Environmental chemistry of aerosols:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Oxford [u.a.]
Blackwell Publ.
2008
|
| Schlagworte: | |
| Online-Zugang: | lizenzfrei lizenzfrei Inhaltsverzeichnis Inhaltsverzeichnis |
| Beschreibung: | Enth. Literaturangaben und Index. |
| Beschreibung: | XII, 255 S. Ill., graph. Darst. |
| ISBN: | 1405139196 9781405139199 |
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| 245 | 1 | 0 | |a Environmental chemistry of aerosols |c ed. by Ian Colbeck |
| 264 | 1 | |a Oxford [u.a.] |b Blackwell Publ. |c 2008 | |
| 300 | |a XII, 255 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 500 | |a Enth. Literaturangaben und Index. | ||
| 650 | 4 | |a Air - Pollution - Aspect de l'environnement | |
| 650 | 4 | |a Aérosols | |
| 650 | 4 | |a Aérosols - Aspect de l'environnement | |
| 650 | 4 | |a Chimie de l'atmosphère | |
| 650 | 4 | |a Chimie de l'environnement | |
| 650 | 4 | |a Umwelt | |
| 650 | 4 | |a Aerosols | |
| 650 | 4 | |a Aerosols |x Environmental aspects | |
| 650 | 4 | |a Air |x Pollution |x Environmental aspects | |
| 650 | 4 | |a Atmospheric chemistry | |
| 650 | 4 | |a Environmental chemistry | |
| 650 | 0 | 7 | |a Ökologische Chemie |0 (DE-588)4135167-8 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Aerosol |0 (DE-588)4000595-1 |2 gnd |9 rswk-swf |
| 689 | 0 | 0 | |a Ökologische Chemie |0 (DE-588)4135167-8 |D s |
| 689 | 0 | 1 | |a Aerosol |0 (DE-588)4000595-1 |D s |
| 689 | 0 | |5 DE-604 | |
| 700 | 1 | |a Colbeck, Ian |e Sonstige |4 oth | |
| 856 | 4 | |u http://www.loc.gov/catdir/enhancements/fy0805/2007042414-b.html |y Contributor biographical information |z lizenzfrei | |
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Datensatz im Suchindex
| _version_ | 1804136597975728128 |
|---|---|
| adam_text | Contents
List of Contributors
ix
Preface
xi
1
Physical and Chemical Properties of Atmospheric Aerosols
1
Jay Turner and Ian Colbeck
1.1
Introduction
1
1.2
Ambient aerosol size distributions
3
1.2.1
Idealised size distributions of aerosol number and mass
3
1.2.2
Size distribution measurements
6
1.2.3
Dynamics of atmospheric aerosol size distributions
8
1.2.4
Features of selected ambient aerosol size distributions
11
1.3
Major chemical components of ambient fine particulate matter
15
1.4
Aerosol composition as a function of size
21
1.5
Summary and conclusions
22
References
25
2
Nudeation
31
Art Laaksonen and
Kari
E.J. Lehtinen
2.1
Introduction
31
2.2
Nucleation kinetics
31
2.2.1
One-component systems
31
2.2.2
Binary systems
34
2.3
Nucleation thermodynamics
36
2.3.1
One-component systems
36
2.3.2
The classical theory
39
2.3.3
Multicomponent systems
40
2.4
The nucleation theorem
41
2.4.1
Scaling properties of critical clusters
42
2.4.2
An application to atmospheric nucleation
45
References
46
Contents
3
Mass Transfer to Aerosols
49
Charles F. Clement
3.1
Introduction
49
3.1.1
Equilibration between aerosol and gas
51
3.2
Transfer to a particle
52
52
53
55
56
56
57
58
64
65
67
68
68
70
73
75
77
79
81
83
83
er
85
4
Organic Aerosols
91
Mihalis
Lazaríais
4.1
Introduction
91
4.2
Carbon-containing aerosols and their sources
93
4.2.1
Elemental carbon
-
primary organic carbon
93
4.2.2
Secondary organic matter formation (secondary organic carbon)
95
4.2.3
Biological aerosols
96
4.2.4
Biogenic aerosols
98
4.2.5
Modelling biogenic aerosol formation
99
4.2.6
Polycyclic aromatic hydrocarbons
100
4.2.7
Emission inventories of primary organic aerosols and
gaseous precursors
102
4.3
Atmospheric chemistry of organic aerosols
-
field studies
102
4.3.1
Measurements of carbonaceous aerosols
102
4.3.2
Organic compounds
-
source apportionment
104
4.4
Carbonaceous aerosols at urban/rural environments
105
4.5
Summary
09
References
1Ό
3.2.1
Molecular motion
3.2.2
Motion in gases: kinetic theory
3.2.3
Diffusion
3.2.4
Diffusion to an aerosol particle
3.2.5
Combined diffusive and kinetic model
3.2.6
Fuchs
mass transfer model
3.2.7
Heat and mass transfer
3.2.8
Multicomponent droplets and binary growth
3.2.9
Chemical model framework
3.2.10
Kinetic coefficients
