Verfügbarkeit: Modern supramolecular gold chemistry

Modern supramolecular gold chemistry: gold-metal interactions and applications

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Weitere Verfasser:	Laguna, Antonio (HerausgeberIn)
Format:	Buch
Sprache:	English
Veröffentlicht:	Weinheim WILEY-VCH 2008
Ausgabe:	1. Aufl.
Schriftenreihe:	Further reading
Schlagworte:	Gold compounds Supramolecular chemistry Supramolekulare Chemie Gold
Online-Zugang:	Inhaltstext Inhaltsverzeichnis
Beschreibung:	XX, 505 S. Ill., graph. Darst.
ISBN:	9783527320295 3527320296

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adam_text	Contents Prefece XI Abbreviation XV List of Contributors XIX 1 The Chemistry of Cold 1 M. Concepción Cimeno 1.1 Introduction 1 1.1.1 History 1 1.1.2 Chemical and Physical Properties 2 1.1.3 Theoretical Considerations 2 1.2 Chemistry 4 1.2.1 Gold(-I) Compounds 5 1.2.2 Gold(O) and Gold Clusters 6 1.2.3 Gold Nanopartides and Nanodusters 8 1.2.4 Gold(I) Complexes 10 1.2.4.1 Mononudear [AuXL], [Aul^]"1" or [AuX2]~ Complexes 10 1.2.4.2 Gold(I) Complexes with Polydentate ligands 14 1.2.4.3 Three and Four-Coordinate Gold(I) Complexes 20 1.2.4.4 Oligomeric Gold(I) Complexes 23 1.2.4.5 Single Heteroatom Bridged Gold(I) Complexes 26 1.2.4.6 Organometallic Gold(I) Complexes 30 1.2.5 Gold(II) Complexes 35 1.2.5.1 Mononudear Gold(II) Complexes 35 1.2.5.2 Polynudear Gold(II) Complexes 38 1.2.6 GoldlHI) Complexes 41 1.2.6.1 Organometallic Gold(III) Complexes 41 1.2.6.2 Gold(III) Complexes with Polydentate Ligands 44 1.2.6.3 Gold(III) Complexes with Chalcogen Ligands 46 1.2.7 Gold in Higher Oxidation States 49 References 50 Modern Supramolecular Gold Chemistry: Gold-Metal Interactions and Applications. Edited by Antonio Laguna Copyright © 2008 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim ISBN: 978-3-527-32O29-5 VI Contents 2 Cold-Cold Interactions 65 Olga Crespo 2.1 Introduction 65 2.2 GoldţlJ-Goldţl) Interactions 66 2.2.1 Aggregation of Mononuclear Dicoordinated Gold Units 67 2.2.1.1 Dinudear Aggregates 68 2.2.1.2 Tri- and Tetranudear Associations 73 2.2.1.3 Formation of Infinite Chains and Supramolecular Arrays 76 2.2.2 Clustering of Gold Atoms at One Center 78 2.2.3 Complexes with Bridging Monodentate Iigands 86 2.2.4 Complexes with Bridging Bidentate Iigands 90 2.2.5 Complexes with Polydentate Iigands 110 2.3 Gold(I)-Gold(III) Interactions 113 2.4 Conduding Remarks 117 References 117 3 Cold Nanomaterials 131 Eduardo J. Fernández and Miguel Monge 3.1 Introduction 131 3.2 Molecular Gold Clusters 131 3.2.1 Synthesis and Structural Characterization of Phosphine-Stabilized Gold Clusters 132 3.2.2 Gold Clusters with Other ligand Stabilizers 136 3.3 Large-Size Gold Clusters. The Au55 Case 139 3.4 Gold Nanopartides 144 3.4.1 Synthesis of Gold Nanopartides 144 3.4.1.1 Monolayer Protected Clusters 144 3.4.1.2 Other Iigands Í46 3.4.1.3 Polymers 149 3.4.1.4 Dendrimers 157 3.4.1.5 Seeded Growth 160 3.4.1.6 Nanopartide-Biomolecule Hybrids 163 3.4.1.7 Nanopartide Assembly 165 3.5 Properties and Applications of Gold Nanopartides 169 3.6 Conduding Remarks 172 References 173 4 Gold-Heterometal Interactions and Bonds 181 Cristian Silvestru 4.1 Introduction 181 4.2 Main Group Metal-Gold Compounds 183 4.2.1 Gold-Group 1 Metal Compounds 183 4.2.2 Gold-Mercury Compounds 186 4.2.3 Gold-Group 13 Metal Compounds 192 4.2.3.1 Gold-Gallium Compounds 192 Contents VII 4.2.3.2 Gold-Indium Compounds 194 