Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
Jülich
Forschungszentrum, Zentralbibliothek
2005
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| Schriftenreihe: | Berichte des Forschungszentrums Jülich
4180 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | VII, 143 S. Ill., graph. Darst. 30 cm |
Internformat
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| 245 | 1 | 0 | |a Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |c Maxim Titov. [Forschungszentrum Jülich in der Helmholtz-Gemeinschaft, Institut für Sicherheitsforschung und Reaktortechnik] |
| 246 | 1 | |a Characterisation and final disposal behaviour of thoria-based fuel kernels in aqueous phases | |
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Datensatz im Suchindex
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| adam_text | CHARACTERISATION AND FINAL DISPOSAL BEHAVIOUR OF THORIA-BASED FUEL
KERNELS IN AQUEOUS PHASES VON DER FAKULTAT FUR GEORESSOURCEN UND
MATERIALTECHNIK DER RHEINISCH-WESTFALISCHEN TECHNISCHEN HOCHSCHULE
AACHEN ZUR ERLANGUNG DES AKADEMISCHEN GRADES EINES DOKTORS DER
NATURWISSENSCHAFTEN GENEHMIGTE DISSERTATION VORGELEGT VON
INGENIEUR-PHYSIKER MAXIM TITOV AUS KRASNOYARSK, RUTLAND BERICHTER:
UNIV.-PROF. DR.RER.NAT. REINHARD ODOJ UNIV.-PROF. DR.RER.NAT.
RAINERTELLE ULB DARMSTADT 111111111111 16232335 TAG DER MUNDLICHEN
PRUFUNG: 12. APRIL 2005 A. INTRODUCTION AND OBJECTIVES B. STATEMENT OF
PROBLEM B.I. THORIUM DIOXIDE: PROPERTIES AND NUCLEAR APPLICATIONS BAA.
THORIUM BA.2. THORIUM DIOXIDE BA.3. THORIA-ACTINIDE OXIDE SOLID
SOLUTIONS BAA. THORIUM FUEL CYCLE 5.7.5. REACTOR EXPERIENCE WITH THO2
AND (TH, U)O2 FUELS B.2. HTR REACTOR B.2.1. FUEL KERNELS B.2.2. COATED
PARTICLES B.2.3. HTR DESIGN AND FEATURES B.3. FINAL DISPOSAL OF HTR
SPENT FUEL B.3A. SPENT FUEL MANAGEMENT B.3.2. FINAL DISPOSAL IN DEEP
GEOLOGICAL FORMATIONS B.3.3. SALT DOME REPOSITORY B.3.4. ACCIDENT
SCENARIO B.4. DISSOLUTION OF THORIA IN AQUEOUS PHASES BAA. DISSOLUTION
MECHANISM OF OXIDES IN AQUEOUS PHASES BA.2. THERMODYNAMIC ASPECTS OFTHO2
STABILITY BA.3. SPECIAL FEATURES OF SPENT FUEL LEACHING BAA. DISSOLUTION
AND LEACHING B.4.5. SIMULATION OF SOLID SOLUTION LEACHING BY THE MONTE
CARLO METHOD C. EXPERIMENTAL PART C.I. TECHNIQUES C.2. REAGENTS AND
MATERIALS C.2.1. PREPARATION OF SALT BRINES C.3. EXPERIMENTAL PROCEDURES
C.3.1. COATED PARTICLE CHARACTERISATION C.3.2. KERNEL ISOLATION C.3.3.
KERNEL CHARACTERISATION C.3.4. INVESTIGATION OF MECHANICAL PROPERTIES OF
OXIDE FUEL KERNELS C.3.5. PREPARATION OF THORIA-URANIA POWDERS C.3.6.
DESCRIPTION OF MONTE CARLO SIMULATION 3 3 5 6 7 9 10 11 12 14 14 15 16
17 19 19 24 28 30 31 .35 35 35 36 36 36 37 37 38 40 40 I C.4. LEACHING
EXPERIMENTS 41 C.4.1. STATIC AND SEQUENTIAL KERNEL LEACHING EXPERIMENTS
43 C.4.2. LEACHING EXPERIMENTS UNDER /-IRRADIATION 44 C.4.3. POWDER
LEACHING EXPERIMENTS 46 C.4.4. LEACHING EXPERIMENTS IN ACIDIC MEDIA 47
D. RESULTS AND DISCUSSION 49 D.I. CHARACTERISATION OF COATED PARTICLES,
KERNELS AND POWDERS 49 DA A. COATED PARTICLE STRUCTURE 4 9 D. 1.2.
