Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
2003
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | München, Techn. Univ., Diss., 2003 |
| Beschreibung: | V, 104 S. Ill., graph. Darst. |
Internformat
MARC
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| 084 | |a CHE 160d |2 stub | ||
| 084 | |a CHE 154d |2 stub | ||
| 100 | 1 | |a Pisliakov, Andrei |d 1976- |e Verfasser |0 (DE-588)128706074 |4 aut | |
| 245 | 1 | 0 | |a Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |c Andrei Pisliakov |
| 246 | 1 | 3 | |a Theory of time- and frequency-gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| 264 | 1 | |c 2003 | |
| 300 | |a V, 104 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 500 | |a München, Techn. Univ., Diss., 2003 | ||
| 650 | 0 | 7 | |a Hexamethylbenzol |0 (DE-588)4587570-4 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Tetracyanoethylen |0 (DE-588)4184867-6 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Spontane Emission |0 (DE-588)4323946-8 |2 gnd |9 rswk-swf |
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
| 689 | 0 | 0 | |a Tetracyanoethylen |0 (DE-588)4184867-6 |D s |
| 689 | 0 | 1 | |a Hexamethylbenzol |0 (DE-588)4587570-4 |D s |
| 689 | 0 | 2 | |a Spontane Emission |0 (DE-588)4323946-8 |D s |
| 689 | 0 | |5 DE-604 | |
| 856 | 4 | 2 | |m DNB Datenaustausch |q application/pdf |u http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010728519&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |3 Inhaltsverzeichnis |
| 940 | 1 | |n oe | |
| 943 | 1 | |a oai:aleph.bib-bvb.de:BVB01-010728519 | |
Datensatz im Suchindex
| _version_ | 1816445219354181632 |
|---|---|
| adam_text |
CONTENTS
1
INTRODUCTION
1
2
TIME
AND
FREQUENCY-GATED
SPONTANEOUS
EMISSION:
GENERAL
THEORY
7
2.1
INTRODUCTION
.
7
2.2
DEFINITION
OF
THE
TIME-RESOLVED
SPECTRUM
.
9
2.3
POLARIZATION
.
11
2.3.1
DEFINITION
.
11
2.3.2
CALCULATION
OF
THE
POLARIZATION:
PERTURBATIVE
APPROACH
.
13
2.3.3
TIME
AND
FREQUENCY-RESOLVED
SIGNAL
IN
TERMS
OF
RESPONSE
FUNCTIONS
15
2.3.4
CALCULATION
OF
RESPONSE
FUNCTIONS
.
16
2.4
DOORWAY-WINDOW
REPRESENTATION
OF
TIME-RESOLVED
SPECTRA
.
17
2.4.1
DOORWAY-WINDOW
PICTURE:
OPERATOR
FORM
.
17
2.4.2
DOORWAY-WINDOW
PICTURE:
COMPUTATIONAL
ASPECTS
.
19
2.4.3
CONNECTION
BETWEEN
THE
TWO
THEORETICAL
APPROACHES
.
20
2.4.4
TRANSIENT
EFFECTS
.
21
2.5
DOORWAY-WINDOW
PICTURE
FOR
DISSIPATIVE
SYSTEMS
.
21
2.6
SUMMARY
.
23
3
TIME-RESOLVED
FLUORESCENCE
OF
SIMPLE
MODEL
SYSTEMS
25
3.1
INTRODUCTION
.
25
3.2
HARMONIC
OSCILLATOR
.
26
3.2.1
ANALYTIC
RESPONSE
FUNCTIONS
.
27
3.2.2
TIME
AND
FREQUENCY
RESOLUTION
EFFECTS
.
28
3.3
BROWNIAN
OSCILLATOR
.
30
3.3.1
ANALYTIC
RESPONSE
FUNCTIONS
.
30
3.3.2
DISSIPATION
EFFECTS
.
31
3.4
DRUDE
OSCILLATOR
.
33
3.4.1
ANALYTIC
RESPONSE
FUNCTIONS
.
34
3.4.2
MEMORY
EFFECTS
.
34
3.5
SUMMARY
.
36
4
TIME-RESOLVED
FLUORESCENCE
OF
ULTRAFAST
ELECTRON
TRANSFER
SYSTEMS
39
4.1
INTRODUCTION
.
39
4.2
ELECTRON
TRANSFER
MODEL
.
40
4.2.1
HAMILTONIANS
.
40
4.2.2
EQUATIONS
OF
MOTION
(REDFIELD
THEORY)
.
42
IV
CONTENTS
4.3
SPECIFIC
EXAMPLES
AND
DISCUSSION
.
43
4.3.1
INTEGRAL
SIGNAL
.
43
4.3.2
ELECTRONIC
COHERENCE
IN
ELECTRON
TRANSFER
.
44
4.3.3
VIBRATIONAL
COHERENCE
IN
ELECTRON
TRANSFER
.
47
4.3.4
TIME
AND
FREQUENCY-GATED
SPONTANEOUS
EMISSION
SPECTRA
.
49
4.3.5
FINITE
PUMP
DURATION
.
52
4.4
SUMMARY
.
53
5
APPLICATION:
TIME-RESOLVED
FLUORESCENCE
OF
THE
TCNE-HMB
COMPLEX
55
5.1
INTRODUCTION
.
55
5.1.1
EXPERIMENTS
.
