Modern spectroscopy:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Chichester [u.a.]
Wiley
2004
|
| Ausgabe: | 4. ed. |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XXVII, 452 S. graph. Darst. |
| ISBN: | 9780470844168 0470844167 0470844159 |
Internformat
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| 100 | 1 | |a Hollas, John Michael |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Modern spectroscopy |c J. Michael Hollas |
| 250 | |a 4. ed. | ||
| 264 | 1 | |a Chichester [u.a.] |b Wiley |c 2004 | |
| 300 | |a XXVII, 452 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
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| 650 | 4 | |a Analyse spectrale | |
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| 650 | 7 | |a Foto-elektronspectrometrie |2 gtt | |
| 650 | 7 | |a Física moderna |2 larpcal | |
| 650 | 7 | |a Kwantummechanica |2 gtt | |
| 650 | 7 | |a Laser spectrometrie |2 gtt | |
| 650 | 7 | |a Molecuulstructuur |2 gtt | |
| 650 | 7 | |a Rotatiespectra |2 gtt | |
| 650 | 7 | |a Spectrometrie |2 gtt | |
| 650 | 7 | |a Vibratiespectra |2 gtt | |
| 650 | 4 | |a Spectrum analysis | |
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Datensatz im Suchindex
| _version_ | 1804130374116179968 |
|---|---|
| adam_text | Contents
Preface to first edition xiii
Preface to second edition xv
Preface to third edition xvii
Preface to fourth edition xix
Units, dimensions and Conventions xxi
Fundamental constants xxiü
Useful conversion factors xxv
1 Some important results in quantum mechanics 1
1.1 Spectroscopy and quantum mechanics 1
1.2 The evolution of quantum theory 2
1.3 The Schrödinger equation and some of its Solutions 8
1.3.1 The Schrödinger equation 9
1.3.2 The hydrogen atom 11
1.3.3 Electron spin and nuclear spin angular momentan 17
1.3.4 The Born-Oppenheimer approximation 19
1.3.5 The rigid rotor 21
1.3.6 The harmonic oscillator 23
Exercises 25
Bibliography 26
2 Electromagnetic radiation and its interaction with atoms
and molecules 27
2.1 Electromagnetic radiation 27
2.2 Absorption and emission of radiation 27
2.3 Line width 34
2.3.1 Natural line broadening 34
2.3.2 Doppier broadening 35
2.3.3 Pressure broadening 36
2.3.4 Power, or Saturation, broadening 36
2.3.5 Removal of line broadening 37
2.3.5.1 Effiisive atomic or molecular beams 37
2.3.5.2 Lamb dip spectroscopy 37
v
vi CONTENTS
Exercises 38
Bibliography 39
3 General features of experimental methods 41
3.1 The electromagnetic spectrum 41
3.2 General components of an absorption experiment 42
3.3 Dispersmg elements 43
3.3.1 Pnsms 43
3.3.2 Diffraction gratings 45
3.3.3 Fourier transformation and interferometers 48
3.3.3.1 Radiofrequency radiation 49
3.3.3.2 Infrared, visible and ultraviolet radiation 55
3.4 Components of absorption experiments in various regions of the spectrum 59
3.4.1 Microwave and millimetre wave 59
3.4.2 Far-infrared 61
3.4.3 Near-infrared and mid-infrared 62
3.4.4 Visible and near-ultraviolet 62
3.4.5 Vacuum- or far-ultraviolet 63
3.5 Other experimental techniques 64
3.5.1 Attenuated total reflectance spectroscopy and
reflection-absorption infrared spectroscopy 64
3.5.2 Atomic absorption spectroscopy 64
3.5.3 Inductively coupled plasma atomic emission spectroscopy 66
3.5.4 Flash photolysis 67