PROPERTIES OF THORIA-URANIA MIXED OXIDE FUEL KERNELS 50 DA.3.
CHARACTERISATION OF THORIA-URANIA POWDERS 54 D.2. MECHANICAL PROPERTIES
OF CERAMIC KERNELS 56 D.2.1. HERTZIAN INDENTATION 56 D.2.2. BEHAVIOUR OF
CERAMIC KERNELS UNDER UNIAXIAL COMPRESSION 57 D.2.3. MECHANISM OF KERNEL
FRACTURE UNDER UNIAXIAL COMPRESSION 60 D.2.4. KERNEL CRUSHING STRENGTH
DISTRIBUTIONS 62 D.3. LEACHING BEHAVIOUR OF (TH,U)C 2 FUEL KERNELS 65
D.3.1. FUEL KERNEL LEACHING IN DEIONISED WATER AND SALT BRINES 65 D.
3.2. SEM INVESTIGATIONS OF LEACHED KERNELS 72 D.3.3. CHANGES OF KERNEL
MECHANICAL PROPERTIES DURING LEACHING 75 D.3.4. THORIA-URANIA POWDER
LEACHING EXPERIMENTS 79 D.3.5. DISSOLUTION OF(TH, U)O2FUEL KERNELS IN
HYDROCHLORIC ACID 81 D.3.6. COMPARISON OF DISSOLUTION RATES IN DIFFERENT
AQUEOUS MEDIA: EFFECT OF COMPOSITION ON MATERIAL LEACHABILITY 86 D.3. 7.
FUEL KERNEL LEACHING UNDER Y-IRRADIATION 90 D.4. MONTE CARLO SIMULATION
OF SOLID SOLUTION LEACHING 97 D.4.1. DISSOLUTION KINETICS OF
ONE-COMPONENT SYSTEM 97 DA.2. SOLID SOLUTION LEACHING 98 E. SUMMARY AND
OUTLOOK 107 F. ACKNOWLEDGEMENTS 111 G. REFERENCES 113 H. APPENDIX 123
H.I. EXPERIMENTAL SCHEMES 123 H.2. XRD INVESTIGATIONS 124 II H.3.
LEACHING EXPERIMENT DATA 124 H.3.1. FUEL KERNEL LEACHING IN DEIONISED
WATER AND SALT BRINES 125 H.3.2. EVOLUTION OF KERNEL MECHANICAL
PROPERTIES DURING LEACHING 128 H.3.3. POWDER LEACHING EXPERIMENTS IN
SALT BRINES 129 H. 3.4. KERNEL DISSOLUTION IN HCL AND HNO 3 130 H.3.5.
KERNEL LEACHING IN WATER UNDER /-IRRADIATION 132 H.4. MONTE CARLO
SIMULATION OF SOLID SOLUTION DISSOLUTION 133 HA A. MONTE CARLO
SIMULATION ROUTINE SOURCE CODE 133 HA. 2. DETERMINATION OF MODEL INPUT
PARAMETERS 137 H.5. LIST OF TABLES 139 H.6. LIST OF FIGURES 140 III
|
| adam_txt |
CHARACTERISATION AND FINAL DISPOSAL BEHAVIOUR OF THORIA-BASED FUEL
KERNELS IN AQUEOUS PHASES VON DER FAKULTAT FUR GEORESSOURCEN UND
MATERIALTECHNIK DER RHEINISCH-WESTFALISCHEN TECHNISCHEN HOCHSCHULE
AACHEN ZUR ERLANGUNG DES AKADEMISCHEN GRADES EINES DOKTORS DER
NATURWISSENSCHAFTEN GENEHMIGTE DISSERTATION VORGELEGT VON
INGENIEUR-PHYSIKER MAXIM TITOV AUS KRASNOYARSK, RUTLAND BERICHTER:
UNIV.-PROF. DR.RER.NAT. REINHARD ODOJ UNIV.-PROF. DR.RER.NAT.