4.2.3.3 Gold-Thallium Compounds 196 4.2.4 Gold-Group 14 Metal Compounds 217 4.2.4.1 Gold-Silicon Compounds 221 4.2.4.2 Gold-Germanium Compounds 222 4.2.4.3 Gold-Tin Compounds 227 4.2.4.4 Gold-Lead Compounds 231 4.2.5 Gold-Group 15 Metal Compounds 231 4.2.5.1 Gold-Antimony Compounds 232 4.2.5.2 Gold-Bismuth Compounds 235 4.3 Transition Metal-Gold Compounds 235 4.3.1 Gold-Titanium Compounds 237 4.3.2 Gold-Group 5 Metal Compounds 237 4.3.2.1 Gold-Vanadium Compounds 238 4.3.2.2 Gold-Niobium Compounds 238 4.3.3 Gold-Group 6 Metal Compounds 238 4.3.3.1 Gold-Chromium Compounds 238 4.3.3.2 Gold-Molybdenum and Gold -Tungsten Compounds 239 4.3.4 Gold-Group 7 Metal Compounds 241 4.3.4.1 Gold-Manganese and Gold-Rhenium Compounds 241 4.3.4.2 Gold-Technetium Compounds 243 4.3.5 Gold-Group 8 Metal Compounds 243 4.3.6 Gold-Group 9 Metal Compounds 251 4.3.7 Gold-Group 10 Metal Compounds 255 4.3.7.1 Gold-Nickel Compounds 255 4.3.7.2 Gold-Palladium Compounds 255 4.3.7.3 Gold-Platinum Compounds 256 4.3.8 Gold-Group 11 Metal Compounds 260 4.3.8.1 Gold-Copper Compounds 260 4.3.8.2 Gold-Silver Compounds 263 4.4 Concluding Remarks 272 References 272 5 Supramolecular Architecture by Secondary Bonds 295 María Elena Olmos 5.1 Introduction 295 5.2 Supramolecular Gold Entities Built with Gold-Non-Metal Secondary Bonds 296 5.2.1 Secondary Bonds: Au· · NM Interactions 296 5.2.2 Hydrogen Bonds: Au- · H-NM Interactions 314 5.2.3 Au- · ·π Interactions 318 5.3 Supramolecular Gold Entities Built with Non-Metal-Non-Metal Secondary Bonds 320 5.3.1 Secondary Bonds: NM· ■ NM Interactions 320 5.3.2 Hydrogen Bonds: NM· · H-NM Interactions 326 VIII Contents 5.3.3 С-Н· · π Interactions and π· · -π Stacking 337 5.4 Concluding Remarks 341 References 342 6 Luminescence of Supramolecular Cold-Containing Materials 347 José María López-de-Luzurìaga 6.1 Introduction. Conditions for Luminescence in Gold Complexes 347 6.2 Luminescent Supramolecular Gold Entities 351 6.2.1 Networks from Mononudear Units 352 6.2.2 Networks from Dinudear Units 359 6.2.3 Networks from Trinudear Units 367 6.2.4 Networks from Higher Nudearity Systems 375 6.3 Luminescent Supramolecular Gold-Heterometal Entities 376 6.3.1 Supramolecular Gold-Group 11 Metal Complexes 377 6.3.2 Other Supramolecular Gold-Heterometal Complexes 385 6.4 Conduding Remarks 398 References 398 7 Liquid Crystals 403 Manuel Bardajt 7.1 Introduction 403 7.1.1 What Are Liquid Crystals? 403 7.1.2 What Are Metallomesogens? 406 7.1.3 Liquid Crystals Characterization 407 7.1.4 Liquid Crystals Applications 407 7.1.5 The Advantages of Gold 408 7.2 Gold Mesogens 408 7.2.1 Alkynyl Ligands 409 7.2.2 Azobenzene Ligands 4J0 7.2.3 Carbene Ligands 430 7.2.4 Dithiobenzoate Ligands 413 7.2.5 Isocyanide Ligands 4J3 7.2.5.1 Combined with an Alkynyl Ugand 4J4 7.2.5.2 Combined with Halides or Pseudohalides 424 7.2.5.3 Combined with a Perhaloaryl ligand 417 7.2.5.4 Cationic bis(Isocyanide) Compounds 419 7.2.5.5 Chiral Isocyanide 420 7.2.5.6 Binary Mixtures of Isocyanide Derivatives 421 7.2.6 Perhaloaryl Ligands 422 7.2.7 Pyrazolate Ligands 423 7.2.8 Stilbazol Ligands 426 7.3 Conduding Remarks 426 References 426 Contents IX 8 Catalysis 429 M. Carmen Blanco Ortiz 8.1 Introduction 429 8.1.1 Transition Metal Catalysis 430 8.1.2 Gold Catalysis 430 8.2 Homogeneous Catalysis 432 8.2.1 Nudeophilic Additions to C -С Multiple Bonds 432 8.2.1.1 Alienes as Substrates 433 8.2.1.2 Alkenes as Substrates 439 8.2.1.3 Alkynes