Tracking coherences in a dissipative ocean: analysing and controlling Br 2 Ar matrix
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Göttingen
Cuvillier
2008
|
| Ausgabe: | 1. Aufl. |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | VIII, 155 S. Ill., graph. Darst. |
| ISBN: | 9783867276481 |
Internformat
MARC
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| 245 | 1 | 0 | |a Tracking coherences in a dissipative ocean |b analysing and controlling Br 2 Ar matrix |c von Heide Nadda Ibrahim |
| 250 | |a 1. Aufl. | ||
| 264 | 1 | |a Göttingen |b Cuvillier |c 2008 | |
| 300 | |a VIII, 155 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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| 338 | |b nc |2 rdacarrier | ||
| 502 | |a Berlin, Freie Univ., Diss., 2008 | ||
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| 999 | |a oai:aleph.bib-bvb.de:BVB01-022207725 | ||
Datensatz im Suchindex
| _version_ | 1804145266163449856 |
|---|---|
| adam_text | IMAGE 1
CONTENTS
CONTENTS
INTRODUCTION 1
1 COHERENCE AND WAVE PACKET INTERFEROMETRY 4
1.1 WAVE PACKETS 4
1.1.1 FRANCK - CONDON PRINCIPLE 5
1.2 COHERENCE 6
ABSORPTION AND WAVE PACKET INTERFEROMETRY IN THE TIME DEPENDENT
FRAMEWORK 1)
1.2.1 AUTO - CORRELATION WITH NS EXCITATION 12
1.2.2 CROSS - CORRELATION WITH FS PULSE TRAIN EXCITATION 14
2 SYSTEM: BR 2/AR 15
2.1 GAS PHASE PROPERTIES 15
2.1.1 PHYSICAL AND CHEMICAL PROPERTIES 15
2.1.2 ELECTRONIC STRUCTURE 15
2.1.3 SPECTROSCOPIC PROPERTIES OF FREE BR2 MOLECULES 16
2.1.4 SELECTION RULES 16
2.2 PROPERTIES OF HALOGENS IN THE CAGE: STATE OF THE ART 17
2.2.1 CAGE EFFECT 18
2.2.2 ELECTRONIC AND VIBRATIONAL COUPLING WITH THE LATTICE 19
2.2.3 ABSORPTION AND EXCITATION SPECTRA OF BR 2/AR 21
2.2.4 EMISSION SPECTROSCOPY OF BR 2/AR 22
2.2.5 PREDISSOCIATION 24
2.2.6 VIBRATIONAL ENERGY RELAXATION 26
2.2.7 COHERENCE TIMES 28
3 EXPERIMENTAL TECHNIQUE 29
3.1 EXPERIMENTAL BASICS 29
3.1.1 SAMPLE PREPARATION 29
3.1.2 FLUORESCENCE DETECTION 29
3.2 FREQUENCY RESOLVED SPECTROSCOPY 30
3.3 TIME RESOLVED SPECTROSCOPY 31
3.3.1 EXPERIMENTAL OVERVIEW 31
3.3.2 ULTRASHORT LASER PULSES 33
3.3.3 SINGLE PUMP - PROBE EXPERIMENT 39
3.4 CONTROL INSTRUMENTS FOR THE GENERATION OF PULSE SEQUENCES 42
3.4.1 MICHELSON INTERFEROMETER 42
3.4.2 PULSE SHAPER 43
3.4.3 DOUBLE PUMP EXPERIMENT 49
GESCANNT DURCH
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/989862305
DIGITALISIERT DURCH
IMAGE 2
CONTENTS
3.4.4 MULTIPLE PUMP - PROBE EXPERIMENT 51
4 ANALYSIS 1: FREQUENCY RESOLVED SPECTROSCOPY 53
4.1 RESULTS 54
4.1.1 EMISSION SPECTRA FROM COVALENT EXCITED STATES B, A AND A 54
4.1.2 EXCITATION OF COVALENT STATES 58
4.1.3 TEMPERATURE DEPENDENCE 65
4.1.4 POLARISATION DEPENDENCE 65
4.1.5 BLEACHING EXPERIMENTS 67
4.2 DISCUSSION 72
5 ANALYSIS 2: TIME RESOLVED SPECTROSCOPY 80
5.1 PUMP - PROBE SPECTROSCOPY RESULTS 80
5.1.1 POLARISATION DEPENDENCE 80
5.1.2 INTENSITY DEPENDENCE 84
5.2 DISCUSSION OF PUMP-PROBE SPECTROSCOPY 86
5.2.1 SIMULATION OF WAVE PACKET DYNAMICS ON THE B-STATE OF FREE BR 2 87
5.2.2 OPEN QUESTIONS 89
6 CONTROL: INTERFERENCE WITH PHASE CONTROLLED PULSE SEQUENCES 93
6.1 TUTORIAL SOLUTION: MICHELSON INTERFEROMETER 93
6.1.1 DOUBLE PULSE EXPERIMENT 93
6.1.2 ELECTRONIC COHERENCE IN THE PLPP SPECTRA 97
6.2 ADVANCED SOLUTION : PULSE SHAPER 99
6.2.1 PULSE TRAIN EXCITATION 99