RAINERTELLE ULB DARMSTADT 111111111111 ' 16232335 TAG DER MUNDLICHEN
PRUFUNG: 12. APRIL 2005 A. INTRODUCTION AND OBJECTIVES B. STATEMENT OF
PROBLEM B.I. THORIUM DIOXIDE: PROPERTIES AND NUCLEAR APPLICATIONS BAA.
THORIUM BA.2. THORIUM DIOXIDE BA.3. THORIA-ACTINIDE OXIDE SOLID
SOLUTIONS BAA. THORIUM FUEL CYCLE 5.7.5. REACTOR EXPERIENCE WITH THO2
AND (TH, U)O2 FUELS B.2. HTR REACTOR B.2.1. FUEL KERNELS B.2.2. COATED
PARTICLES B.2.3. HTR DESIGN AND FEATURES B.3. FINAL DISPOSAL OF HTR
SPENT FUEL B.3A. SPENT FUEL MANAGEMENT B.3.2. FINAL DISPOSAL IN DEEP
GEOLOGICAL FORMATIONS B.3.3. SALT DOME REPOSITORY B.3.4. ACCIDENT
SCENARIO B.4. DISSOLUTION OF THORIA IN AQUEOUS PHASES BAA. DISSOLUTION
MECHANISM OF OXIDES IN AQUEOUS PHASES BA.2. THERMODYNAMIC ASPECTS OFTHO2
STABILITY BA.3. SPECIAL FEATURES OF SPENT FUEL LEACHING BAA. DISSOLUTION
AND LEACHING B.4.5. SIMULATION OF SOLID SOLUTION LEACHING BY THE MONTE
CARLO METHOD C. EXPERIMENTAL PART C.I. TECHNIQUES C.2. REAGENTS AND
MATERIALS C.2.1. PREPARATION OF SALT BRINES C.3. EXPERIMENTAL PROCEDURES
C.3.1. COATED PARTICLE CHARACTERISATION C.3.2. KERNEL ISOLATION C.3.3.
KERNEL CHARACTERISATION C.3.4. INVESTIGATION OF MECHANICAL PROPERTIES OF
OXIDE FUEL KERNELS C.3.5. PREPARATION OF THORIA-URANIA POWDERS C.3.6.
DESCRIPTION OF MONTE CARLO SIMULATION 3 3 5 6 7 9 10 11 12 14 14 15 16
17 19 19 24 28 30 31 .35 35 35 36 36 36 37 37 38 40 40 I C.4. LEACHING
EXPERIMENTS 41 C.4.1. STATIC AND SEQUENTIAL KERNEL LEACHING EXPERIMENTS
43 C.4.2. LEACHING EXPERIMENTS UNDER /-IRRADIATION 44 C.4.3. POWDER
LEACHING EXPERIMENTS 46 C.4.4. LEACHING EXPERIMENTS IN ACIDIC MEDIA 47
D. RESULTS AND DISCUSSION 49 D.I. CHARACTERISATION OF COATED PARTICLES,
KERNELS AND POWDERS 49 DA A. COATED PARTICLE STRUCTURE 4 9 D. 1.2.
PROPERTIES OF THORIA-URANIA MIXED OXIDE FUEL KERNELS 50 DA.3.
CHARACTERISATION OF THORIA-URANIA POWDERS 54 D.2. MECHANICAL PROPERTIES
OF CERAMIC KERNELS 56 D.2.1. HERTZIAN INDENTATION 56 D.2.2. BEHAVIOUR OF
CERAMIC KERNELS UNDER UNIAXIAL COMPRESSION 57 D.2.3. MECHANISM OF KERNEL
FRACTURE UNDER UNIAXIAL COMPRESSION 60 D.2.4. KERNEL CRUSHING STRENGTH
DISTRIBUTIONS 62 D.3. LEACHING BEHAVIOUR OF (TH,U)C 2 FUEL KERNELS 65
D.3.1. FUEL KERNEL LEACHING IN DEIONISED WATER AND SALT BRINES 65 D.