3.3
Transfer
to an aerosol
3.3.1
Aerosol description
3.3.2
Mean field approximation
3.3.3
Growth equations
3.3.4
Empirical atmospheric timescales
3.3.5
Redistributive
processes
3.3.6
Nucleation mode mass transfer
3.3.7
Source terms
Appendix: water data
Nomenclature
References
Contents
5 Metals in Aerosols 117
Irena
Grgić
5.1
Introduction
П7
5.2
Physico-chemical characteristics of metals in aerosols
118
5.2.1
Size distribution
118
5.2.2
Chemical speciation
122
5.3
Reactivity of transition metals
128
5.3.1
Photochemical/chemical cycling
128
5.3.2
Interactions of transition metals with S( IV) species
129
References
133
6
Thermodynamics of Aqueous Systems
141
David Topping
6.1
Introduction
141
6.2
Equilibrium
141
6.2.1
The chemical potential
143
6.2.2
Activity
145
6.3
Mixed solvent systems-
abrief
outline
147
6.4
Aqueous systems
148
6.4.1
Water content in the regime subsaturated with respect to
water vapour
148
6.5
General aqueous thermodynamic equilibrium models for
atmospheric aerosols
152
6.6
Inorganic systems
153
6.6 1
Activity coefficients
153
6.6.2
Bulk inorganic contributions to particulate water content in
the regime subsaturated with respect to water vapour
155
6.7
Organic systems
157
6.7.1
Activity coefficients
157
6.7.2
Bulk organic contributions to particulate water content in the
regime subsaturated with respect to water vapour
161
6.8
Mixed inorganic/organic systems
164
6.8.1
Activity coefficients
-
coupled thermodynamics
164
6.8.2
Activity coefficients
-
uncoupled thermodynamics
166
6.8.3
Bulk mixed inorganic/organic contributions to particulate
water content in the regime subsaturated with respect to
water vapour
166
6.8.4
Deliquescence
169
6.9
Temperature-dependent equilibrium
171
6.9 1
Deliquescence
171
6.9.2
Gas-to-particle partitioning
173
6.9.3
Activity
174
6.10
The influence of curvature
175
6.10.1
The Kelvin effect
175
Contents
6.10.2 The Köhler
equation
-
describing the equilibrium between a
curved particle and its humid environment: basic equilibrium
considerations
177
References
181
7
Stratospheric Chemistry: Aerosols and the Ozone Layer
193
Rob MacKenzie
7.1
Introduction
193
7.2
General properties of the stratospheric aerosol layer
195
7.3
General stratospheric chemistry
197
7.3.1
Catalysed ozone loss
197
7.3.2
Initiation, null cycles, and termination of stratospheric
chain reactions
199
7.4
Heterogeneous stratospheric chemistry
200
7.5
Polar stratospheric clouds and the ozone hole
201
7.6
Volcanic aerosol
203
7.7
Meteoritic aerosol
207
7.8
Interactions between stratospheric chemistry and climate
208
References
210
8
Aerosol Chemistry in Remote Locations
217
Urs Baltensperger
and
Markus Furger
8.1
Introduction
217
8.1.1
Definition of remote locations
217
8.1.2
Aerosol measurement and monitoring
219
8.1.3
Processes and mechanisms
220
8.2
Observations
224
8.2.1
Oceans and marine locations
225
8.2.2
Antarctica
228
8.2.3
Arctic
232
8.2.4
Tropical forests
235
8.2.5
Boreal forests
238
8.2.6
High elevation and free troposphere
239
8.3
Summary
242
References 244
Index
253
The colour plate section follows page
228
|
| adam_txt |
Contents
List of Contributors
ix
Preface
xi
1
Physical and Chemical Properties of Atmospheric Aerosols
1
Jay Turner and Ian Colbeck
1.1
Introduction
1
1.2
Ambient aerosol size distributions
3
1.2.1
Idealised size distributions of aerosol number and mass
3
1.2.2
Size distribution measurements
6
1.2.3
Dynamics of atmospheric aerosol size distributions
8
1.2.4
Features of selected ambient aerosol size distributions
11
1.3
Major chemical components of ambient fine particulate matter
15
1.4
Aerosol composition as a function of size
21
1.5
Summary and conclusions
22
References
25
2
Nudeation
31
Art Laaksonen and
Kari
E.J. Lehtinen
2.1
Introduction
31
2.2
Nucleation kinetics
31
2.2.1
One-component systems
31
2.2.2
Binary systems
34
2.3
Nucleation thermodynamics
36
2.3.1
One-component systems
36
2.3.2
The classical theory
39
2.3.3
Multicomponent systems
40
2.4
The nucleation theorem
41
2.4.1
Scaling properties of critical clusters
42
2.4.2
An application to atmospheric nucleation
