Lithium ion batteries: solid electrolyte interphase
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
London
Imperial College Press
2004
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Hier auch später erschienene, unveränderte Nachdrucke |
| Beschreibung: | XV, 407 S. Ill., graph. Darst. |
| ISBN: | 1860943624 |
Internformat
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| 245 | 1 | 0 | |a Lithium ion batteries |b solid electrolyte interphase |c ed.: Perla B. Balbuena ... |
| 246 | 1 | 3 | |a Lithium-ion batteries |
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Datensatz im Suchindex
| _version_ | 1804132812164431872 |
|---|---|
| adam_text | EDITORS PERLA B. BALBUENA YIXUAN WANG UNIVERSITY OF SOUTH CAROLINA
LITHIUM-ION BATTERIES SOLID-ELECTROLYTE INTERPHASE IMPERIAL COLLEGE
PRESS CONTENTS PREFACE XIII CHAPTER 1. SEI ON LITHIUM, GRAPHITE,
DISORDERED CARBONS AND TIN-BASED ALLOYS 1 EMANUEL PELED AND DIANA
GOLODNITSKY 1. INTRODUCTION 1 2. SEI FORMATION 3 2.1 THE MAIN PRINCIPLES
AND ROUTES OF THE SEI FORMATION 3 2.2 STRUCTURE OF THE SEI 5 3. CHEMICAL
COMPOSITION AND PROPERTIES OF THE SEI ON INERT SUBSTRATE AND ON LITHIUM
7 3.1 INERT METAL SUBSTRATE 7 3.2 LITHIUM COVERED BY A NATIVE FILM 10
3.3 SEI FORMATION IN SOLID POLYMER AND GEL ELECTROLYTES 11 4.
CARBONACEOUS ELECTRODES 13 4.1 PRINCIPLES OF SEI FORMATION 13 4.2 SEI
COMPOSITION AND MORPHOLOGY 16 4.2.1 HOPG 16 4.2.2 SLX20 28 4.2.3
DISORDERED CARBONS 32 4.2.4 OVERVIEW OF SEI COMPOSITION AND PROPERTIES
IN DIFFERENT CARBON/NON-AQUEOUS ELECTROLYTE SYSTEMS 45 4.2.5 EFFECT
OFCARBONMODIFICATIONON SEI FORMATION 49 5. SEI FORMATION ON LITHIUM-TIN
ALLOYS 53 6. CONCLUSIONS 59 CHAPTER 2. IDENTIFICATION OF SURFACE FILMS
ON ELECTRODES IN NON-AQUEOUS ELECTROLYTE SOLUTIONS: SPECTROSCOPIC,
ELECTRONIC AND MORPHOLOGICAL STUDIES 70 DORON AURBACH AND YARON S. COHEN
1. INTRODUCTION 70 LA. PASSIVATION OF SURFACE FILMS: A GENERAL
PHENOMENON 70 VI LITHIUM-ION BATTERIES: SOLID-ELECTROLYTE INTERPHASE IB.
MODES OF GROWTH OF SURFACE FILM PHENOMENA, AND THEIR TRANSPORT
PROPERTIES 72 LC. ON THE EFFECT OF THE ELECTROLYTE SOLUTIONS 73 ID. THE
ROLE OF THE CATION IN SURFACE PHENOMENA IN NON-AQUEOUS ELECTROLYTE
SOLUTIONS 74 LE. ON THE IMPACT OF THE ELECTRODE S MATERIAL 75 LF. SOME
COMMENTS ON APPLICATIONS 76 2. METHODS FOR IDENTIFICATION OF SURFACE
FILMS ON ELECTRODES 77 2A. INTRODUCTORY REMARKS 77 2B. FAST FOURIER
TRANSFORM INFRARED SPECTROSCOPY (FTIR) 78 2C. RAMAN SPECTROSCOPY 80 2D.
ULTRAVIOLET, VISIBLE LIGHT (UV-VIS) 81 2E. EXTENDED X-RAY ABSORPTION
FINE STRUCTURE (EXAFS), X-RAY ABSORPTION NEAR-EDGE STRUCTURE (XANES) 82
2F. X-RAY PHOTOELECTRON SPECTROSCOPY (XPS) AND AUGER (AES) ELECTRON
SPECTROSCOPY 82 2G. ENERGY DISPERSIVE ANALYSISOF X-RAYS (ED AX) 82 2H.