3.2. SEM INVESTIGATIONS OF LEACHED KERNELS 72 D.3.3. CHANGES OF KERNEL
MECHANICAL PROPERTIES DURING LEACHING 75 D.3.4. THORIA-URANIA POWDER
LEACHING EXPERIMENTS 79 D.3.5. DISSOLUTION OF(TH, U)O2FUEL KERNELS IN
HYDROCHLORIC ACID 81 D.3.6. COMPARISON OF DISSOLUTION RATES IN DIFFERENT
AQUEOUS MEDIA: EFFECT OF COMPOSITION ON MATERIAL LEACHABILITY 86 D.3. 7.
FUEL KERNEL LEACHING UNDER Y-IRRADIATION 90 D.4. MONTE CARLO SIMULATION
OF SOLID SOLUTION LEACHING 97 D.4.1. DISSOLUTION KINETICS OF
ONE-COMPONENT SYSTEM 97 DA.2. SOLID SOLUTION LEACHING 98 E. SUMMARY AND
OUTLOOK 107 F. ACKNOWLEDGEMENTS 111 G. REFERENCES 113 H. APPENDIX 123
H.I. EXPERIMENTAL SCHEMES 123 H.2. XRD INVESTIGATIONS 124 II H.3.
LEACHING EXPERIMENT DATA 124 H.3.1. FUEL KERNEL LEACHING IN DEIONISED
WATER AND SALT BRINES 125 H.3.2. EVOLUTION OF KERNEL MECHANICAL
PROPERTIES DURING LEACHING 128 H.3.3. POWDER LEACHING EXPERIMENTS IN
SALT BRINES 129 H. 3.4. KERNEL DISSOLUTION IN HCL AND HNO 3 130 H.3.5.
KERNEL LEACHING IN WATER UNDER /-IRRADIATION 132 H.4. MONTE CARLO
SIMULATION OF SOLID SOLUTION DISSOLUTION 133 HA A. MONTE CARLO
SIMULATION ROUTINE SOURCE CODE 133 HA. 2. DETERMINATION OF MODEL INPUT
PARAMETERS 137 H.5. LIST OF TABLES 139 H.6. LIST OF FIGURES 140 III |
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| index_date | 2024-07-02T13:37:47Z |
| indexdate | 2024-07-09T20:33:42Z |
| institution | BVB |
| language | English |
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| spelling | Titov, Maxim Verfasser aut Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases Maxim Titov. [Forschungszentrum Jülich in der Helmholtz-Gemeinschaft, Institut für Sicherheitsforschung und Reaktortechnik] Characterisation and final disposal behaviour of thoria-based fuel kernels in aqueous phases Jülich Forschungszentrum, Zentralbibliothek 2005 VII, 143 S. Ill., graph. Darst. 30 cm txt rdacontent n rdamedia nc rdacarrier Berichte des Forschungszentrums Jülich 4180 Zugl.: Aachen, Techn. Hochsch., Diss., 2005 Abgebranntes Brennelement swd Endlagerung swd (DE-588)4113937-9 Hochschulschrift gnd-content Berichte des Forschungszentrums Jülich 4180 (DE-604)BV004194732 4180 HEBIS Datenaustausch Darmstadt application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=014565953&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Titov, Maxim Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases Berichte des Forschungszentrums Jülich Abgebranntes Brennelement swd Endlagerung swd |
| subject_GND | (DE-588)4113937-9 |
| title | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| title_alt | Characterisation and final disposal behaviour of thoria-based fuel kernels in aqueous phases |
| title_auth | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| title_exact_search | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| title_exact_search_txtP | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| title_full | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases Maxim Titov. [Forschungszentrum Jülich in der Helmholtz-Gemeinschaft, Institut für Sicherheitsforschung und Reaktortechnik] |
| title_fullStr | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases Maxim Titov. [Forschungszentrum Jülich in der Helmholtz-Gemeinschaft, Institut für Sicherheitsforschung und Reaktortechnik] |
| title_full_unstemmed | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases Maxim Titov. [Forschungszentrum Jülich in der Helmholtz-Gemeinschaft, Institut für Sicherheitsforschung und Reaktortechnik] |
| title_short | Characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| title_sort | characterisation and final disposal behaviour of thoria based fuel kernels in aqueous phases |
| topic | Abgebranntes Brennelement swd Endlagerung swd |
| topic_facet | Abgebranntes Brennelement Endlagerung Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=014565953&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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