6.2.2 DOUBLE PUMP - PROBE EXPERIMENT - TIME RESOLVED 102
6.2.3 PULSE TRAIN PUMP - PROBE EXPERIMENT 106
6.3 DISCUSSION OF CONTROL EXPERIMENTS 112
6.3.1 PHASE RECONSTRUCTION 113
6.3.2 PREDISSOCIATION 122
6.3.3 WAVE PACKET INTERFEROMETRY 126
6.3.4 ELECTRONIC COHERENCE 130
SUMMARY 132
BIBLIOGRAPHY 135
APPENDIX A 150
H. IBRAHIM, FU BERLIN
|
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| author | Ibrahim, Heide Nadda 1978- |
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| bvnumber | BV026658487 |
| ctrlnum | (OCoLC)263416946 (DE-599)BVBBV026658487 |
| dewey-full | 535.15 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 535 - Light and related radiation |
| dewey-raw | 535.15 |
| dewey-search | 535.15 |
| dewey-sort | 3535.15 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| edition | 1. Aufl. |
| format | Thesis Book |
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| id | DE-604.BV026658487 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T23:16:43Z |
| institution | BVB |
| isbn | 9783867276481 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-022207725 |
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| owner_facet | DE-188 |
| physical | VIII, 155 S. Ill., graph. Darst. |
| publishDate | 2008 |
| publishDateSearch | 2008 |
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| spelling | Ibrahim, Heide Nadda 1978- Verfasser (DE-588)136374085 aut Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix von Heide Nadda Ibrahim 1. Aufl. Göttingen Cuvillier 2008 VIII, 155 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Berlin, Freie Univ., Diss., 2008 Pump-Probe-Technik (DE-588)4601119-5 gnd rswk-swf VIS-Spektroskopie (DE-588)4117385-5 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Pump-Probe-Technik (DE-588)4601119-5 s VIS-Spektroskopie (DE-588)4117385-5 s DE-188 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022207725&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Ibrahim, Heide Nadda 1978- Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix Pump-Probe-Technik (DE-588)4601119-5 gnd VIS-Spektroskopie (DE-588)4117385-5 gnd |
| subject_GND | (DE-588)4601119-5 (DE-588)4117385-5 (DE-588)4113937-9 |
| title | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix |
| title_auth | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix |
| title_exact_search | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix |
| title_full | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix von Heide Nadda Ibrahim |
| title_fullStr | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix von Heide Nadda Ibrahim |
| title_full_unstemmed | Tracking coherences in a dissipative ocean analysing and controlling Br 2 Ar matrix von Heide Nadda Ibrahim |
| title_short | Tracking coherences in a dissipative ocean |
| title_sort | tracking coherences in a dissipative ocean analysing and controlling br 2 ar matrix |
| title_sub | analysing and controlling Br 2 Ar matrix |
| topic | Pump-Probe-Technik (DE-588)4601119-5 gnd VIS-Spektroskopie (DE-588)4117385-5 gnd |
| topic_facet | Pump-Probe-Technik VIS-Spektroskopie Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022207725&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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