45
References
46
Contents
3
Mass Transfer to Aerosols
49
Charles F. Clement
3.1
Introduction
49
3.1.1
Equilibration between aerosol and gas
51
3.2
Transfer to a particle
52
52
53
55
56
56
57
58
64
65
67
68
68
70
73
75
77
79
81
83
83
er
85
4
Organic Aerosols
91
Mihalis
Lazaríais
4.1
Introduction
91
4.2
Carbon-containing aerosols and their sources
93
4.2.1
Elemental carbon
-
primary organic carbon
93
4.2.2
Secondary organic matter formation (secondary organic carbon)
95
4.2.3
Biological aerosols
96
4.2.4
Biogenic aerosols
98
4.2.5
Modelling biogenic aerosol formation
99
4.2.6
Polycyclic aromatic hydrocarbons
100
4.2.7
Emission inventories of primary organic aerosols and
gaseous precursors
102
4.3
Atmospheric chemistry of organic aerosols
-
field studies
102
4.3.1
Measurements of carbonaceous aerosols
102
4.3.2
Organic compounds
-
source apportionment
104
4.4
Carbonaceous aerosols at urban/rural environments
105
4.5
Summary
'09
References
1Ό
3.2.1
Molecular motion
3.2.2
Motion in gases: kinetic theory
3.2.3
Diffusion
3.2.4
Diffusion to an aerosol particle
3.2.5
Combined diffusive and kinetic model
3.2.6
Fuchs
mass transfer model
3.2.7
Heat and mass transfer
3.2.8
Multicomponent droplets and binary growth
3.2.9
Chemical model framework
3.2.10
Kinetic coefficients
3.3
Transfer
to an aerosol
3.3.1
Aerosol description
3.3.2
Mean field approximation
3.3.3
Growth equations
3.3.4
Empirical atmospheric timescales
3.3.5
Redistributive
processes
3.3.6
Nucleation mode mass transfer
3.3.7
Source terms
Appendix: water data
Nomenclature
References
Contents
5 Metals in Aerosols 117
Irena
Grgić
5.1
Introduction
П7
5.2
Physico-chemical characteristics of metals in aerosols
118
5.2.1
Size distribution
118
5.2.2
Chemical speciation
122
5.3
Reactivity of transition metals
128
5.3.1
Photochemical/chemical cycling
128
5.3.2
Interactions of transition metals with S( IV) species
129
References
133
6
Thermodynamics of Aqueous Systems
141
David Topping
6.1
Introduction
141
6.2
Equilibrium
141
6.2.1
The chemical potential
143
6.2.2
Activity
145
6.3
Mixed solvent systems-
abrief
outline
147
6.4
Aqueous systems
148
6.4.1
Water content in the regime subsaturated with respect to
water vapour
148
6.5
General aqueous thermodynamic equilibrium models for
atmospheric aerosols
152
6.6
Inorganic systems
153
6.6 1
Activity coefficients
153
6.6.2
Bulk inorganic contributions to particulate water content in
the regime subsaturated with respect to water vapour
155
6.7
Organic systems
157
6.7.1
Activity coefficients
157
6.7.2
Bulk organic contributions to particulate water content in the
regime subsaturated with respect to water vapour
161
6.8
Mixed inorganic/organic systems
164
6.8.1
Activity coefficients
-
coupled thermodynamics
164
6.8.2
Activity coefficients
-
uncoupled thermodynamics
166
6.8.3
Bulk mixed inorganic/organic contributions to particulate
water content in the regime subsaturated with respect to
water vapour
166
6.8.4
Deliquescence
169
6.9
Temperature-dependent equilibrium
171
6.9 1
Deliquescence
171
6.9.2
Gas-to-particle partitioning
173
6.9.3
Activity
174
6.10
The influence of curvature
175
6.10.1
The Kelvin effect
175
Contents
6.10.2 The Köhler
equation
-
describing the equilibrium between a
curved particle and its humid environment: basic equilibrium
considerations
177
References
181
7
Stratospheric Chemistry: Aerosols and the Ozone Layer
193
Rob MacKenzie
7.1
Introduction
193
7.2
General properties of the stratospheric aerosol layer
195
7.3
General stratospheric chemistry
197
7.3.1
Catalysed ozone loss
197
7.3.2
Initiation, null cycles, and termination of stratospheric
chain reactions
199
7.4
Heterogeneous stratospheric chemistry
200
7.5
Polar stratospheric clouds and the'ozone hole'
201
7.6
Volcanic aerosol
203
7.7
Meteoritic aerosol
207
7.8
Interactions between stratospheric chemistry and climate
208
References
210
8
Aerosol Chemistry in Remote Locations
217
Urs Baltensperger
and
Markus Furger
8.1
Introduction
217
8.1.1
Definition of'remote locations'
217
8.1.2
Aerosol measurement and monitoring
219