as Substrates 446 8.2.1.4 Enynes as Substrates 466 8.2.2 Activation of Carbonyl Groups and Alcohols 472 8.2.3 Hydrogénation Reactions 474 8.3 Heterogeneous Catalysis 476 8.3.1 Hydrogénation Reactions 476 8.3.1.1 Alkenes Hydrogénation 476 8.3.1.2 Hydrogénation of oc, ß-Unsaturated Aldehydes 478 8.3.2 Oxidation Reactions 478 8.3.2.1 C -Н Bond Activation 478 8.3.2.2 Oxidation of Alcohols and Aldehydes 479 8.3.2.3 Epoxidation 479 8.3.2.4 Direct Synthesis of Hydrogen Peroxide 480 8.3.3 Reactions Involving Carbon Monoxide 481 8.3.3.1 Carbon Monoxide Oxidation 481 8.3.3.2 Water Gas Shift Reaction 481 8.4 Concluding Remarks 482 References 482 9 Concluding Remarks 491 M. Concepción Gimeno and Antonio Laguna References 494 Index 495
adam_txt	Contents Prefece XI Abbreviation XV List of Contributors XIX 1 The Chemistry of Cold 1 M. Concepción Cimeno 1.1 Introduction 1 1.1.1 History 1 1.1.2 Chemical and Physical Properties 2 1.1.3 Theoretical Considerations 2 1.2 Chemistry 4 1.2.1 Gold(-I) Compounds 5 1.2.2 Gold(O) and Gold Clusters 6 1.2.3 Gold Nanopartides and Nanodusters 8 1.2.4 Gold(I) Complexes 10 1.2.4.1 Mononudear [AuXL], [Aul^]"1" or [AuX2]~ Complexes 10 1.2.4.2 Gold(I) Complexes with Polydentate ligands 14 1.2.4.3 Three and Four-Coordinate Gold(I) Complexes 20 1.2.4.4 Oligomeric Gold(I) Complexes 23 1.2.4.5 Single Heteroatom Bridged Gold(I) Complexes 26 1.2.4.6 Organometallic Gold(I) Complexes 30 1.2.5 Gold(II) Complexes 35 1.2.5.1 Mononudear Gold(II) Complexes 35 1.2.5.2 Polynudear Gold(II) Complexes 38 1.2.6 GoldlHI) Complexes 41 1.2.6.1 Organometallic Gold(III) Complexes 41 1.2.6.2 Gold(III) Complexes with Polydentate Ligands 44 1.2.6.3 Gold(III) Complexes with Chalcogen Ligands 46 1.2.7 Gold in Higher Oxidation States 49 References 50 Modern Supramolecular Gold Chemistry: Gold-Metal Interactions and Applications. Edited by Antonio Laguna Copyright © 2008 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim ISBN: 978-3-527-32O29-5 VI Contents 2 Cold-Cold Interactions 65 Olga Crespo 2.1 Introduction 65 2.2 GoldţlJ-Goldţl) Interactions 66 2.2.1 Aggregation of Mononuclear Dicoordinated Gold Units 67 2.2.1.1 Dinudear Aggregates 68 2.2.1.2 Tri- and Tetranudear Associations 73 2.2.1.3 Formation of Infinite Chains and Supramolecular Arrays 76 2.2.2 Clustering of Gold Atoms at One Center 78 2.2.3 Complexes with Bridging Monodentate Iigands 86 2.2.4 Complexes with Bridging Bidentate Iigands 90 2.2.5 Complexes with Polydentate Iigands 110 2.3 Gold(I)-Gold(III) Interactions 113 2.4 Conduding Remarks 117 References 117 3 Cold Nanomaterials 131 Eduardo J. Fernández and Miguel Monge 3.1 Introduction 131 3.2 Molecular Gold Clusters 131 3.2.1 Synthesis and Structural Characterization of Phosphine-Stabilized Gold Clusters 132 3.2.2 Gold Clusters with Other ligand Stabilizers 136 3.3 Large-Size Gold Clusters. The Au55 Case 139 3.4 Gold Nanopartides 144 3.4.1 Synthesis of Gold Nanopartides 144 3.4.1.1 Monolayer Protected Clusters 144 3.4.1.2 Other Iigands Í46 3.4.1.3 Polymers 149 3.4.1.4 Dendrimers 157 3.4.1.5 Seeded Growth 160 3.4.1.6 Nanopartide-Biomolecule Hybrids 163 3.4.1.7 Nanopartide Assembly 165 3.5 Properties and Applications of Gold Nanopartides 169 3.6 Conduding Remarks 172 References 173 4 Gold-Heterometal Interactions and Bonds 181 Cristian Silvestru 4.1 Introduction 181 4.2 Main Group Metal-Gold Compounds 183 4.2.1 Gold-Group 1 Metal Compounds 183 4.2.2 Gold-Mercury Compounds 186 