SECONDARY ION MASS SPECTROMETRY (SIMS) 83 2I. ELECTROCHEMICAL QUARTE
CRYSTAL MICROBALANCE (EQCM) 83 2J. X-RAY DIFFRACTOMETRY (XRD) 85 2K.
NMR, ESR SPECTROSCOPY 86 21. SCANNING PROBE MICROSCOPIES (AFM, STM) 86
2M. THE USE OF UHV SYSTEMS FOR IDENTIFICATION OF SURFACE FILMS FORMED ON
LITHIUM 87 3. THE GENERAL STRUCTURE OF SURFACE FILMS ON REACTIVE
SURFACES 87 3A. INTRODUCTION 87 3B. SURFACE FILM FORMATION ON ACTIVE
METALS 88 3C. SURFACE FILM FORMATION ON NON-REACTIVE METAL AND CARBON
ELECTRODES 90 3D. ON TRANSPORT PROPERTIES OF SURFACE FILMS 93 4.
IMPEDANCE SPECTROSCOPY OF ELECTRODES COVERED BY SURFACE FILMS 93 4A.
INTRODUCTORY REMARKS 93 4B. ACTIVE METAL ELECTRODES 94 4B. 1 LITHIUM 94
4B.2 MG ELECTRODES 95 4C. NON-ACTIVE METAL ELECTRODES POLARIZED TO LOW
POTENTIALS 97 5. IDENTIFICATION OF SURFACE FILMS FORMED ON LITHIUM AND
NON-ACTIVE ELECTRODES POLARIZED TO LOW POTENTIALS IN LI SALT SOLUTIONS
100 CONTENTS VN 5A. THE PREPARATION OF A LIBRARY OF FTIR SPECTRA 100 5B.
IDENTIFICATION OF SURFACE FILMS FORMED ON LI ELECTRODES IN ETHER
SOLUTIONS 102 5C. IDENTIFICATION OF SURFACE FILMS FORMED ON LI AND
NON-ACTIVE ELECTRODES AT LOW POTENTIALS IN ESTER SOLUTIONS 105 5D.
IDENTIFICATION OF SURFACE FILMS FORMED ON LI AND NON-ACTIVE METALS AT
LOW POTENTIALS IN ALKYL CARBONATE SOLUTIONS 107 5E. THE IMPACT OF SALT
ANIONS AND CONTAMINANT REACTIONS ON THE SURFACE CHEMISTRY OF LITHIUM AND
NOBLE METAL ELECTRODES IN NON-AQUEOUS LI SALT SOLUTIONS 111 5F. ON
SURFACE FILMS FORMED ON LI ELECTRODES IN POLYMERIC ELECTROLYTES 116 6.
SURFACE FILMS ON LITHIATED CARBON ELECTRODES 116 6A. INTRODUCTORY
REMARKS: SURFACE FILM FORMATION ON CARBON ELECTRODES, THE INFLUENCE OF
THE TYPE OF CARBON, AND THE IMPACT OF THE SURFACE FILMS ON LI INSERTION
PROCESSES 116 6B. ON THE IDENTIFICATION OF SURFACE FILMS FORMED ON
LITHIATED GRAPHITE ELECTRODES 117 6C. ON THE CORRELATION BETWEEN THE
PERFORMANCE OF LITHIATED GRAPHITE ANODES AND THEIR SURFACE CHEMISTRY 120
7. SURFACE STUDIES OF LITHIUM AND LITHIATED CARBON ELECTRODES BY
SCANNING PROBE MICROSCOPY 124 7A. IMAGING OF LI ELECTRODES BYAFM 124 7B.