8.1.3
Processes and mechanisms
220
8.2
Observations
224
8.2.1
Oceans and marine locations
225
8.2.2
Antarctica
228
8.2.3
Arctic
232
8.2.4
Tropical forests
235
8.2.5
Boreal forests
238
8.2.6
High elevation and free troposphere
239
8.3
Summary
242
References 244
Index
253
The colour plate section follows page
228 |
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| id | DE-604.BV022499505 |
| illustrated | Illustrated |
| index_date | 2024-07-02T17:54:57Z |
| indexdate | 2024-07-09T20:58:56Z |
| institution | BVB |
| isbn | 1405139196 9781405139199 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-015706591 |
| oclc_num | 175218012 |
| open_access_boolean | |
| owner | DE-703 DE-83 |
| owner_facet | DE-703 DE-83 |
| physical | XII, 255 S. Ill., graph. Darst. |
| publishDate | 2008 |
| publishDateSearch | 2008 |
| publishDateSort | 2008 |
| publisher | Blackwell Publ. |
| record_format | marc |
| spelling | Environmental chemistry of aerosols ed. by Ian Colbeck Oxford [u.a.] Blackwell Publ. 2008 XII, 255 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Enth. Literaturangaben und Index. Air - Pollution - Aspect de l'environnement Aérosols Aérosols - Aspect de l'environnement Chimie de l'atmosphère Chimie de l'environnement Umwelt Aerosols Aerosols Environmental aspects Air Pollution Environmental aspects Atmospheric chemistry Environmental chemistry Ökologische Chemie (DE-588)4135167-8 gnd rswk-swf Aerosol (DE-588)4000595-1 gnd rswk-swf Ökologische Chemie (DE-588)4135167-8 s Aerosol (DE-588)4000595-1 s DE-604 Colbeck, Ian Sonstige oth http://www.loc.gov/catdir/enhancements/fy0805/2007042414-b.html Contributor biographical information lizenzfrei http://www.loc.gov/catdir/enhancements/fy0805/2007042414-d.html Publisher description lizenzfrei http://www.loc.gov/catdir/enhancements/fy0805/2007042414-t.html lizenzfrei Inhaltsverzeichnis Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=015706591&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Environmental chemistry of aerosols Air - Pollution - Aspect de l'environnement Aérosols Aérosols - Aspect de l'environnement Chimie de l'atmosphère Chimie de l'environnement Umwelt Aerosols Aerosols Environmental aspects Air Pollution Environmental aspects Atmospheric chemistry Environmental chemistry Ökologische Chemie (DE-588)4135167-8 gnd Aerosol (DE-588)4000595-1 gnd |
| subject_GND | (DE-588)4135167-8 (DE-588)4000595-1 |
| title | Environmental chemistry of aerosols |
| title_auth | Environmental chemistry of aerosols |
| title_exact_search | Environmental chemistry of aerosols |
| title_exact_search_txtP | Environmental chemistry of aerosols |
| title_full | Environmental chemistry of aerosols ed. by Ian Colbeck |
| title_fullStr | Environmental chemistry of aerosols ed. by Ian Colbeck |
| title_full_unstemmed | Environmental chemistry of aerosols ed. by Ian Colbeck |
| title_short | Environmental chemistry of aerosols |
| title_sort | environmental chemistry of aerosols |
| topic | Air - Pollution - Aspect de l'environnement Aérosols Aérosols - Aspect de l'environnement Chimie de l'atmosphère Chimie de l'environnement Umwelt Aerosols Aerosols Environmental aspects Air Pollution Environmental aspects Atmospheric chemistry Environmental chemistry Ökologische Chemie (DE-588)4135167-8 gnd Aerosol (DE-588)4000595-1 gnd |
| topic_facet | Air - Pollution - Aspect de l'environnement Aérosols Aérosols - Aspect de l'environnement Chimie de l'atmosphère Chimie de l'environnement Umwelt Aerosols Aerosols Environmental aspects Air Pollution Environmental aspects Atmospheric chemistry Environmental chemistry Ökologische Chemie Aerosol |
| url | http://www.loc.gov/catdir/enhancements/fy0805/2007042414-b.html http://www.loc.gov/catdir/enhancements/fy0805/2007042414-d.html http://www.loc.gov/catdir/enhancements/fy0805/2007042414-t.html http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=015706591&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT colbeckian environmentalchemistryofaerosols |
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