4.2.3 Gold-Group 13 Metal Compounds 192 4.2.3.1 Gold-Gallium Compounds 192 Contents VII 4.2.3.2 Gold-Indium Compounds 194 4.2.3.3 Gold-Thallium Compounds 196 4.2.4 Gold-Group 14 Metal Compounds 217 4.2.4.1 Gold-Silicon Compounds 221 4.2.4.2 Gold-Germanium Compounds 222 4.2.4.3 Gold-Tin Compounds 227 4.2.4.4 Gold-Lead Compounds 231 4.2.5 Gold-Group 15 Metal Compounds 231 4.2.5.1 Gold-Antimony Compounds 232 4.2.5.2 Gold-Bismuth Compounds 235 4.3 Transition Metal-Gold Compounds 235 4.3.1 Gold-Titanium Compounds 237 4.3.2 Gold-Group 5 Metal Compounds 237 4.3.2.1 Gold-Vanadium Compounds 238 4.3.2.2 Gold-Niobium Compounds 238 4.3.3 Gold-Group 6 Metal Compounds 238 4.3.3.1 Gold-Chromium Compounds 238 4.3.3.2 Gold-Molybdenum and Gold -Tungsten Compounds 239 4.3.4 Gold-Group 7 Metal Compounds 241 4.3.4.1 Gold-Manganese and Gold-Rhenium Compounds 241 4.3.4.2 Gold-Technetium Compounds 243 4.3.5 Gold-Group 8 Metal Compounds 243 4.3.6 Gold-Group 9 Metal Compounds 251 4.3.7 Gold-Group 10 Metal Compounds 255 4.3.7.1 Gold-Nickel Compounds 255 4.3.7.2 Gold-Palladium Compounds 255 4.3.7.3 Gold-Platinum Compounds 256 4.3.8 Gold-Group 11 Metal Compounds 260 4.3.8.1 Gold-Copper Compounds 260 4.3.8.2 Gold-Silver Compounds 263 4.4 Concluding Remarks 272 References 272 5 Supramolecular Architecture by Secondary Bonds 295 María Elena Olmos 5.1 Introduction 295 5.2 Supramolecular Gold Entities Built with Gold-Non-Metal Secondary Bonds 296 5.2.1 Secondary Bonds: Au· · NM Interactions 296 5.2.2 Hydrogen Bonds: Au- · H-NM Interactions 314 5.2.3 Au- · ·π Interactions 318 5.3 Supramolecular Gold Entities Built with Non-Metal-Non-Metal Secondary Bonds 320 5.3.1 Secondary Bonds: NM· ■ NM Interactions 320 5.3.2 Hydrogen Bonds: NM· · H-NM Interactions 326 VIII Contents 5.3.3 С-Н· · π Interactions and π· · -π Stacking 337 5.4 Concluding Remarks 341 References 342 6 Luminescence of Supramolecular Cold-Containing Materials 347 José María López-de-Luzurìaga 6.1 Introduction. Conditions for Luminescence in Gold Complexes 347 6.2 Luminescent Supramolecular Gold Entities 351 6.2.1 Networks from Mononudear Units 352 6.2.2 Networks from Dinudear Units 359 6.2.3 Networks from Trinudear Units 367 6.2.4 Networks from Higher Nudearity Systems 375 6.3 Luminescent Supramolecular Gold-Heterometal Entities 376 6.3.1 Supramolecular Gold-Group 11 Metal Complexes 377 6.3.2 Other Supramolecular Gold-Heterometal Complexes 385 6.4 Conduding Remarks 398 References 398 7 Liquid Crystals 403 Manuel Bardajt 7.1 Introduction 403 7.1.1 What Are Liquid Crystals? 403 7.1.2 What Are Metallomesogens? 406 7.1.3 Liquid Crystals Characterization 407 7.1.4 Liquid Crystals Applications 407 7.1.5 The Advantages of Gold 408 7.2 Gold Mesogens 408 7.2.1 Alkynyl Ligands 409 7.2.2 Azobenzene Ligands 4J0 7.2.3 Carbene Ligands 430 7.2.4 Dithiobenzoate Ligands 413 7.2.5 Isocyanide Ligands 4J3 7.2.5.1 Combined with an Alkynyl Ugand 4J4 7.2.5.2 Combined with Halides or Pseudohalides 424 7.2.5.3 Combined with a Perhaloaryl ligand 417 7.2.5.4 Cationic bis(Isocyanide) Compounds 419 7.2.5.5 Chiral Isocyanide 420 7.2.5.6 Binary Mixtures of Isocyanide Derivatives 421 7.2.6 Perhaloaryl Ligands 422 7.2.7 Pyrazolate Ligands 423 7.2.8 Stilbazol Ligands 426 7.3 Conduding Remarks 426 References 426 Contents IX 8 Catalysis 429 M. Carmen Blanco Ortiz 8.1 Introduction 429 8.1.1 Transition Metal Catalysis 430 8.1.2 Gold Catalysis 430 8.2 Homogeneous Catalysis 432 8.2.1 Nudeophilic