Fuel cell catalysis: a surface science approach
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Hoboken, NJ
Wiley
2009
|
| Schriftenreihe: | The Wiley series on electrocatalysis and electrochemistry
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis Klappentext |
| Beschreibung: | XIII, 697 S. Ill., graph. Darst. |
| ISBN: | 9780470131169 |
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Datensatz im Suchindex
| _version_ | 1804138051889266688 |
|---|---|
| adam_text | A CORE REFERENCE ON FUEL CELL CATALYSIS
Fuel cells represent an important alternative energy source and a very
active area of research. Fuel Cell Catalysis brings together world leaders
in this field, providing a unique combination of state-of-the-art theory
and computational and experimental methods. With an emphasis on under¬
standing fuel cell catalysis at the molecular level, this text covers fundamen¬
tal principles, future challenges, and important current research themes.
Fuel Cell Catalysis:
•
Provides a molecular-level description of catalysis for low-temperature
polymer-electrolyte membrane fuel cells, including both hydrogen-
oxygen cells and direct alcohol cells
•
Examines catalysis issues of both anode and cathode such as oxygen
reduction, alcohol oxidation, and CO tolerance
•
Features a timely and forward-looking approach through emphasis on
novel aspects such as computation and bio-inspiration
•
Reviews the use and potential of surface-sensitive techniques like vibra-
tional spectroscopy
(IR,
Raman, nonlinear spectroscopy, laser), scanning
tunneling microscopy, X-ray scattering, NMR, electrochemical tech¬
niques, and more
•
Reviews the use and potential of such modern computational tech¬
niques as DFT, ah initio MD, kinetic Monte Carlo simulations, and more
•
Surveys important trends in reactivity and structure sensitivity, nano-
particles, dynamic
catalysis, electrocatalysis vs. gas-phase catalysis, new
experimental techniques, and
nontraditional
catalysts
This cutting-edge collection offers a core reference for electrochemists,
electrocatalysis researchers, surface and physical chemists, chemical and
automotive engineers, and researchers in
academia,
research institutes,
and industry.
MARC: T. M.
KOPER
obtained his PhD (cum
laude)
with Professor J. H.
Sluyters from Utrecht University in
1994
on Far-from-equilibrium phenom¬
ena in electrochemical systems: instabilities, oscillations and chaos. He is
currently a Full Professor in Fundamental Surface Science at Leiden University,
where he studies electrochemistry, electrocatalysis, electrochemical surface
science, and theoretical and computational electrochemistry.
CONTENTS
Preface
to the Wiley Series on Electrocatalysis and
Electrochemistry
vii
Preface
ix
List of Contributors
xi
1.
Electrocatalysis of Oxygen Reduction in Polymer
Electrolyte Fuel Cells: A Brief History and a Critical
Examination of Present Theory and Diagnostics
1
Shimshon
Gottesfeld
2.
Electrochemical Electron Transfer:
From Marcus Theory to Electrocatalysis
31
E. Santos and W. Schmickler
3.
Electrocatalysis and Catalyst Screening from Density
Functional Theory Calculations
57
J. Rossmeisl, J. Greeley, and G.S.
Karlberg
4.
First-Principles Simulation of the Active Sites and Reaction
Environment in Electrocatalysis
93
Michael J.
Janik,
Sally A. Wasileski, Christopher D. Taylor,
and Matthew Neurock
5. Ab Initio
Atomistic Thermodynamics for Fuel Cell Catalysis
129
Timo
Jacob
6.
Mechanisms of the Oxidation of Carbon Monoxide and
Small Organic Molecules at Metal Electrodes
159
Marc
T.M. Koper,
Stanley C.S. Lai, and Enrique
Herrero
7.
Clues for the Molecular-Level Understanding of Electrocatalysis on
Single-Crystal Platinum Surfaces Modified by p-Block
Adatoms 209
V. Climent,
N.
García-Aráez,
and J.M. Feliu
8.
Electrochemistry at Well-Characterized Bimetallic Surfaces
245
Vojislav
R.
Stamenkovic and Nenad M. Markovic
VÍ
CONTENTS
9.
Recent
Developments
¡η
the Electrocatalysis of the O2
Reduction Reaction
271
Ye Xu, Minhua Shao,
Manos Mavrikakis,
and
Radoslav R.
Adzie
10.
Electrocatalysis at Platinum and Bimetallic Alloys
317
Masahiro Watanabe and Hiroyuki Uchida
11.