GRAPHITE ELECTRODES 126 8. ABOUT SURFACE FILM FORMATION ON TRANSITION
METAL OXIDE CATHODES IN NON-AQUEOUS SALT SOLUTIONS 128 9. IDENTIFICATION
OF SURFACE FILMS ON CALCIUM AND MAGNESIUM ELECTRODES 129 10. CONCLUDING
REMARKS 131 CHAPTER 3. SPECTROSCOPY STUDIES OF SOLID-ELECTROLYTE
INTERPHASE ON POSITIVE AND NEGATIVE ELECTRODES FOR LITHIUM ION BATTERIES
140 ZHAOXIANG WANG, XUEJIE HUANG ANDLIQUAN CHEN 1. INTRODUCTION 140 2.
SEI ON TIN OXIDE ANODE IN VARIOUS ELECTROLYTES 141 2.1 SAMPLE
PREPARATION AND INSTRUMENTAL 143 2.2 CAPACITY LOSS AND ELECTROLYTE
DECOMPOSITION IN FIRST CYCLE 144 VLLL LITHIUM-ION BATTERIES:
SOLID-ELECTROLYTE INTERPHASE 2.3 HRTEM STUDY OF SEI STRUCTURE ON
NANO-SNO SURFACE 145 2.4 IDENTIFICATION OFLI 2 C0 3 AND ROC0 2 LI ON
NANO-SNO ANODES 146 2.5 FORMATION OFLI 2 C03 AND ROC0 2 LI ON NANO-SNO
ANODES 150 2.6 QUESTION: WHAT IS THE REDUCTION SEQUENCE OF SNO AND
ELECTROLYTE? 152 2.7 ELECTROLYTE-DEPENDENT SEI COMPOSITION 154 2.8
CONCLUSION 157 3. SURFACE ENHANCED RAMAN SCATTERING (SERS) ON ROUGH
ELECTRODES 157 3.1 NORMAL RAMAN SCATTERING AND SERS STUDIES ON BATTERY
MATERIALS 158 3.2 EXPERIMENTAL 159 3.3 ELECTROCHEMICAL PERFORMANCE
OFAGELECTRODE 160 3.4 SERS STUDY OF PASSIVATING FILM ON AG ELECTRODE IN
LITHIUM BATTERIES 160 3.5 PROSPECTS AND CONCLUSIONS ON RAMAN SCATTERING
IN SEI INVESTIGATION 166 4. INFRARED ABSORPTION AND X-RAY PHOTELECTRON
SPECTROSCOPIC INVESTIGATION ON PERFORMANCE IMPROVEMENT OF
SURFACE-MODIFIED LICO0 2 CATHODE MATERIALS 167 4.1 SAMPLE PREPARATION
170 4.2 COMPARISON OF EC ADSORBED ON DIFFERENT SUBSTRATES 172 4.3 IR
SPECTRAOFECON ELECTRODES CHARGEDTO DIFFERENT VOLTAGES 180 4.4 XPS STUDY
ON EVOLUTION OF ELECTRONIC STRUCTURE OF CATHODE MATERIALS WITH CHARGE
VOLTAGES 185 4.5 CONCLUSIONS 189 5. SUMMARY AND COMMENTS 190 6.
ACKNOWLEDGEMENTS 190 CHAPTER 4. SCANNING PROBE MICROSCOPY ANALYSIS OF
THE SEI FORMATION ON GRAPHITE ANODES 198 MINORU INABA AND ZEMPACHI OGUMI
1. INTRODUCTION 198 2. CHARGE AND DISCHARGE CHARACTERISTICS OF GRAPHITE
ANODE IN EC- AND PC-BASED SOLUTIONS 201 3. MORPHOLOGY CHANGES OF HOPG
BASAL PLANES IN THE INITIAL STAGE OF SOLVENT DECOMPOSITION 203 4. SEI
FORMATION IN EC-BASED SOLUTIONS 206 CONTENTS IX 5. EFFECT OF CO-SOLVENT
ON SOLVENT CO-INTERCALATION IN EC-BASED SOLUTIONS 211 6. ADDITIVES IN
PC-BASED SOLUTIONS 214 6.1 ROLES OF VC, FEC, AND ES AS ADDITIVES 216 6.2
ROLES OFOTHER ADDITIVES IN PC-BASED SOLUTIONS 220 7. SUMMARY AND OUTLOOK
221 CHAPTER 5. THEORETICAL INSIGHTS INTO THE SEI COMPOSITION AND
FORMATION MECHANISM: DENSITY FUNCTIONAL THEORY STUDIES 227 YIXUAN
WANGANDPERLASS. BALBUENA 1 . INTRODUCTION 227 2. THEORETICAL MODEIS AND
COMPUTATIONAL DETAILS 229 3. INITIAL REDUCTION OF LI + (EC), LI + (PC),
AND LI + (VC) 231 4. COMPARISON OF REDUCTIVE DECOMPOSITION BETWEEN EC
AND PC: LI + (EC) N AND LI + (PC) N (N = 2, 3) 232 4.1 REDUCTION
POTENTIALS AND RING OPENING BARRIERS OF EC AND PC 233 4.2 DECOMPOSITION
PRODUCTS OF EC AND PC: LI + (EC) 2 AND LI + (PC) 2 235 THE EFFECT OF VC
ON THE REDUCTIVE DECOMPOSITION OF EC AND 5. PC: (S) N LI + (VC) (S = EC
AND PC; N = 1 AND 2) CLUSTERS 238 5.1 INITIAL REDUCTION 238 5.2
TERMINATIONREACTIONOFRADICALANIONS 241 5.3 SUMMARY OF REDUCTIVE
DECOMPOSITION OF SOLVENTS IN THE PRESENCE OF VC 246 6. ASSOCIATIONS OF
LITHIUM ALKYL DICARBONATES THROUGH 0~»»LI + »»»0~ BRIDGES 247 6.1
GEOMETRIES AND ENERGETICS 247 6.2 VIBRATIONAL FREQUENCIES 255 7.