Additions to C -С Multiple Bonds 432 8.2.1.1 Alienes as Substrates 433 8.2.1.2 Alkenes as Substrates 439 8.2.1.3 Alkynes as Substrates 446 8.2.1.4 Enynes as Substrates 466 8.2.2 Activation of Carbonyl Groups and Alcohols 472 8.2.3 Hydrogénation Reactions 474 8.3 Heterogeneous Catalysis 476 8.3.1 Hydrogénation Reactions 476 8.3.1.1 Alkenes Hydrogénation 476 8.3.1.2 Hydrogénation of oc, ß-Unsaturated Aldehydes 478 8.3.2 Oxidation Reactions 478 8.3.2.1 C -Н Bond Activation 478 8.3.2.2 Oxidation of Alcohols and Aldehydes 479 8.3.2.3 Epoxidation 479 8.3.2.4 Direct Synthesis of Hydrogen Peroxide 480 8.3.3 Reactions Involving Carbon Monoxide 481 8.3.3.1 Carbon Monoxide Oxidation 481 8.3.3.2 Water Gas Shift Reaction 481 8.4 Concluding Remarks 482 References 482 9 Concluding Remarks 491 M. Concepción Gimeno and Antonio Laguna References 494 Index 495
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physical	XX, 505 S. Ill., graph. Darst.
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publishDateSearch	2008
publishDateSort	2008
publisher	WILEY-VCH
record_format	marc
series2	Further reading
spelling	Modern supramolecular gold chemistry gold-metal interactions and applications Hrsg. Antonio Laguna 1. Aufl. Weinheim WILEY-VCH 2008 XX, 505 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Further reading Gold compounds Supramolecular chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd rswk-swf Gold (DE-588)4157819-3 gnd rswk-swf Gold (DE-588)4157819-3 s Supramolekulare Chemie (DE-588)4306141-2 s DE-604 Laguna, Antonio edt text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3089585&prov=M&dok_var=1&dok_ext=htm Inhaltstext Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016741216&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Modern supramolecular gold chemistry gold-metal interactions and applications Gold compounds Supramolecular chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd Gold (DE-588)4157819-3 gnd
subject_GND	(DE-588)4306141-2 (DE-588)4157819-3
title	Modern supramolecular gold chemistry gold-metal interactions and applications
title_auth	Modern supramolecular gold chemistry gold-metal interactions and applications
title_exact_search	Modern supramolecular gold chemistry gold-metal interactions and applications
title_exact_search_txtP	Modern supramolecular gold chemistry gold-metal interactions and applications
title_full	Modern supramolecular gold chemistry gold-metal interactions and applications Hrsg. Antonio Laguna
title_fullStr	Modern supramolecular gold chemistry gold-metal interactions and applications Hrsg. Antonio Laguna
title_full_unstemmed	Modern supramolecular gold chemistry gold-metal interactions and applications Hrsg. Antonio Laguna
title_short	Modern supramolecular gold chemistry
title_sort	modern supramolecular gold chemistry gold metal interactions and applications
title_sub	gold-metal interactions and applications
topic	Gold compounds Supramolecular chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd Gold (DE-588)4157819-3 gnd
topic_facet	Gold compounds Supramolecular chemistry Supramolekulare Chemie Gold
url	http://deposit.dnb.de/cgi-bin/dokserv?id=3089585&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016741216&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
work_keys_str_mv	AT lagunaantonio modernsupramoleculargoldchemistrygoldmetalinteractionsandapplications

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