Electrocatalysis for the Direct Alcohol Fuel Cell
343
J.-M.
Leger,
С.
Coutanceau, and
C.
Lamy
12.
Broadband Sum Frequency Generation Studies of Surface
Intermediates Involved in Fuel Cell Electrocatalysis
375
G.Q.
Lu,
A. Lagutchev, T. Takeshita, R.L.
Behrens, Dana D.
Dlott,
and A. Wieckowski
13. Methanol,
Formaldehyde, and Formic Acid Adsorption/Oxidation
on a Carbon-Supported Pt Nanoparticle Fuel Cell Catalyst:
A Comparative Quantitative DEMS Study
411
Z. Jusys and R.J. Behm
14.
The Effect of Structurally Well-Defined Pt Modification
on the Electrochemical and Electrocatalytic Properties
of Ru(0001) Electrodes
465
HE. Hosier and R.J. Behm
15.
Size Effects in Electrocatalysis of Fuel Cell Reactions
on Supported Metal Nanoparticles
507
Frederic
Maillard,
Sergey Pronkin, and Elena R. Savinova
16.
Support and Particle Size Effects in Electrocatalysis
567
Brian E. Hayden and Jens-Peter
Suchsland
17.
Electrocatalysis for Fuel Cells at Enzyme-Modified Electrodes
593
K.A. Vincent, S.C. Barton, G.W. Canters, and
H.A.
Heering
18.
Metalloporphyrin Catalysts of Oxygen Reduction
637
Roman Boulatov
Index
695
|
| adam_txt |
A CORE REFERENCE ON FUEL CELL CATALYSIS
Fuel cells represent an important alternative energy source and a very
active area of research. Fuel Cell Catalysis brings together world leaders
in this field, providing a unique combination of state-of-the-art theory
and computational and experimental methods. With an emphasis on under¬
standing fuel cell catalysis at the molecular level, this text covers fundamen¬
tal principles, future challenges, and important current research themes.
Fuel Cell Catalysis:
•
Provides a molecular-level description of catalysis for low-temperature
polymer-electrolyte membrane fuel cells, including both hydrogen-
oxygen cells and direct alcohol cells
•
Examines catalysis issues of both anode and cathode such as oxygen
reduction, alcohol oxidation, and CO tolerance
•
Features a timely and forward-looking approach through emphasis on
novel aspects such as computation and bio-inspiration
•
Reviews the use and potential of surface-sensitive techniques like vibra-
tional spectroscopy
(IR,
Raman, nonlinear spectroscopy, laser), scanning
tunneling microscopy, X-ray scattering, NMR, electrochemical tech¬
niques, and more
•
Reviews the use and potential of such modern computational tech¬
niques as DFT, ah initio MD, kinetic Monte Carlo simulations, and more
•
Surveys important trends in reactivity and structure sensitivity, nano-
particles, "dynamic
"
catalysis, electrocatalysis vs. gas-phase catalysis, new
experimental techniques, and
nontraditional
catalysts
This cutting-edge collection offers a core reference for electrochemists,
electrocatalysis researchers, surface and physical chemists, chemical and
automotive engineers, and researchers in
academia,
research institutes,
and industry.
MARC: T. M.
KOPER
obtained his PhD (cum
laude)
with Professor J. H.
Sluyters from Utrecht University in
1994
on "Far-from-equilibrium phenom¬
ena in electrochemical systems: instabilities, oscillations and chaos." He is
currently a Full Professor in Fundamental Surface Science at Leiden University,
where he studies electrochemistry, electrocatalysis, electrochemical surface
science, and theoretical and computational electrochemistry.
CONTENTS
Preface
to the Wiley Series on Electrocatalysis and
Electrochemistry
vii
Preface
ix
List of Contributors
xi
1.
Electrocatalysis of Oxygen Reduction in Polymer
Electrolyte Fuel Cells: A Brief History and a Critical
Examination of Present Theory and Diagnostics
1
Shimshon
Gottesfeld
2.
Electrochemical Electron Transfer:
From Marcus Theory to Electrocatalysis
31
E. Santos and W. Schmickler
3.
Electrocatalysis and Catalyst Screening from Density
Functional Theory Calculations
57
J. Rossmeisl, J. Greeley, and G.S.
Karlberg
4.
First-Principles Simulation of the Active Sites and Reaction
Environment in Electrocatalysis
93
Michael J.
Janik,
Sally A. Wasileski, Christopher D. Taylor,
and Matthew Neurock
5. Ab Initio
Atomistic Thermodynamics for Fuel Cell Catalysis
129
Timo
Jacob
6.