3.6 Typical recording spectrophotometers for the near-infrared, mid-infrared,
visible and near-ultraviolet regions 68
Exercise 70
Bibliography 70
4 Molecular symmetry 73
4.1 Elements of symmetry 3
4.1.1 n-Fold axis of symmetry, C„ *
4.1.2 Plane of symmetry, a 75
4.1.3 Centre of inversion, / 6
4.1.4 n-Fold rotation-reflection axis of symmetry, Sn
4.1.5 The identity element of symmetry, / (or E)
4.1.6 Generation of elements
4.1.7 Symmetry conditions for molecular chirality
4.2 Point groups 81
4.2.1 C„ point groups °^
4.2.2 Sn point groups °
4.2.3 Cni point groups
4.2.4 Dn point groups
4.2.5 Cnh point groups ^
4.2.6 Dnd point groups S4
4.2.7 D„h point groups ^4
CONTENTS vii
4.2.8 Td point group 85
4.2.9 Oh point group 85
4.2.10 Kh point group 86
4.2.11 4 point group 86
4.2.12 Other point groups 87
4.3 Point group character tables 87
4.3.1 C2l. character table ¦ 87
4.3.2 C3l. character table 92
4.3.3 Cxr character table 96
4.3.4 4 character table 97
4.4 Symmetry and dipole moments 97
Exercises 102
Bibliography 102
5 Rotational spectroscopy 103
5.1 Linear, Symmetrie rotor, spherical rotor and asymmetric rotor molecules 103
5.2 Rotational infrared, millimetre wave and microwave spectra 105
5.2.1 Diatomic and linear polyatomic molecules 105
5.2.1.1 Transition frequencies or wavenumbers 105
5.2.1.2 Intensities 110
5.2.1.3 Centrifugal distortion 111
5.2.1.4 Diatomic molecules in excited vibrational states 112
5.2.2 Symmetrie rotor molecules 113
5.2.3 Stark effect in diatomic, linear and Symmetrie rotor molecules 115
5.2.4 Asymmetric rotor molecules 116
5.2.5 Spherical rotor molecules 117
5.2.6 Interstellar molecules detected by their radiofrequency, microwave
or millimetre wave spectra 119
5.3 Rotational Raman spectroscopy 122
5.3.1 Experimental methods 122
5.3.2 Theory of rotational Raman scattering 124
5.3.3 Rotational Raman spectra of diatomic and linear polyatomic
molecules 126
5.3.4 Nuclear spin statistical weights 128
5.3.5 Rotational Raman spectra of Symmetrie and asymmetric rotor
molecules 131
5.4 Structure determination from rotational constants 131
Exercises 134
Bibliography 135
6 Vibrational spectroscopy 137
6.1 Diatomic molecules 137
6.1.1 Infrared spectra 138
6.1.2 Raman spectra 140
6.1.3 Anharmonicity 142
6.1.3.1 Electrical anharmonicity 142
6.1.3.2 Mechanical anharmonicity 142
viü CONTENTS
6.1.4 Vibration-rotation spectroscopy 147
6.1.4.1 Infirared spectra 147
6.1.4.2 Raman spectra 151
6.2 Polyatomic molecules 154
6.2.1 Group vibrations 154
6.2.2 Number of normal vibrations of each symmetry species 162
6.2.2.1 Non-degenerate vibrations 163
6.2.2.2 Degenerate vibrations 165
6.2.3 Vibrational selection rules 166
6.2.3.1 Infrared spectra 166
6.23.2 Raman spectra 172
6.2.4 Vibration-rotation spectroscopy 173
6.2.4.1 Infrared spectra of linear molecules 174
6.2.4.2 Infrared spectra of Symmetrie rotors 1 °
6.2.4.3 Infrared spectra of spherical rotors 180
6.2.4.4 Infrared spectra of asymmetric rotors 181
6.2.5 Anharmonicity 184
6.2.5.1 Potential energy surfaces 184
6.2.5.2 Vibrational term values 186
6.2.5.3 Local mode treatment of vibrations 1°
6.2.5.4 Vibrational potential funetions with more than one minimum 188
6.2.5.4(a) Inversion vibrations ^°
6.2.5.4(b) Ring-puckering vibrations 1 !
