH |c 2009 | |
| 300 | |a XVII, 322 S. |b Ill., graph. Darst. |c 240 mm x 170 mm | ||
| 336 | |b txt |2 rdacontent | ||
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| 338 | |b nc |2 rdacarrier | ||
| 650 | 4 | |a Catalysts |x Design | |
| 650 | 4 | |a Heterogeneous catalysis | |
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Datensatz im Suchindex
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CONTENTS PREFACE XIII LIST OFCONTRIBUTORS XV 1 USE OF OXIDE LIGANDS IN
DESIGNING CATALYTIC ACTIVE SITES 1 EDWARD L LEE AND ISRAEL E. WACHS 1.1
INTRODUCTION 1 1.2 MOLECULAR STRUCTURAL DETERMINATION OF SUPPORTED METAL
OXIDE CATALYSTS WITH IN SITU RAMAN SPECTROSCOPY 3 1.3 CHARACTERIZATION
OF ALO % , TIO X , AND ZRO X SURFACE-MODIFIED SIO 2 3 1.4 ANCHORING SITE
OF SURFACE M,O X . SPECIES ON SUPPORTED M 2 O V /SIO 2 5 1.5 MOLECULAR
STRUCTURE OF DEHYDRATED SUPPORTED V 2 O 5 /SIO 2 AND V 2 O 5 /M 2 O X
/SIO 2 CATALYST SYSTEMS 5 1.6 MOLECULAR STRUCRURE OF DEHYDRATED
SUPPORTED MOO S /SIO 2 AND MOO,/M 2 O X /SIO 2 CATALYST SYSTEMS 8 1.7
MOLECULAR STRUCTURE OF DEHYDRATED SUPPORTED RE 2 BIBLIOGRAFISCHE
INFORMATIONEN HTTP://D-NB.INFO/990245926 DIGITALISIERT DURCH VI CONTENTS
2.1.3 POROUS CATALYST ARCHITECTURE AND OPTIMIZATION METHODS 27 2.1.4
LEARNING FROM NATURE 28 2.2 OPTIMIZING MESOPORE CONNECTIVITY AND SHAPE
30 2.2.1 TOPOLOGY, ORDER, AND RANDOMNESS 30 2.2.2 SURFACE ROUGHNESS AND
FRACTAL MORPHOLOGY 32 2.3 OPTIMIZING CATALYSTS BY MACROSCOPIC
DISTRIBUTIONS IN ACTIVITY 34 2.4 OPTIMAL DESIGN OF THE HIGHWAY NETWORK
36 2.4.1 NOVEL CAPABILITIES IN SYNTHESIZING HIERARCHICAL PORE SPACES 37
2.4.2 THEORETICAL OPTIMIZATION STUDIES: OPPORTUNITIES FOR OPTIMAL DESIGN
39 2.4.3 APPLICATION TO THE DESIGN OF A BIMODAL POROUS CATALYST FOR NO X
ABATEMENT 47 2.5 CONCLUSIONS 49 REFERENCES 50 3 USE OF DENDRIMERS IN
CATALYST DESIGN 59 BERT D. CHANDLER, JEONG-KYU LEE, HAROLD H. KUNG, AND
MAYFAIR C KUNG 3.1 INTRODUCTION 59 3.2 MODIFIED DENDRIMER CATALYSTS 60
3.2.1 DENDRIMER SYNTHESIS 60 3.2.2 DENDRIMER PROPERTIES IMPORTANT FOR
CATALYSIS 61 3.2.3 COOPERATIVE CATALYSIS 61 3.2. CONTENTS VII 4.3.4
AGING STUDIES 86 4.3.5 KINETICS 87 4.3.6 CATALYST SCALE-UP 88 4.3.7
QUALITY CONTROL 89 4.4 EXAMPLE 1: AUTOMOBILE POLLUTION ABATEMENT
CATALYST SYSTEM 89 4.4.1 THE QUALITY OF THE FUEL 90 4.4.2 BASE METALS
VERSUS PRECIOUS METALS 90 4.4.3 PARTICULATE VERSUS MONOLITHIC STRUCTURES