Mechanisms of the Oxidation of Carbon Monoxide and
Small Organic Molecules at Metal Electrodes
159
Marc
T.M. Koper,
Stanley C.S. Lai, and Enrique
Herrero
7.
Clues for the Molecular-Level Understanding of Electrocatalysis on
Single-Crystal Platinum Surfaces Modified by p-Block
Adatoms 209
V. Climent,
N.
García-Aráez,
and J.M. Feliu
8.
Electrochemistry at Well-Characterized Bimetallic Surfaces
245
Vojislav
R.
Stamenkovic and Nenad M. Markovic
VÍ
CONTENTS
9.
Recent
Developments
¡η
the Electrocatalysis of the O2
Reduction Reaction
271
Ye Xu, Minhua Shao,
Manos Mavrikakis,
and
Radoslav R.
Adzie
10.
Electrocatalysis at Platinum and Bimetallic Alloys
317
Masahiro Watanabe and Hiroyuki Uchida
11.
Electrocatalysis for the Direct Alcohol Fuel Cell
343
J.-M.
Leger,
С.
Coutanceau, and
C.
Lamy
12.
Broadband Sum Frequency Generation Studies of Surface
Intermediates Involved in Fuel Cell Electrocatalysis
375
G.Q.
Lu,
A. Lagutchev, T. Takeshita, R.L.
Behrens, Dana D.
Dlott,
and A. Wieckowski
13. Methanol,
Formaldehyde, and Formic Acid Adsorption/Oxidation
on a Carbon-Supported Pt Nanoparticle Fuel Cell Catalyst:
A Comparative Quantitative DEMS Study
411
Z. Jusys and R.J. Behm
14.
The Effect of Structurally Well-Defined Pt Modification
on the Electrochemical and Electrocatalytic Properties
of Ru(0001) Electrodes
465
HE. Hosier and R.J. Behm
15.
Size Effects in Electrocatalysis of Fuel Cell Reactions
on Supported Metal Nanoparticles
507
Frederic
Maillard,
Sergey Pronkin, and Elena R. Savinova
16.
Support and Particle Size Effects in Electrocatalysis
567
Brian E. Hayden and Jens-Peter
Suchsland
17.
Electrocatalysis for Fuel Cells at Enzyme-Modified Electrodes
593
K.A. Vincent, S.C. Barton, G.W. Canters, and
H.A.
Heering
18.
Metalloporphyrin Catalysts of Oxygen Reduction
637
Roman Boulatov
Index
695 |
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| spelling | Fuel cell catalysis a surface science approach ed. by Marc T. M. Koper Hoboken, NJ Wiley 2009 XIII, 697 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier The Wiley series on electrocatalysis and electrochemistry Fuel cells Catalysis Brennstoffzelle (DE-588)4008195-3 gnd rswk-swf Elektrokatalyse (DE-588)4151819-6 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Brennstoffzelle (DE-588)4008195-3 s Elektrokatalyse (DE-588)4151819-6 s DE-604 Koper, Marc T. M. 1967- Sonstige (DE-588)138227381 oth Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016761679&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016761679&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext |
| spellingShingle | Fuel cell catalysis a surface science approach Fuel cells Catalysis Brennstoffzelle (DE-588)4008195-3 gnd Elektrokatalyse (DE-588)4151819-6 gnd |
| subject_GND | (DE-588)4008195-3 (DE-588)4151819-6 (DE-588)4143413-4 |
| title | Fuel cell catalysis a surface science approach |
| title_auth | Fuel cell catalysis a surface science approach |
| title_exact_search | Fuel cell catalysis a surface science approach |
| title_exact_search_txtP | Fuel cell catalysis a surface science approach |
| title_full | Fuel cell catalysis a surface science approach ed. by Marc T. M. Koper |
| title_fullStr | Fuel cell catalysis a surface science approach ed. by Marc T. M. Koper |
| title_full_unstemmed | Fuel cell catalysis a surface science approach ed. by Marc T. M. Koper |
| title_short | Fuel cell catalysis |
| title_sort | fuel cell catalysis a surface science approach |
| title_sub | a surface science approach |
| topic | Fuel cells Catalysis Brennstoffzelle (DE-588)4008195-3 gnd Elektrokatalyse (DE-588)4151819-6 gnd |
| topic_facet | Fuel cells Catalysis Brennstoffzelle Elektrokatalyse Aufsatzsammlung |
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