ADSORPTION AND TWO-DIMENSIONAL ASSOCIATION OF LITHIUM ALKYL DICARBONATES
ON GRAPHITE SURFACES THROUGH 0~ »»»LI + »»»»7T (ARENE) INTERACTIONS 260
7.1 - H-TRUNCATED CLUSTER MODEIS 261 7.2 ADSORPTION OF LITHIUM ALKYL
DICARBONATES ON THE BASAL PLANE OFTHE NEUTRAL GRAPHITE SURFACE 262 7.3
ADSORPTION OF LITHIUM ALKYL DICARBONATES ON THE BASAL PLANE OF
NEGATIVELY CHARGED GR 54 AND EDGE PLANE OF GR 78 ^ 267 X LITHIUM-ION
BATTERIES: SOLID-ELECTROLYTE INTERPHASE 7.4 TWO-DIMENSIONAL ASSOCIATION
OF LITHIUM ALKYL DICARBONATES ON THE BASAL PLANE OF THE GRAPHITE SURFACE
(GR 96 ) 269 7.5 SUMMARY ABOUT ADSORPTIONS OF LVD, LED AND LPD ON ANODE
SURFACE 271 8. REMARKS ON THE FAILURE OF PC AND THE EFFICIENCY OF VC FOR
THE SEI LAYER FORMATION IN EC/PC-BASED SOLUTIONS 272 CHAPTER 6.
CONTINUUM AND STATISTICAL MECHANICS-BASED MODEIS FOR SOLID-ELECTROLYTE
INTERPHASES IN LITHIUM-ION BATTERIES 276 HARRY J. PLOEHN, PREMANAND
RAMADASS, RALPH E. WHITE, DIEGO ALTOMARE ANDPERLA B. BALBUENA 1.
INTRODUCTION 276 2. CONTINUUM MODEIS FOR SEI GROWTH 277 2.1 OVERVIEW
OFPREVIOUS MACROSCOPIC MODEIS 277 2.2 ELEMENTS OF CONTINUUM MECHANICS
280 2.2.1 KINEMATICS 282 2.2.2 CONSERVATIONOFMASS 285 2.3 DYNAMIC
CONTINUUM MODEIS FOR SEI FORMATION AND GROWTH 287 2.3.1 GROWTH LIMITED
BY SEI ELECTRONIC CONDUCTIVITY 288 2.3.2 GROWTH LIMITED BY SOLVENT
DIFFUSION 291 3. STATISTICAL MECHANICS-BASED MODEL 296 3.1 DESCRIPTION
OF THE LATTICE-GAS MODEL 297 3.1.1 IMPLEMENTATION OF THE MODEL 299 3.2
RESULTS AND DISCUSSIONS 299 3.3 REMARKS WITH RESPECT TO THE LATTICE
MODEL 305 CHAPTER 7. DEVELOPMENT OF NEW ANODES FOR RECHARGEABLE LITHIUM
BATTERIES AND THEIR SEI CHARACTERIZATION BY RAMAN AND NEXAFS
SPECTROSCOPY 308 GISELLE SAUDI 1. INTRODUCTION 308 2. CARBON AS A HOST
IN LITHIUM ION CELLS 310 3. ALTERNATIVE ANODE MATERIALS 319 4. UV RAMAN
SPECTROSCOPY OFTEMPLATED-DISORDEREDCARBONS 321 5. SEI CHARACTERIZATION
BY NEXAFS 323 CONTENTS XI 1. 2. 3. 4. 5. BACKGROUND LIMN 2 0 4 2.1
XPSANALYSIS 2.2 ELEVATED TEMPERATURE EFFECTS FOR LIMN 2 0 4 LICO0 2 ,
LINI0 2 AND LINIO. 8 CO 0 . 2 0 2 LIFEP0 4 SUMMARY 6. CONCLUSIONS 331 7.