91 4.4.4 THE FIRST GENERATION 91 4.4.5 THE FINAL TEST 92 4.5 EXAMPLE 2:
DEHYDROGENATION OF LIGHT ALKANES 93 4.5.1 UNDERSTANDING REACTION
KINETICS, THERMODYNAMICS, AND PROCESS CONSTRAINTS 94 4.5.2 FORMULATING
THE CATALYST 95 4.5.3 PILOT PLANT TESTING 97 4.5.4 FIELD TESTING 98
4.5.5 COMMERCIAL LAUNCH 99 4.6 EXAMPLE 3: PETROLEUM REFINING - FLUID
CATALYTIC CRACKING 100 4.6.1 UNDERSTANDING DEACTIVATION 101 4.6.2 AGE
DISTRIBUTION 105 4.6.3 ATTRITION 105 4.6.4 FEED EFFECTS 107 4.6.5
SCALE-UP AND COMMERCIALIZATION 209 4. VIII CONTENTS 6 CATALYTIC
NANOMOTORS 242 JOHN CIBBS AND YIPING ZHAO 6.1 INTRODUCTION 142 6.1.1
BIOLOGICAL MOTORS 142 6.1.2 ARTIFICIAL CATALYTIC NANOMOTORS 142 6.2 THE
PROPULSION MECHANISM OF CATALYTIC NANOMOTORS 244 6.2.1 DIFFUSIOPHORESIS
244 6.2.2 SELF-ELECTROPHORESIS 245 6.2.3 BUBBLE PROPULSION 248 6.2.4
INTERFACIAL TENSION GRADIENTS 149 6.2.5 BIOELECTROCHEMICAL PROPULSION
150 6.3 ADVANCED DESIGN OF CATALYTIC NANOMOTORS 252 6.3.1 DYNAMIC
SHADOWING GROWTH 151 6.3.2 ROTARY SI-PT NANOROD NANOMOTORS 252 6.3.3
L-SHAPED NANOROD NANOMOTORS 152 6.3.4 ROLLING NANOSPRING 253 6.3.5
HINGED NANORODS 254 6.4 APPLICATIONS, CHALLENGES, AND PERSPECTIVES 257
REFERENCES 258 7 RATIONAL DESIGN AND HIGH-THROUGHPUT SCREENING OF METAL
OPEN FRAMEWORKS FOR GAS SEPARATION AND CATALYSIS 262 DAVID FARRUSSENG
AND CLAUDE MIRODATOS 7.1 INTRODUCTION 161 7.2 MOF GENERAL FEATURES AND
BRIEF STATE OF THE ART 162 7.2.1 A BUILDING BLOCK CONSTRUCTION 262 7.2.2
ROBUST OPEN, FUNCTIONALIZED, AND SIZEABLE FRAMEWORKS 262 7.2.3 MOFS
SYNTHESIS 264 7.2.4 ADSORPTION PROPERTIES OF MOF 266 7.2. CONTENTS IX
7.4.1 PROPERTIES OF MOF IN CATALYSIS 179 7.4.1.1 LEWIS ACID CATALYSIS
280 7.4.1.2 BROENSTED ACID CATALYSIS 182 7.4.1.3 BASIC AND
ENANTIOSELECTIVE CATALYSIS 182 7.4.1.4 C-C COUPLING 183 7.4.1.5 METAL
CATALYSIS 183 7.4.1.6 WALL FUNCTIONALIZATION 183 7.4.1.7
POSTFUNCTIONALIZATION 184 7.4.2 MOFS - ARE THEY "HETEROGENIZED"
CATALYSTS OR SOLID CATALYSTS? 285 7.4.2.1 ENGINEERING OF STRUCTURAL
DEFECTS IN MOF 285 7.4.2.2 PROBING ACID CENTERS BY ALKYLATION REACTIONS
285 7.4.2.3 CATALYST CHARACTERIZATION 187 7.4.2.4 GENERA] STATEMENTS ON
MOF APPLICATION FOR CATALYSIS 288 7.5 CONCLUSION 288 REFERENCES 189 8
DESIGN OF BIMETALLIC CATALYSTS: FROM MODEL SURFACES TO SUPPORTED
CATALYSTS 295 JEFFREY P. BOSCO, MICHAEL P. HUMBERT, AND JINGGUANG C.