55
5.1.2
PREVIOUS
SIMULATIONS
AND
THEORETICAL
INTERPRETATIONS
.
56
5.1.3
OUR
GOALS
.
57
5.2
COMPUTATIONAL
DETAILS
.
58
5.3
RESULTS
AND
INTERPRETATIONS
.
59
5.3.1
CUT
AT
A
=
774
NM
.
59
5.3.2
PEAK-SHIFT
.
60
5.3.3
COMPARISON
OF
SEVERAL
CUTS
.
62
5.3.4
INTEGRAL
SIGNAL
.
64
5.3.5
TIME-RESOLVED
FLUORESCENCE
SPECTRUM
.
66
5.3.6
COMPARISON
WITH
THE
SINGLE-EXCITED-STATE
MODEL
.
66
5.4
POSSIBLE
IMPROVEMENTS
OF
THE
MODEL
.
67
5.5
SUMMARY
.
68
6
PHENOMENOLOGICAL
RELAXATION
MODEL
69
6.1
INTRODUCTION
.
69
6.2
THE
MODEL
.
69
6.3
ANALYTIC
EXPRESSIONS
FOR
NONLINEAR
RESPONSE
FUNCTIONS
.
72
6.4
TIME
AND
FREQUENCY-GATED
SPONTANEOUS
EMISSION
IN
THE
FRAMEWORK
OF
THE
PHENOMENOLOGICAL
RELAXATION
MODEL
.
74
6.5
APPLICATIONS
OF
THE
MODEL
.
76
6.5.1
COMPARISON
WITH
A
BROWNIAN
OSCILLATOR
MODEL
.
77
6.5.2
COMPARISON
WITH
REDFIELD
THEORY
FOR
ELECTRON
TRANSFER
SYSTEMS
.
78
6.6
SUMMARY
.
83
7
CONCLUSIONS
85
A
TIME
AND
FREQUENCY-GATED
SPONTANEOUS
EMISSION
SPECTRA
IN
TERMS
OF
WIGNER
SPECTROGRAMS
89
B
NONPERTURBATIVE
TREATMENT
OF
THE
EXCITATION
PROCESS
91
C
PUMP-PROBE
SIGNAL
IN
THE
FRAMEWORK
OF
THE
PHENOMENOLOGICAL
RELAX
ATION
MODEL
95
BIBLIOGRAPHY
97 |
| any_adam_object | 1 |
| author | Pisliakov, Andrei 1976- |
| author_GND | (DE-588)128706074 |
| author_facet | Pisliakov, Andrei 1976- |
| author_role | aut |
| author_sort | Pisliakov, Andrei 1976- |
| author_variant | a p ap |
| building | Verbundindex |
| bvnumber | BV017887737 |
| classification_tum | CHE 160d CHE 154d |
| ctrlnum | (OCoLC)645633262 (DE-599)BVBBV017887737 |
| discipline | Physik Chemie |
| format | Book |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV017887737 |
| illustrated | Illustrated |
| indexdate | 2024-11-22T17:39:12Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-010728519 |
| oclc_num | 645633262 |
| open_access_boolean | |
| owner | DE-91 DE-BY-TUM DE-12 |
| owner_facet | DE-91 DE-BY-TUM DE-12 |
| physical | V, 104 S. Ill., graph. Darst. |
| publishDate | 2003 |
| publishDateSearch | 2003 |
| publishDateSort | 2003 |
| record_format | marc |
| spelling | Pisliakov, Andrei 1976- Verfasser (DE-588)128706074 aut Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation Andrei Pisliakov Theory of time- and frequency-gated spontaneous emission from systems with nonadiabatic coupling and dissipation 2003 V, 104 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier München, Techn. Univ., Diss., 2003 Hexamethylbenzol (DE-588)4587570-4 gnd rswk-swf Tetracyanoethylen (DE-588)4184867-6 gnd rswk-swf Spontane Emission (DE-588)4323946-8 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Tetracyanoethylen (DE-588)4184867-6 s Hexamethylbenzol (DE-588)4587570-4 s Spontane Emission (DE-588)4323946-8 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010728519&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Pisliakov, Andrei 1976- Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation Hexamethylbenzol (DE-588)4587570-4 gnd Tetracyanoethylen (DE-588)4184867-6 gnd Spontane Emission (DE-588)4323946-8 gnd |
| subject_GND | (DE-588)4587570-4 (DE-588)4184867-6 (DE-588)4323946-8 (DE-588)4113937-9 |
| title | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| title_alt | Theory of time- and frequency-gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| title_auth | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| title_exact_search | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| title_full | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation Andrei Pisliakov |
| title_fullStr | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation Andrei Pisliakov |
| title_full_unstemmed | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation Andrei Pisliakov |
| title_short | Theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| title_sort | theory of time and frequency gated spontaneous emission from systems with nonadiabatic coupling and dissipation |
| topic | Hexamethylbenzol (DE-588)4587570-4 gnd Tetracyanoethylen (DE-588)4184867-6 gnd Spontane Emission (DE-588)4323946-8 gnd |
| topic_facet | Hexamethylbenzol Tetracyanoethylen Spontane Emission Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010728519&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT pisliakovandrei theoryoftimeandfrequencygatedspontaneousemissionfromsystemswithnonadiabaticcouplinganddissipation |