ACKNOWLEDGEMENTS 331 CHAPTER 8. THE CATHODE-ELECTROLYTE INTERFACE IN A
LI-ION BATTERY 337 KRISTINA EDSTROEM, TORBJOERN GUSTAFSSON AND JOSH THOMAS
337 338 340 344 353 358 360 CHAPTER 9. THEORETICAL STUDIES ON THE
SOLVENT STRUCTURE AND ASSOCIATION PROPERTIES, AND ON THE LI-ION
SOLVATION: IMPLICATIONS FOR SEI LAYER PHENOMENA 365 YIXUAN WANG ANDPERLA
B. BALBUENA 1. INTRODUCTION 365 2. COMPUTATIONAL DETAILS 367 3.
GEOMETRIE STRUCTURES OF VARIOUS CYCLIC/LINEAR CARBONATES, AND EFFECTIVE
ADDITIVES AND CO-SOLVENTS TO PC-BASED SOLUTIONS 368 4. SEIF AND CROSS
ASSOCIATIONS OF CYCLIC/LINEAR CARBONATES VIA C-H»»0 INTERACTIONS 373
4.1 GEOMETRIE AND ENERGETIC PROPERTIES 374 4.2 C-H BOND LENGTHS AND
VIBRATIONAL FREQUENCIES 380 4.3 C=0 BOND LENGTHS AND VIBRATIONAL
FREQUENCIES 384 4.4 CHARACTERISTICS OF C-H»»»0 INTERACTIONS USING AIM
384 5. LI + SOLVATION FROM ALKYL CARBONATES 387 5.1 INTERACTIONS BETWEEN
LI + AND ORGANIC SOLVENTS 387 5.2 SOLVATION MUMBEROFLI + 390 6.
CONCLUSION: IMPLICATIONS FOR SEI LAYER PHENOMENA 393 INDEX 398
|
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| id | DE-604.BV019372299 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T19:58:46Z |
| institution | BVB |
| isbn | 1860943624 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-012835677 |
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| owner_facet | DE-703 DE-91 DE-BY-TUM DE-91G DE-BY-TUM |
| physical | XV, 407 S. Ill., graph. Darst. |
| publishDate | 2004 |
| publishDateSearch | 2004 |
| publishDateSort | 2004 |
| publisher | Imperial College Press |
| record_format | marc |
| spelling | Lithium ion batteries solid electrolyte interphase ed.: Perla B. Balbuena ... Lithium-ion batteries London Imperial College Press 2004 XV, 407 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Hier auch später erschienene, unveränderte Nachdrucke Electrochemistry Electrolytes Conductivity Lithium cells Lithiumbatterie (DE-588)4167901-5 gnd rswk-swf Lithiumbatterie (DE-588)4167901-5 s DE-604 Balbuena, Perla B. Sonstige oth GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=012835677&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Lithium ion batteries solid electrolyte interphase Electrochemistry Electrolytes Conductivity Lithium cells Lithiumbatterie (DE-588)4167901-5 gnd |
| subject_GND | (DE-588)4167901-5 |
| title | Lithium ion batteries solid electrolyte interphase |
| title_alt | Lithium-ion batteries |
| title_auth | Lithium ion batteries solid electrolyte interphase |
| title_exact_search | Lithium ion batteries solid electrolyte interphase |
| title_full | Lithium ion batteries solid electrolyte interphase ed.: Perla B. Balbuena ... |
| title_fullStr | Lithium ion batteries solid electrolyte interphase ed.: Perla B. Balbuena ... |
| title_full_unstemmed | Lithium ion batteries solid electrolyte interphase ed.: Perla B. Balbuena ... |
| title_short | Lithium ion batteries |
| title_sort | lithium ion batteries solid electrolyte interphase |
| title_sub | solid electrolyte interphase |
| topic | Electrochemistry Electrolytes Conductivity Lithium cells Lithiumbatterie (DE-588)4167901-5 gnd |
| topic_facet | Electrochemistry Electrolytes Conductivity Lithium cells Lithiumbatterie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=012835677&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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