6.2.5.4(c) Torsional vibrations ¦ ¦^
Exercises 195
Bibliography 196
7 Electronic spectroscopy 1
7.1 Atomic spectroscopy 199
7.1.1 The periodic table 1
7.1.2 Vector representation of momenta and vector coupling approximations 201
7.1.2.1 Angular momenta and magnetic moments 201
7.1.2.2 Coupling of angular momenta 20S
7.1.2.3 Russell-Saunders coupling approximation ^
7.1.2.3(a) Non-equivalent electrons 206
7.1.2.3(b) Equivalent electrons 210
7.1.3 Spectra of alkali metal atoms 213
7.1.4 Spectrum of the hydrogen atom 216
7.1.5 Spectra of helium and the alkaline earth metal atoms 219
999
7.1.6 Spectra of other polyelectronic atoms /zz
7.2 Electronic spectroscopy of diatomic molecules 225
7.2.1 Molecular Orbitals ^
7.2.1.1 Homonuclear diatomic molecules
732
7.2.1.2 Heteronuclear diatomic molecules
9T^
7.2.2 Classification of electronic states
7.2.3 Electronic selection rules 236
9^7
7.2.4 Derivation of states arising frorn configurations z
7.2.5 Vibrational coarse strueture
7.2.5.1 Potential energy curves in excited electronic states ^
7.2.5.2 Progressions and sequences
CONTENTS ix
7.2.5.3 The Franck-Condon principle 246
7.2.5.4 Deslandres tables 250
7.2.5.5 Dissociation energies 250
7.2.5.6 Repulsive states and continuous spectra 253
7.2.6 Rotational fine structure 254
7.2.6.1 Z — £ electronic and vibronic transitions 254
7.2.6.2 n — £ electronic and vibronic transitions 257
7.3 Electronic spectroscopy of polyatomic molecules 260
7.3.1 Molecular Orbitals and electronic states 260
7.3.1.1 AH2 molecules 261
7.3.U(a) ZHAH= 180° 261
7.3.1.1(b) ZHAH = 90c 263
7.3.1.2 Formaldehyde (H2CO) 265
7.3.1.3 Benzene 267
7.3.1.4 Crystal field and ligand field molecular Orbitals 270
7.3.1.4(a) Crystal field theory 271
7.3.1.4(b) Ligand field theory 273
7.3.1.4(c) Electronic transitions 275
7.3.2 Electronic and vibronic selection rules 275
7.3.3 Chromophores 278
7.3.4 Vibrational coarse structure 278
7.3.4.1 Sequences 278
7.3.4.2 Progressions 279
7.3.4.2(a) Totally Symmetrie vibrations 279
7.3.4.2(b) Non-totally Symmetrie vibrations 279
7.3.5 Rotational fine structure 283
7.3.6 Diffuse spectra 284
Exercises 287
Bibliography 288
8 Photoelectron and related spectroscopies 289
8.1 Photoelectron spectroscopy 289
8.1.1 Experimental methods 291
8.1.1.1 Sources of monochromatic ionizing radiation 291
8.1.1.2 Electron velocity analysers 294
8.1.1.3 Electron detectors 294
8.1.1.4 Resolution 294
8.1.2 Ionization processes and Koopmans theorem 295
8.1.3 Photoelectron spectra and their interpretation 297
8.1.3.1 Ultraviolet photoelectron spectra of atoms 297
8.1.3.2 Ultraviolet photoelectron spectra of molecules 298
8.1.3.2(a) Hydrogen 298
8.1.3.2(b) Nitrogen 300
8.1.3.2(c) Hydrogen bromide 302
8.1.3.2(d) Water 305
8.1.3.2(e) Benzene 305
8.1.3.3 X-ray photoelectron spectra of gases 307
8.1.3.4 X-ray photoelectron spectra of solids 313
8.2 Auger electron and X-ray fluorescence spectroscopy 315
8.2.1 Auger electron spectroscopy 317
8.2.1.1 Experimental method 317
x CONTENTS
8.2.1.2 Processes in Auger electron ejection 318
8.2.1.3 Examples of Auger electron spectra 319
8.2.2 X-ray fluorescence spectroscopy 322
8.2.2.1 Experimental method 322
8.2.2.2 Processes in X-ray fluorescence 324
8.2.2.3 Examples of X-ray fluorescence spectra 325
8.3 Extended X-ray absorption fine structure 327
Exercises 334
Bibliography 335
9 Lasers and laser spectroscopy 337
9.1 General discussion of lasers 337
9.1.1 General features and properties 337
9.1.2 Methods of obtaming population Inversion 340
9.1.3 Laser cavity modes 341
9.1.4 ß-switching 342
9.1.5 Modelocking 344
9.1.6 Harmonie generation 345
9.2 Examples of lasers 346
9.2.1 The ruby and alexandrite lasers 346
9.2.2 The titanium-sapphire laser 348
9.2.3 The neodymmm-YAG laser 349
9.2.4 The diode or semiconduetor laser 350
9.2.5 The helium-neon laser 352
9.2.6 The argon ion and krypton ion lasers 354
9.2.7 The nitrogen (N2) laser 355
9.2.8 The excimer and exciplex lasers 356
9.2.9 The carbon dioxide laser 358
9.2.10 The dye lasers 359
9.2.11 Laser materials in general 362
9.3 Uses of lasers in spectroscopy 362