CHEN 8.1 INTRODUCTION 295 8.2 EXPERIMENTAL AND THEORETICAL METHODS 196
8.2.1 EXPERIMENTAL TECHNIQUES 296 8.2.2 DFTMODELING 199 8.3 RESULTS AND
DISCUSSION 299 8.3.1 UHV AND DFT SRUDIES ON PT-NI MODEL SURFACES 1 99
8.3.1.1 ADSORPTION AND DESORPTION OF HYDROGEN 200 8.3.1.2
DISPROPORTIONATION AND HYDROGENATION OF CYCLOHEXENE 202 CONTENTS 9.2.4
SELF-ASSEMBLY OF ZEOLITE SEEDS INTO MESOPHASE 223 9.2.5 ORGANIC
FUNCTIONAL GROUPS AS CATALYSTS 224 9.3 DESIGNING CATALYSTS AT THE
NANOPARTICLE SURFACES 225 9.3.1 POLYOXOMETALATES: NANOPARTIDES WITH
CATIONS 225 9.3.2 DENDRIMER-STABILIZED METAL NANOPARTICLES 226 9.4
PERSPECTIVES 226 REFERENCES 227 10 THEORY-AIDED CATALYST DESIGN 232
MATTHEW NEUROCK 10.1 INTRODUCTION 231 10.2 CATALYTIC DESCRIPTORS 234
10.2.1 ELECTRONIC DESCRIPTORS 234 10.2.2 ENERGETIC DESCRIPTORS 235
10.2.3 ADSORPTION ENERGIES OR BINDING ENERGIES 236 10.2.4
HIGH-THROUGHPUT SCREENING 238 10.3 HIGH-THROUGHPUT SIMULATION AND DESIGN
242 10.3.1 NO DECOMPOSITION 244 10.3.2 VINYL ACETATE (VAM) SYNTHESIS 249
10.4 CONTROLLED PATTERNING 252 10.5 CATALYST SYNTHESIS AND STABILITY 252
10.6 CONCLUSIONS 253 REFERENCES 254 11 USE OF IN SITU XA CONTENTS XI 12
CATALYST DESIGN THROUGH DUAL TEMPLATING 295 MOISES A. CARREON AND VADIM
V. CULIANTS 12.1 INTRODUCTION 295 12.2 SURFACTANT-ASSISTED SELF-ASSEMBLY
OF MESOPOROUS METAL OXIDES 297 12.2.1 FUNDAMENTALS 297 12.2.2 THERMAL
STABILITY CONSIDERATIONS 297 12.2.3 MESOSTRUCTURING VIA
EVAPORATION-INDUCED SELF-ASSEMBLY 299 12.3 COLLOIDAL SPHERE TEMPLATING
OF MACROPOROUS METAL OXIDES 301 12.4 DUAL TEMPLATING OF METAL OXIDES 303
12.5 CATALYTIC APPLICATIONS 305 12.5.1 MESOPOROUS METAL OXIDES 305
12.5.2 MACROPOROUS METAL OXIDES 310 12.5.3 METAL OXIDES OBTAINED VIA
DUAL TEMPLATING 311 12.6 CONCLUDING REMARKS 312 REFERENCES 313 INDEX 315 |
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| language | English |
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| spelling | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling ed. by Umit S. Ozkan Weinheim WILEY-VCH 2009 XVII, 322 S. Ill., graph. Darst. 240 mm x 170 mm txt rdacontent n rdamedia nc rdacarrier Catalysts Design Heterogeneous catalysis Heterogene Katalyse (DE-588)4123377-3 gnd rswk-swf Molekulardesign (DE-588)4265444-0 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf Katalysator (DE-588)4029919-3 s Molekulardesign (DE-588)4265444-0 s Heterogene Katalyse (DE-588)4123377-3 s DE-604 Ozkan, Umit S. Sonstige (DE-588)137297947 oth text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3152684&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017076988&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling Catalysts Design Heterogeneous catalysis Heterogene Katalyse (DE-588)4123377-3 gnd Molekulardesign (DE-588)4265444-0 gnd Katalysator (DE-588)4029919-3 gnd |
| subject_GND | (DE-588)4123377-3 (DE-588)4265444-0 (DE-588)4029919-3 |
| title | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling |
| title_auth | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling |
| title_exact_search | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling |
| title_full | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling ed. by Umit S. Ozkan |
| title_fullStr | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling ed. by Umit S. Ozkan |
| title_full_unstemmed | Design of heterogeneous catalysts new approaches based on synthesis, characterization and modeling ed. by Umit S. Ozkan |
| title_short | Design of heterogeneous catalysts |
| title_sort | design of heterogeneous catalysts new approaches based on synthesis characterization and modeling |
| title_sub | new approaches based on synthesis, characterization and modeling |
| topic | Catalysts Design Heterogeneous catalysis Heterogene Katalyse (DE-588)4123377-3 gnd Molekulardesign (DE-588)4265444-0 gnd Katalysator (DE-588)4029919-3 gnd |
| topic_facet | Catalysts Design Heterogeneous catalysis Heterogene Katalyse Molekulardesign Katalysator |
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