9.3.1 Hyper Raman spectroscopy 363
9.3.2 Stimulated Raman spectroscopy 365
9.3.3 Coherent anti-Stokes Raman scattering spectroscopy 367
9.3.4 Laser Stark (or laser electron resonance) spectroscopy 368
9.3.5 Two-photon and multiphoton absorption 371
9.3.6 Multiphoton dissociation and laser Separation of isotopes 374
9.3.7 Single vibronic level, or dispersed, fluorescence 377
9.3.8 Light detection and ranging (LIDAR) 379
9.3.9 Cavity ring-down spectroscopy 382
9.3.10 Femtosecond spectroscopy 3o7
9.3.11 Spectroscopy of molecules in supersonic jets 393
9.3.11.1 Properties of a supersonic jet 393
9.3.11.2 Fluorescence excitation spectroscopy 370
9.3.11.3 Single vibronic level, or dispersed, fluorescence
spectroscopy ™
9.3.11.4 Zero kinetic energy photoelectron spectroscopy 402
Exercises 404
Bibliography 405
CONTENTS xi
Appendix
A Character tables 407
B Symmetry species of vibrations 423
Index of Atoms and Molecules 429
Subject Index 439
|
| any_adam_object | 1 |
| author | Hollas, John Michael |
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| dewey-full | 543.0858 535.8/4 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 543 - Analytical chemistry 535 - Light and related radiation |
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| dewey-search | 543.0858 535.8/4 |
| dewey-sort | 3543.0858 |
| dewey-tens | 540 - Chemistry and allied sciences 530 - Physics |
| discipline | Chemie / Pharmazie Physik Chemie |
| edition | 4. ed. |
| format | Book |
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| genre | (DE-588)4123623-3 Lehrbuch gnd-content |
| genre_facet | Lehrbuch |
| id | DE-604.BV017618479 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T19:20:01Z |
| institution | BVB |
| isbn | 9780470844168 0470844167 0470844159 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-010600285 |
| oclc_num | 54817480 |
| open_access_boolean | |
| owner | DE-29 DE-91G DE-BY-TUM DE-703 DE-526 DE-83 DE-188 |
| owner_facet | DE-29 DE-91G DE-BY-TUM DE-703 DE-526 DE-83 DE-188 |
| physical | XXVII, 452 S. graph. Darst. |
| publishDate | 2004 |
| publishDateSearch | 2004 |
| publishDateSort | 2004 |
| publisher | Wiley |
| record_format | marc |
| spelling | Hollas, John Michael Verfasser aut Modern spectroscopy J. Michael Hollas 4. ed. Chichester [u.a.] Wiley 2004 XXVII, 452 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd rswk-swf Molekülspektroskopie (DE-588)4128850-6 gnd rswk-swf Theorie (DE-588)4059787-8 gnd rswk-swf Atomspektroskopie (DE-588)4143333-6 gnd rswk-swf (DE-588)4123623-3 Lehrbuch gnd-content Molekülspektroskopie (DE-588)4128850-6 s DE-604 Atomspektroskopie (DE-588)4143333-6 s Spektroskopie (DE-588)4056138-0 s Theorie (DE-588)4059787-8 s 1\p DE-604 Erscheint auch als Online-Ausgabe 9780470094716 (DE-604)BV046662001 HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010600285&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Hollas, John Michael Modern spectroscopy Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Theorie (DE-588)4059787-8 gnd Atomspektroskopie (DE-588)4143333-6 gnd |
| subject_GND | (DE-588)4056138-0 (DE-588)4128850-6 (DE-588)4059787-8 (DE-588)4143333-6 (DE-588)4123623-3 |
| title | Modern spectroscopy |
| title_auth | Modern spectroscopy |
| title_exact_search | Modern spectroscopy |
| title_full | Modern spectroscopy J. Michael Hollas |
| title_fullStr | Modern spectroscopy J. Michael Hollas |
| title_full_unstemmed | Modern spectroscopy J. Michael Hollas |
| title_short | Modern spectroscopy |
| title_sort | modern spectroscopy |
| topic | Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Theorie (DE-588)4059787-8 gnd Atomspektroskopie (DE-588)4143333-6 gnd |
| topic_facet | Analyse spectrale Análise espectral Foto-elektronspectrometrie Física moderna Kwantummechanica Laser spectrometrie Molecuulstructuur Rotatiespectra Spectrometrie Vibratiespectra Spectrum analysis Spektroskopie Molekülspektroskopie Theorie Atomspektroskopie Lehrbuch |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010600285&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT hollasjohnmichael modernspectroscopy |